Time-integrated optical emission analysis of laser-induced plasma on Teflon is presented.Plasma was induced under atmospheric pressure air using transversely excited atmospheric CO_(2) laser pulses.Teflon is a C-based...Time-integrated optical emission analysis of laser-induced plasma on Teflon is presented.Plasma was induced under atmospheric pressure air using transversely excited atmospheric CO_(2) laser pulses.Teflon is a C-based polymer that is,among other things,interesting as a substrate for laser-induced breakdown spectroscopy analysis of liquid samples.This study aimed to determine the optimal experimental conditions for obtaining neutral and ionized C spectral lines and C2 and CN molecular band emission suitable for spectrochemical purposes.Evaluation of plasma parameters was done using several spectroscopic techniques.Stark profiles of appropriate C ionic lines were used to determine electron number density.The ratio of the integral intensity of ionic-to-atomic C spectral lines was used to determine the ionization temperature.A spectral emission of C2 Swan and CN violet bands system was used to determine the temperature of the colder,peripheral parts of plasma.We critically analyzed the use of molecular emission bands as a tool for plasma diagnostics and suggested methods for possible improvements.展开更多
We report on the phenomena of the periodic spontaneous collapse and revival in the dynamics of an atomic beam interacting with a single-mode and coherent-state light field. Conventional collapse and revival by Eberly ...We report on the phenomena of the periodic spontaneous collapse and revival in the dynamics of an atomic beam interacting with a single-mode and coherent-state light field. Conventional collapse and revival by Eberly et al. [Phys. Rev. Lett. 44(1980)1323 ] are presented in the case of the evolution with time of the population inversion. Here, we study the evolution with coupling strength of population inversion. We define the collapse and revival coupling strengths as characteristic parameters to describe the above collapse and revival. Furthermore, we present the analytic formulas for the population inversion, the collapse and revival coupling strengths.展开更多
We illustrate our experimental observation of coexisting the controllable spatial splitting and intensity suppression of four-wave mixing (FWM) beam in a V-type three-level atomic system. The peak number and separat...We illustrate our experimental observation of coexisting the controllable spatial splitting and intensity suppression of four-wave mixing (FWM) beam in a V-type three-level atomic system. The peak number and separation distance of the FWM beam are controlled by the intensities and frequencies of the laser beams, as well as atomic density.展开更多
Cross sections for charge transfer and ionization of atomic hydrogen by highly charged ions A^q+ (q =6 9) are evaluated using a simple and classical method based on the previous works by Bohr and Lindhard [K. Dan. ...Cross sections for charge transfer and ionization of atomic hydrogen by highly charged ions A^q+ (q =6 9) are evaluated using a simple and classical method based on the previous works by Bohr and Lindhard [K. Dan. Vidensk. Selsk. Mat. Fys. Medd 28 (1954) No 7], Brandt [Nucl. Instrum. Methods Phys. Res. 214 (1983) 93] and Ben-Itzhak et al. [J. Phys. B: At. Mol. Opt. Phys. 26 (1993) 1711]. It is proved that the present calculations are feasible to some extent in comparison with available experimental data and quantum calculations.展开更多
Segmented all-electron basis set of triple zeta valence quality plus polarization functions(TZP)for the elements of the fifth row to be used together with the zero-order regular approximation(ZORA)is carefully constru...Segmented all-electron basis set of triple zeta valence quality plus polarization functions(TZP)for the elements of the fifth row to be used together with the zero-order regular approximation(ZORA)is carefully constructed.To correctly describe electrons distant from atomic nuclei,the basis set is augmented with diffuse functions giving rise to a set designated as ATZP-ZORA.At the ZORA-B3LYP theoretical level,these sets are used to calculate the ionization energy and mean dipole polarizability of some atoms,bond length,dissociation energy,and harmonic vibrational frequency of diatomic molecules.Then,these results are compared with the theoretical and experimental data found in the literature.Even considering that our sets are relatively compact,they are sufficiently accurate and reliable to perform property calculations involving simultaneously electrons from the inner shell and outer shell.The performances of the ZORA and second-order Douglas-Kroll-Hess Hamiltonians are evaluated and the results are also discussed.展开更多
