期刊文献+
共找到148,986篇文章
< 1 2 250 >
每页显示 20 50 100
Scheme for implementing quantum dense coding with W-class state in cavity QED 被引量:3
1
作者 何娟 叶柳 倪致祥 《Chinese Physics B》 SCIE EI CAS CSCD 2008年第5期1597-1600,共4页
An experimentally feasible protocol for realizing dense coding by using a class of W-state in cavity quantum electrodynamics (QED) is proposed in this paper. The prominent advantage of our scheme is that the success... An experimentally feasible protocol for realizing dense coding by using a class of W-state in cavity quantum electrodynamics (QED) is proposed in this paper. The prominent advantage of our scheme is that the successful probability of the dense coding with a W-class state can reach 1. In addition, the scheme can be implemented by the present cavity QED techniques. 展开更多
关键词 quantum dense coding w-class state cavity quantum electrodynamics (QED)
下载PDF
Scheme for implementing perfect remote state preparation with W-class state in cavity QED 被引量:1
2
作者 王学文 彭朝晖 《Chinese Physics B》 SCIE EI CAS CSCD 2008年第7期2346-2351,共6页
In this paper we present a remote state preparation scheme with a three-qubit W-class state in cavity QED. It has been shown that a special single-qubit state and a special two-qubit entangled state can be remotely pr... In this paper we present a remote state preparation scheme with a three-qubit W-class state in cavity QED. It has been shown that a special single-qubit state and a special two-qubit entangled state can be remotely prepared perfectly. Furthermore, the classical information cost in this scheme is less than that in the corresponding teleportation scheme and only a single-qubit projective measurement is made by the sender. We also generalize this idea to the multiqubit W-class state. 展开更多
关键词 remote state preparation w-class state cavity QED
下载PDF
Deterministic quantum teleportation and information splitting via a peculiar W-class state 被引量:1
3
作者 梅锋 於亚飞 张智明 《Chinese Physics B》 SCIE EI CAS CSCD 2010年第2期62-66,共5页
In the paper (Phys. Rev. 2006 A 4 062320) Agrawal et al. have introduced a kind of W-class state which can be used for the quantum teleportation of single-particle state via a three-particle von Neumann measurement,... In the paper (Phys. Rev. 2006 A 4 062320) Agrawal et al. have introduced a kind of W-class state which can be used for the quantum teleportation of single-particle state via a three-particle von Neumann measurement, and they thought that the state could not be used to teleport an unknown state by making two-particle and one-particle measurements. Here we reconsider the features of the W-class state and the quantum teleportation process via the W-class state. We show that, by introducing a unitary operation, the quantum teleportation can be achieved deterministically by making two-particle and one-particle measurements. In addition, our protocol is extended to the process of teleporting two-particle state and splitting information. 展开更多
关键词 w-class state quantum teleportation quantum information splitting
下载PDF
Quantum Teleportation and Superdense Coding via W-Class States 被引量:1
4
作者 WU Huai-Zhi YANG Zhen-Biao ZHENG Shi-Biao 《Communications in Theoretical Physics》 SCIE CAS CSCD 2008年第4期901-904,共4页
根据 Agrawal 等的协议,我们为远距传物并且稠密的编码的实现建议一个洞证完计划。而不是使用 EPR 状态和 GHZ 状态,我们的计划对由把一个 W 班状态用作一条量隧道的一个粒子的损失更感觉迟钝。而且,我们的计划对热地有免疫力,并且... 根据 Agrawal 等的协议,我们为远距传物并且稠密的编码的实现建议一个洞证完计划。而不是使用 EPR 状态和 GHZ 状态,我们的计划对由把一个 W 班状态用作一条量隧道的一个粒子的损失更感觉迟钝。而且,我们的计划对热地有免疫力,并且不要求洞在整个过程留在真空状态。 展开更多
关键词 量子无线电技术 电子传播 密度点 电子技术
下载PDF
Distillation of GHZ State from Multiple Copies of Arbitrary W-Class State
5
作者 WU Chun-Wang CHEN Ping-Xing LI Cheng-Zu 《Communications in Theoretical Physics》 SCIE CAS CSCD 2008年第6期1502-1504,共3页
W。D ü r 等。证明了经由本地操作和古典通讯(LOCC ) 从任意的 W 班状态的一个拷贝获得一个 GHZ 状态是不可能的[W。D ü r, G。Vidal,和 J.I Cirac, Phys。加快。一 62 (2000 ) 062314 ] 。在我们的纸,更一般的案例小心... W。D ü r 等。证明了经由本地操作和古典通讯(LOCC ) 从任意的 W 班状态的一个拷贝获得一个 GHZ 状态是不可能的[W。D ü r, G。Vidal,和 J.I Cirac, Phys。加快。一 62 (2000 ) 062314 ] 。在我们的纸,更一般的案例小心地被调查。我们首先证明与任意的 W 班状态的二个拷贝的供应,我们能总是构造一个明确的过程与非零可能性提取一个 GHZ 状态。然后基于这结果,为从任意的 W 班状态的 n 拷贝提取 GHZ 状态的一个简单过程被介绍。最后,我们简短讨论应用。 展开更多
关键词 蒸馏 GHZ状态 W类状态 物理研究
下载PDF
Scheme for Implementing Perfect Quantum Teleportation with Non-maximally Entangled W-Class State in Cavity QED
6
作者 PENG Zhao-Hui JIA Chun-Xia LI Jun-Gang 《Communications in Theoretical Physics》 SCIE CAS CSCD 2008年第8期375-378,共4页
