Phosphorous (P) fraction characteristics in sediment resuspension were investigated under adequately hydrodynamic conditions. Four forms of P in overlying water, including dissolved inorganic P, dissolved total P, t...Phosphorous (P) fraction characteristics in sediment resuspension were investigated under adequately hydrodynamic conditions. Four forms of P in overlying water, including dissolved inorganic P, dissolved total P, total P, and particulate P, and six fractions of P in suspended particulate matter (SPM), including loosely sorbed P (NH4Cl-P), redox-sensitive P (BD-P), aluminum-bound P (Al- P), organic P (NaOH-nrP), calcium-bound P (Ca-P) and residual P (Res-P), were quantified, respectively. Different hydrodynamic conditions resulted in different P form changes. Four states could be ascribed: (1) P desorption by sediment and SPM, and P adsorption by overlying water; (2) P desorption by SPM, and P adsorption by overlying water; (3) P adsorption by SPM, and P desorption by overlying water; and (4) P equilibrium between SPM and overlying water. The contents of P in overlying water acquired peak values in the middle position of the vertical P distribution due to the combined actions of SPM and sediment. P fractions in SPM were in the following order: BD-P 〉 NaOH-nrp 〉 Ca-P 〉 Al-P 〉 Res-P 〉 NH4Cl-P. BD-P in SPM frequently exchanged with P forms in overlying water. Resuspension was favorable to forming Ca-P in SPM.展开更多
The lattice Boltzmann method was used to investigate numerically the fiber orientation distributions in slit channel flows with abrupt expansion for fiber suspensions even in the concentrated regime. The channels have...The lattice Boltzmann method was used to investigate numerically the fiber orientation distributions in slit channel flows with abrupt expansion for fiber suspensions even in the concentrated regime. The channels have a thin slit geometry with 1:4 and 1:3 expansions. Both the interactions between fibers and that between fibers and channel walls were taken into consideration. Some of numerical results are qualitatively in agreement with the experiment data. It is found that most of fibers are aligned in the flow direction in all the suspensions in the entrance region of the expansion. Fiber orientation distributions, having different patterns in different regions of the flow, depend on the expansion ratio of the channel. The mechanical fiber-fiber interaction largely affects the fiber orientation in the downstream of the expansion and in the salient corner for the cases of concentrated suspensions. The hydrodynamic interaction plays an important role on the fiber orientation in the dilute suspension.展开更多
Experiments on Phosphorus (P) fraction characteristics in sediment resuspension were performed under adequate hydrodynamic conditions. It is found that the concentration of Suspended Particulate Matter (SPM) in th...Experiments on Phosphorus (P) fraction characteristics in sediment resuspension were performed under adequate hydrodynamic conditions. It is found that the concentration of Suspended Particulate Matter (SPM) in the eddy current region exhibits the "Matthew effect". Velocity is an impact factor of the Equilibrium Phosphate Concentration (EPC), which is related to other hydraulic conditions. Overall bioavailable dissolved P in the SPM causes migration to overlying water and sediment, eventually being converted into a chemical speciation of P. Conditions of resuspension promote A1-P of SPM that migrated to the sediment and water. Concentrations of A1-P in SPM are reduced. P is released from SPM to water bodies, mainly through conversion into particulate P and dissolved total P. Meanwhile, exchange between SPM and sediments occur mainly through Ca-P migration. A1-P and BD-P possess similar geochemical characteristics or source. Ca-P and A1-P exhibit a negative correlation between migration and conversion.展开更多
Sediments are ultimate sinks of nutrients in lakes that record the pollution history evolutionary processes, and anthropogenic activities of a lake. However, sediments are considered as inner sources of environmental ...Sediments are ultimate sinks of nutrients in lakes that record the pollution history evolutionary processes, and anthropogenic activities of a lake. However, sediments are considered as inner sources of environmental factor changes such as the variation in hydrodynamic conditions because of the nutrients they release. How does this process happen? This study investigates a typical nutrient phosphorus (P) exchange among sediment, suspended particle matter (SPM), and water. Compared with numerical and experimental studies, this study confirms that the critical velocity that occurs at a lower flow rate state exists in the range of 7 to 15 crn/sec. Critical velocity below the critical flow rate promotes the migration of particulate phosphorus (PP) to the SPM. On the other hand, critical velocity above the critical flow rate promotes the release of PP in water.展开更多
