In this study, regional persistent haze events(RPHEs) in the Beijing–Tianjin–Hebei(BTH) region were identified based on the Objective Identification Technique for Regional Extreme Events for the period 1980–201...In this study, regional persistent haze events(RPHEs) in the Beijing–Tianjin–Hebei(BTH) region were identified based on the Objective Identification Technique for Regional Extreme Events for the period 1980–2013. The formation mechanisms of the severe RPHEs were investigated with focus on the atmospheric circulation and dynamic mechanisms. Results indicated that:(1) 49 RPHEs occurred during the past 34 years.(2) The severe RPHEs could be categorized into two types according to the large-scale circulation, i.e. the zonal westerly airflow(ZWA) type and the high-pressure ridge(HPR) type. When the ZWA-type RPHEs occurred, the BTH region was controlled by near zonal westerly airflow in the mid–upper troposphere.Southwesterly winds prevailed in the lower troposphere, and near-surface wind speeds were only 1–2 ms^-1. Warm and humid air originating from the northwestern Pacific was transported into the region, where the relative humidity was 70% to 80%, creating favorable moisture conditions. When the HPR-type RPHEs appeared, northwesterly airflow in the mid–upper troposphere controlled the region. Westerly winds prevailed in the lower troposphere and the moisture conditions were relatively weak.(3) Descending motion in the mid-lower troposphere caused by the above two circulation types provided a crucial dynamic mechanism for the formation of the two types of RPHEs. The descending motion contributed to a reduction in the height of the planetary boundary layer(PBL), which generated an inversion in the lower troposphere. This inversion trapped the abundant pollution and moisture in the lower PBL, leading to high concentrations of pollutants.展开更多
In this paper, the relation between Asian summer monsoon circulation and sea surface temperature anomalies over equatorial central-eastern Pacific is investigated by using a global spectral model. This model has nine ...In this paper, the relation between Asian summer monsoon circulation and sea surface temperature anomalies over equatorial central-eastern Pacific is investigated by using a global spectral model. This model has nine layers in the vertical and the model variables are represented in the horizontal as truncated expansions of the surface spherical harmonics with rhomboidal truncation at wave number 15. The model involves comparatively complete physical processes and parameterizations with mountains.Using the above model, two experimental schemes are designed, namely control case and anomalous sea surface temperature case. The above two schemes are respectively integrated for forty days and the simulated results are obtained from the last 30-day averaged simulations.The simulations show that positive SST anomalies over equatorial central-eastern Pacific weakens Indian monsoon circulation,decreases precipitation in Indian sub-continent whereas it intensifies East Asian monsoon circulation and increases precipitation in East Asian area. All these results reflect the characteristics of Asian summer monsoon during the El Nino period. In this paper, SST anomalies over equatorial central-eastern Pacific have a direct influence on the intensity and position of subtropical high via the wave train over Northern Hemisphere, which is similar to that suggested by Nitta(1987) and the wave train over Southern Hemisphere has an influence on the intensity of Muscarene high and Australia high resulting in affecting cross equatorial flow. As a result, atmospheric interior heat sources and sinks are redistributed because of the change of cross equatorial flow. And the response of atmosphere to the new heat source and sink has a significant influence on Asian summer monsoon.展开更多
By reviewing the mechanisms of drilling fluid lost circulation and its control in fractured formations, the applicability and working mechanisms of different kinds of lost circulation materials in plugging fractured f...By reviewing the mechanisms of drilling fluid lost circulation and its control in fractured formations, the applicability and working mechanisms of different kinds of lost circulation materials in plugging fractured formations have been summarized. Meanwhile, based on the types of lost circulation materials, the advantages, disadvantages, and application effects of corresponding plugging technologies have been analyzed to sort out the key problems existing in the current lost circulation control technologies. On this basis, the development direction of plugging technology for severe loss have been pointed out. It is suggested that that the lost circulation control technology should combine different disciplines such as geology, engineering and materials to realize integration, intelligence and systematization in the future. Five research aspects should be focused on:(1) the study on mechanisms of drilling fluid lost circulation and its control to provide basis for scientific selection of lost circulation material formulas, control methods and processes;(2) the research and development of self-adaptive lost circulation materials to improve the matching relationship between lost control materials and fracture scales;(3) the research and development of lost circulation materials with strong retention and strong filling in three-dimensional fracture space, to enhance the retention and filling capacities of materials in fractures and improve the lost circulation control effect;(4) the research and development of lost circulation materials with high temperature tolerance, to ensure the long-term plugging effect of deep high-temperature formations;(5) the study on digital and intelligent lost circulation control technology, to promote the development of lost circulation control technology to digital and intelligent direction.展开更多