We propose an experimentally feasible teleportation scheme with three-atom W-class state,which was first proposed by Agrawal and Pati [P.Agrawal and A.Pati,Phys.Rev.A 74 (2006) 062320 ],in cavity QED.In this scheme at... We propose an experimentally feasible teleportation scheme with three-atom W-class state,which was first proposed by Agrawal and Pati [P.Agrawal and A.Pati,Phys.Rev.A 74 (2006) 062320 ],in cavity QED.In this scheme atoms interact simultaneously with a nonresonant cavity and there is no energy exchange between the atoms and the cavity.Thus it is insensitive to the cavity decay,which is of importance in view of experiment. 展开更多
关键词 量子 远距传物 缠结 物理
下载PDF
Semi-analytical solution for drained expansion analysis of a hollow cylinder of critical state soils 被引量:1
7
作者 He Yang Jialiang Zhang +1 位作者 Haisui Yu Peizhi Zhuang 《Journal of Rock Mechanics and Geotechnical Engineering》 SCIE CSCD 2024年第6期2326-2340,共15页
The expansion of a thick-walled hollow cylinder in soil is of non-self-similar nature that the stress/deformation paths are not the same for different soil material points.As a result,this problem cannot be solved by ... The expansion of a thick-walled hollow cylinder in soil is of non-self-similar nature that the stress/deformation paths are not the same for different soil material points.As a result,this problem cannot be solved by the common self-similar-based similarity techniques.This paper proposes a novel,exact solution for rigorous drained expansion analysis of a hollow cylinder of critical state soils.Considering stress-dependent elastic moduli of soils,new analytical stress and displacement solutions for the nonself-similar problem are developed taking the small strain assumption in the elastic zone.In the plastic zone,the cavity expansion response is formulated into a set of first-order partial differential equations(PDEs)with the combination use of Eulerian and Lagrangian descriptions,and a novel solution algorithm is developed to efficiently solve this complex boundary value problem.The solution is presented in a general form and thus can be useful for a wide range of soils.With the new solution,the non-self-similar nature induced by the finite outer boundary is clearly demonstrated and highlighted,which is found to be greatly different to the behaviour of cavity expansion in infinite soil mass.The present solution may serve as a benchmark for verifying the performance of advanced numerical techniques with critical state soil models and be used to capture the finite boundary effect for pressuremeter tests in small-sized calibration chambers. 展开更多
关键词 Cavity expansion Drained analysis Boundary effect Critical state soil Non-self-similar Eulerian-Lagrangian approach
下载PDF
Whole-process case management effects on mental state and selfcare ability in patients with liver cancer 被引量:1
8
作者 Man-Di Ju Qin Qin Meng Li 《World Journal of Gastrointestinal Surgery》 SCIE 2024年第3期833-841,共9页
BACKGROUND Regarding the incidence of malignant tumors in China,the incidence of liver cancer ranks fourth,second only to lung,gastric,and esophageal cancers.The case fatality rate ranks third after lung and cervical ... BACKGROUND Regarding the incidence of malignant tumors in China,the incidence of liver cancer ranks fourth,second only to lung,gastric,and esophageal cancers.The case fatality rate ranks third after lung and cervical cancer.In a previous study,the whole-process management model was applied to patients with breast cancer,which effectively reduced their negative emotions and improved treatment adherence and nursing satisfaction.METHODS In this single-center,randomized,controlled study,60 randomly selected patients with liver cancer who had been admitted to our hospital from January 2021 to January 2022 were randomly divided into an observation group(n=30),who received whole-process case management on the basis of routine nursing mea-sures,and a control group(n=30),who were given routine nursing measures.We compared differences between the two groups in terms of anxiety,depression,the level of hope,self-care ability,symptom distress,sleep quality,and quality of life.RESULTS Post-intervention,Hamilton anxiety scale,Hamilton depression scale,memory symptom assessment scale,and Pittsburgh sleep quality index scores in both groups were lower than those pre-intervention,and the observation group had lower scores than the control group(P<0.05).Herth hope index,self-care ability assessment scale-revision in Chinese,and quality of life measurement scale for patients with liver cancer scores in both groups were higher than those pre-intervention,with higher scores in the observation group compared with the control group(P<0.05).CONCLUSION Whole-process case management can effectively reduce anxiety and depression in patients with liver cancer,alleviate symptoms and problems,and improve the level of hope,self-care ability,sleep quality,and quality of life,as well as provide feasible nursing alternatives for patients with liver cancer. 展开更多
