With the global ambition of moving towards carbon neutrality,this sets to increase significantly with most of the energy sources from renewables.As a result,cost-effective and resource efficient energy conversion and ...With the global ambition of moving towards carbon neutrality,this sets to increase significantly with most of the energy sources from renewables.As a result,cost-effective and resource efficient energy conversion and storage will have a great role to play in energy decarbonization.This review focuses on the most recent developments of one of the most promising energy conversion and storage technologies-the calcium-looping.It includes the basics and barriers of calcium-looping beyond CO_(2) capture and storage(CCS)and technological solutions to address the associated challenges from material to system.Specifically,this paper discusses the flexibility of calcium-looping in the context of CO_(2) capture,combined with the use of H_(2)-rich fuel gas conversion and thermochemical heat storage.To take advantage of calcium-looping based energy integrated utilization of CCS(EIUCCS)in carbon neutral power generation,multiple-scale process innovations will be required,starting from the material level and extending to the system level.展开更多
Cigarette butts(CBs)are one of the most common types of litter in the world.Due to the toxic substances they contain,the waste generated poses a harmful risk to the environment,and therefore there is an urgent need fo...Cigarette butts(CBs)are one of the most common types of litter in the world.Due to the toxic substances they contain,the waste generated poses a harmful risk to the environment,and therefore there is an urgent need for alternative solutions to landfill storage.Thus,this work presents a possible revalorization of this waste material,which implies interesting environmental benefits.CBs were used as sacrificial templates for the preparation of CaO-based materials by impregnation with calcium and magnesium nitrates followed by flaming combustion.These materials presented enhanced porosity for their use in the Calcium Looping process applied either to thermochemical energy storage or CO_(2)capture applications.The influence of the concentration of Ca and Mg in the impregnating solutions on the multicycle reactivity of the samples was studied.An improved multicycle performance was obtained in terms of conversion for both applications.展开更多
基金supported by the National Science Fund for Distinguished Young Scholars[51925604]the National Natural Science Foundation of China[52176210,51820105010]+1 种基金the Bureau of International Cooperation of Chinese Academy of Sciences[182211KYSB20170029]the Cooperation Foundation of Dalian National Laboratory for Clean Energy[DNL202017].
文摘With the global ambition of moving towards carbon neutrality,this sets to increase significantly with most of the energy sources from renewables.As a result,cost-effective and resource efficient energy conversion and storage will have a great role to play in energy decarbonization.This review focuses on the most recent developments of one of the most promising energy conversion and storage technologies-the calcium-looping.It includes the basics and barriers of calcium-looping beyond CO_(2) capture and storage(CCS)and technological solutions to address the associated challenges from material to system.Specifically,this paper discusses the flexibility of calcium-looping in the context of CO_(2) capture,combined with the use of H_(2)-rich fuel gas conversion and thermochemical heat storage.To take advantage of calcium-looping based energy integrated utilization of CCS(EIUCCS)in carbon neutral power generation,multiple-scale process innovations will be required,starting from the material level and extending to the system level.
基金supported by MCIN/AEI/10.13039/501100011033 and European Union Next Generation EU/PRTR(Nos.PDC2021121552-C21 and PID2022-140815OB-C22)Ministerio de Ciencia e Innovación(No.TED2021-131839B-C22)+1 种基金the Spanish Government Agency Ministerio de Ciencia,Innovación y Universidades(No.PRE2018-085866)the APOSTD program co-funded by ESF Investing in your future(No.CIAPOS/2021/67)。
文摘Cigarette butts(CBs)are one of the most common types of litter in the world.Due to the toxic substances they contain,the waste generated poses a harmful risk to the environment,and therefore there is an urgent need for alternative solutions to landfill storage.Thus,this work presents a possible revalorization of this waste material,which implies interesting environmental benefits.CBs were used as sacrificial templates for the preparation of CaO-based materials by impregnation with calcium and magnesium nitrates followed by flaming combustion.These materials presented enhanced porosity for their use in the Calcium Looping process applied either to thermochemical energy storage or CO_(2)capture applications.The influence of the concentration of Ca and Mg in the impregnating solutions on the multicycle reactivity of the samples was studied.An improved multicycle performance was obtained in terms of conversion for both applications.
