Remote sensing of air pollution incorporating integrated-path differential-absorption and coherent-Doppler lidar

An innovative complex lidar system deployed on an airborne rotorcraft platform for remote sensing of atmospheric pollution is proposed and demonstrated.The system incorporates integrated-path differential absorption lidar(DIAL) and coherent-doppler lidar(CDL) techniques using a dual tunable TEA CO_(2)laser in the 9—11 μm band and a 1.55 μm fiber laser.By combining the principles of differential absorption detection and pulsed coherent detection,the system enables agile and remote sensing of atmospheric pollution.Extensive static tests validate the system’s real-time detection capabilities,including the measurement of concentration-path-length product(CL),front distance,and path wind speed of air pollution plumes over long distances exceeding 4 km.Flight experiments is conducted with the helicopter.Scanning of the pollutant concentration and the wind field is carried out in an approximately 1 km slant range over scanning angle ranges from 45°to 65°,with a radial resolution of 30 m and10 s.The test results demonstrate the system’s ability to spatially map atmospheric pollution plumes and predict their motion and dispersion patterns,thereby ensuring the protection of public safety.

Distribution of Atmospheric Pollution in Southern Benin

This study focuses on air quality in southern Benin in order to show public authorities what the Beninese populations are exposed to for efficient decision-making. Two sampling campaigns were carried out, one in the wet period and the other in the dry season. The measurements were taken using a monitor called an “Air Quality Monitor”. For data processing, the multiple comparison methods of Dun (1961) and the Wilcoxon test were used. To maintain legitimacy, all spatial data were included in the official cartographic repository of Benin: WGS 1984, Transverse Mercator Universe Projection (UTM), Zone 31 North. The Moran statistic was used to measure the levels of spatial autocorrelation of the variables studied and to test the significance. In order to locate the spatial subsets, the local spatial association indices of Anselin Local Moran and Getis-Ord, Gi* were used. In terms of results, on the 13 monitoring sites and the 8 parameters chosen to determine air quality, we do not note any significant inter-seasonal difference. Of the eight parameters, only three parameters present spatial autocorrelation leading to predictions of ambient air quality over the entire study area based on the distance separating the points, namely, PM2.5, PM10 and ambient air quality index (AQI). The localities affected by atmospheric pollution in South Benin are located in the south-western part of Benin, headed by Cotonou, which is heavily polluted by CO2, TCOV, PM10 and PM2.5.

Level of Exposure of Populations to Atmospheric Pollution in Southern Benin

This study focuses on monitoring the exposure of populations in South Benin to atmospheric pollution. Thirteen (13) monitoring points were identified where the Air quality measurements were taken using autonomous electronic devices called “Air Quality Monitor”. Calibrated and turned on, the measuring device automatically determines the concentrations of carbon dioxide CO2, Total Organic Compounds, methanal (HCHO), particulate matter PM2.5 and PM10, temperature in degrees Fahrenheit and relative humidity (RH). Per site, air pollution levels are recorded for 5 minutes every 30 minutes from 7 a.m. to 6 p.m. After the analyses, it appears that the carbon dioxide CO2 contents vary from 400 to 1444 ppm with an average of 486.80 ± 184.3 ppm, the daily contents of Total Volatile Organic Compounds from 0.01 to 6 .91 mg/m3 with a daily average of 0.36 ± 0.65 mg/m3, aldehydes from 0.005 to 3 mg/m3 with an average of 0.05 ± 0.17 mg/m3, for particulate matter of diameters less than or equal to 2.5 μm (PM2.5) pollution levels vary between 5 and 173.8 μg/m3 with an average of 21.5 ± 17.62 μg/m3. On the other hand, for PM10, the contents vary from 5 to 449.6 μg/m3 with an average of 28.17 ± 31.74 μg/m3, the Air Quality Index (AQI) varies from 0, 3 to 243 with an average of 39 ± 33.16. From the results observed, it appears that the south-western part of South Benin is heavily polluted by CO2, Total Volatile Organic Compounds, PM10 and especially PM2.5 with the city of Cotonou at its head, in particular the Red Star crossroads, the Toyota crossroads and the crossroads after the friendship stadium. The impacts of this pollution could be significant on sensitive people such as the elderly, newborns and patients with acute and chronic respiratory illnesses.

