Molecular self-assembly is extremely important in many fields, but the characterization of their corresponding intermolecular interactions is still lacking. The C-H stretching Raman band can reflect the hydrophobic in...Molecular self-assembly is extremely important in many fields, but the characterization of their corresponding intermolecular interactions is still lacking. The C-H stretching Raman band can reflect the hydrophobic interactions during the self-assembly process of sodium dodecyl sulfate （SDS） in aqueous solutions. However, the Raman spectra in this region are seriously overlapped by the OH stretching band of water. In this work, vertically polarized Raman spectra were used to improve the detection sensitivity of spectra of C-H region for the first time. The spectral results showed that the first critical micelle concentration and the second critical micelle concentration of SDS in water were 8.5 and 69 mmol/L, respectively, which were consistent with the results given by surface tension measurements. Because of the high sensitivity of vertically polarized Raman spectra, the critical micelle concentration of SDS in a relatively high concentration of salt solution could be obtained in our experiment. The two critical concentrations of SDS in 100 mmol/L NaCl solution were recorded to be 1.8 and 16.5 mmol/L, respectively. Through comparing the spectra and surface tension of SDS in water and in NaCl solution, the self-assembly process in bulk phase and at interface were discussed. The interactions among salt ions, SDS and water molecules were also analyzed. These results demonstrated the vertically polarized Raman spectra could be employed to study the self-assembly process of SDS in water.展开更多
We present an alternative scheme for preparing the superpositions of coherent states along a straight line of a cavity field using degenerate atom-cavity field Raman interaction. In the scheme, a collection of A-type ...We present an alternative scheme for preparing the superpositions of coherent states along a straight line of a cavity field using degenerate atom-cavity field Raman interaction. In the scheme, a collection of A-type three-level atoms is orderly sent through the cavity to interact with the cavity field adjusted by a microwave source connected to it, followed by state-selective measurements. In this way, we can prepare the superpositions of several coherent states along a straight line with arbitrary weighting factors for the cavity field. In the scheme, the coherence of the atom-cavity system may be maintained and the second microwave field is unnecessary, which is prior to the previous scheme.展开更多
A scheme is reported for the teleportation of entangled coherent states through the degenerate Raman interaction. The scheme uses an entangled state of an atom and two coherent states as a quantum channel. It makes lu...A scheme is reported for the teleportation of entangled coherent states through the degenerate Raman interaction. The scheme uses an entangled state of an atom and two coherent states as a quantum channel. It makes lull use of coherent cavity fields. Furthermore, it does not need any classical field to transform the atom states.展开更多
A method is presented for generating highly squeezed states of a cavity field via the atom-cavity field interaction of the Raman type. In the scheme a sequence of three-level -type atoms interacts with a cavity field,...A method is presented for generating highly squeezed states of a cavity field via the atom-cavity field interaction of the Raman type. In the scheme a sequence of three-level -type atoms interacts with a cavity field, displaced by a classical source, in a Raman manner. Then the atomic states are measured. By this way the cavity field may collapse onto a superposition of several coherent states, which exhibits strong squeezing. The scheme can also be used to prepare superpositions of many two-mode coherent states for two cavity fields. The coherent states in each mode are on a straight line. This is the first way for preparing multi-component entangled coherent states of this type in cavity QED.展开更多
A scheme for generating cluster states via Raman interaction is proposed. In the scheme, we firstly prepare cluster states of multi-cavities with information encoded in the coherent states and then generate cluster st...A scheme for generating cluster states via Raman interaction is proposed. In the scheme, we firstly prepare cluster states of multi-cavities with information encoded in the coherent states and then generate cluster states of multiatoms, which encode the information in the ground states of A-type atoms. The advantages of our scheme are that the atomic spontaneous radiation can be efficiently reduced since the cavity frequency is largely detuned from the atomic transition frequency and the Hadamard gate operation of the coherent states is replaced by measuring the coherent states.展开更多
A scheme is presented for generating a four-photon coherent state via the degenerate Raman interaction. The scheme does not need classical fields to manipulate the atoms. Its another advantage is that the atomic spont...A scheme is presented for generating a four-photon coherent state via the degenerate Raman interaction. The scheme does not need classical fields to manipulate the atoms. Its another advantage is that the atomic spontaneous emission can be neglected. Therefore, the coherence of the system may be better maintained. The scheme can be generalized to generate superposition of 2^n coherent states and superposition of 2^n two-mode coherent states. The coherent states in each mode are on a circle symmetrically.展开更多