Dressed four-wave mixing (DFWM) spectroscopy is investigated theoretically in some micrometric thin cells. It is found that DFWM spectra can be modified by polarization interference of atoms and transient effects in...Dressed four-wave mixing (DFWM) spectroscopy is investigated theoretically in some micrometric thin cells. It is found that DFWM spectra can be modified by polarization interference of atoms and transient effects induced by atom-wall collision. This modification can lead to width-narrowing of DFWM lines and facilitates to implement experiment of high resolution DFWM spectroscopy in a confined atomic system.展开更多
The comparison between single-point energy scanning (SPES) and geometry optimization (OPT) in determining the equilibrium geometries of c^3∑g^+ and B^1-Пu states of dimer 7Li2 is made at numerous basis sets by ...The comparison between single-point energy scanning (SPES) and geometry optimization (OPT) in determining the equilibrium geometries of c^3∑g^+ and B^1-Пu states of dimer 7Li2 is made at numerous basis sets by using a symmetryadapted-cluster configuration-interaztion (SAC-CI) method in the Gaussian 03 program package. In this paper the difference of the equilibrium geometries obtained by SPES and by OPT is reported. The results obtained by SPES are found to be more reasonable than those obtained by OPT in full active space at the present SAC-CI level of theory. And the conclusion is attained that the cc-PVTZ is a most suitable basis set for these states. The calculated dissociation energies and equilibrium geometries are 0.8818 eV and 0.3090 nm for c^3∑g^+ state, and 0.3668 eV and 0.2932 nm for B^1-Пu state respectively. The potential energy curves are calculated over a wide internuclear distance range from about 2.5α0 to 37α0 and have a least-squares fit into the Murrell-Sorbie function. According to the calculated analytic potential energy functions, the harmonic frequencies (We) and other spectroscopic data (ωeXe, Be and αe) are calculated. Comparison of the theoretical determinations at present work with the experiments and other theories clearly shows that the present work is the most complete effort and thus represents an improvement over previous theoretical results.展开更多
The generation of various entangled states is an essential task in quantum information processing. Recently, a scheme (PRA 79, 022304) has been suggested for generating Greenberger-Horne-Zeilinger state and cluster ...The generation of various entangled states is an essential task in quantum information processing. Recently, a scheme (PRA 79, 022304) has been suggested for generating Greenberger-Horne-Zeilinger state and cluster state with atomic ensembles based on the Rydberg blockade. Using similar resources as the earlier scheme, here we propose an experimentally feasible scheme of preparing arbitrary four-qubit W class of maximally and non- maximally entangled states with atomic ensembles in a single step. Moreover, we carefully analyze the realistic noises and predict that four-qubit W states can be produced with high fidelity (F - 0.994) via our scheme.展开更多
Using the single-atom induced dipole moment under strong field approximation as a source, we suggest a model to simulate the macroscopic high-order harmonic generation (HHG) from the mixed gases (He and Ne) intera...Using the single-atom induced dipole moment under strong field approximation as a source, we suggest a model to simulate the macroscopic high-order harmonic generation (HHG) from the mixed gases (He and Ne) interacting with intense infrared laser by solving the three-dimensional Maxwell's equation of the harmonic field. Regular destructive interference (DI) and constructive interference (CI) are observed in the macroscopic HHG spectra when the gas jet is put at a good phase-matching position. A semiclassical model of short and long electron trajectories is applied to interpret the DI and CI of HHG qualitatively.展开更多
