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Dynamics and vibration reduction performance of asymmetric tristable nonlinear energy sink 被引量:3
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作者 Hongyan CHEN Youcheng ZENG +2 位作者 Hu DING Siukai LAI Liqun CHEN 《Applied Mathematics and Mechanics(English Edition)》 SCIE EI CSCD 2024年第3期389-406,共18页
With its complex nonlinear dynamic behavior,the tristable system has shown excellent performance in areas such as energy harvesting and vibration suppression,and has attracted a lot of attention.In this paper,an asymm... With its complex nonlinear dynamic behavior,the tristable system has shown excellent performance in areas such as energy harvesting and vibration suppression,and has attracted a lot of attention.In this paper,an asymmetric tristable design is proposed to improve the vibration suppression efficiency of nonlinear energy sinks(NESs)for the first time.The proposed asymmetric tristable NES(ATNES)is composed of a pair of oblique springs and a vertical spring.Then,the three stable states,symmetric and asymmetric,can be achieved by the adjustment of the distance and stiffness asymmetry of the oblique springs.The governing equations of a linear oscillator(LO)coupled with the ATNES are derived.The approximate analytical solution to the coupled system is obtained by the harmonic balance method(HBM)and verified numerically.The vibration suppression efficiency of three types of ATNES is compared.The results show that the asymmetric design can improve the efficiency of vibration reduction through comparing the chaotic motion of the NES oscillator between asymmetric steady states.In addition,compared with the symmetrical tristable NES(TNES),the ATNES can effectively control smaller structural vibrations.In other words,the ATNES can effectively solve the threshold problem of TNES failure to weak excitation.Therefore,this paper reveals the vibration reduction mechanism of the ATNES,and provides a pathway to expand the effective excitation amplitude range of the NES. 展开更多
关键词 asymmetric nonlinear energy sink(NES) tristable vibration control po-tential barrier
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Activation Redistribution Based Hybrid Asymmetric Quantization Method of Neural Networks 被引量:1
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作者 Lu Wei Zhong Ma Chaojie Yang 《Computer Modeling in Engineering & Sciences》 SCIE EI 2024年第1期981-1000,共20页
The demand for adopting neural networks in resource-constrained embedded devices is continuously increasing.Quantization is one of the most promising solutions to reduce computational cost and memory storage on embedd... The demand for adopting neural networks in resource-constrained embedded devices is continuously increasing.Quantization is one of the most promising solutions to reduce computational cost and memory storage on embedded devices.In order to reduce the complexity and overhead of deploying neural networks on Integeronly hardware,most current quantization methods use a symmetric quantization mapping strategy to quantize a floating-point neural network into an integer network.However,although symmetric quantization has the advantage of easier implementation,it is sub-optimal for cases where the range could be skewed and not symmetric.This often comes at the cost of lower accuracy.This paper proposed an activation redistribution-based hybrid asymmetric quantizationmethod for neural networks.The proposedmethod takes data distribution into consideration and can resolve the contradiction between the quantization accuracy and the ease of implementation,balance the trade-off between clipping range and quantization resolution,and thus improve the accuracy of the quantized neural network.The experimental results indicate that the accuracy of the proposed method is 2.02%and 5.52%higher than the traditional symmetric quantization method for classification and detection tasks,respectively.The proposed method paves the way for computationally intensive neural network models to be deployed on devices with limited computing resources.Codes will be available on https://github.com/ycjcy/Hybrid-Asymmetric-Quantization. 展开更多
关键词 QUANTIZATION neural network hybrid asymmetric ACCURACY
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Asymmetric Drying and Wetting Trends in Eastern and Western China 被引量:1
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作者 Wen WU Fei JI +1 位作者 Shujuan HU Yongli HE 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第2期221-232,共12页