Atmospheric lead pollution in fine particulate matter in Shanghai, China

The Pb-monitoring program was extended for 6 years from 2002 to 2007 at 17 representative urban sites （6 traffic, 5 industrial, and 6 residential sites）, and 3 suburban sites to assess the lead pollution in fine particulate matter （PM2.5） after phasing out leaded gasoline in Shanghai. Compared with Pb levels reported in other places, the Pb pollution in Shanghai is still serious after phasing out leaded gasoline, which remains at high concentration range （213-176 ng/m^3） in PM2.5 in winter. Significant spatial variation of Pb concentrations and strong seasonal variation of higher Pb concentration in winter than that in summer were detected. The size distribution of Pb in particulate matter has a unimodat mode that peaks at approximately 0.154-1.59 μm particle diameter, indicating that Pb is mainly concentrated in fine fraction. Lead in the fine fraction is enriched by a factor of 103-104 relative to Pb abundance in crust. Eight categories of Pb pollution sources were identified in the PM2.5 in the winter of 2007 in Shanghai. The important emission sources among them are vehicle exhaust derived from combustion of unleaded gasoline, metaUurgic industry emission, and coal combustion emission.

Relationship between Environmental Pollution of Coal Mine and Spectral Characteristics of Nearby Plants

Remote sensing technology, as the most advanced method for collecting data, along with the common ways often used in the past on research of environmental science, was integrated to study the relationship between environmental pollution of coal mine and spectral characteristics of nearby plants. With compositive index and mean reflectivity at near infrared, a regression equation was established, and a conclusion was made that spectral reflectivity can be used to distinguish regions with different pollution degree. Through testing with real status of the research region, it is verified that this kind of integration and conclusion not only are helpful for human being in controlling the movement law of pollutants and the corresponding change of coal mine environmental quality but also bring a new way for the research of environment problems of coal mine.

Transport Patterns and Potential Sources of Atmospheric Pollution during the ⅩⅩⅣ Olympic Winter Games Period

The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the ⅩⅩⅣ Olympic Winter Games(OWG). Transport patterns and potential sources of pollutants in Zhangjiakou(ZJK) were investigated using pollutant monitoring datasets and a dispersion model. The PM_(2.5) concentration during February in ZJK has increased slightly(28%) from 2018 to 2021, mostly owing to the shift of main potential source regions of west-central Inner Mongolia and Mongolian areas(2015–18) to the North China Plain and northern Shanxi Province(NCPS) after 2018.Using CO as an indicator, the relative contributions of the different regions to the receptor site(ZJK) were evaluated based on the source-receptor-relationship method(SRR) and an emission inventory. We found that the relative contribution of pollutants from NCPS increased from 33% to 68% during 2019–21. Central Inner Mongolia(CIM) also has an important impact on ZJK under unfavorable weather conditions. This study demonstrated that the effect of pollution control measures in the NCPS and CIM should be strengthened to ensure that the air quality meets the standard during the ⅩⅩⅣ OWG.

Atmospheric pollution in Beijing, China, as recorded in sediments of the Kunming Lake

The fluxes of heavy metals and magnetite, a fly-ash component, from coal burning, to sediments of the Kunming Lake in Beijing have increased measurably over the last fifty years. Ages were introduced to the sediment strata through Pb-210 geochronologies. Even with a doubling of coal usage by the year 2000, the anthropogenic metal fluxes will still be less than those recorded in metropolitan Tokyo and U.S. lakes.

