Increasing energy consumption in the transportation sector results in challenging greenhouse gas(GHG)emissions and environmental problems.This paper involved integrated assessments on GHG emissions and emergy of the l...Increasing energy consumption in the transportation sector results in challenging greenhouse gas(GHG)emissions and environmental problems.This paper involved integrated assessments on GHG emissions and emergy of the life cycle for the internal combustion engine(ICE)and electric automobiles in the USA over the entire assumed fifteen-year lifetime.The hotspots of GHG emissions as well as emergy indices for the major processes of automobile life cycle within the defined system boundaries have been investigated.The potential strategies for reducing GHG emissions and emergy in the life cycle of both ICE and electric automobiles were further proposed.Based on the current results,the total GHG emissions from the life cycle of ICE automobiles are 4.48 E+07 kg CO2-e which is320 times higher than that of the electric automobiles.The hotspot area of the GHG emissions from ICE and electric automobiles are operation phase and manufacturing process,respectively.Interesting results were observed that comparable total emergy of the ICE automobiles and electric automobiles have been calculated which were 1.54 E+17 and 2.20 E+17 sej,respectively.Analysis on emergy index evidenced a better environmental sustainability of electric automobiles than ICE automobiles over the life cycle due to its higher ESI.To the authors’knowledge,it is the first time to integrate the analysis of GHG emissions together with emergy in industrial area of automobile engineering.It is expected that the integration of emergy and GHG emissions analysis may provide a comprehensive perspective on eco-industrial sustainability of automobile engineering.展开更多
Automobile exhaust contributes the largest sources of carbon monoxide(CO)into the environment.To control this CO pollution,the catalytic converters have been discovered.The catalytic converters have been invented for ...Automobile exhaust contributes the largest sources of carbon monoxide(CO)into the environment.To control this CO pollution,the catalytic converters have been discovered.The catalytic converters have been invented for regulating the CO discharge.There are many types of catalysts have been investigated for CO emission control purposes.Inorganic perovskite-type oxides are fascinating nanomaterials for wide applications in catalysis,fuel cells,and electrochemical sensing.Perovskites prepared in the nanoscale have recently received more attention due to their catalytic nature when used as electrode modifiers.Perovskite catalysts show great potential for CO oxidation catalyst in a catalytic converter for their low cost,high thermal stability and tailoring flexibility.It is active for CO oxidation at a lower temperature.The catalytic activity of these oxides is higher than that of many transition metals compounds and even some precious metal oxides.They represents attractive physical and chemical characteristics such as electronic conductivity,electrically active structure,the oxide ions mobility through the crystal lattice,variations on the content of the oxygen,thermal and chemical stability,and supermagnetic,photocatalytic,thermoelectric and dielectric properties.The surface sites and lattice oxygen species present in perovskite catalysts play an important role in chemical transformations.The partial replacement of cations A and B by different elements,which changes the atomic distance,causes unit cell disturbances,stabilizes various oxidation states or added cationic or anionic vacancies inside the lattice.The novel things disturb the solid reactivity by varying the reaction mechanism on the catalyst surface.Thus,the better cations replacement may represent more activity.There are lots of papers available to CO oxidation over perovskite catalysts but no review paper available in the literature that is represented to CO oxidation.展开更多
基金financially supported by National Natural Science Foundation for Young Scientists of China(Grant No.51608531)
文摘Increasing energy consumption in the transportation sector results in challenging greenhouse gas(GHG)emissions and environmental problems.This paper involved integrated assessments on GHG emissions and emergy of the life cycle for the internal combustion engine(ICE)and electric automobiles in the USA over the entire assumed fifteen-year lifetime.The hotspots of GHG emissions as well as emergy indices for the major processes of automobile life cycle within the defined system boundaries have been investigated.The potential strategies for reducing GHG emissions and emergy in the life cycle of both ICE and electric automobiles were further proposed.Based on the current results,the total GHG emissions from the life cycle of ICE automobiles are 4.48 E+07 kg CO2-e which is320 times higher than that of the electric automobiles.The hotspot area of the GHG emissions from ICE and electric automobiles are operation phase and manufacturing process,respectively.Interesting results were observed that comparable total emergy of the ICE automobiles and electric automobiles have been calculated which were 1.54 E+17 and 2.20 E+17 sej,respectively.Analysis on emergy index evidenced a better environmental sustainability of electric automobiles than ICE automobiles over the life cycle due to its higher ESI.To the authors’knowledge,it is the first time to integrate the analysis of GHG emissions together with emergy in industrial area of automobile engineering.It is expected that the integration of emergy and GHG emissions analysis may provide a comprehensive perspective on eco-industrial sustainability of automobile engineering.
文摘Automobile exhaust contributes the largest sources of carbon monoxide(CO)into the environment.To control this CO pollution,the catalytic converters have been discovered.The catalytic converters have been invented for regulating the CO discharge.There are many types of catalysts have been investigated for CO emission control purposes.Inorganic perovskite-type oxides are fascinating nanomaterials for wide applications in catalysis,fuel cells,and electrochemical sensing.Perovskites prepared in the nanoscale have recently received more attention due to their catalytic nature when used as electrode modifiers.Perovskite catalysts show great potential for CO oxidation catalyst in a catalytic converter for their low cost,high thermal stability and tailoring flexibility.It is active for CO oxidation at a lower temperature.The catalytic activity of these oxides is higher than that of many transition metals compounds and even some precious metal oxides.They represents attractive physical and chemical characteristics such as electronic conductivity,electrically active structure,the oxide ions mobility through the crystal lattice,variations on the content of the oxygen,thermal and chemical stability,and supermagnetic,photocatalytic,thermoelectric and dielectric properties.The surface sites and lattice oxygen species present in perovskite catalysts play an important role in chemical transformations.The partial replacement of cations A and B by different elements,which changes the atomic distance,causes unit cell disturbances,stabilizes various oxidation states or added cationic or anionic vacancies inside the lattice.The novel things disturb the solid reactivity by varying the reaction mechanism on the catalyst surface.Thus,the better cations replacement may represent more activity.There are lots of papers available to CO oxidation over perovskite catalysts but no review paper available in the literature that is represented to CO oxidation.