关键词 Liver cancer Mental state Self-care ability Whole-process case management Life quality NURSING
下载PDF
Target layer state estimation in multi-layer complex dynamical networks considering nonlinear node dynamics
9
作者 吴亚勇 王欣伟 蒋国平 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第4期245-252,共8页
In many engineering networks, only a part of target state variables are required to be estimated.On the other hand,multi-layer complex network exists widely in practical situations.In this paper, the state estimation ... In many engineering networks, only a part of target state variables are required to be estimated.On the other hand,multi-layer complex network exists widely in practical situations.In this paper, the state estimation of target state variables in multi-layer complex dynamical networks with nonlinear node dynamics is studied.A suitable functional state observer is constructed with the limited measurement.The parameters of the designed functional observer are obtained from the algebraic method and the stability of the functional observer is proven by the Lyapunov theorem.Some necessary conditions that need to be satisfied for the design of the functional state observer are obtained.Different from previous studies, in the multi-layer complex dynamical network with nonlinear node dynamics, the proposed method can estimate the state of target variables on some layers directly instead of estimating all the individual states.Thus, it can greatly reduce the placement of observers and computational cost.Numerical simulations with the three-layer complex dynamical network composed of three-dimensional nonlinear dynamical nodes are developed to verify the effectiveness of the method. 展开更多
关键词 multi-layer complex dynamical network nonlinear node dynamics target state estimation functional state observer
下载PDF
Topological edge and corner states of valley photonic crystals with zipper-like boundary conditions
10
作者 沈云峰 许孝芳 +2 位作者 孙铭 周文佶 常雅箐 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第4期480-491,共12页
We present a stable valley photonic crystal(VPC)unit cell with C_(3v)symmetric quasi-ring-shaped dielectric columns and realize its topological phase transition by breaking mirror symmetry.Based on this unit cell stru... We present a stable valley photonic crystal(VPC)unit cell with C_(3v)symmetric quasi-ring-shaped dielectric columns and realize its topological phase transition by breaking mirror symmetry.Based on this unit cell structure,topological edge states(TESs)and topological corner states(TCSs)are realized.We obtain a new type of wave transmission mode based on photonic crystal zipper-like boundaries and apply it to a beam splitter assembled from rectangular photonic crystals(PCs).The constructed beam splitter structure is compact and possesses frequency separation functions.In addition,we construct a box-shaped triangular PC structures with zipper-like boundaries and discover phenomena of TCSs in the corners,comparing its corner states with those formed by other boundaries.Based on this,we explore the regularities of the electric field patterns of TESs and TCSs,explain the connection between the characteristic frequencies and locality of TCSs,which helps better control photons and ensures low power consumption of the system. 展开更多
关键词 valley photonic crystal topological edge states topological corner states higher-order topological insulators topological phase transition
下载PDF
Predicted Critical State Based on Invariance of the Lyapunov Exponent in Dual Spaces
11
作者 刘通 夏旭 《Chinese Physics Letters》 SCIE EI CAS CSCD 2024年第1期68-76,共9页