Spatio-temporal Characteristics of Atmospheric Pollution and Cause Analysis of Haze Events in Sichuan Basin,China

This study analyzed the spatio-temporal variability of air quality data for six standard air pollutants(Particulate Matter 2.5(PM2.5),Particulate Matter 10(PM10),SO2,NO2,CO,and O3)in the Sichuan Basin(SCB),China from 2015 to 2018 in relation to the formation of haze using conventional meteorological data(temperature,wind speed,and relative humidity),satellite data(fire point data,vertical profiles of aerosol subtypes,and aerosol optical depth),planetary boundary layer height,and backward trajectories.The results indicated that the spatio-temporal evolution of the air quality index(AQI)had notable seasonality for the pollution severity in descending order:winter,spring,summer,and autumn.Autumn and winter severe haze events occurred in November and January,respectively,and were caused by higher local pollution emissions under stagnant air conditions.Spring severe haze events occurred in May and were caused by dust from Northwest China and local regions.Severe summer haze events occurred in July and were caused by local burning.Therefore,the analyses showed that local burning,stagnant meteorological conditions,air mass transport and anthropogenic pollution emissions played a key role in haze in the SCB.This study provides scientific insights for fully analyzing heavy air pollution in SCB,China,and also provides a scientific basis for pollution research in regions of complex terrain as basins and mountains.

Influence of Temperature and Relative Humidity on Air Pollution in Addis Ababa, Ethiopia

In this paper we access the effects of two atmospheric variables (temperatureand relative humidity) on two important pollutants in the atmosphere(Nitrogen oxides (NOx) and carbon monoxide (CO)) by using one year(2016) data of Addis Ababa. Temperature has impact on atmosphericmixing and cause for the reduction of NOx as temperature increases.There are positive correlation between temperature and CO concentrationfrom January to April with (R^2 = 0.69), negative correlation from Mayto August with (R2 = 0.92) and no correlation for the remaining months.NOx and CO have moderate positive and negative correlation with relativehumidity during the months January-April (R^2 = 0.294 for NOx and R^2 =0291 for CO) and in the months May-August are R2 = 0.97 and R2 = 0.15for NOx and CO respectively. But there are no clear correlation betweenthe NOx and CO with relative humidity from September-December.NOx concentrations during wet season was almost about twice that of thedry season, but no such difference was observed in the case of CO. Theseasonal average air temperature in wet season is relatively lower than dryseason. NOx exhibited positive and CO negative seasonal correlations withrelative humidity.

Pollution Characteristics and Health Risk Assessment of Heavy Metals in PM2.5 during Winter in the Suburb of Cangzhou, China

The heavy metals in atmospheric fine particles are of great concern to human health. To understand the pollution characteristics and health risks of heavy metals in particulate matter with an aerodynamic equivalent diameter ≤2.5 μm (PM2.5) during winter in the suburb of Cangzhou, PM2.5 samples were collected with an intelligent medium-flow atmospheric particulate matter sampler from January to February 2019. The Fe, Cu, Mn, Pb and Zn contents in PM2.5 were determined via inductively coupled plasma optical emission spectrometry (ICP-OES). The sources and health risks of heavy metals in PM2.5 were analysed via the enrichment factor (EF) method and the United States Environmental Protection Agency (US EPA) health risk assessment model. The results showed that the average PM2.5 concentration in the suburb of Cangzhou reached 71.6 μg/m3, ranging from 23.7 to 169.5 μg/m3. The exceeding standard rate was 29.4% during the sampling period. The PM2.5 concentration during the nighttime was higher than that during the daytime. The heavy metal concentrations in PM2.5 decreased in the order of Fe > Mn > Zn > Cu > Pb, and the Fe, Mn, Pb and Zn concentrations decreased in the order of clean days < pollution days < heavy pollution days. The Fe and Mn concentrations were higher during the daytime than those during the nighttime, while the Cu, Pb and Zn concentrations were higher during the nighttime than those during the daytime. EF analysis revealed that Zn, Pb and Cu were significantly enriched, and Pb was highly enriched on heavy pollution days with increasing pollution degree. The enrichment level of heavy metals during the nighttime was higher than that during the daytime. Health risk assessment demonstrated that Mn posed non-carcinogenic risks to both adults and children, following the sequence of clean days < pollution days < heavy pollution days. Pb posed a carcinogenic risk to adults on heavy pollution days. The study revealed that the pollution levels of heavy metals in PM2.5 in the suburb of Cangzhou were low, and Pb and Mn in PM2.5 posed certain health risks to the population.