In order to further improve the catalytic performance of zeolite catalyst for methanol to aromatics(MTA)technology, the double-tier SAPO-34/ZSM-5/quartz composite zeolite films were successfully synthesized via hydrot...In order to further improve the catalytic performance of zeolite catalyst for methanol to aromatics(MTA)technology, the double-tier SAPO-34/ZSM-5/quartz composite zeolite films were successfully synthesized via hydrothermal crystallization. The Si/Al ratio of SAPO-34 film was used as the only variable to study this material. The composite zeolite material with 0.6Si/Al ratio of SAPO-34 has the largest mesoporous specific surface area and the most suitable acid distribution. The catalytic performance for the MTA process showed that 0.6-SAPO-34/ZSM-5/quartz film has as high as 50.3% benzene-toluenexylene selectivity and 670 min lifetime. The MTA reaction is carried out through the path we designed to effectively avoid the hydrocarbon pool circulation of ZSM-5 zeolite, so as to improve the aromatics selectivity and inhibit the occurrence of deep side reactions to a great extent. The coke deposition behavior was monitored by thermogravimetric analysis and gas chromatograph/mass spectrometer, it is found that with the increase of Si/Al ratio, the active intermediates changed from low-substituted methylbenzene to high-substituted methylbenzene, which led to the rapid deactivation of the catalyst. This work provides a possibility to employ the synergy effect of composite zeolite film synthesizing anti-carbon deposition catalyst in MTA reaction.展开更多
The propagation and underlying mechanisms of the boreal summer quasi-biweekly oscillation(QBWO)over the entire Asian monsoon region are investigated,based on ECMWF Interim reanalysis(ERA-Interim)data,GPCP precipit...The propagation and underlying mechanisms of the boreal summer quasi-biweekly oscillation(QBWO)over the entire Asian monsoon region are investigated,based on ECMWF Interim reanalysis(ERA-Interim)data,GPCP precipitation data,and an atmospheric general circulation model(AGCM).Statistical analyses indicate that the QBWO over the Asian monsoon region derives its main origin from the equatorial western Pacific and moves northwestward to the Bay of Bengal and northern India,and then northward to the Tibetan Plateau(TP)area,with a baroclinic vertical structure.Northward propagation of the QBWO is promoted by three main mechanisms:barotropic vorticity,boundary moisture advection,and surface sensible heating(SSH).It is dominated by the barotropic vorticity effect when the QBWO signals are situated to the south of 20°N.During the propagation taking place farther north toward the TP,the boundary moisture advection and SSH are the leading mechanisms.We use an AGCM to verify the importance of SSH on the northward propagation of the QBWO.Numerical simulations confirm the diagnostic conclusion that the equatorial western Pacific is the source of the QBWO.Importantly,the model can accurately simulate the propagation pathway of the QBWO signals over the Asian monsoon region.Simultaneously,sensitivity experiments demonstrate that the SSH over northern India and the southern slope of the TP greatly contributes to the northward propagation of the QBWO as far as the TP area.展开更多
The present work is intended to simulate, in a rotating annulus of stratified liquid, the me-chanical effect of the Xizang (Tibetan) Plateau on the zonal circulation. The main featuresof three flow patterns around the...The present work is intended to simulate, in a rotating annulus of stratified liquid, the me-chanical effect of the Xizang (Tibetan) Plateau on the zonal circulation. The main featuresof three flow patterns around the plateau for different Rossby number R and rotating Eulernumber E are analysed. and a division diagram of the flow pattern in (R, E) plane is given.It has been found that under the condition that similarity criterions R and E of the experimentalfluid are the same as those existing in the atmosphere for monthly mean states in spring, au-tumn and winter months, the experimental results are satisfied for the following weathersystems over the plateau and its vicinities: the low vortex, trough and shear line over thesoutheast part of the plateau, the tilted ridge over the northwest part of the plateau, the troughpatterns over the upstream and dewnstream of the plateau, the vertical circulation structure, thejets on both north and southeast sides of the plateau, and so on. This shows that the展开更多
基金jointly sponsored by the National Basic Research Program of China(973 Program)(Grant No.2013CB430202)the National Natural Science Foundation of China(Grant No.41401056)+1 种基金the China Meteorological Administration Special Public Welfare Research Fund(Grant No.GYHY201406001)the Research Innovation Program for College Graduates of Jiangsu Province(Grant No.KYLX15 0858)