The interactions of lanthanoid ions with dipalmitoylphosphatidylcholine bilayer were studied by DSC and Raman spectroscopy.The results show that the addition of lanthanoid ions causes a considerable increase of the ge...The interactions of lanthanoid ions with dipalmitoylphosphatidylcholine bilayer were studied by DSC and Raman spectroscopy.The results show that the addition of lanthanoid ions causes a considerable increase of the gel to liquid crystalline transition temperature of phospholipid and a reduction of order of lateral packing and conformation of acyl chains in SUVs.展开更多
In order to produce millimeter-scale plasmas for the research of laser-plasma interactions （LPIs）, gasbag target is designed and tested on Shenguang-III prototype laser facility. The x-ray pinhole images show that m...In order to produce millimeter-scale plasmas for the research of laser-plasma interactions （LPIs）, gasbag target is designed and tested on Shenguang-III prototype laser facility. The x-ray pinhole images show that millimeter-scale plasmas are produced with the gasbag. The electron temperature inferred from the stimulated Raman scattering （SRS） spectrum is about 1.6 keV. The SRS spectrum also indicates that the electron density has a fiat region within the duration of 200 ps. The obvious differences between the results of the gasbag and that of the void half hohlraum show the feasibility of the gasbag target in creating millimeter-scale plasmas. The LPIs in these millimeter-scale plasmas may partially mimic those in the ignition condition because the duration of the existence of a flat plasma density is much larger than the growth time of the two main instabilities, i.e., SRS and stimulated Brillouin scattering （SBS）. So we make the conclusion that the gasbag target can be used to research the large-scale LPIs.展开更多
We present our recent laser-plasmas instability(LPI)comparison experiment at the SGIII laser facility between the spherical and cylindrical hohlraums.Three kinds of filling are considered:vacuum,gas-filling with or wi...We present our recent laser-plasmas instability(LPI)comparison experiment at the SGIII laser facility between the spherical and cylindrical hohlraums.Three kinds of filling are considered:vacuum,gas-filling with or without a capsule inside.A spherical hohlraum of 3.6 mm in diameter,and a cylindrical hohlraum of 2.4 mm?4.3 mm are used.The capsule diameter is 0.96 mm.A flat-top laser pulse with 3 ns duration and up to 92.73 kJ energy is used.The experiment has shown that the LPI level in the spherical hohlraum is close to that of the outer beam in the cylindrical hohlraum,while much lower than that of the inner beam.The experiment is further simulated by using our 2-dimensional radiation hydrodynamic code LARED-Integration,and the laser back-scattering fraction and the stimulated Raman scatter(SRS)spectrum are post-processed by the high efficiency code of laser interaction with plasmas HLIP.According to the simulation,the plasma waves are strongly damped and the SRS is mainly developed at the plasma conditions of electron density from 0.08 n_(c) to 0.1 n_(c) and electron temperature from 1.5 keV to 2.0 keV inside the hohlraums.However,obvious differences between the simulation and experiment are found,such as that the SRS back-scattering is underestimated,and the numerical SRS spectrum peaks at a larger wavelength and at a later time than the data.These dif-ferences indicate that the development of a 3D radiation hydrodynamic code,with more accurate physics models,is mandatory for spherical hohlraum study.展开更多
基金This work is supported by the National Natural Science Foundation of China （No.21473171 and No.21573208）, the Pundamental Research Funds for the Central Universities （No.JB160508）, and the Huashan Mountain Scholar Program.
文摘Molecular self-assembly is extremely important in many fields, but the characterization of their corresponding intermolecular interactions is still lacking. The C-H stretching Raman band can reflect the hydrophobic interactions during the self-assembly process of sodium dodecyl sulfate （SDS） in aqueous solutions. However, the Raman spectra in this region are seriously overlapped by the OH stretching band of water. In this work, vertically polarized Raman spectra were used to improve the detection sensitivity of spectra of C-H region for the first time. The spectral results showed that the first critical micelle concentration and the second critical micelle concentration of SDS in water were 8.5 and 69 mmol/L, respectively, which were consistent with the results given by surface tension measurements. Because of the high sensitivity of vertically polarized Raman spectra, the critical micelle concentration of SDS in a relatively high concentration of salt solution could be obtained in our experiment. The two critical concentrations of SDS in 100 mmol/L NaCl solution were recorded to be 1.8 and 16.5 mmol/L, respectively. Through comparing the spectra and surface tension of SDS in water and in NaCl solution, the self-assembly process in bulk phase and at interface were discussed. The interactions among salt ions, SDS and water molecules were also analyzed. These results demonstrated the vertically polarized Raman spectra could be employed to study the self-assembly process of SDS in water.
文摘We present an alternative scheme for preparing the superpositions of coherent states along a straight line of a cavity field using degenerate atom-cavity field Raman interaction. In the scheme, a collection of A-type three-level atoms is orderly sent through the cavity to interact with the cavity field adjusted by a microwave source connected to it, followed by state-selective measurements. In this way, we can prepare the superpositions of several coherent states along a straight line with arbitrary weighting factors for the cavity field. In the scheme, the coherence of the atom-cavity system may be maintained and the second microwave field is unnecessary, which is prior to the previous scheme.