The equation of motion of two-level chromium atoms in Gauss standing laser wave is discussed and the distribution of chromium atoms is given under different transverse velocity conditions. The results show that the fo...The equation of motion of two-level chromium atoms in Gauss standing laser wave is discussed and the distribution of chromium atoms is given under different transverse velocity conditions. The results show that the focusing position of atoms will be affected by the transverse velocity of atoms. Based on the four-order Runge- Kutta method, the locus of chromium atoms in Gauss standing laser wave is simulated. The three-dimensional characteristics of nanometer structures are stimulated under perfect and emanative conditions.展开更多
The molecular dynamics (MD) method is used to simulate the interactions of energetic C20 clusters with the dense plasma targets within the framework of the linear Vlasov-Poisson theory. The influences of various clu...The molecular dynamics (MD) method is used to simulate the interactions of energetic C20 clusters with the dense plasma targets within the framework of the linear Vlasov-Poisson theory. The influences of various clusters (H2, N2, C20 and C60 respectively) on stopping power are discussed. The simulation results show that the vicinage effects in the Coulomb explosion dynamics and the stopping power are strongly affected by the variations in the cluster speed and the plasma parameters. Coulomb explosions are found to proceed faster for higher speeds, lower plasma densities and higher electron temperatures. In addition, the cluster stopping power is strongly enhanced in the early stages of Coulomb explosions due to the vicinage effect, but this enhancement eventually diminishes, after the cluster constituent ions are sufficiently separated. For the large and heavy clusters, the stopping power ratio reaches much higher values in the early stage of Coulomb explosion owing to the constructive interferences in the vicinage effect.展开更多
One-dimensional deposition of a neutral chromium atomic beam focused by a near-resonant Gaussian standing- laser field is discussed by using a fourth-order Runge-Kutta type algorithm. The deposition pattern of neutral...One-dimensional deposition of a neutral chromium atomic beam focused by a near-resonant Gaussian standing- laser field is discussed by using a fourth-order Runge-Kutta type algorithm. The deposition pattern of neutral chromium atoms in a laser standing wave with different laser power is discussed and the simulation result shows that the full width at half maximum (FWHM) of a nanometer stripe is 115nm and the contrast is 2.5:1 with laser power 3.93mW; the FWHM is 0.8nm and the contrast is 27:1 with laser power 16mW, the optimal laser power; but with laser power increasing to 50mW, the nanometer structure forms multi-crests and the quality worsens quickly with increasing laser power.展开更多
By using a pump-probe technique, the nascent rotational and vibrational state distributions of CsH are obtained in the Cs(6^2 D,7^2 D) plus H2 reaction. The nascent CsH molecules are found to populate the lowest two...By using a pump-probe technique, the nascent rotational and vibrational state distributions of CsH are obtained in the Cs(6^2 D,7^2 D) plus H2 reaction. The nascent CsH molecules are found to populate the lowest two vibrational (v″ = 0 and 1) levels of the ground electronic state. By comparing the spectral intensities of the CsH action spectra with those of pertinent Cs atomic fluorescence excitation spectra, the relative reactivity with 1-12 is in an order of6^2D3/2 〉 6^2D5/2 〉 7^2D3/2 〉 7^2D5/2. The rotational temperatures are found to be slightly below the cell temperature. The relative fractions (〈fV〉, 〈fR〉, 〈fT〉) of average energy disposal are derived as (0.2,0.12,0.68), (0.2,0.12,0.68), (0.07,0.04,0.89) and (0.07,0.04,0.89) for the 6^2D3/2, 6^2D5/2, 7^2D3/2 and 7^2D5/2, respectively. The major available energy is released as translation. These results support that the reaction mechanism of Cs(6^2 D,7^2 D) plus 112 is primarily a eollinear abstraction and not an insertion.展开更多
A complex optical model potential modified by incorporating the concept of bonded atom, which takes into consideration the overlapping effect of electron clouds between two atoms in a molecule, is first employed to ca...A complex optical model potential modified by incorporating the concept of bonded atom, which takes into consideration the overlapping effect of electron clouds between two atoms in a molecule, is first employed to calculate the total cross sections for electrons scattering from such complex molecules as C2H6, C2F6, C6H6 and C6F6 using the aclditivity rule model at Hartree-Fock level over the energy range from 100 eV to 5000 eV. The total cross sections are quantitatively compared with those obtained by experiments wherever available, and they are in good agreement with each other over a wide energy range. It is shown that the modified potential together with the additivity rule model is completely suitable for the calculation of total cross sections of electrons scattering from such complex molecules as C2H6, C2F6, C6H6 and C6F6 above 200 eV-300 eV.展开更多
