Research of caged dynamics of clusters center atoms in Pd_(82)Si_(18) amorphous alloy

To date,there is still a lack of a comprehensive explanation for caged dynamics which is regarded as one of the intricate dynamic behaviors in amorphous alloys.This study focuses on Pd_(82)Si_(18)as the research object to further elucidate the underlying mechanism of caged dynamics from multiple perspectives,including the cage's lifetime,atomic local environment,and atomic potential energy.The results reveal that Si atoms exhibit a pronounced cage effect due to the hindrance of Pd atoms,resulting in an anomalous peak in the non-Gaussian parameters.An in-depth investigation was conducted on the caged dynamics differences between fast and slow Si atoms.In comparison to fast Si atoms,slow Si atoms were surrounded by more Pd atoms and occupied lower potential energy states,resulting in smaller diffusion displacements for the slow Si atoms.Concurrently,slow Si atoms tend to be in the centers of smaller clusters with coordination numbers of 9 and 10.During the isothermal relaxation process,clusters with coordination numbers 9 and 10 have longer lifetimes,suggesting that the escape of slow Si atoms from their cages is more challenging.The findings mentioned above hold significant implications for understanding the caged dynamics.

Efficient loading of cesium atoms in a magnetic levitated dimple trap

We report a detailed study of magnetically levitated loading of ultracold ^(133)Cs atoms in a dimple trap.The atomic sample was produced in a combined red-detuned optical dipole trap and dimple trap formed by two small waist beams crossing a horizontal plane.The magnetic levitation for the ^(133)Cs atoms forms an effective potential for a large number of atoms in a high spatial density.Dependence of the number of atoms loaded and trapped in the dimple trap on the magnetic field gradient and bias field is in good agreement with the theoretical analysis.This method has been widely used to obtain the Bose–Einstein condensation atoms for many atomic species.

Simulation of space heavy-ion induced primary knock-on atoms in bipolar devices

Bipolar junction transistors(BJTs) are often used in spacecraft due to their excellent working characteristics. However,the complex space radiation environment induces primary knock-on atoms(PKAs) in BJTs through collisions, resulting in hard-to-recover displacement damage and affecting the performance of electronic components. In this paper, the properties of PKAs induced by typical space heavy ions(C, N, O, Fe) in BJTs are investigated using Monte Carlo simulations. The simulated results show that the energy spectrum of ion-induced PKAs is primarily concentrated in the low-energy range(17eV–100eV) and displays similar features across all tested ions. The PKAs induced by the collision of energetic ions have large forward scattering angles, mainly around 88°. Moreover, the distribution of PKAs within a transistor as a function of depth displays a peak characteristic, and the peak position is linearly proportional to the incident energy at a certain energy range. These simulation outcomes serve as crucial theoretical support for long-term semiconductor material defect evolution and ground testing of semiconductor devices.

Improved Plasmonic Hot‑Electron Capture in Au Nanoparticle/Polymeric Carbon Nitride by Pt Single Atoms for Broad‑Spectrum Photocatalytic H_(2)Evolution

ABSTRACT Rationally designing broad-spectrum photocatalysts to harvest whole visible-light region photons and enhance solar energy conversion is a“holy grail”for researchers,but is still a challenging issue.Herein,based on the common polymeric carbon nitride(PCN),a hybrid co-catalysts system comprising plasmonic Au nanoparticles(NPs)and atomically dispersed Pt single atoms(PtSAs)with different functions was constructed to address this challenge.For the dual co-catalysts decorated PCN(PtSAs–Au_(2.5)/PCN),the PCN is photoexcited to generate electrons under UV and short-wavelength visible light,and the synergetic Au NPs and PtSAs not only accelerate charge separation and transfer though Schottky junctions and metal-support bond but also act as the co-catalysts for H_(2) evolution.Furthermore,the Au NPs absorb long-wavelength visible light owing to its localized surface plasmon resonance,and the adjacent PtSAs trap the plasmonic hot-electrons for H_(2) evolution via direct electron transfer effect.Consequently,the PtSAs–Au_(2.5)/PCN exhibits excellent broad-spectrum photocatalytic H_(2) evolution activity with the H_(2) evolution rate of 8.8 mmol g^(−1) h^(−1) at 420 nm and 264μmol g^(−1) h^(−1) at 550 nm,much higher than that of Au_(2.5)/PCN and PtSAs–PCN,respectively.This work provides a new strategy to design broad-spectrum photocatalysts for energy conversion reaction.

Fine and hyperfine structures of pionic helium atoms

The fine and hyperfine structures of pionic helium metastable states is calculated within the formalism of the Breit-Pauli Hamiltonian by using the variationally generated wave functions in Hylleraas coordinates.Our results not only verify the existing values of Hori et al.[Phys.Rev.A 89,042515(2014)]for the fine structure of π^(4)He^(+),but also determine the hyperfine structure of π^(3)He^(+).