As an important factor that directly affects agricultural production, the social economy, and policy implementation,observed changes in dry/wet conditions have become a matter of widespread concern. However, previous ... As an important factor that directly affects agricultural production, the social economy, and policy implementation,observed changes in dry/wet conditions have become a matter of widespread concern. However, previous research has mainly focused on the long-term linear changes of dry/wet conditions, while the detection and evolution of the non-linear trends related to dry/wet changes have received less attention. The non-linear trends of the annual aridity index, obtained by the Ensemble Empirical Mode Decomposition(EEMD) method, reveal that changes in dry/wet conditions in China are asymmetric and can be characterized by contrasting features in both time and space in China. Spatially, most areas in western China have experienced transitions from drying to wetting, while opposite changes have occurred in most areas of eastern China. Temporally, the transitions occurred earlier in western China compared to eastern China. Research into the asymmetric spatial characteristics of dry/wet conditions compensates for the inadequacies of previous studies, which focused solely on temporal evolution;at the same time, it remedies the inadequacies of traditional research on linear trends over centennial timescales. Analyzing the non-linear trend also provides for a more comprehensive understanding of the drying/wetting changes in China. 展开更多
关键词 aridity index EEMD dry/wet conditions asymmetric evolution
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Asymmetric Electrolytes Design for Aqueous Multivalent Metal Ion Batteries 被引量:1
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作者 Xiaochen Yang Xinyu Wang +2 位作者 Yue Xiang Longtao Ma Wei Huang 《Nano-Micro Letters》 SCIE EI CSCD 2024年第3期227-253,共27页
With the rapid development of portable electronics and electric road vehicles,high-energy-density batteries have been becoming front-burner issues.Traditionally,homogeneous electrolyte cannot simultaneously meet diame... With the rapid development of portable electronics and electric road vehicles,high-energy-density batteries have been becoming front-burner issues.Traditionally,homogeneous electrolyte cannot simultaneously meet diametrically opposed demands of high-potential cathode and low-potential anode,which are essential for high-voltage batteries.Meanwhile,homogeneous electrolyte is difficult to achieve bi-or multi-functions to meet different requirements of electrodes.In comparison,the asymmetric electrolyte with bi-or multi-layer disparate components can satisfy distinct requirements by playing different roles of each electrolyte layer and meanwhile compensates weakness of individual electrolyte.Consequently,the asymmetric electrolyte can not only suppress by-product sedimentation and continuous electrolyte decomposition at the anode while preserving active substances at the cathode for high-voltage batteries with long cyclic lifespan.In this review,we comprehensively divide asymmetric electrolytes into three categories:decoupled liquid-state electrolytes,bi-phase solid/liquid electrolytes and decoupled asymmetric solid-state electrolytes.The design principles,reaction mechanism and mutual compatibility are also studied,respectively.Finally,we provide a comprehensive vision for the simplification of structure to reduce costs and increase device energy density,and the optimization of solvation structure at anolyte/catholyte interface to realize fast ion transport kinetics. 展开更多
关键词 asymmetric electrolyte Aqueous multivalent metal ion batteries Electrochemical stability windows Electrolyte interface
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Acoustic Bilayer Gradient Metasurfaces for Perfect and Asymmetric Beam Splitting
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作者 权家琪 孙宝印 +2 位作者 伏洋洋 高雷 徐亚东 《Chinese Physics Letters》 SCIE EI CAS CSCD 2024年第1期39-50,共12页
We experimentally and theoretically present a paradigm for the accurate bilayer design of gradient metasurfaces for wave beam manipulation,producing an extremely asymmetric splitting effect by simply tailoring the int... We experimentally and theoretically present a paradigm for the accurate bilayer design of gradient metasurfaces for wave beam manipulation,producing an extremely asymmetric splitting effect by simply tailoring the interlayer size.This concept arises from anomalous diffraction in phase gradient metasurfaces and the precise combination of the phase gradient in bilayer metasurfaces.Ensured by different diffraction routes in momentum space for incident beams from opposite directions,extremely asymmetric acoustic beam splitting can be generated in a robust way,as demonstrated in experiments through a designed bilayer system.Our work provides a novel approach and feasible platform for designing tunable devices to control wave propagation. 展开更多