A diamond-shaped shock wave was created in a helium arcjet plasma. Visi- ble/ultraviolet emission spectroscopy was used to investigate the condition for the formation of stable shocks and to determine characteristics ...A diamond-shaped shock wave was created in a helium arcjet plasma. Visi- ble/ultraviolet emission spectroscopy was used to investigate the condition for the formation of stable shocks and to determine characteristics of the plasma. Dependence of the position of the shock front on the gas pressure in the expansion region was investigated. It was found that the shock wave arises from the collision of plasma particles and residual neutral atoms in that region. Continuum and line spectra of neutral helium were measured, from which the electron temper- atures were derived. The electron density was deduced from the Inglis-Teller limit of the He I 2p3p-3d3D series. The temperature and density were found to have almost constant values of 0.2 eV and 8.5x 1013 cm-3, respectively, across the shock front.展开更多
We present a simple scheme for the probabilistic generation of the $n$-qubit W state of three-level systems in cavity quantum electrodynamics. Once the W state is prepared, it will be insensitive to the spontaneous em...We present a simple scheme for the probabilistic generation of the $n$-qubit W state of three-level systems in cavity quantum electrodynamics. Once the W state is prepared, it will be insensitive to the spontaneous emission of atoms due to the fact that only the two degenerate ground states of the three-level atoms are involved. With time evolution of the system, the success probability and the experimental feasibility are also discussed.展开更多
We explore the effects of atomic memory on quantum correlations of two-mode light fields from four-wave mixing. A three-level atomic system in A configuration is considered, in which the atomic relaxation times are co...We explore the effects of atomic memory on quantum correlations of two-mode light fields from four-wave mixing. A three-level atomic system in A configuration is considered, in which the atomic relaxation times are comparable to or longer than the cavity relaxation times and thus there exists the atomic memory. The quantum correlation spectrum in the output is calculated without the adiabatic elimination of atomic variables. It is shown that the continuous variable entanglement is enhanced over a wide range of the normalized detuning in the intermediate and bad cavity cases compared with the good cavity case. In some situations more significant enhancement occurs at sidebands.展开更多
The experiment of measuring the spin depolarized time and light storage time in a Rb vapor under different conditions is performed. Typically, these measurements are accomplished in three different containers: atoms ...The experiment of measuring the spin depolarized time and light storage time in a Rb vapor under different conditions is performed. Typically, these measurements are accomplished in three different containers: atoms in a bare glass cell, atoms in a buffer gas cell, and atoms in a tetracontane (C4oH82) coating cell. The increasing depolarization and storage times are observed in both the buffer gas cell and the tetracontane coating cell. In the latter case, a storage time greater than 400μs is obtained.展开更多
Using a linearly polarized, phase-stabilized 3-fs driving pulse of 800 nm central wavelength shape-optimized on its'ascending edge by its an amplitude-reduced pulse irradiating on a superposition state of the helium ...Using a linearly polarized, phase-stabilized 3-fs driving pulse of 800 nm central wavelength shape-optimized on its'ascending edge by its an amplitude-reduced pulse irradiating on a superposition state of the helium atom, we demonstrate theoretically the generation of a super strong isolated 176-attosecond pulse in the spectral region of 93-124 eV. The unusually high intensity of this attosecond pulse is marked by the Rabi-like oscillations emerging in the time-dependent populations of the ground state and the continuum during the occurrence of the electron recombination, which is for the first time observed in this work.展开更多