文摘In this study, regional persistent haze events(RPHEs) in the Beijing–Tianjin–Hebei(BTH) region were identified based on the Objective Identification Technique for Regional Extreme Events for the period 1980–2013. The formation mechanisms of the severe RPHEs were investigated with focus on the atmospheric circulation and dynamic mechanisms. Results indicated that:(1) 49 RPHEs occurred during the past 34 years.(2) The severe RPHEs could be categorized into two types according to the large-scale circulation, i.e. the zonal westerly airflow(ZWA) type and the high-pressure ridge(HPR) type. When the ZWA-type RPHEs occurred, the BTH region was controlled by near zonal westerly airflow in the mid–upper troposphere.Southwesterly winds prevailed in the lower troposphere, and near-surface wind speeds were only 1–2 ms^-1. Warm and humid air originating from the northwestern Pacific was transported into the region, where the relative humidity was 70% to 80%, creating favorable moisture conditions. When the HPR-type RPHEs appeared, northwesterly airflow in the mid–upper troposphere controlled the region. Westerly winds prevailed in the lower troposphere and the moisture conditions were relatively weak.(3) Descending motion in the mid-lower troposphere caused by the above two circulation types provided a crucial dynamic mechanism for the formation of the two types of RPHEs. The descending motion contributed to a reduction in the height of the planetary boundary layer(PBL), which generated an inversion in the lower troposphere. This inversion trapped the abundant pollution and moisture in the lower PBL, leading to high concentrations of pollutants.
文摘In this paper, the relation between Asian summer monsoon circulation and sea surface temperature anomalies over equatorial central-eastern Pacific is investigated by using a global spectral model. This model has nine layers in the vertical and the model variables are represented in the horizontal as truncated expansions of the surface spherical harmonics with rhomboidal truncation at wave number 15. The model involves comparatively complete physical processes and parameterizations with mountains.Using the above model, two experimental schemes are designed, namely control case and anomalous sea surface temperature case. The above two schemes are respectively integrated for forty days and the simulated results are obtained from the last 30-day averaged simulations.The simulations show that positive SST anomalies over equatorial central-eastern Pacific weakens Indian monsoon circulation,decreases precipitation in Indian sub-continent whereas it intensifies East Asian monsoon circulation and increases precipitation in East Asian area. All these results reflect the characteristics of Asian summer monsoon during the El Nino period. In this paper, SST anomalies over equatorial central-eastern Pacific have a direct influence on the intensity and position of subtropical high via the wave train over Northern Hemisphere, which is similar to that suggested by Nitta(1987) and the wave train over Southern Hemisphere has an influence on the intensity of Muscarene high and Australia high resulting in affecting cross equatorial flow. As a result, atmospheric interior heat sources and sinks are redistributed because of the change of cross equatorial flow. And the response of atmosphere to the new heat source and sink has a significant influence on Asian summer monsoon.
基金Supported by National Natural Science Foundation of China(51991361,52074327,U1762212)Major Engineering Technology Field Tes Project of CNPC(2020F-45)。
文摘By reviewing the mechanisms of drilling fluid lost circulation and its control in fractured formations, the applicability and working mechanisms of different kinds of lost circulation materials in plugging fractured formations have been summarized. Meanwhile, based on the types of lost circulation materials, the advantages, disadvantages, and application effects of corresponding plugging technologies have been analyzed to sort out the key problems existing in the current lost circulation control technologies. On this basis, the development direction of plugging technology for severe loss have been pointed out. It is suggested that that the lost circulation control technology should combine different disciplines such as geology, engineering and materials to realize integration, intelligence and systematization in the future. Five research aspects should be focused on:(1) the study on mechanisms of drilling fluid lost circulation and its control to provide basis for scientific selection of lost circulation material formulas, control methods and processes;(2) the research and development of self-adaptive lost circulation materials to improve the matching relationship between lost control materials and fracture scales;(3) the research and development of lost circulation materials with strong retention and strong filling in three-dimensional fracture space, to enhance the retention and filling capacities of materials in fractures and improve the lost circulation control effect;(4) the research and development of lost circulation materials with high temperature tolerance, to ensure the long-term plugging effect of deep high-temperature formations;(5) the study on digital and intelligent lost circulation control technology, to promote the development of lost circulation control technology to digital and intelligent direction.