关键词 SURFACES SPLITTING asymmetric
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Effects of asymmetric coupling and boundary on the dynamic behaviors of a random nearest neighbor coupled system
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作者 徐玲 姜磊 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第6期309-322,共14页
This study investigates the dynamical behaviors of nearest neighbor asymmetric coupled systems in a confined space.First, the study derivative analytical stability and synchronization conditions for the asymmetrically... This study investigates the dynamical behaviors of nearest neighbor asymmetric coupled systems in a confined space.First, the study derivative analytical stability and synchronization conditions for the asymmetrically coupled system in an unconfined space, which are then validated through numerical simulations. Simulation results show that asymmetric coupling has a significant impact on synchronization conditions. Moreover, it is observed that irrespective of whether the system is confined, an increase in coupling asymmetry leads to a hastened synchronization pace. Additionally, the study examines the effects of boundaries on the system's collective behaviors via numerical experiments. The presence of boundaries ensures the system's stability and synchronization, and reducing these boundaries can expedite the synchronization process and amplify its effects. Finally, the study reveals that the system's output amplitude exhibits stochastic resonance as the confined boundary size increases. 展开更多
关键词 asymmetric coupled confined space SYNCHRONIZATION stochastic resonance stability
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Nickel catalysts with asymmetric steric hindrance for ethylene polymerization
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作者 Wanlu Tian Fuzhou Wang Chen Zou 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第6期48-52,59,I0010,I0011,共8页
α-Diimide catalysts have attracted widespread attention due to their unique chain walking characteristics.A series ofα-diimide nickel/palladium catalysts with different electronic effects and steric hindrances were ... α-Diimide catalysts have attracted widespread attention due to their unique chain walking characteristics.A series ofα-diimide nickel/palladium catalysts with different electronic effects and steric hindrances were designed and synthesized for olefin polymerization.In this work,we synthesized a series of asymmetricα-diimide nickel complexes with different steric hindrances and used them for ethylene polymerization.These nickel catalysts have high ethylene polymerization activity,up to 6.51×10^(6)g·mol^(−1)·h^(−1),and the prepared polyethylene has a moderate melting point and high molecular weight(up to 38.2×10^(4)g·mol^(−1)),with a branching density distribution between 7 and 94 branches per 1000 carbons.More importantly,the polyethylene prepared by these catalysts exhibits excellent tensile properties,with strain and stress reaching 800%and 30 MPa,respectively. 展开更多
关键词 Α-DIIMINE nickel complex POLYETHYLENE POLYMERIZATION asymmetric steric hindrance
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Enhanced and asymmetric signatures of hybridization at climatic margins: Evidence from closely related dioecious fig species
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作者 Jian-Feng Huang Clive T.Darwell Yan-Qiong Peng 《Plant Diversity》 SCIE CAS CSCD 2024年第2期181-193,共13页
Hybridization plays a significant role in biological evolution. However, it is not clear whether ecological contingency differentially influences likelihood of hybridization, particularly at ecological margins where p... Hybridization plays a significant role in biological evolution. However, it is not clear whether ecological contingency differentially influences likelihood of hybridization, particularly at ecological margins where parental species may exhibit reduced fitnesses. Moreover, it is unknown whether future ecosystem change will increase the prevalence of hybridization. Ficus heterostyla and F. squamosa are closely related species co-distributed from southern Thailand to southwest China where hybridization, yielding viable seeds, has been documented. As a robust test of ecological factors driving hybridization, we investigated spatial hybridization signatures based on nuclear microsatellites from extensive population sampling across a widespread contact range. Both species showed high population differentiation and strong patterns of isolation by distance. Admixture estimates exposed asymmetric interspecific gene flow.Signatures of hybridization increase significantly towards higher latitude zones, peaking at the northern climatic margins. Geographic variation in reproductive phenology combined with ecologically challenging marginal habitats may promote this phenomenon. Our work is a first systematic evaluation of such patterns in a comprehensive, latitudinally-based clinal context, and indicates that tendency to hybridize appears strongly influenced by environmental conditions. Moreover, that future climate change scenarios will likely alter and possibly augment cases of hybridization at ecosystem scales. 展开更多