The formulae of photon angular distribution and polarization degree for radiative recombination are presented to include the contribution of multipoles and their correlations. A fully relativistic code is then develop...The formulae of photon angular distribution and polarization degree for radiative recombination are presented to include the contribution of multipoles and their correlations. A fully relativistic code is then developed to calculate the photon angular distribution and polarization. The calculated polarization degree and differential cross-sections agree well with that of Scofild's results within 10%. The effects of multipoles on polarization and angular distribution are investigated. The polarization and the angular distribution become asymmetric when the multipoles are accounted as the electron energy increases.展开更多
基金funded by the Ministry of Education,Science and Technological Development of the Republic of Serbia(Nos.451-03-68/2022-14/200017 and 451-03-68/2022-14/200146)the financial support of the State Committee on Science and Technology of the Republic of Belarusthe Belarusian Republican Foundation for Fundamental Research(No.F20SRBG-001)。
文摘Time-integrated optical emission analysis of laser-induced plasma on Teflon is presented.Plasma was induced under atmospheric pressure air using transversely excited atmospheric CO_(2) laser pulses.Teflon is a C-based polymer that is,among other things,interesting as a substrate for laser-induced breakdown spectroscopy analysis of liquid samples.This study aimed to determine the optimal experimental conditions for obtaining neutral and ionized C spectral lines and C2 and CN molecular band emission suitable for spectrochemical purposes.Evaluation of plasma parameters was done using several spectroscopic techniques.Stark profiles of appropriate C ionic lines were used to determine electron number density.The ratio of the integral intensity of ionic-to-atomic C spectral lines was used to determine the ionization temperature.A spectral emission of C2 Swan and CN violet bands system was used to determine the temperature of the colder,peripheral parts of plasma.We critically analyzed the use of molecular emission bands as a tool for plasma diagnostics and suggested methods for possible improvements.
基金Supported by the National Basic Research Program of China under Grant No 2005CB724500, the National Natural Science Foundation of China under No 10874009, and Open Research Found of State Key Laboratory of Precision Spectroscopy (East China Normal University).
文摘We report on the phenomena of the periodic spontaneous collapse and revival in the dynamics of an atomic beam interacting with a single-mode and coherent-state light field. Conventional collapse and revival by Eberly et al. [Phys. Rev. Lett. 44(1980)1323 ] are presented in the case of the evolution with time of the population inversion. Here, we study the evolution with coupling strength of population inversion. We define the collapse and revival coupling strengths as characteristic parameters to describe the above collapse and revival. Furthermore, we present the analytic formulas for the population inversion, the collapse and revival coupling strengths.
基金Supported by the National Natural Science Foundation of China under Grant No 10974151, the New Century Excellent Talent Project (NCET) of the Ministry of Education of China under Grant No 08-0431, the Cross-Disciplinary Project of Xi'an Jiaotong University under Grant No 2009xjtujc08.
文摘We illustrate our experimental observation of coexisting the controllable spatial splitting and intensity suppression of four-wave mixing (FWM) beam in a V-type three-level atomic system. The peak number and separation distance of the FWM beam are controlled by the intensities and frequencies of the laser beams, as well as atomic density.
基金Supported by the National Natural Science Foundation of China under Grant No 10704030the Natural Science Foundation of Gansu Province under Grant No 0710RJZA014.
文摘Cross sections for charge transfer and ionization of atomic hydrogen by highly charged ions A^q+ (q =6 9) are evaluated using a simple and classical method based on the previous works by Bohr and Lindhard [K. Dan. Vidensk. Selsk. Mat. Fys. Medd 28 (1954) No 7], Brandt [Nucl. Instrum. Methods Phys. Res. 214 (1983) 93] and Ben-Itzhak et al. [J. Phys. B: At. Mol. Opt. Phys. 26 (1993) 1711]. It is proved that the present calculations are feasible to some extent in comparison with available experimental data and quantum calculations.
