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Broadening of Cr nanostructures in laser-focused atomic deposition 被引量:1
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作者 卢向东 李同保 马艳 《Chinese Physics B》 SCIE EI CAS CSCD 2010年第12期168-173,共6页
This paper presents the experimental progress of laser-focused Cr atomic deposition and the experimental condition. The result is an accurate array of lines with a periodicity of 212.8±0.2 nm and mean full-width ... This paper presents the experimental progress of laser-focused Cr atomic deposition and the experimental condition. The result is an accurate array of lines with a periodicity of 212.8±0.2 nm and mean full-width at half maximum as approximately 95 nm. Surface growth in laser-focused Cr atomic deposition is modeled and studied by kinetic Monte Carlo simulation including two events: the one is that atom trajectories in laser standing wave are simulated with the semiclassical equations of motion to obtain the deposition position; the other is that adatom diffuses by considering two major diffusion processes, namely, terrace diffusion and step-edge descending. Comparing with experimental results (Anderson W R, Bradley C C, McClelland J J and Celotta R J 1999 Phys. Rev. A 59 2476), it finds that the simulated trend of dependence on feature width is in agreement with the power of standing wave, the other two simulated trends are the same in the initial stage. These results demonstrate that some surface diffusion processes play important role in feature width broadening. Numerical result also shows that high incoming beam flux of atoms deposited redounds to decrease the distance between adatoms which can diffuse to minimize the feature width and enhance the contrast. 展开更多
关键词 atom optics laser-focused atomic deposition kinetic Monte Carlo simulation surface growth
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Effect of nitrogen pressure on optical properties and microstructure of diamond-like carbon films grown by pulsed laser deposition 被引量:2
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作者 丁旭丽 李清山 孔祥和 《Optoelectronics Letters》 EI 2009年第2期117-119,共3页
The effect of nitrogen pressure on optical properties of hydrogen-free diamond-like carbon (DLC) films deposited by pulsed laser ablation graphite in different background pressures of nitrogen is reported. By varying ... The effect of nitrogen pressure on optical properties of hydrogen-free diamond-like carbon (DLC) films deposited by pulsed laser ablation graphite in different background pressures of nitrogen is reported. By varying nitrogen pressures from 0.05 to 15.00 Pa, the photoluminescence is gradually increased and optical transmittance is gradually decreased. Atomic force microscopy (AFM) is used to observe the surface morphology of the DLC films. The results indicate that the surface becomes unsmoothed and there are some globose particles on the films surface with the rise of nitrogen pressures. The microstructure of the films is characterized using Raman spectroscopy. 展开更多
关键词 Effect of nitrogen pressure on optical properties and microstructure of diamond-like carbon films grown by pulsed laser deposition DLC
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光学玻璃基底原子层同质材料沉积薄膜光谱及激光诱导损伤特性研究 被引量:2
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作者 程海鹏 耿锋 +2 位作者 刘民才 张清华 李亚国 《光谱学与光谱分析》 SCIE EI CAS CSCD 北大核心 2021年第7期2307-2313,共7页
通过原子层沉积技术在熔石英玻璃表面制备了同质材料的单层SiO_(2)薄膜,对光学薄膜的物理化学性质和强激光辐照下的激光诱导损伤性能进行了深入研究。实验中采用双叔丁基氨基硅烷(BTBAS)和臭氧(O_(3))作为反应前驱体,在熔石英光学元件... 通过原子层沉积技术在熔石英玻璃表面制备了同质材料的单层SiO_(2)薄膜,对光学薄膜的物理化学性质和强激光辐照下的激光诱导损伤性能进行了深入研究。实验中采用双叔丁基氨基硅烷(BTBAS)和臭氧(O_(3))作为反应前驱体,在熔石英光学元件表面进行了SiO_(2)薄膜的原子层沉积工艺研究,以不同沉积温度条件制备了一系列膜样品。首先对原子层沉积特性和薄膜均匀性展开了研究,发现薄膜生长厚度与沉积循环次数之间符合线性生长规律,验证了制备薄膜的原子级逐层生长特性,并且表面沉积膜层的均匀性很好,其测得膜厚波动不超过2%。然后针对不同温度条件下沉积的SiO_(2)薄膜,对其粗糙度及各类光谱特性展开了研究,对比结果表明:样品的表面粗糙度在镀膜后有轻微的降低;薄膜样品在200~1000 nm范围内具有出色的透过率,均超过90%并逐渐趋近于93.3%,且其透射光谱与在裸露熔石英衬底上测得的光谱没有明显差异;镀膜前后荧光光谱和傅里叶变换红外光谱的差异证实了原子层沉积SiO_(2)膜中点缺陷(非桥键氧、氧空位、羟基等)的存在,这将会影响薄膜耐损伤性能。最后对衬底和膜样品进行了紫外激光诱导损伤测试,损伤阈值的变化表明熔石英元件表面沉积薄膜后的激光损伤性能有所降低,其零概率损伤阈值从31.8 J·cm^(-2)减小到20 J·cm^(-2)左右,与光谱缺陷情况表征相符合。薄膜中点缺陷部位会吸收紫外激光能量,导致局域温度升高,进而出现激光诱导损伤现象并降低抗激光损伤阈值。在选定的沉积温度范围内,较高温度条件下沉积的SiO_(2)薄膜其激光诱导损伤性能更好,可以控制沉积温度条件使得元件的抗损伤性能更为接近衬底本身,后续有望通过其他反应参数的优化来获得薄膜抗损伤性能的进一步提升。 展开更多
关键词 原子层沉积 二氧化硅 沉积温度 光学特性 激光诱导损伤
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激光汇聚Cr原子沉积的原子光学特性研究 被引量:9
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作者 卢向东 李同保 +1 位作者 马艳 汪黎栋 《物理学报》 SCIE EI CAS CSCD 北大核心 2009年第12期8205-8211,共7页
利用激光汇聚原子沉积技术,实验上获得了一维Cr层光栅结构.经原子力显微镜测试,其周期常数为(212.8±0.2)nm,约等于激光驻波场波长的一半.根据半经典理论模型,采用Adams-Bashforth-Moulton算法进行数值求解,模拟了同等实验参数条件... 利用激光汇聚原子沉积技术,实验上获得了一维Cr层光栅结构.经原子力显微镜测试,其周期常数为(212.8±0.2)nm,约等于激光驻波场波长的一半.根据半经典理论模型,采用Adams-Bashforth-Moulton算法进行数值求解,模拟了同等实验参数条件下的Cr原子运动轨迹,并对其原子光学特性进行分析.结果表明,模拟分析与实验结果符合得较好. 展开更多
关键词 原子光学 激光汇聚原子沉积 原子光学特性
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