Atmospheric Pollution Control Effect of Key Cities in Inner Mongolia in 2014

APEC conference was held in Beijing during November 3- 12,2014. Hohhot City and Baotou City fall into the peripheral key air pollution control cities in the ＂ Beijing- Tianjin- Hebei＂ region. Inner Mongolia government adopted powerful pollution control measures in the period of the conference. According to pollutant concentration data and meteorological data etc. in the course of the event and the same period of last year,the atmospheric pollution variations and control effect were discussed in this study. The results showed that during October 1- 25,2014,there were 16 days with air pollution in Hohhot City and 15 days with air pollution in Baotou City,respectively increasing by 8% and 34% compared with the same period of 2013,and the concentration of particulate matter was also higher than that of last year. During October 22- 24,2014,Hohhot and Baotou cities were polluted persistently. The variation features of hourly concentration of main pollutants PM（10） and PM2. 5were similar to those in the same period of 2013. That is,the pollutant concentration reached the maximum from 21：00 to 23：00,and the minimum appeared from 15： 00 to 19： 00 in the next day. In the course of the event,the concentration of particulate matter in the two cities stared to reduce greatly on October 26. From October 26 to November 13,there were no days with air pollution in Hohhot City,decreasing by 100% compared with the same period of 2013; there were five days with air pollution in Baotou City,and the numbers of days with slight,moderate and severe pollution reduced by 37%,100% and67% respectively compared with the same period of last year. The persistent air pollution from October 22 to the first 10 days of November was related to unfavorable meteorological conditions,and the meteorological condition in the same period of 2014 was even worse. In the course of the event,the Inner Mongolia Government adopted air pollution control measures around October 25 and began to adopt some powerful pollution control measures on November 1. As a result,air pollution in key cities has been controlled effectively. This event showed that urban atmospheric pollution problem can be resolved,and we should take an optimistic attitude towards this matter.

Airborne Microorganisms Present in the Atmosphere in Valladolid, Spain

Over the past few years, research on the quality of air and microorganisms present in the atmosphere and spore composition of the environment has increased significantly, due to concerns over health risks for humans, plants, and animals. This study shows the abundance and diversity of microorganisms and the atmosphere of an urban nucleus, that is, the city of Valladolid (Spain). We considered the conditions of precipitation, humidity and wind, and the presence of some atmospheric pollutants such as nitrogen dioxide and nitrogen monoxide (NO2/NO), carbon monoxide (CO), sulfur dioxide, and particulate matter (PM10 and PM2.5). After their deposition present at five geographic points with different environmental conditions, differences were observed in the proportion of bacteria growth which was characterized by growth in several specific culture media. Most identified the Gram-negative bacteria identified in the air samples collected belong to the genera Staphylococcus and Streptococcus. Gram-positive bacteria were present at a low rate.

Management of Air Pollution by a System of Transferable Individual Emission Permits with Overlapping Generations

The purpose of this article is to analyze the effectiveness of a pollution management system through individual permits that are distributed to young people with overlapping generations.From a general equilibrium model,the results show that such a system provides the conditions for optimal pollution management.But because of the non-cooperative behavior of the actors,this policy cannot institute intergenerational altruism.Incentives such as tax or subsidy are needed to get the receiving population to better choose between the physical good whose production satisfies their needs and the quality of the environment that depends on their option to sell the permits to firms or the future generation.