Critical states in disordered systems,fascinating and subtle eigenstates,have attracted a lot of research interests.However,the nature of critical states is difficult to describe quantitatively,and in general,it canno... Critical states in disordered systems,fascinating and subtle eigenstates,have attracted a lot of research interests.However,the nature of critical states is difficult to describe quantitatively,and in general,it cannot predict a system that hosts the critical state.We propose an explicit criterion whereby the Lyapunov exponent of the critical state should be 0 simultaneously in dual spaces,namely the Lyapunov exponent remains invariant under the Fourier transform.With this criterion,we can exactly predict a one-dimensional quasiperiodic model which is not of self-duality,but hosts a large number of critical states.Then,we perform numerical verification of the theoretical prediction and display the self-similarity of the critical state.Due to computational complexity,calculations are not performed for higher dimensional models.However,since the description of extended and localized states by the Lyapunov exponent is universal and dimensionless,utilizing the Lyapunov exponent of dual spaces to describe critical states should also be universal.Finally,we conjecture that some kind of connection exists between the invariance of the Lyapunov exponent and conformal invariance,which can promote the research of critical phenomena. 展开更多
关键词 state EXPONENT CRITICAL
下载PDF
Screening of Rodents from Rural Communities of Lagos and Ogun State Nigeria of Lassa Virus RNA
12
作者 Fatai Sarafa Emmanuel Tochukwu Onyeje +3 位作者 Joseph Ojonugwa Shaibu Olumuyiwa Babalola Salu Rosemary Ajuma Audu Sunday Aremu Omilabu 《Open Journal of Medical Microbiology》 2024年第2期120-130,共11页
Background: In recent times, there has been an increase in the number of Lassa fever cases resulting from the several episodes of Lassa fever epidemics ravaging Nigeria and other West African countries. The presence o... Background: In recent times, there has been an increase in the number of Lassa fever cases resulting from the several episodes of Lassa fever epidemics ravaging Nigeria and other West African countries. The presence of Lassa virus in rodents other than the major reservoir (Mastomys natalensis) has been a public health concern as to the actual burden of the disease. It is therefore of a public health necessity to explore the LASV RNA habouring potential of several species of rodents in endemic as well as non-endemic areas for proper prevention of emergence of outbreaks in non-endemic areas. Objectives: The aim of this study was to detect the presence of LASV RNA in different species of rodents in Ikorodu, Lagos state and Abeokuta, Ogun state. Methods: A total of ninety one (91) rodents were captured from Ikorodu, Lagos State (61 rodents) and Abeokuta, Ogun State (30 rodents), euthanized, bled, and plasma obtained for the detection of LASV RNA by Reverse Transcriptase Polymerase Chain Reaction. Results: A total of 91 rodents consisting of 77 Rattus rattus and 14 Crocidura spp. The S segment of LASV RNA was not in any of the 91 rodents’ plasma samples. Conclusion: The rodents captured within the rural communities of Ikorodu, Lagos State and Abeokuta, Ogun State were found not to habour the LASV RNA. This study is limited by the relatively small sample size. Similar studies should be encouraged both in endemic and non-endemic areas in order to understand the actual burden of Lassa fever as well as put into check future epidemics. 展开更多
关键词 Lassa Virus Lassa Fever Mastomys natalensis TRANSMISSION Lagos state Ogun state
下载PDF
Comparative Study of the Socioeconomic Characteristics and Digital Literacy Level of Agricultural Extension Personnel in Imo and Ebonyi States, South-East, Nigeria
13
作者 Ogbonnaya Okoro Aja Cyril Chigozie Asiabaka +1 位作者 Anthony Okorie Ani Edna Chioma Matthews-Njoku 《Agricultural Sciences》 2024年第2期230-245,共16页