基金the Conselho Nacional de Desenvolvimento Científico Tecnológico(Brazilian Agency)。
文摘Segmented all-electron basis set of triple zeta valence quality plus polarization functions(TZP)for the elements of the fifth row to be used together with the zero-order regular approximation(ZORA)is carefully constructed.To correctly describe electrons distant from atomic nuclei,the basis set is augmented with diffuse functions giving rise to a set designated as ATZP-ZORA.At the ZORA-B3LYP theoretical level,these sets are used to calculate the ionization energy and mean dipole polarizability of some atoms,bond length,dissociation energy,and harmonic vibrational frequency of diatomic molecules.Then,these results are compared with the theoretical and experimental data found in the literature.Even considering that our sets are relatively compact,they are sufficiently accurate and reliable to perform property calculations involving simultaneously electrons from the inner shell and outer shell.The performances of the ZORA and second-order Douglas-Kroll-Hess Hamiltonians are evaluated and the results are also discussed.
基金Support from the National Natural Science Foundation of China under Grant No 10874139, and the Major Program of Science Foundation of Xi'an University of Arts and Science.
文摘Dressed four-wave mixing (DFWM) spectroscopy is investigated theoretically in some micrometric thin cells. It is found that DFWM spectra can be modified by polarization interference of atoms and transient effects induced by atom-wall collision. This modification can lead to width-narrowing of DFWM lines and facilitates to implement experiment of high resolution DFWM spectroscopy in a confined atomic system.
基金Project supported by the National Natural Science Foundation of China (Grant No 10574039), the Henan Innovation for University Prominent Research Talents (Grant No 2006KYCX002) and the National Natural Science Foundation of Education Bureau of Henan Province, China (Grant No 2007140015). We heartily thank Professor Zhu Zheng-Hem of Sichuan University for his helpful discussion about the reasonable dissociation stages of these calculations limits during the planning
文摘The comparison between single-point energy scanning (SPES) and geometry optimization (OPT) in determining the equilibrium geometries of c^3∑g^+ and B^1-Пu states of dimer 7Li2 is made at numerous basis sets by using a symmetryadapted-cluster configuration-interaztion (SAC-CI) method in the Gaussian 03 program package. In this paper the difference of the equilibrium geometries obtained by SPES and by OPT is reported. The results obtained by SPES are found to be more reasonable than those obtained by OPT in full active space at the present SAC-CI level of theory. And the conclusion is attained that the cc-PVTZ is a most suitable basis set for these states. The calculated dissociation energies and equilibrium geometries are 0.8818 eV and 0.3090 nm for c^3∑g^+ state, and 0.3668 eV and 0.2932 nm for B^1-Пu state respectively. The potential energy curves are calculated over a wide internuclear distance range from about 2.5α0 to 37α0 and have a least-squares fit into the Murrell-Sorbie function. According to the calculated analytic potential energy functions, the harmonic frequencies (We) and other spectroscopic data (ωeXe, Be and αe) are calculated. Comparison of the theoretical determinations at present work with the experiments and other theories clearly shows that the present work is the most complete effort and thus represents an improvement over previous theoretical results.
基金Supported by the National Natural Science Foundation of China under Grant No 10774192, the Fund of Innovation of Graduate School of National University of Defense Technology under Grant No 080201.
文摘The generation of various entangled states is an essential task in quantum information processing. Recently, a scheme (PRA 79, 022304) has been suggested for generating Greenberger-Horne-Zeilinger state and cluster state with atomic ensembles based on the Rydberg blockade. Using similar resources as the earlier scheme, here we propose an experimentally feasible scheme of preparing arbitrary four-qubit W class of maximally and non- maximally entangled states with atomic ensembles in a single step. Moreover, we carefully analyze the realistic noises and predict that four-qubit W states can be produced with high fidelity (F - 0.994) via our scheme.
基金Supported by the National Natural Science Foundation of China under Grant No 10674112, the Specialized Research Fund for the Doctoral Program of Higher Education of China under Grant No 20096203110001, the Foundation of Center of Theoretical Nuclear Physics of National Laboratory of Heavy Ion Accelerator of Lanzhou, and Foundation of Northwest Normal University under Grant No NWNU-KJCXGC-03-62.