基金supported by the National Basic Research Program(973) of China(No.2008CB418203)
文摘Phosphorous (P) fraction characteristics in sediment resuspension were investigated under adequately hydrodynamic conditions. Four forms of P in overlying water, including dissolved inorganic P, dissolved total P, total P, and particulate P, and six fractions of P in suspended particulate matter (SPM), including loosely sorbed P (NH4Cl-P), redox-sensitive P (BD-P), aluminum-bound P (Al- P), organic P (NaOH-nrP), calcium-bound P (Ca-P) and residual P (Res-P), were quantified, respectively. Different hydrodynamic conditions resulted in different P form changes. Four states could be ascribed: (1) P desorption by sediment and SPM, and P adsorption by overlying water; (2) P desorption by SPM, and P adsorption by overlying water; (3) P adsorption by SPM, and P desorption by overlying water; and (4) P equilibrium between SPM and overlying water. The contents of P in overlying water acquired peak values in the middle position of the vertical P distribution due to the combined actions of SPM and sediment. P fractions in SPM were in the following order: BD-P 〉 NaOH-nrp 〉 Ca-P 〉 Al-P 〉 Res-P 〉 NH4Cl-P. BD-P in SPM frequently exchanged with P forms in overlying water. Resuspension was favorable to forming Ca-P in SPM.
基金Project supported by the Major Program of the National Natural Science Foundation of China (Grant No.10632070).
文摘The lattice Boltzmann method was used to investigate numerically the fiber orientation distributions in slit channel flows with abrupt expansion for fiber suspensions even in the concentrated regime. The channels have a thin slit geometry with 1:4 and 1:3 expansions. Both the interactions between fibers and that between fibers and channel walls were taken into consideration. Some of numerical results are qualitatively in agreement with the experiment data. It is found that most of fibers are aligned in the flow direction in all the suspensions in the entrance region of the expansion. Fiber orientation distributions, having different patterns in different regions of the flow, depend on the expansion ratio of the channel. The mechanical fiber-fiber interaction largely affects the fiber orientation in the downstream of the expansion and in the salient corner for the cases of concentrated suspensions. The hydrodynamic interaction plays an important role on the fiber orientation in the dilute suspension.
基金supported by the National Basic Research Program of China (973 Program,Grant No.2008CB418203)the National Science and Technology Specific Project of China (Grant No.20080ZX07422-005)
文摘Experiments on Phosphorus (P) fraction characteristics in sediment resuspension were performed under adequate hydrodynamic conditions. It is found that the concentration of Suspended Particulate Matter (SPM) in the eddy current region exhibits the "Matthew effect". Velocity is an impact factor of the Equilibrium Phosphate Concentration (EPC), which is related to other hydraulic conditions. Overall bioavailable dissolved P in the SPM causes migration to overlying water and sediment, eventually being converted into a chemical speciation of P. Conditions of resuspension promote A1-P of SPM that migrated to the sediment and water. Concentrations of A1-P in SPM are reduced. P is released from SPM to water bodies, mainly through conversion into particulate P and dissolved total P. Meanwhile, exchange between SPM and sediments occur mainly through Ca-P migration. A1-P and BD-P possess similar geochemical characteristics or source. Ca-P and A1-P exhibit a negative correlation between migration and conversion.
基金supported by the Major State Basic Research Development Program of China(No.2011CB013101)the National Natural Science Foundation of China(No.10872003,10932001,11172001)+2 种基金the National Excellent Doctoral Dissertation of China(No.2007B2)the National Basic Research Program (973) of China(No.2008CB418203)the National Science and Technology Specific Project of China(No.20080ZX07422)
文摘Sediments are ultimate sinks of nutrients in lakes that record the pollution history evolutionary processes, and anthropogenic activities of a lake. However, sediments are considered as inner sources of environmental factor changes such as the variation in hydrodynamic conditions because of the nutrients they release. How does this process happen? This study investigates a typical nutrient phosphorus (P) exchange among sediment, suspended particle matter (SPM), and water. Compared with numerical and experimental studies, this study confirms that the critical velocity that occurs at a lower flow rate state exists in the range of 7 to 15 crn/sec. Critical velocity below the critical flow rate promotes the migration of particulate phosphorus (PP) to the SPM. On the other hand, critical velocity above the critical flow rate promotes the release of PP in water.