中国首个地基高分辨率傅里叶变换光谱观测站的大气成分长期观测研究

长期观测主要大气成分的体积混合比(VMR)廓线和柱总量对掌握中国气候变化和碳收支具有重要意义。本文对我国首个TCCON高分辨率傅里叶变换光谱(FTS)地基观测站——合肥观测站开展了系统性研究,该观测站可观测30多种大气成分的柱总量和VMR廓线。本文公布了2014年以来合肥观测站观测到的部分关键大气成分的时间序列,总结了迄今为止该站点取得的主要研究成果,包括光谱反演表征和归一化、关键大气成分的总体演变特征、排放估计、卫星和化学传输模式(CTM)校验以及对大气污染来源和传输的相关研究。同时,本文还对合肥观测站的观测、科学研究和未来研究计划进行了展望。中国明确提出2030年二氧化碳排放达到峰值,2060年实现碳中和。合肥观测站将为中国政府制定绿色经济政策、实现碳中和及《巴黎协定》目标提供科学支撑。

THE RELATION OF THE THRESHOLD VELOCITY OF COAL DUST TO ITS SIZE AND HUMIDITY

On the ground of wharf and a station where coal is piled up, the sources polluting the atmosphere are mainly the raised coal dust. According to the principle of mechanics, with the consideration of the gravities of coal dust particles and liquid droplets, coal dust size and humidity, under the condition of force balance when the coal dust was raised, the authors obtaineda theoretical formula for the threshold velocity of coal dust with humidity,Finally, the theoretical values from the formula gave a good agreement with the experimental data from some wind tunnels.

基于GIS的大气污染应急监测方案自动生成研究(英文)

Based on emergency monitoring work flow analysis of atmospheric pollution incidents, key technical problems involved in the atmospheric pollution monitoring scheme based on GIS was studied, including the orientation of the accident site, the inquiry of the distribution of the emergency monitoring units and the groups of experts and the determination of the shortest path of emergency monitoring researchers and equipments arriving to the accident site as well as the integrated technology of Gaussian model with GIS which was mainly researched. The automatic prototype system of the emergency monitoring optimized scheme of the atmospheric pollution based on GIS was analyzed with the case of atmospheric pollution accident in Kunshan.

Concentrations and isotopic characteristics of atmospheric reactive nitrogen around typical sources in Beijing,China

With rapid economic growth in China, anthropogenic reactive nitrogen （Nr） emissions have more than doubled over the last two or three decades. Atmospheric Nr pollution is an environmental concern in China especially in megacities such as Beijing. In order to identify the impact of emission sources on atmospheric Nr pollution, we measured atmospheric Nr concentrations and their isotopic composition （δ15N） dynamics at three typical sites： landfill, pig farm and road traffic sites in Beijing from April 2010 to March 2011. Passive samplers were used for monitoring ammonia （NH3） and nitrogen dioxide （NO2）, two major Nr species, while their δ15N values were measured by a diffusion method combined with mass spectrometer approach. The raw water pool of the landfill and fattening house of the pig farm were important NH3 sources with mean NH3 concentrations being 2,829 and 2,369 μg/m3, respectively, while the road traffic site was a minor NH3 source （10.6 μg/m3）. NH3 concentrations at sites besides the landfill and roads were high in summer and low in winter due to the annual variation of temperature and the change of emission source intensity. In contrast, the NH3 concentrations inside the pig farm house were high in winter and low in summer, for the barn windows were open in summer and closed in winter. The mean NO2 concentrations were 89.8, 32.9 and 23.0 μg/m3 at the road traffic, the landfill and pig farm sites, respectively. Due to vehicle fuel combustion, NO2 concentration at the road traffic was the highest among the three sources, and the road traffic was a main NO2 emission source. PM10, pNH4＊ and pNO3- concentrations in particulate matter were higher in summer than in winter （except PM10 for the pig farm）. The δ15NH3 values ranged from -19.14‰ to 7.82‰, with an average of-0.05‰ for the landfill site, and the lowest values were observed in June and July. The δ15NH3 values for the pig farm site ranged from -29.78‰ to-14.05‰ with an average of-24.51‰, and the 515NH3 values were more negative in summer than in the other seasons. The （515NO2 values were -9.63%o to 7.04‰ with an average of -3.72%0 for the road traffic site. The δ15NO2 values were more negative in summer than those in the other seasons. The different δ15N values for the various Nr species in different sources may serve as important indicators for identifying atmospheric Nr sources in megacities. The results may also provide the theoretical basis for research on the atmospheric N deposition and its sources.

