This study focuses on the degradation behaviour of metallised film capacitors,which are the essential components for the stability of converter valves in flexible ultra-high voltage direct current(HVDC)transmission sy...This study focuses on the degradation behaviour of metallised film capacitors,which are the essential components for the stability of converter valves in flexible ultra-high voltage direct current(HVDC)transmission systems.Through systematic experimentation,we investigated the failure mechanisms of MFCs under HVDC fields with superimposed harmonics,considering both equipment and material perspectives.The experiments subjected capacitors to 500 h of ageing under two conditions:a DC/AC-superimposed field with a constant DC component of 290 kV/mm and an AC ripple rate varying from 12%to 28%,and a control group aged solely under a DC field.Our findings indicate that capacitors aged under the DC/AC-superimposed field exhibited shorter lifespans and more significant capacitance loss than those aged under only the DC field.This difference in performance is primarily attributed to the distinct electrode loss behaviours observed under each ageing condition,which are key factors in the capacitors'capacitance decay.Moreover,the biaxially oriented polypropylene films in the DC-aged samples showed more severe deterioration,characterised by more noticeable molecular chain scission and reduced breakdown strength,compared to those aged under the DC/AC superimposed field.This difference is partly due to the moderate temperature increase caused by harmonics,which benefits the aggregation structure,and partly to the reduced molecular structure damage from the AC field.展开更多
High-order harmonic generation(HHG) of Ar atom in an elliptically polarized intense laser field is experimentally investigated in this work.Interestingly,the anomalous ellipticity dependence on the laser ellipticity(...High-order harmonic generation(HHG) of Ar atom in an elliptically polarized intense laser field is experimentally investigated in this work.Interestingly,the anomalous ellipticity dependence on the laser ellipticity(ε) in the lower-order harmonics is observed,specifically in the 13rd-order,which displays a maximal harmonic intensity at ε ≈ 0.1,rather than at ε = 0 as expected.This contradicts the general trend of harmonic yield,which typically decreases with the increase of laser ellipticity.In this study,we attribute this phenomenon to the disruption of the symmetry of the wave function by the Coulomb effect,leading to the generation of a harmonic with high ellipticity.This finding provides valuable insights into the behavior of elliptically polarized harmonics and opens up a potential way for exploring new applications in ultrafast spectroscopy and light–matter interactions.展开更多
In generator design field,waveform total harmonic distortion(THD)and telephone harmonic factor(THF)are parameters commonly used to measure the impact of generator no-load voltage harmonics on the power communication q...In generator design field,waveform total harmonic distortion(THD)and telephone harmonic factor(THF)are parameters commonly used to measure the impact of generator no-load voltage harmonics on the power communication quality.Tubular hydrogenerators are considered the optimal generator for exploiting low-head,high-flow hydro resources,and they have seen increasingly widespread application in China's power systems recent years.However,owing to the compact and constrained internal space of such generators,their internal magnetic-field harmonics are pronounced.Therefore,accurate calculation of their THD and THF is crucial during the analysis and design stages to ensure the quality of power communication.Especially in the electromagnetic field finite element modeling analysis of such generators,the type and order of the finite element meshes may have a significant impact on the THD and THF calculation results,which warrants in-depth research.To address this,this study takes a real 34 MW large tubular hydrogenerator as an example,and establishes its electromagnetic field finite element model under no-load conditions.Two types of meshes,five mesh densities,and two mesh orders are analyzed to reveal the effect of electromagnetic field finite element mesh types and orders on the calculation results of THD and THF for such generators.展开更多
