We carry out the first time-resolved measurement of Rb atoms desorbing from octadecyltrichlorosilane coated sur- faces by polarizing the atoms near the surface using an evanescent wave pump pulse and watching the subs...We carry out the first time-resolved measurement of Rb atoms desorbing from octadecyltrichlorosilane coated sur- faces by polarizing the atoms near the surface using an evanescent wave pump pulse and watching the subsequent intensity change of another evanescent wave probe beam, and find the mean adsorption （dwell） time to be about 400ns at a cell body temperature of 112℃. The adsorption energy is found to be 0.19eV from the surface tem- perature dependence of the adsorption time. This method can be extended to study the adsorption/desorption process of other alkali atoms on other surfaces of transparent substrates with an ultimate time resolution limited by the flight time of atoms in the evanescent wave which is of the order of nanoseconds.展开更多
基金Supported by the National Natural Science Foundation of China under Grant No 11074050
文摘We carry out the first time-resolved measurement of Rb atoms desorbing from octadecyltrichlorosilane coated sur- faces by polarizing the atoms near the surface using an evanescent wave pump pulse and watching the subsequent intensity change of another evanescent wave probe beam, and find the mean adsorption （dwell） time to be about 400ns at a cell body temperature of 112℃. The adsorption energy is found to be 0.19eV from the surface tem- perature dependence of the adsorption time. This method can be extended to study the adsorption/desorption process of other alkali atoms on other surfaces of transparent substrates with an ultimate time resolution limited by the flight time of atoms in the evanescent wave which is of the order of nanoseconds.