High efficient Raman sideband cooling and strong three-body recombination of atoms

We report a highly efficient three-dimensional degenerated Raman sideband cooling(3D dRSC)that enhances the loading of a magnetically levitated optical dipole trap,and observe the strong atom loss due to the three-body recombination.The 3D dRSC is implemented to obtain 5×10^(7)Cs atoms with the temperature of~480 nK.The cold temperature enables 1.8×10^(7)atoms loaded into a crossed dipole trap with an optimized excessive levitation magnetic gradient.Compared to the loading of atoms from a bare magneto-optical trap or the gray-molasses cooling,there is a significant increase in the number of atoms loaded into the optical dipole trap.We derive for the three-body recombination coefficient of L_(3)=7.73×10^(-25)cm^(6)/s by analyzing the strong atom loss at a large scattering length of 1418 Bohr radius,and discover the transition from the strong three-body loss to the dominant one-body loss.Our result indicates that the lifetime of atoms in the optical dipole trap is finally decided by the one-body loss after the initial strong three-body loss.

Investigation of cyclohexane catalytic degradation driven by N atoms from N_(2)discharges

The effect of N_(2)discharge products on cyclohexane degradation over a MnO_(2)/γ-Al_(2)O_(3)catalyst has been evaluated by feeding N_(2)discharge products to the catalyst using a specially designed dielectric barrier discharge reactor.At a reaction temperature of 100℃,the cyclohexane conversion increased from 2.46%(without N_(2)discharge products)to 26.3%(with N_(2)discharge products).N-and O-containing by-product(3,4-dehydroproline)was found on the catalyst surface using gas chromatograph-mass spectrometry identification,in which C=N–C and C=N–H bonds were also confirmed from x-ray photoelectron spectroscopy analysis results.Operando analysis results using diffuse reflectance infrared Fourier transform spectroscopy revealed that N atoms can react with surface H_(2)O possibly to NH and OH reactive species that have reactivities to promote CO oxidation to CO_(2).The mechanism of N-atom-driven cyclohexane degradation to CO and CO_(2)is proposed.

Electric field intensity measurement by using doublet electromagnetically induced transparency of cold Rb Rydberg atoms

We demonstrate a simple method to measure electric field intensity by using doublet electromagnetically induced transparency(EIT) spectra of cold Rb Rydberg atoms, where the frequency of the coupling laser does not need to be locked. Based on the Stark splitting of the Rb Rydberg state, 10D_(3/2), under electric fields and the corresponding calculated polarizabilities, the real electric field intensity is calculated using the difference in radio-frequency diffraction between two acousto-optic modulators, which acts as a frequency criterion that allows us to measure the electrical field without locking the coupling laser. The value measured by this simple method shows a good agreement with our previous work [Opt.Express 29 1558(2021)] where the frequency of the coupling laser needs to be locked with an additional EIT spectrum based on atom vapor and a proportional–integral–differential feedback circuit. Our presented method can also be extended to the measurement of electric field based on hot Rydberg atom vapor, which has application in industry.

Experimental Realization of Degenerate Fermi Gases of 87Sr Atoms with 10 or Two Spin Components

We report the experimental realization of quantum degenerate Fermi gases of87Sr atoms under controlled 10-and dual-nuclear-spin configurations.Based on laser cooling and evaporative cooling,we achieve an ultracold Fermi gas of 105 atoms equally distributed over 10 spin states,with a temperature of T/TF = 0.21.We further prepare a dual-spin gas by optically pumping atoms to the mF = 9/2 and mF = 7/2 states and observe a slightly lower T/TF than that for a 10-spin gas under the same trapping condition,showing efficient evaporative cooling under a decreasing number N of spin states(N≥2)despite the increasing importance of Pauli exclusion.Given that rethermalization becomes less efficient with N approaching unity,we evaporatively cool an almost polarized gas to 130 nK.The simple and efficient preparation of ultracold Fermi gases of 87Sr with tunable spin configurations provides a first step towards engineering topological quantum systems.

Erratum and Note: Measurement of Zeeman Shift of Cesium Atoms Using an Optical Nanofiber [Chin. Phys. Lett. 35(2018) 083201]

Our recent article (Chin. Phys. Lett. 35 (2018)083201) measured the Zeeman shift of cesium atoms using an optical nanofiber. Before our work, Watkins et al.(Ref.[17] in our article) had demonstrated the Zeeman shift also using an optical nanofiber in rubidium atoms. Watkins et al. reported on the

Study of optical clocks based on ultracold ^171Yb atoms

The optical atomic clocks have the potential to transform global timekeeping,relying on the state-of-the-art accuracy and stability,and greatly improve the measurement precision for a wide range of scientific and technological applications.Herein we report on the development of the optical clock based on 171Yb atoms confined in an optical lattice.A minimum width of 1.92-Hz Rabi spectra has been obtained with a new 578-nm clock interrogation laser.The in-loop fractional instability of the 171Yb clock reaches 9.1×10-18 after an averaging over a time of 2.0×104 s.By synchronous comparison between two clocks,we demonstrate that our 171Yb optical lattice clock achieves a fractional instability of 4.60×10-16/√τ.

