Non-thermal plasmas under atmospheric pressure are of great interest in polymer surface processing because of their convenience, effectiveness and low cost. In this paper, the treatment of Polyethylene terephthalate (...Non-thermal plasmas under atmospheric pressure are of great interest in polymer surface processing because of their convenience, effectiveness and low cost. In this paper, the treatment of Polyethylene terephthalate (PET) film surface for improving hydrophilicity using the non-thermal plasma generated by atmospheric pressure glow discharge (APGD) in air is conducted. The discharge characteristics of APGD are shown by measurement of their electrical discharge parameters and observation of light-emission phenomena, and the surface properties of PET before and after the APGD treatment are studied using contact angle measurement, x-ray photoelectron spectroscopy (XPS) and scanning electron microscopy (SEM). It is found that the APGD is homogeneous and stable in the whole gas gap, which differs from the commonly filamentary dielectric barrier discharge (DBD). A short time (several seconds) APGD treatment can modify the surface characteristics of PET film markedly and uniformly. After 10 s APGD treatment, the展开更多
A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-li...A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-like discharge was achieved. Two kinds of typical bacteria, i.e., the Staphylococcus aureus (S. aureus) and Escherichia coil (E. coil), were employed to study the bacterial inactivation mechanism by means of the non-thermal plasma. The killing log value (KLV) of S. aureus reached up to 5.38 with a treatment time of 90 s and that of E. coil up to 5.36 with 60 s, respectively. According to the argon emission spectra of the plasma jet and the scanning electron microscope (SEM) images of the two bacteria before and after the plasma treatment, it is concluded that the reactive species in the argon plasma played a major role in the bacterial inactivation, while the heat, electric field and UV photons had little effect.展开更多
Dielectric barrier discharge (DBD) excitated by pulsed power is a promising method for producing nonthermal plasma at atmospheric pressure. Discharge characteristic in a DBD with salt water as electrodes by a home-m...Dielectric barrier discharge (DBD) excitated by pulsed power is a promising method for producing nonthermal plasma at atmospheric pressure. Discharge characteristic in a DBD with salt water as electrodes by a home-made unipolar nanosecond-pulse power source is presented in this paper. The generator is capable of providing repetitive pulses with the voltage up to 30 kV and duration of 70 ns at a 300 Ω resistive load. Applied voltage and discharge current are measured under various experimental conditions. The DBD created between two liquid electrodes shows that the discharge is homogeneous and diffuse in the whole discharge regime, Spectra diagnosis is conducted by an optical emission spectroscopy. The air plasma has strong emission from nitrogen species below 400 nm, notably the nitrogen second positive system.展开更多
文摘Non-thermal plasmas under atmospheric pressure are of great interest in polymer surface processing because of their convenience, effectiveness and low cost. In this paper, the treatment of Polyethylene terephthalate (PET) film surface for improving hydrophilicity using the non-thermal plasma generated by atmospheric pressure glow discharge (APGD) in air is conducted. The discharge characteristics of APGD are shown by measurement of their electrical discharge parameters and observation of light-emission phenomena, and the surface properties of PET before and after the APGD treatment are studied using contact angle measurement, x-ray photoelectron spectroscopy (XPS) and scanning electron microscopy (SEM). It is found that the APGD is homogeneous and stable in the whole gas gap, which differs from the commonly filamentary dielectric barrier discharge (DBD). A short time (several seconds) APGD treatment can modify the surface characteristics of PET film markedly and uniformly. After 10 s APGD treatment, the
基金supported in part by China Foundation for the Author of National Excellent Doctoral Dissertation(No.200338)New Century Excellent Talents in University(No.NCET-04-0943)
文摘A coaxial dielectric barrier discharge plasma jet was designed, which can be operated in atmospheric pressure argon under an intermediate frequency sinusoidal resonant power supply, and an atmospheric pressure glow-like discharge was achieved. Two kinds of typical bacteria, i.e., the Staphylococcus aureus (S. aureus) and Escherichia coil (E. coil), were employed to study the bacterial inactivation mechanism by means of the non-thermal plasma. The killing log value (KLV) of S. aureus reached up to 5.38 with a treatment time of 90 s and that of E. coil up to 5.36 with 60 s, respectively. According to the argon emission spectra of the plasma jet and the scanning electron microscope (SEM) images of the two bacteria before and after the plasma treatment, it is concluded that the reactive species in the argon plasma played a major role in the bacterial inactivation, while the heat, electric field and UV photons had little effect.
基金supported by National Natural Science Foundation of China(Nos.11076026,50707032)the Knowledge Innovation Program of the Chinese Academy of Sciences(No.KGCX2-YW-339)Opening Project of State Key Laboratory of Polymer Materials Engineering in Sichuan University(No.KF201103)
文摘Dielectric barrier discharge (DBD) excitated by pulsed power is a promising method for producing nonthermal plasma at atmospheric pressure. Discharge characteristic in a DBD with salt water as electrodes by a home-made unipolar nanosecond-pulse power source is presented in this paper. The generator is capable of providing repetitive pulses with the voltage up to 30 kV and duration of 70 ns at a 300 Ω resistive load. Applied voltage and discharge current are measured under various experimental conditions. The DBD created between two liquid electrodes shows that the discharge is homogeneous and diffuse in the whole discharge regime, Spectra diagnosis is conducted by an optical emission spectroscopy. The air plasma has strong emission from nitrogen species below 400 nm, notably the nitrogen second positive system.