By analyzing GPS, leveling and gravity observation data from the Minle, Huazangsi and Shagouhe profiles across the Qilian Mountain-Haiyuan fault during 2005 - 2009, the changes of these data and activity characteristi...By analyzing GPS, leveling and gravity observation data from the Minle, Huazangsi and Shagouhe profiles across the Qilian Mountain-Haiyuan fault during 2005 - 2009, the changes of these data and activity characteristics of the main faults in different time are obtained. The results show that the Changma-Erbo, Maomaoshan, Zhunglanghe and Haiyuan faults have been active in recent years. The relationship between the vertical displacement and mobile gravity data is analyzed, and the results reveal the gravity changes are mainly due to mass transfer. The results of GPS observation show that the direction of the horizontal movement velocity was almost along the fault strike in 2006 - 2007, while the horizontal velocity deviated from the fault direction in 2007 - 2008, characterized by increased eastward displacement. Further analysis upon removal of the linear trend on the time series of the N and E coordinate values of the continuous observation stations of the Crustal Movement Observation Network of China near the three profiles reveals that the Wenchuan earthquake had an effect on the observations in 2007 - 2008. Comparing the gravitational changes in 2008 - 2009 with the Bouguer gravity anomaly background, we find that the area near Minle profile is in the stage of adjustment and recovery, while the anomaly is not completely recovered around Huazangsi and Shagouhe profiles.展开更多
Vehicle evaporation is an essential source of VOCs in cities but is not well understood in China.Reported emission factors from previous studies are not enough for understanding the atmospheric chemical process of veh...Vehicle evaporation is an essential source of VOCs in cities but is not well understood in China.Reported emission factors from previous studies are not enough for understanding the atmospheric chemical process of vehicular evaporative VOCs.In this work,a serious of detailed VOCs speciation profiles are developed based on test processes and emission processes.A mass balance method was used to divide different emission processes during diurnal tests.The results show that headspace vapor of gasoline cannot represent the real-world vehicle evaporation because of the significant differences in VOCs speciation profiles,especially for aromatics.To further distinguish emissions from evaporation and exhaust,only the ratios of MTBE/benzene and MTBE/toluene can serve as indicators when considering species from all evaporative processes.Besides,emissions from different sources change significantly with the seasons.To solve these problems,we developed a monthly comprehensive evaporation speciation profile.The individual profiles at the emission processes are weighted by the emission of the in-use vehicle fleet in Beijing to derive the comprehensive speciation profile of evaporative VOCs.Ozone formation potential(OFP)and secondary organic aerosol potential(SOAP)were used to evaluate the environmental impact.For SOAP,100 g evaporative emissions are equal to 6.05-12.71 g toluene in different months,much higher than that given using headspace vapors,especially in winter(7.2 times higher in December).These findings would improve our understanding of the evaporative VOCs emissions in China and their environmental impacts(e.g.,O3 and SOA formation).展开更多
基金sponsored by Special Scientific Research Project,China Earthquake Administration(200908029)National Natural Science Foundation of China(40674057)
文摘By analyzing GPS, leveling and gravity observation data from the Minle, Huazangsi and Shagouhe profiles across the Qilian Mountain-Haiyuan fault during 2005 - 2009, the changes of these data and activity characteristics of the main faults in different time are obtained. The results show that the Changma-Erbo, Maomaoshan, Zhunglanghe and Haiyuan faults have been active in recent years. The relationship between the vertical displacement and mobile gravity data is analyzed, and the results reveal the gravity changes are mainly due to mass transfer. The results of GPS observation show that the direction of the horizontal movement velocity was almost along the fault strike in 2006 - 2007, while the horizontal velocity deviated from the fault direction in 2007 - 2008, characterized by increased eastward displacement. Further analysis upon removal of the linear trend on the time series of the N and E coordinate values of the continuous observation stations of the Crustal Movement Observation Network of China near the three profiles reveals that the Wenchuan earthquake had an effect on the observations in 2007 - 2008. Comparing the gravitational changes in 2008 - 2009 with the Bouguer gravity anomaly background, we find that the area near Minle profile is in the stage of adjustment and recovery, while the anomaly is not completely recovered around Huazangsi and Shagouhe profiles.
基金supported by the National Key R&D Program(2016YFC0201504)the National Natural Science Foundation of China(Nos.41822505 and 41571447)+2 种基金National Research Program for Key Issues in Air Pollution Control(DQGG0201&0207)Beijing Nova Program(Z181100006218077)SEE Foundation.
文摘Vehicle evaporation is an essential source of VOCs in cities but is not well understood in China.Reported emission factors from previous studies are not enough for understanding the atmospheric chemical process of vehicular evaporative VOCs.In this work,a serious of detailed VOCs speciation profiles are developed based on test processes and emission processes.A mass balance method was used to divide different emission processes during diurnal tests.The results show that headspace vapor of gasoline cannot represent the real-world vehicle evaporation because of the significant differences in VOCs speciation profiles,especially for aromatics.To further distinguish emissions from evaporation and exhaust,only the ratios of MTBE/benzene and MTBE/toluene can serve as indicators when considering species from all evaporative processes.Besides,emissions from different sources change significantly with the seasons.To solve these problems,we developed a monthly comprehensive evaporation speciation profile.The individual profiles at the emission processes are weighted by the emission of the in-use vehicle fleet in Beijing to derive the comprehensive speciation profile of evaporative VOCs.Ozone formation potential(OFP)and secondary organic aerosol potential(SOAP)were used to evaluate the environmental impact.For SOAP,100 g evaporative emissions are equal to 6.05-12.71 g toluene in different months,much higher than that given using headspace vapors,especially in winter(7.2 times higher in December).These findings would improve our understanding of the evaporative VOCs emissions in China and their environmental impacts(e.g.,O3 and SOA formation).