关键词 HYBRIDIZATION Heterospecific visitation FIG Pollinator wasp asymmetric gene flow
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Dual-negative-objective Coordinated Control of Brushless Doubly Fed Induction Generator under Unbalanced Grid Voltage
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作者 Ming Cheng Zheng Cao Xiaoming Yan 《CES Transactions on Electrical Machines and Systems》 EI CSCD 2024年第3期347-355,共9页
This article proposes a dual-negative-objective coordinated control strategy for brushless doubly fed induction generator(BDFIG)based wind power generation system under unbalanced grid voltage.To alleviate the mechani... This article proposes a dual-negative-objective coordinated control strategy for brushless doubly fed induction generator(BDFIG)based wind power generation system under unbalanced grid voltage.To alleviate the mechanical stress and impaction on rotating shaft,the negative control objective(NCO)of machine side converter(MSC)is set to suppress the ripple of electromagnetic torque.While the NCO of grid side converter(GSC)is selected to suppress the oscillation of total output active power or the unbalanced degree of total output current for BDFIG generation system.In comparison with traditional single converter control scheme of the MSC or GSC,dual NCOs can be satisfied at the same time due to the enlarged freedom degree in the proposed improved coordinated control system for back-toback converters.The effectiveness of proposed control strategy is validated by simulation and experimental results on a dual-cagerotor BDFIG(DCR-BDFIG)prototype. 展开更多
关键词 Brushless doubly fed induction generator Dual-negative-objective Freedom degree unbalanced grid voltage
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A Hybrid Dung Beetle Optimization Algorithm with Simulated Annealing for the Numerical Modeling of Asymmetric Wave Equations
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作者 Wei Xu-ruo Bai Wen-lei +2 位作者 Liu Lu Li You-ming Wang Zhi-yang 《Applied Geophysics》 SCIE CSCD 2024年第3期513-527,618,共16页
In the generalized continuum mechanics(GCM)theory framework,asymmetric wave equations encompass the characteristic scale parameters of the medium,accounting for microstructure interactions.This study integrates two th... In the generalized continuum mechanics(GCM)theory framework,asymmetric wave equations encompass the characteristic scale parameters of the medium,accounting for microstructure interactions.This study integrates two theoretical branches of the GCM,the modified couple stress theory(M-CST)and the one-parameter second-strain-gradient theory,to form a novel asymmetric wave equation in a unified framework.Numerical modeling of the asymmetric wave equation in a unified framework accurately describes subsurface structures with vital implications for subsequent seismic wave inversion and imaging endeavors.However,employing finite-difference(FD)methods for numerical modeling may introduce numerical dispersion,adversely affecting the accuracy of numerical modeling.The design of an optimal FD operator is crucial for enhancing the accuracy of numerical modeling and emphasizing the scale effects.Therefore,this study devises a hybrid scheme called the dung beetle optimization(DBO)algorithm with a simulated annealing(SA)algorithm,denoted as the SA-based hybrid DBO(SDBO)algorithm.An FD operator optimization method under the SDBO algorithm was developed and applied to the numerical modeling of asymmetric wave equations in a unified framework.Integrating the DBO and SA algorithms mitigates the risk of convergence to a local extreme.The numerical dispersion outcomes underscore that the proposed SDBO algorithm yields FD operators with precision errors constrained to 0.5‱while encompassing a broader spectrum coverage.This result confirms the efficacy of the SDBO algorithm.Ultimately,the numerical modeling results demonstrate that the new FD method based on the SDBO algorithm effectively suppresses numerical dispersion and enhances the accuracy of elastic wave numerical modeling,thereby accentuating scale effects.This result is significant for extracting wavefield perturbations induced by complex microstructures in the medium and the analysis of scale effects. 展开更多