Highly sensitive detection of Rydberg atoms with fluorescence loss spectrum in cold atoms

Fluorescence loss spectrum for detecting cold Rydberg atoms with high sensitivity has been obtained based on lock-in detection of fluorescence of 6 P3/2 state when cooling lasers of the magneto-optical trap are modulated.The experiment results show that the signal to noise ratio has been improved by 32.64 dB when the modulation depth(converted to laser frequency)and frequency are optimized to 4 MHz and 6 kHz,respectively.This technique enables us to perform a highly sensitive non-destructive detection of Rydberg atoms.

Magnetism of Metals, Alloys and of Clusters of Transition Metal Atoms

A condition for local moment formation in metals derived by Stoddart and March (Ann. Phys. NY 1972 64, 174) is first used to discuss the ferromagnetism of body-centred-cubic Fe. A less detailed discussion is also added on Ni and Co. This leads into a treatment of the non- linear response of such 3d ferromagnets to dilute substitutional impurities. Antiferromagnets responding to local changes in the exchange field caused by such impurities are also studied, Mn in Cr being one such system discussed. The paper concludes with a brief summary of clusters of transition metal atoms, with most attention devoted to Cr and to Mn.

Entanglement and Quantum Discord of Two Moving Atoms

In this paper we discuss two measures for the quantumness of correlations (quantum discord and entanglement) of two isolated moving atoms which are initially in Werner state. We compare and analyze the effect of the atomic motion in quantum discord and entanglement. The results show that the atomic motion related to the field mode structure parameter can make the entanglement and quantum discord evolve periodically. The results also indicate that the entanglement suddenly disappears during the evaluation but quantum discord remains non zero, so quantum discord is considered as indicator of disentanglement.

Ionization of Atoms and the Thomas-Fermi Model for the Electric Field in Crystal Planar Channels

The electric field in the crystal planar channels is studied by the Thomas Fermi method. The Thomas-Fermi equation and the corresponding boundary conditions are derived for the crystal planar channels. The numericalsolution for the electric field in the channels between (110) planes of the single crystal silicon and the critical angles ofchannelling protons in them are shown. Reasonable agreements with the experimental data are obtained. The resultsshow that the Thomas-Fermi method for the crystal works well in this study, and a microscopic research of the channelelectric field with the contribution of all atoms and the atomic ionization being taken into account is practical.

ACCELERATOR-BASED ATOMIC PHYSICS AT THE LAWRENCE BERKELEY LABORATOTY:COLLISIONS OF FAST,HIGHLY-CHARGED IONS WITH ATOMS

Research on accelerator-based atomic physics at the Lawrence Berkeley Laboratory super-HILAC and Bevalac accelerators is described. This research covers several important topics in collisions of fast, highly charged ions with atoms: charge transfer, ionization, and excitation. Multiple - electron processes are emphasized. Electron correlation is important in some of these processes, e.g., resonance transfer and excitation (RTE) multiple-electron capture in close collisions. A variety of experiments and results for energies from 1 to 420 MeV/u are presented.

Intrinsic transverse relaxation mechanisms of polarized alkali atoms enclosed in radio-frequency magnetometer cell

The intrinsic transverse relaxation mechanisms of polarized alkali atoms enclosed in the radio-frequency magnetometer cell are investigated.The intrinsic transverse relaxation rate of cesium atoms as a function of cell temperature is obtained.The absorption of alkali atoms by the glass wall and the reservoir effect are the main error factors which contribute to the disagreements between theory and experiments.A modified relaxation model is presented, in which both the absorption of alkali atoms by the glass wall and the reservoir effect are included.This study provides a more accurate description of the intrinsic transverse relaxation mechanisms of polarized alkali atoms, and enlightens the optimization of the cell design.

Insight into the Relationship Between Local Coordination of Isolated Pt Atoms and Chemical Reactivity

The supported isolated Pt atoms(Pt iso)and other rare metals have attracted intensive concern due to their maximized metal utilization efficiency,unique reactivity or selectivity,connection to organometallic catalysis and the potential for making well-defined active sites[1-3].As catalytic active sites,oxide-supported isolated Pt-group metal atoms are well known for their unique reactivity and efficient metal utilization[4-6].Even continuous efforts have been made,it is still challenging to characterize the intrinsic ca-talytic activity of these dispersed active sites on oxide supports at a level that relates local electronic and geometric structure to function,because of their atomic dispersion,heterogeneity in the local coordination,dynamic changes in local coordination under reactive environments and low loading of metal[7-9].

Strange Attractors in the Resonance Interaction of Two-State Atoms with Single-Mode Laser Field

The resonance Interaction or two-state atoms with single mode rleld is described theoretically byusing the semi-classical theory and Jaynes-Cummings model. The nonlinear characteristics of this system arecalculated by using FFT and Runge-Kutta methods. The chaotic strange attractors in this system are obtainedfrom the numerical results.