The study comparatively analysed the socioeconomic characteristics and digital literacy level of Agricultural Extension personnel (AEP) in Ebonyi and Imo States, South-East, Nigeria. The specific objectives were to de... The study comparatively analysed the socioeconomic characteristics and digital literacy level of Agricultural Extension personnel (AEP) in Ebonyi and Imo States, South-East, Nigeria. The specific objectives were to describe the socioeconomic characteristics of agricultural extension personnel in Ebonyi and Imo States, and to ascertain the digital literacy level of AEP in the studied states. Purposive sampling technique was used to select 312 Agricultural Extension personnel (132 from Ebonyi State Agricultural Development Program and 180 from Imo State Agricultural Development Program) for the study. Data were collected through the use of validated and structured questionnaire, and administered through the help of well-trained enumerators. Data were analysed using simple descriptive statistical tools such as percentages mean score, standard deviation and weighted mean. Findings indicated that they were more male in the both States (55.3% and 57.8%) for Ebonyi and Imo State respectively and that the average age of AEP in Ebonyi and Imo States were 44.7 years and 49.2 years respectively. It was further revealed that the majority (77.3% and 82.8%) had B.Sc./HND as their highest academic qualifications, belonged to professional organisations (62.1% and 75%), and were earning an average monthly income of N58,798 and N62,648 for Ebonyi and Imo State respectively. Also, it was revealed that their mean years of service were 12.4 years and 13.4 years for Ebonyi and Imo State respectively. Almost all of them (87.9% and 95.0%) own a smartphone, had access to the internet (80.3% and 90.0%), but do not own a laptop/ipad (82.6% and 72.8%) for Ebon-yi and Imo State respectively. Results further revealed that Agricultural extension personnel in both Ebonyi and Imo State respectively had low digital literacy level ( = 2.41 and 2.32). The study concluded that AEP in Ebonyi and Imo State respectively had similar socioeconomic characteristics and low level of digital literacy. The study recommended that the management of ADPs in both Ebonyi and Imo State should ensure the training of AEP in digital skills to enhance their digital literacy level to enable them use digital technologies in their work. 展开更多
关键词 Agricultural Extension Personnel Digital Literacy Ebonyi state Imo state Socioeconomic Characteristics
下载PDF
The 5αcondensate state in 20Ne
14
作者 Takahiro Kawabata 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第2期3-5,共3页
Theclustering phenomenon,in which nucleons are arranged intoparticles(4 He nuclei)within a nuclear system,is one of the most intriguing aspects of nuclear structure.It has been observed in various light nuclei,such as... Theclustering phenomenon,in which nucleons are arranged intoparticles(4 He nuclei)within a nuclear system,is one of the most intriguing aspects of nuclear structure.It has been observed in various light nuclei,such as^(8)Be,^(12)C,^(16)O,and^(20)Ne,and is responsible for many exotic and fascinating phenomena,such as the Hoyle state in^(12)C,which plays an essential role in stellar nucleosynthesis[1-6]as well as in heavy-ion collisions[7-9]. 展开更多
关键词 STRUCTURE state
下载PDF
Deep learning for determining pure isotropic proton spectra from solidstate spectra
15
作者 Mengjie Qiu Zhong Chen Yanqin Lin 《Magnetic Resonance Letters》 2024年第1期63-64,共2页
Recently,an article on ^(1)H solid-state NMR spectra was published,in which the authors proposed a deep learning approach to infer the pure isotropic proton NMR spectra obtained at an infinite magic angle spinning(MAS... Recently,an article on ^(1)H solid-state NMR spectra was published,in which the authors proposed a deep learning approach to infer the pure isotropic proton NMR spectra obtained at an infinite magic angle spinning(MAS)rate.This approach even allowed to obtain,by far,the best resolved ^(1)H spectra of molecular solids[1](https://doi.org/10.1002/anie.202216607).Deep learning based artificial intelligence is developing rapidly,and its application is deepening.Currently,there are many applications of deep learning in the field of magnetic resonance,such as the reconstruction of the under-sampled multidimensional spectra[2-4],the deconvolution of two-dimensional NMR spectra[5]and noise suppression and weak peak retrial[6],etc. 展开更多
关键词 SPECTRA ISOTROPIC state
下载PDF
Preparation and interface state of phosphate tailing-based geopolymers
16
作者 ZHANG Shou-xun XIE Xian +4 位作者 XIE Rui-qi TONG Xiong WU Yu-yao LI Jia-wen LI Yue 《Journal of Central South University》 SCIE EI CAS CSCD 2024年第6期1900-1914,共15页