关键词 FINITE-DIFFERENCE asymmetric wave equation Numerical modeling DBO algorithm SA algorithm
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Decentralized Optimal Control and Stabilization of Interconnected Systems With Asymmetric Information
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作者 Na Wang Xiao Liang +1 位作者 Hongdan Li Xiao Lu 《IEEE/CAA Journal of Automatica Sinica》 SCIE EI CSCD 2024年第3期698-707,共10页
The paper addresses the decentralized optimal control and stabilization problems for interconnected systems subject to asymmetric information.Compared with previous work,a closed-loop optimal solution to the control p... The paper addresses the decentralized optimal control and stabilization problems for interconnected systems subject to asymmetric information.Compared with previous work,a closed-loop optimal solution to the control problem and sufficient and necessary conditions for the stabilization problem of the interconnected systems are given for the first time.The main challenge lies in three aspects:Firstly,the asymmetric information results in coupling between control and estimation and failure of the separation principle.Secondly,two extra unknown variables are generated by asymmetric information(different information filtration)when solving forward-backward stochastic difference equations.Thirdly,the existence of additive noise makes the study of mean-square boundedness an obstacle.The adopted technique is proving and assuming the linear form of controllers and establishing the equivalence between the two systems with and without additive noise.A dual-motor parallel drive system is presented to demonstrate the validity of the proposed algorithm. 展开更多
关键词 asymmetric information decentralized control forwardbackward stochastic difference equations interconnected system stalibization
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A Multifunctional Chiral Metasurface with Asymmetric Transmission and Linear-Polarization Conversion
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作者 AFZAL Ahmed CAO Qunsheng MUHAMMAD Sajjad 《Transactions of Nanjing University of Aeronautics and Astronautics》 EI CSCD 2024年第S01期21-26,共6页
In this paper,a multifunctional chiral metasurface is presented to achieve asymmetric transmission(AT)and linear-polarization conversion(LPC).The designed metasurface consists of a cross swords-like shape and two hole... In this paper,a multifunctional chiral metasurface is presented to achieve asymmetric transmission(AT)and linear-polarization conversion(LPC).The designed metasurface consists of a cross swords-like shape and two holes in the lower side of the unit cell.In the frequency band from 8.3 GHz to 10.4 GHz,AT is realized with more than 90%efficiency and the same chiral metasurface transforms linear polarized wave into its orthogonal counterpart with high efficiency.For LPC,the polarization conversion ratio(PCR)is greater than 95%.The proposed metasurface is stable against the incident angles of striking electromagnetic(EM)waves up to 60°for both operations of AT and LPC. 展开更多
关键词 chiral metasurface polarization conversion asymmetric tranmission plasmon resonances
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Dynamics of information diffusion and disease transmission in time-varying multiplex networks with asymmetric activity levels
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作者 谢笑笑 霍良安 +1 位作者 董雅芳 程英英 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第3期690-699,共10页
While the interaction between information and disease in static networks has been extensively investigated,many studies have ignored the characteristics of network evolution.In this study,we construct a new two-layer ... While the interaction between information and disease in static networks has been extensively investigated,many studies have ignored the characteristics of network evolution.In this study,we construct a new two-layer coupling model to explore the interactions between information and disease.The upper layer describes the diffusion of disease-related information,and the lower layer represents the disease transmission.We then use power-law distributions to examine the influence of asymmetric activity levels on dynamic propagation,revealing a mapping relationship characterizing the interconnected propagation of information and diseases among partial nodes within the network.Subsequently,we derive the disease outbreak threshold by using the microscopic Markov-chain approach(MMCA).Finally,we perform extensive Monte Carlo(MC)numerical simulations to verify the accuracy of our theoretical results.Our findings indicate that the activity levels of individuals in the disease transmission layer have a more significant influence on disease transmission compared with the individual activity levels in the information diffusion layer.Moreover,reducing the damping factor can delay disease outbreaks and suppress disease transmission,while improving individual quarantine measures can contribute positively to disease control.This study provides valuable insights into policymakers for developing outbreak prevention and control strategies. 展开更多