文摘Using the single-atom induced dipole moment under strong field approximation as a source, we suggest a model to simulate the macroscopic high-order harmonic generation (HHG) from the mixed gases (He and Ne) interacting with intense infrared laser by solving the three-dimensional Maxwell's equation of the harmonic field. Regular destructive interference (DI) and constructive interference (CI) are observed in the macroscopic HHG spectra when the gas jet is put at a good phase-matching position. A semiclassical model of short and long electron trajectories is applied to interpret the DI and CI of HHG qualitatively.
基金Supported by the National Natural Science Foundation of China under Grant No 11064002.
文摘The equation of motion of two-level chromium atoms in Gauss standing laser wave is discussed and the distribution of chromium atoms is given under different transverse velocity conditions. The results show that the focusing position of atoms will be affected by the transverse velocity of atoms. Based on the four-order Runge- Kutta method, the locus of chromium atoms in Gauss standing laser wave is simulated. The three-dimensional characteristics of nanometer structures are stimulated under perfect and emanative conditions.
基金Supported by the National Natural Science Foundation of China under Grant No 10705007, and the Doctorial Start-up Foundation of Liaoning Province under Grant No 20071067.
文摘The molecular dynamics (MD) method is used to simulate the interactions of energetic C20 clusters with the dense plasma targets within the framework of the linear Vlasov-Poisson theory. The influences of various clusters (H2, N2, C20 and C60 respectively) on stopping power are discussed. The simulation results show that the vicinage effects in the Coulomb explosion dynamics and the stopping power are strongly affected by the variations in the cluster speed and the plasma parameters. Coulomb explosions are found to proceed faster for higher speeds, lower plasma densities and higher electron temperatures. In addition, the cluster stopping power is strongly enhanced in the early stages of Coulomb explosions due to the vicinage effect, but this enhancement eventually diminishes, after the cluster constituent ions are sufficiently separated. For the large and heavy clusters, the stopping power ratio reaches much higher values in the early stage of Coulomb explosion owing to the constructive interferences in the vicinage effect.
文摘One-dimensional deposition of a neutral chromium atomic beam focused by a near-resonant Gaussian standing- laser field is discussed by using a fourth-order Runge-Kutta type algorithm. The deposition pattern of neutral chromium atoms in a laser standing wave with different laser power is discussed and the simulation result shows that the full width at half maximum (FWHM) of a nanometer stripe is 115nm and the contrast is 2.5:1 with laser power 3.93mW; the FWHM is 0.8nm and the contrast is 27:1 with laser power 16mW, the optimal laser power; but with laser power increasing to 50mW, the nanometer structure forms multi-crests and the quality worsens quickly with increasing laser power.
基金Supported by the National Natural Science Foundation of China under Grand No 10664003.
文摘By using a pump-probe technique, the nascent rotational and vibrational state distributions of CsH are obtained in the Cs(6^2 D,7^2 D) plus H2 reaction. The nascent CsH molecules are found to populate the lowest two vibrational (v″ = 0 and 1) levels of the ground electronic state. By comparing the spectral intensities of the CsH action spectra with those of pertinent Cs atomic fluorescence excitation spectra, the relative reactivity with 1-12 is in an order of6^2D3/2 〉 6^2D5/2 〉 7^2D3/2 〉 7^2D5/2. The rotational temperatures are found to be slightly below the cell temperature. The relative fractions (〈fV〉, 〈fR〉, 〈fT〉) of average energy disposal are derived as (0.2,0.12,0.68), (0.2,0.12,0.68), (0.07,0.04,0.89) and (0.07,0.04,0.89) for the 6^2D3/2, 6^2D5/2, 7^2D3/2 and 7^2D5/2, respectively. The major available energy is released as translation. These results support that the reaction mechanism of Cs(6^2 D,7^2 D) plus 112 is primarily a eollinear abstraction and not an insertion.
基金Project supported by the National Natural Science Foundation of China (Grant No 10574039).