The long-term storage of phosphate tailings will occupy a large amount of land,pollute soil and groundwater,thus,it is crucial to achieve the harmless disposal of phosphate tailings.In this study,high-performance geop... The long-term storage of phosphate tailings will occupy a large amount of land,pollute soil and groundwater,thus,it is crucial to achieve the harmless disposal of phosphate tailings.In this study,high-performance geopolymers with compressive strength of 38.8 MPa were prepared by using phosphate tailings as the main raw material,fly ash as the active silicon-aluminum material,and water glass as the alkaline activator.The solid content of phosphate tailings and fly ash was 60% and 40%,respectively,and the water-cement ratio was 0.22.The results of XRD,FTIR,SEM-EDS and XPS show that the reactivity of phosphate tailings with alkaline activator is weak,and the silicon-aluminum material can react with alkaline activator to form zeolite and gel,and encapsulate/cover the phosphate tailings to form a dense phosphate tailings-based geopolymer.During the formation of geopolymers,part of the aluminum-oxygen tetrahedron replaced the silicon-oxygen tetrahedron,causing the polycondensation reaction between geopolymers and increasing the strength of geopolymers.The leaching toxicity test results show that the geopolymer has a good solid sealing effect on heavy metal ions.The preparation of geopolymer from phosphate tailings is an important way to alleviate the storage pressure and realize the resource utilization of phosphate tailings. 展开更多
关键词 phosphate tailing GEOPOLYMER interface state toxicity leaching
下载PDF
Numerical simulation for the initial state of avalanche in polydisperse particle systems
17
作者 韩韧 李亭 +2 位作者 迟志鹏 杨晖 李然 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第2期405-412,共8页
Numerical simulation is employed to investigate the initial state of avalanche in polydisperse particle systems.Nucleation and propagation processes are illustrated for pentadisperse and triadisperse particle systems,... Numerical simulation is employed to investigate the initial state of avalanche in polydisperse particle systems.Nucleation and propagation processes are illustrated for pentadisperse and triadisperse particle systems,respectively.In these processes,particles involved in the avalanche grow slowly in the early stage and explosively in the later stage,which is clearly different from the continuous and steady growth trend in the monodisperse system.By examining the avalanche propagation,the number growth of particles involved in the avalanche and the slope of the number growth,the initial state can be divided into three stages:T1(nucleation stage),T2(propagation stage),T3(overall avalanche stage).We focus on the characteristics of the avalanche in the T2 stage,and find that propagation distances increase almost linearly in both axial and radial directions in polydisperse systems.We also consider the distribution characteristics of the average coordination number and average velocity for the moving particles.The results support that the polydisperse particle systems are more stable in the T2 stage. 展开更多
关键词 AVALANCHE initial state polydisperse particle systems PROPAGATION
下载PDF
Morphology and valence state evolution of Cu:Unraveling the impact on nitric oxide electroreduction
18
作者 Ting Sun Fengyu Gao +4 位作者 Ya Wang Honghong Yi Qingjun Yu Shunzheng Zhao Xiaolong Tang 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第4期276-286,共11页
Ammonia(NH3)serves as a critical component in the fertilizer industry and fume gas denitrification.However,the conventional NH3production process,namely the Haber-Bosch process,leads to considerable energy consumption... Ammonia(NH3)serves as a critical component in the fertilizer industry and fume gas denitrification.However,the conventional NH3production process,namely the Haber-Bosch process,leads to considerable energy consumption and waste gas emissions.To address this,electrocatalytic nitric oxide reduction reaction(NORR)has emerged as a promising strategy to bridge NH3consumption to NH3production,harnessing renewable electricity for a sustainable future.Copper(Cu)stands out as a prominent electrocatalyst for NO reduction,given its exceptional NH3yield and selectivity.However,a crucial aspect that remains insufficiently explored is the effects of morphology and valence states of Cu on the NORR performance.In this investigation,we synthesized CuO nanowires(CuO-NF)and Cu nanocubes(Cu-NF)as cathodes through an in situ growth method.Remarkably,CuO-NF exhibited an impressive NH3yield of 0.50±0.02 mg cm^(-2)h^(-1)at-0.6 V vs.reversible hydrogen electrode(RHE)with faradaic