关键词 information diffusion disease transmission asymmetric activity levels quarantine strength
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Constraints on Asymmetric Dark Matter in Quintessence Model
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作者 Sujuan Qiu Hoernisa Iminniyaz 《Journal of High Energy Physics, Gravitation and Cosmology》 CAS 2024年第2期599-608,共10页
The modified cosmology like quintessence model with kination phase predicted the Hubble expansion rate of the universe before Big Bang Nucleosynthesis is different from the standard cosmological scenario. The modified... The modified cosmology like quintessence model with kination phase predicted the Hubble expansion rate of the universe before Big Bang Nucleosynthesis is different from the standard cosmological scenario. The modified expansion rate leaves its imprint on the relic density of asymmetric dark matter. In this work, we review the calculation of relic density of asymmetric WIMP dark matter in the standard cosmological scenario and quintessence model with kination phase. Then we use the Planck data to find constraints on the annihilation cross section and the mass of the asymmetric dark matter in those models. 展开更多
关键词 asymmetric Dark Matter Standard Model Quintessence Model
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Negative Stiffness Mechanism on An Asymmetric Wave Energy Converter by Using A Weakly Nonlinear Potential Model
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作者 Sunny Kumar POGULURI Dongeun KIM Yoon Hyeok BAE 《China Ocean Engineering》 SCIE EI CSCD 2024年第4期689-700,共12页
Salter's duck,an asymmetrical wave energy converter(WEC)device,showed high efficiency in extracting energy from 2D regular waves in the past;yet,challenges remain for fluctuating wave conditions.These can potentia... Salter's duck,an asymmetrical wave energy converter(WEC)device,showed high efficiency in extracting energy from 2D regular waves in the past;yet,challenges remain for fluctuating wave conditions.These can potentially be addressed by adopting a negative stiffness mechanism(NSM)in WEC devices to enhance system efficiency,even in highly nonlinear and steep 3D waves.A weakly nonlinear model was developed which incorporated a nonlinear restoring moment and NSM into the linear formulations and was applied to an asymmetric WEC using a time domain potential flow model.The model was initially validated by comparing it with published experimental and numerical computational fluid dynamics results.The current results were in good agreement with the published results.It was found that the energy extraction increased in the range of 6%to 17%during the evaluation of the effectiveness of the NSM in regular waves.Under irregular wave conditions,specifically at the design wave conditions for the selected test site,the energy extraction increased by 2.4%,with annual energy production increments of approximately 0.8MWh.The findings highlight the potential of NSM in enhancing the performance of asymmetric WEC devices,indicating more efficient energy extraction under various wave conditions. 展开更多
关键词 asymmetric wave energy converter negative stiffness mechanism weakly nonlinear potential flow POWER
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Coexistence behavior of asymmetric attractors in hyperbolic-type memristive Hopfield neural network and its application in image encryption
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作者 李晓霞 何倩倩 +2 位作者 余天意 才壮 徐桂芝 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第3期302-315,共14页