基金supported by the National Natural Science Foundation of China (51974312, 51974308)the National Key Research & Development Program of China (2019YFE0100100)。
文摘In order to further improve the catalytic performance of zeolite catalyst for methanol to aromatics(MTA)technology, the double-tier SAPO-34/ZSM-5/quartz composite zeolite films were successfully synthesized via hydrothermal crystallization. The Si/Al ratio of SAPO-34 film was used as the only variable to study this material. The composite zeolite material with 0.6Si/Al ratio of SAPO-34 has the largest mesoporous specific surface area and the most suitable acid distribution. The catalytic performance for the MTA process showed that 0.6-SAPO-34/ZSM-5/quartz film has as high as 50.3% benzene-toluenexylene selectivity and 670 min lifetime. The MTA reaction is carried out through the path we designed to effectively avoid the hydrocarbon pool circulation of ZSM-5 zeolite, so as to improve the aromatics selectivity and inhibit the occurrence of deep side reactions to a great extent. The coke deposition behavior was monitored by thermogravimetric analysis and gas chromatograph/mass spectrometer, it is found that with the increase of Si/Al ratio, the active intermediates changed from low-substituted methylbenzene to high-substituted methylbenzene, which led to the rapid deactivation of the catalyst. This work provides a possibility to employ the synergy effect of composite zeolite film synthesizing anti-carbon deposition catalyst in MTA reaction.
基金Supported by the Startup Fund for Introducing Talent of Nanjing University of Information Science&Technology(2015r032)Open Research Fund of the Plateau Atmosphere and Environment Key Laboratory of Sichuan Province(PAEKL-2017-K4)National Natural Science Foundation of China(91337218 and 41605039)
文摘The propagation and underlying mechanisms of the boreal summer quasi-biweekly oscillation(QBWO)over the entire Asian monsoon region are investigated,based on ECMWF Interim reanalysis(ERA-Interim)data,GPCP precipitation data,and an atmospheric general circulation model(AGCM).Statistical analyses indicate that the QBWO over the Asian monsoon region derives its main origin from the equatorial western Pacific and moves northwestward to the Bay of Bengal and northern India,and then northward to the Tibetan Plateau(TP)area,with a baroclinic vertical structure.Northward propagation of the QBWO is promoted by three main mechanisms:barotropic vorticity,boundary moisture advection,and surface sensible heating(SSH).It is dominated by the barotropic vorticity effect when the QBWO signals are situated to the south of 20°N.During the propagation taking place farther north toward the TP,the boundary moisture advection and SSH are the leading mechanisms.We use an AGCM to verify the importance of SSH on the northward propagation of the QBWO.Numerical simulations confirm the diagnostic conclusion that the equatorial western Pacific is the source of the QBWO.Importantly,the model can accurately simulate the propagation pathway of the QBWO signals over the Asian monsoon region.Simultaneously,sensitivity experiments demonstrate that the SSH over northern India and the southern slope of the TP greatly contributes to the northward propagation of the QBWO as far as the TP area.
文摘The present work is intended to simulate, in a rotating annulus of stratified liquid, the me-chanical effect of the Xizang (Tibetan) Plateau on the zonal circulation. The main featuresof three flow patterns around the plateau for different Rossby number R and rotating Eulernumber E are analysed. and a division diagram of the flow pattern in (R, E) plane is given.It has been found that under the condition that similarity criterions R and E of the experimentalfluid are the same as those existing in the atmosphere for monthly mean states in spring, au-tumn and winter months, the experimental results are satisfied for the following weathersystems over the plateau and its vicinities: the low vortex, trough and shear line over thesoutheast part of the plateau, the tilted ridge over the northwest part of the plateau, the troughpatterns over the upstream and dewnstream of the plateau, the vertical circulation structure, thejets on both north and southeast sides of the plateau, and so on. This shows that the