efficiency of29,68%±1,35%,surpassing that of Cu-NF(0.17±0.01 mg cm^(-2)h^(-1),16.18%±1.40%).Throughout the electroreduction process,secondary cubes were generated on the CuO-NF surface,preserving their nanosheet cluster morphology,sustained by an abundant supply of subsurface oxygen(s-O)even after an extended duration of 10 h,until s-O depletion ensued.Conversely,Cu-NF exhibited inadequate s-O content,leading to rapid crystal collapse within the same timeframe.The distinctive current-potential relationship,akin to a volcano-type curve,was attributed to distinct NO hydrogenation mechanisms.Further Tafel analysis revealed the exchange current density(i0)and standard heterogeneous rate constant(k0)for CuO-NF,yielding 3.44×10^(-6)A cm^(-2)and 3.77×10^(-6)cm^(-2)s^(-1)when NORR was driven by overpotentials.These findings revealed the potential of CuO-NF for NO reduction and provided insights into the intricate interplay between crystal morphology,valence states,and electrochemical performance. 展开更多
关键词 NORR Ammonia Synthesis COPPER MORPHOLOGY Valence states Mechanism
下载PDF
Spectroscopy and molecule opacity investigation on excited states of SiS
19
作者 李瑞 吕浩男 +3 位作者 桑纪群 刘晓华 梁桂颖 吴勇 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第5期381-387,共7页
The SiS molecule,which plays a significant role in space,has attracted a great deal of attention for many years.Due to complex interactions among its low-lying electronic states,precise information regarding the molec... The SiS molecule,which plays a significant role in space,has attracted a great deal of attention for many years.Due to complex interactions among its low-lying electronic states,precise information regarding the molecular structure of SiS is limited.To obtain accurate information about the structure of its excited states,the high-precision multireference configuration interaction(MRCI)method has been utilized.This method is used to calculate the potential energy curves(PECs)of the 18Λ–S states corresponding to the lowest dissociation limit of SiS.The core–valence correlation effect,Davidson’s correction and the scalar relativistic effect are also included to guarantee the precision of the MRCI calculation.Based on the calculated PECs,the spectroscopic constants of quasi-bound and bound electronic states are calculated and they are in accordance with previous experimental results.The transition dipole moments(TDMs)and dipole moments(DMs)are determined by the MRCI method.In addition,the abrupt variations of the DMs for the 1^(5)Σ^(+)and 2^(5)Σ^(+)states at the avoided crossing point are attributed to the variation of the electronic configuration.The opacity of SiS at a pressure of 100 atms is presented across a series of temperatures.With increasing temperature,the expanding population of excited states blurs the band boundaries. 展开更多
关键词 SIS OPACITY excited state spectroscopic constant configuration interaction
下载PDF
Observation of flat-band localized state in a one-dimensional diamond momentum lattice of ultracold atoms
20
作者 曾超 石悦然 +5 位作者 毛一屹 武菲菲 谢岩骏 苑涛 戴汉宁 陈宇翱 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第1期212-217,共6页
We investigated the one-dimensional diamond ladder in the momentum lattice platform. By inducing multiple twoand four-photon Bragg scatterings among specific momentum states, we achieved a flat band system based on th... We investigated the one-dimensional diamond ladder in the momentum lattice platform. By inducing multiple twoand four-photon Bragg scatterings among specific momentum states, we achieved a flat band system based on the diamond model, precisely controlling the coupling strength and phase between individual lattice sites. Utilizing two lattice sites couplings, we generated a compact localized state associated with the flat band, which remained localized throughout the entire time evolution. We successfully realized the continuous shift of flat bands by adjusting the corresponding nearest neighbor hopping strength, enabling us to observe the complete localization process. This opens avenues for further exploration of more complex properties within flat-band systems, including investigating the robustness of flat-band localized states in disordered flat-band systems and exploring many-body localization in interacting flat-band systems. 展开更多
关键词 diamond lattice flat band momentum lattice localized state
下载PDF
上一页 1 2 250 下一页 到第
使用帮助 返回顶部