The neuron model has been widely employed in neural-morphic computing systems and chaotic circuits.This study aims to develop a novel circuit simulation of a three-neuron Hopfield neural network(HNN)with coupled hyper... The neuron model has been widely employed in neural-morphic computing systems and chaotic circuits.This study aims to develop a novel circuit simulation of a three-neuron Hopfield neural network(HNN)with coupled hyperbolic memristors through the modification of a single coupling connection weight.The bistable mode of the hyperbolic memristive HNN(mHNN),characterized by the coexistence of asymmetric chaos and periodic attractors,is effectively demonstrated through the utilization of conventional nonlinear analysis techniques.These techniques include bifurcation diagrams,two-parameter maximum Lyapunov exponent plots,local attractor basins,and phase trajectory diagrams.Moreover,an encryption technique for color images is devised by leveraging the mHNN model and asymmetric structural attractors.This method demonstrates significant benefits in correlation,information entropy,and resistance to differential attacks,providing strong evidence for its effectiveness in encryption.Additionally,an improved modular circuit design method is employed to create the analog equivalent circuit of the memristive HNN.The correctness of the circuit design is confirmed through Multisim simulations,which align with numerical simulations conducted in Matlab. 展开更多
关键词 hyperbolic-type memristor Hopfield neural network(HNN) asymmetric attractors image encryption
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12.6μm-Thick Asymmetric Composite Electrolyte with Superior Interfacial Stability for Solid-State Lithium-Metal Batteries
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作者 Zheng Zhang Jingren Gou +4 位作者 Kaixuan Cui Xin Zhang Yujian Yao Suqing Wang Haihui Wang 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期397-409,共13页
Solid-state lithium metal batteries(SSLMBs)show great promise in terms of high-energy-density and high-safety performance.However,there is an urgent need to address the compatibility of electrolytes with high-voltage ... Solid-state lithium metal batteries(SSLMBs)show great promise in terms of high-energy-density and high-safety performance.However,there is an urgent need to address the compatibility of electrolytes with high-voltage cathodes/Li anodes,and to minimize the electrolyte thickness to achieve highenergy-density of SSLMBs.Herein,we develop an ultrathin(12.6μm)asymmetric composite solid-state electrolyte with ultralight areal density(1.69 mg cm^(−2))for SSLMBs.The electrolyte combining a garnet(LLZO)layer and a metal organic framework(MOF)layer,which are fabricated on both sides of the polyethylene(PE)separator separately by tape casting.The PE separator endows the electrolyte with flexibility and excellent mechanical properties.The LLZO layer on the cathode side ensures high chemical stability at high voltage.The MOF layer on the anode side achieves a stable electric field and uniform Li flux,thus promoting uniform Li^(+)deposition.Thanks to the well-designed structure,the Li symmetric battery exhibits an ultralong cycle life(5000 h),and high-voltage SSLMBs achieve stable cycle performance.The assembled pouch cells provided a gravimetric/volume energy density of 344.0 Wh kg^(−1)/773.1 Wh L^(−1).This simple operation allows for large-scale preparation,and the design concept of ultrathin asymmetric structure also reveals the future development direction of SSLMBs. 展开更多
关键词 Solid-state lithium metal batteries Composite solid-state electrolyte Ultrathin asymmetric structure Pouch cells
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Asymmetric Zn-N_4 atomic sites embedded hollow fibers as stable Zn anode for high-performance Zn-ion hybrid capacitor
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作者 Yukun Liu Bing Li +5 位作者 Jin Wang Caiyun Li Hongrui Yang Yang Song Sen Zhang Chao Deng 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第10期460-469,I0009,共11页
Zn based electrochemical energy storage systems(EES)have attracted tremendous interests owing to their low cost and high intrinsic safety.Nevertheless,the uncontrolled growth of Zn dendrites and the side reactions of ... Zn based electrochemical energy storage systems(EES)have attracted tremendous interests owing to their low cost and high intrinsic safety.Nevertheless,the uncontrolled growth of Zn dendrites and the side reactions of Zn metal anodes(ZMAs)severely restrict their applications.To address these issues,we design the asymmetric Zn-N_(4) atomic sites embedded hollow fibers(AS-IHF)as the flexible host for stable ZMAs.Through introducing different nitrogen resources in the synthesis,two kinds of coordination,i,e.Zn-N(pyridinic)and Zn-N(pyrrolic),are introduced in the Zn-N_(4) atomic module synchronously.The asymmetric Zn-N_(4) module with regulated micro-environment facilitates the superior zincophilic features and promotes the Zn adsorption.Meanwhile,the highly porous structure of the hollow fiber effectively reduces local current density,homogenize Zn ion flux,and