Study on the Total Amount Control of Atmospheric Pollutant Based on GIS

To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.

Preliminary Analysis of Influencing Factors of Low Visibility on a Hazy Day in Winter in Binzhou City

Based on the monitoring data of visibility,particulate matter（ PM2. 5 and PM10） and atmospheric pollutants（ SO2,NO2,CO,and O3）,and meteorological factors（ temperature,humidity,and wind speed） at the six automatic air monitoring stations in Binzhou City from December 2016 to February 2017,the correlations between visibility and influencing factors were analyzed to study the main influencing factors of atmospheric visibility. The results showed that the daily average concentration of particulate matter negatively correlated with atmospheric visibility,and the correlation between PM2. 5 concentration and atmospheric visibility was more obvious than that of PM10 concentration. Among atmospheric pollutants,the daily average concentration of CO,NO2 and SO2 also negatively correlated with atmospheric visibility,while there was a positive correlation between visibility and the daily average concentration of O3. Daily average temperature and wind speed positively correlated with visibility,while relative humidity negatively correlated with visibility. Wind speed,relative humidity and PM2. 5 had strong correlation with visibility,and the linear correlation coefficient R2 was 0. 501 6,0. 446 6,and 0. 205 8 respectively,so wind speed,relative humidity,and PM2. 5 were the main factors influencing the decrease of atmospheric visibility on a hazy day in winter.

Concentrations,sources,and influential factors of water-soluble ions of atmospheric particles in Dunhuang Mogao Grottoes,a world heritage site in China

Atmospheric particle pollution is one of the major factors leading to degradation of ancient wall paintings,particularly heritage sites in arid and semi-arid regions.However,current systematic research on the changes,sources,and influential factors of atmospheric particulate matter and its water-soluble ion concentrations is not sufficient.Thus,the major water-soluble ion concentrations,sources,and influential factors of atmospheric particles PM_(2.5) and PM_(10)(particulate matter with an aerodynamic equivalent diameter≤2.5 and 10.0μm,respectively,in ambient air)were collected from Cave 16 and its ambient exterior environment in the Dunhuang Mogao Grottoes,China,between April 2015 and March 2016.Results showed that the concentrations of PM_(2.5) and PM_(10) inside and outside the cave were the highest in March 2016 and the lowest in December 2015.The higher particle concentration from March to May was related to the frequent occurrence of sand and dust events,and the lower particle concentration from June to September was associated with good diffusion conditions,increased precipitation,and an established cave shelterbelt.The concentration of particulate matter inside the cave was affected by the concentration of particles in the air outside the cave.Ca2+,NH+4,Na+,Cl-,and SO2-4were the main components of the total ions of PM_(2.5) and PM_(10) both inside and outside the cave.The total ions inside the cave were frequently affected by the disturbance of tourists'activities during the peak tourist season from May to August.Under the influence of dust,the total concentrations of Cl-,SO2-4,Na+,NH+4,and Ca2+in particles of different sizes inside and outside the cave increased,and the concentrations of Cl-,SO2-4,Na+,and Ca2+decreased during precipitation period.Backward air mass trajectory analysis suggested that the pollutants were mainly from Xinjiang,China.The pollutant sources of air particulates are straw burning,secondary pollution sources,soil dust,dry spring rivers,and tourist activities.