文摘A complex optical model potential modified by incorporating the concept of bonded atom, which takes into consideration the overlapping effect of electron clouds between two atoms in a molecule, is first employed to calculate the total cross sections for electrons scattering from such complex molecules as C2H6, C2F6, C6H6 and C6F6 using the aclditivity rule model at Hartree-Fock level over the energy range from 100 eV to 5000 eV. The total cross sections are quantitatively compared with those obtained by experiments wherever available, and they are in good agreement with each other over a wide energy range. It is shown that the modified potential together with the additivity rule model is completely suitable for the calculation of total cross sections of electrons scattering from such complex molecules as C2H6, C2F6, C6H6 and C6F6 above 200 eV-300 eV.
文摘A diamond-shaped shock wave was created in a helium arcjet plasma. Visi- ble/ultraviolet emission spectroscopy was used to investigate the condition for the formation of stable shocks and to determine characteristics of the plasma. Dependence of the position of the shock front on the gas pressure in the expansion region was investigated. It was found that the shock wave arises from the collision of plasma particles and residual neutral atoms in that region. Continuum and line spectra of neutral helium were measured, from which the electron temper- atures were derived. The electron density was deduced from the Inglis-Teller limit of the He I 2p3p-3d3D series. The temperature and density were found to have almost constant values of 0.2 eV and 8.5x 1013 cm-3, respectively, across the shock front.
文摘We present a simple scheme for the probabilistic generation of the $n$-qubit W state of three-level systems in cavity quantum electrodynamics. Once the W state is prepared, it will be insensitive to the spontaneous emission of atoms due to the fact that only the two degenerate ground states of the three-level atoms are involved. With time evolution of the system, the success probability and the experimental feasibility are also discussed.
基金Supported by the National Natural Science Foundation of China under Grant No 60778005.
文摘We explore the effects of atomic memory on quantum correlations of two-mode light fields from four-wave mixing. A three-level atomic system in A configuration is considered, in which the atomic relaxation times are comparable to or longer than the cavity relaxation times and thus there exists the atomic memory. The quantum correlation spectrum in the output is calculated without the adiabatic elimination of atomic variables. It is shown that the continuous variable entanglement is enhanced over a wide range of the normalized detuning in the intermediate and bad cavity cases compared with the good cavity case. In some situations more significant enhancement occurs at sidebands.
基金Supported by the National Natural Science Foundation of China under No 10834007, and the Key Program of Chinese Academy of Sciences (KJCX2-SW-T12)
文摘The experiment of measuring the spin depolarized time and light storage time in a Rb vapor under different conditions is performed. Typically, these measurements are accomplished in three different containers: atoms in a bare glass cell, atoms in a buffer gas cell, and atoms in a tetracontane (C4oH82) coating cell. The increasing depolarization and storage times are observed in both the buffer gas cell and the tetracontane coating cell. In the latter case, a storage time greater than 400μs is obtained.
基金Supported by the National Natural Science Foundation of China under Grant No 10474028 and 10604021, Specialized Research Fund for the Doctoral Programme of Higher Education of China under Grant No 20040183041, and the Research Fund for the Innovative Project of Jilin University.
文摘Using a linearly polarized, phase-stabilized 3-fs driving pulse of 800 nm central wavelength shape-optimized on its'ascending edge by its an amplitude-reduced pulse irradiating on a superposition state of the helium atom, we demonstrate theoretically the generation of a super strong isolated 176-attosecond pulse in the spectral region of 93-124 eV. The unusually high intensity of this attosecond pulse is marked by the Rabi-like oscillations emerging in the time-dependent populations of the ground state and the continuum during the occurrence of the electron recombination, which is for the first time observed in this work.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10674020 and 10878008, Science and Technology Funds of CAEP (2008A0102005 and 2009A0102006), and the National High-Technology ICF Committee of China.
文摘The formulae of photon angular distribution and polarization degree for radiative recombination are presented to include the contribution of multipoles and their correlations. A fully relativistic code is then developed to calculate the photon angular distribution and polarization. The calculated polarization degree and differential cross-sections agree well with that of Scofild's results within 10%. The effects of multipoles on polarization and angular distribution are investigated. The polarization and the angular distribution become asymmetric when the multipoles are accounted as the electron energy increases.