alleviate structure stress.All the advantages endow the high efficiency and good stability for Zn plating/stripping.Both theoretical and experimental results demonstrate the high reversibility,low nucleation overpotential,and dendritefree behavior of the AS-IHF@Zn anode,which afford the high stability in high-rate and long-term cycling.Moreover,the solid-state Zn-ion hybrid capacitor(ZIHC)based on AS-IHF@Zn anode shows the high flexibility,reliability,and superior long-term cycling capability in a wide-range of temperatures(-20-25℃).Therefore,the present work not only gives a new strategy for modulating local environments of single atomic sites,but also propels the development of flexible power sources for diverse electronics. 展开更多
关键词 asymmetric coordination Single atomic sites Zincophilic sites Dendrite free behavior Zn-ion hybrid capacitor
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Alkyl chain modulation of asymmetric hexacyclic fused acceptor synergistically with wide bandgap third component for high efficiency ternary organic solar cells
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作者 Shufang Li Huilan Guan +4 位作者 Can Zhu Chaoyuan Sun Qingya Wei Jun Yuan Yingping Zou 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2024年第7期1713-1719,共7页
Herein,two asymmetric hexacyclic fused small molecule acceptors(SMAs),namely BP4F-HU and BP4F-UU,were synthesized.The elongated outside chains in the BP4F-UU molecule played a crucial role in optimizing the morphology... Herein,two asymmetric hexacyclic fused small molecule acceptors(SMAs),namely BP4F-HU and BP4F-UU,were synthesized.The elongated outside chains in the BP4F-UU molecule played a crucial role in optimizing the morphology of blend film,thereby improving charge mobility and reducing energy loss within the corresponding film.Notably,the PM6:BP4F-UU device exhibited a higher open-circuit voltage(V_(oc))of 0.878 V compared to the PM6:BP4F-HU device with a V_(oc)of 0.863 V.Further,a new wide bandgap SMA named BTP-TA was designed and synthesized as the third component to the PM6:BP4F-UU host binary devices,which showed an ideal complementary absorption spectrum in PM6:BP4F-UU system.In addition,BTP-TA can achieve efficient intermolecular energy transfer to BP4F-UU by fluorescence resonance energy transfer(FRET)pathway,due to the good overlap between the photoluminescence(PL)spectrum of BTP-TA and the absorption region of BP4F-UU.Consequently,ternary devices with 15wt%BTP-TA exhibits broader photon utilization,optimal blend morphology,and reduced charge recombination compared to the corresponding binary devices.Consequently,PM6:BP4F-UU:BTP-TA ternary device achieved an optimal power conversion efficiency(PCE)of 17.83%with simultaneously increased V_(oc)of 0.905 V,short-circuit current density(J_(sc))of 26.14 mA/cm^(2),and fill factor(FF)of 75.38%. 展开更多
关键词 asymmetric hexacyclic acceptor outside chain wide bandgap acceptor ternary organic solar cells
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Study of a Hydraulic Jump in an Asymmetric Trapezoidal Channel with Different Sluice Gates
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作者 Bouthaina Debabeche Sonia Cherhabil 《Fluid Dynamics & Materials Processing》 EI 2024年第7期1499-1516,共18页
In this study,the main properties of the hydraulic jump in an asymmetric trapezoidal flume are analyzed experimentally,including the so-called sequent depths,characteristic lengths,and efficiency.In particular,an asym... In this study,the main properties of the hydraulic jump in an asymmetric trapezoidal flume are analyzed experimentally,including the so-called sequent depths,characteristic lengths,and efficiency.In particular,an asymmetric trapezoidal flume with a length of 7 m and a width of 0.304 m is considered,with the bottom of the flume transversely inclined at an angle of m=0.296 and vertical lateral sides.The corresponding inflow Froude number is allowed to range in the interval(1.40<F1<6.11).The properties of this jump are compared to those of hydraulic jumps in channels with other types of cross-sections.A relationship for calculating hydraulic jump efficiency is proposed for the considered flume.For F1>5,the hydraulic jump is found to be more effective than that occurring in triangular and symmetric trapezoidal channels.Also,when■mes>8 and■>5,the hydraulic jump in the asymmetrical trapezoidal channel downstream of a parallelogram sluice gate is completely formed as opposed to the situation where a triangular sluice is considered. 展开更多
关键词 asymmetric trapezoidal channel characteristic lengths EFFICIENCY Froude hydraulic jump sequent depths sluice gate
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