基金The project supported by the Natural Science Foundation of Fujian Province of China under Grant No. 2006J0234
文摘A scheme is reported for the teleportation of entangled coherent states through the degenerate Raman interaction. The scheme uses an entangled state of an atom and two coherent states as a quantum channel. It makes lull use of coherent cavity fields. Furthermore, it does not need any classical field to transform the atom states.
文摘A method is presented for generating highly squeezed states of a cavity field via the atom-cavity field interaction of the Raman type. In the scheme a sequence of three-level -type atoms interacts with a cavity field, displaced by a classical source, in a Raman manner. Then the atomic states are measured. By this way the cavity field may collapse onto a superposition of several coherent states, which exhibits strong squeezing. The scheme can also be used to prepare superpositions of many two-mode coherent states for two cavity fields. The coherent states in each mode are on a straight line. This is the first way for preparing multi-component entangled coherent states of this type in cavity QED.
基金The project supported by National Natural Science Foundation of China under Grant No. 10574022 and the Natural Science Foundation of Fujian Province of China under Grant No. Z0512006
文摘A scheme for generating cluster states via Raman interaction is proposed. In the scheme, we firstly prepare cluster states of multi-cavities with information encoded in the coherent states and then generate cluster states of multiatoms, which encode the information in the ground states of A-type atoms. The advantages of our scheme are that the atomic spontaneous radiation can be efficiently reduced since the cavity frequency is largely detuned from the atomic transition frequency and the Hadamard gate operation of the coherent states is replaced by measuring the coherent states.
基金The author is grateful to professor ZHENG Shi-Biao for his help.
文摘A scheme is presented for generating a four-photon coherent state via the degenerate Raman interaction. The scheme does not need classical fields to manipulate the atoms. Its another advantage is that the atomic spontaneous emission can be neglected. Therefore, the coherence of the system may be better maintained. The scheme can be generalized to generate superposition of 2^n coherent states and superposition of 2^n two-mode coherent states. The coherent states in each mode are on a circle symmetrically.
文摘The interactions of lanthanoid ions with dipalmitoylphosphatidylcholine bilayer were studied by DSC and Raman spectroscopy.The results show that the addition of lanthanoid ions causes a considerable increase of the gel to liquid crystalline transition temperature of phospholipid and a reduction of order of lateral packing and conformation of acyl chains in SUVs.
基金Project supported by the National Natural Science Foundation of China (Grant No. 10625523)the Innovation Project of the Chinese Academy of Sciences (Grant No. KJCX2-YW-N36)National High-Tech Program of China
文摘In order to produce millimeter-scale plasmas for the research of laser-plasma interactions （LPIs）, gasbag target is designed and tested on Shenguang-III prototype laser facility. The x-ray pinhole images show that millimeter-scale plasmas are produced with the gasbag. The electron temperature inferred from the stimulated Raman scattering （SRS） spectrum is about 1.6 keV. The SRS spectrum also indicates that the electron density has a fiat region within the duration of 200 ps. The obvious differences between the results of the gasbag and that of the void half hohlraum show the feasibility of the gasbag target in creating millimeter-scale plasmas. The LPIs in these millimeter-scale plasmas may partially mimic those in the ignition condition because the duration of the existence of a flat plasma density is much larger than the growth time of the two main instabilities, i.e., SRS and stimulated Brillouin scattering （SBS）. So we make the conclusion that the gasbag target can be used to research the large-scale LPIs.
基金This work is supported by the National Natural Science Foundation of China under grants Nos.11405011 and 11475033.
文摘We present our recent laser-plasmas instability(LPI)comparison experiment at the SGIII laser facility between the spherical and cylindrical hohlraums.Three kinds of filling are considered:vacuum,gas-filling with or without a capsule inside.A spherical hohlraum of 3.6 mm in diameter,and a cylindrical hohlraum of 2.4 mm?4.3 mm are used.The capsule diameter is 0.96 mm.A flat-top laser pulse with 3 ns duration and up to 92.73 kJ energy is used.The experiment has shown that the LPI level in the spherical hohlraum is close to that of the outer beam in the cylindrical hohlraum,while much lower than that of the inner beam.The experiment is further simulated by using our 2-dimensional radiation hydrodynamic code LARED-Integration,and the laser back-scattering fraction and the stimulated Raman scatter(SRS)spectrum are post-processed by the high efficiency code of laser interaction with plasmas HLIP.According to the simulation,the plasma waves are strongly damped and the SRS is mainly developed at the plasma conditions of electron density from 0.08 n_(c) to 0.1 n_(c) and electron temperature from 1.5 keV to 2.0 keV inside the hohlraums.However,obvious differences between the simulation and experiment are found,such as that the SRS back-scattering is underestimated,and the numerical SRS spectrum peaks at a larger wavelength and at a later time than the data.These dif-ferences indicate that the development of a 3D radiation hydrodynamic code,with more accurate physics models,is mandatory for spherical hohlraum study.