We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position...We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position in the harmonic emission by adjusting the absolute phase parameter within the frequency domain of the shaping pulse.This phenomenon holds potential significance for experimental setups necessitating precisely tuned single harmonics.Notably,we observe a modulated shift in the created harmonic photon energy,spanning an impressive range of 1.2 eV.This frequency peak shift is rooted in the asymmetry exhibited by the rising and falling edges of the laser pulse,directly influencing the position of the peak frequency emission.Our study quantifies the dependence of this tuning range and the asymmetry of the laser pulse,offering valuable insights into the underlying mechanisms driving this phenomenon.Furthermore,our investigation uncovers the emergence of semi-integer order harmonics as the phase parameter is altered.We attribute this discovery to the intricate interference between harmonics generated by the primary and secondary return cores.This observation introduces an innovative approach for generating semi-integer order harmonics,thus expanding our understanding of high-order harmonic generation.Ultimately,our work contributes to the broader comprehension of complex phenomena in laser-matter interactions and provides a foundation for harnessing these effects in various applications,particularly those involving precise spectral control and the generation of unique harmonic patterns.展开更多
Electric field is an important parameter of plasma,which is related to electron temperature,electron density,excited species density,and so on.In this work,the electric field of an atmospheric pressure plasma jet is d...Electric field is an important parameter of plasma,which is related to electron temperature,electron density,excited species density,and so on.In this work,the electric field of an atmospheric pressure plasma jet is diagnosed by the electric field induced second harmonic(E-FISH)method,and the time-resolved electric field under different conditions is investigated.When positive pulse voltage is applied,the electric field has a peak of about 25 kV cm-1at the rising edge of the voltage pulse.A dark channel is left behind the plasma bullet and the electric field in the dark channel is about 5 kV cm-1.On the other hand,when negative pulse voltage is applied,the electric field has a peak of-16 kV cm-1when the negative voltage is increased to-8 kV.A relatively bright channel is left behind the plasma head and the electric field in this relatively bright channel is about-6 kV cm-1.When the pulse rising time increases from 60 to 200 ns,the peak electric field at both the rising edge and the falling edge of the voltage decreases significantly.When 0.5%of oxygen is added to the main working gas helium,the peak electric field at the rising edge is only about 15 kV cm-1.On the other hand,when 0.5%nitrogen is added,the peak electric field increases especially at the falling edge of the voltage pulse,where it increases reversely from-12 to-16 kV cm-1(the minus sign only represents the direction of electric field).展开更多
The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation ...The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation process of highorder harmonic from the He atom under the action of orthogonal two-color combined pulse of fundamental frequency and higher intensity second harmonic fields is studied.In this paper,we propose to achieve quasi-chirp-free isolated attosecond pulses by superimposing a higher second-harmonic field on the orthogonal direction of the fundamental frequency field.It is found that the high-energy part of its harmonic emission exhibits small chirp characteristics,which can be used to synthesize isolated attosecond pulses.Through the analysis of the wave packets evolution and the classical motion trajectories of the electron,it is demonstrated that the quasi-chirp-free harmonic can be attributed to the simultaneous return of electrons ionized at different times to the parent particle.The influence of the relative phase of the two pulses on the harmonics is further analyzed,and it is observed that this phenomenon is sensitive to the relative phase,but it can still generate isolated attosecond pulses within a certain phase.展开更多
This paper theoretically investigates the high-order harmonic generation cutoff extension using intense few-cycle linearly chirped laser pulses. It shows that the cutoff of the harmonic can be extended remarkably by o...This paper theoretically investigates the high-order harmonic generation cutoff extension using intense few-cycle linearly chirped laser pulses. It shows that the cutoff of the harmonic can be extended remarkably by optimising the chirping parameters. The time-frequency characteristics of high-order harmonics with different chirping parameters are analysed by means of wavelet transform of the dipole acceleration. It also gives out the classical three-step model pictures of electron. By superposing a properly selected range of the harmonic spectrum, it obtains an isolated 65as pulse.展开更多
We theoretically study the selection of the quantum path in high-order harmonics(HHG) and isolated attosecond pulse generation from a one-dimensional(1D) model of a H_2~+ molecule in few-cycle inhomogeneous laser...We theoretically study the selection of the quantum path in high-order harmonics(HHG) and isolated attosecond pulse generation from a one-dimensional(1D) model of a H_2~+ molecule in few-cycle inhomogeneous laser fields.We show that the inhomogeneity of the laser fields play an important role in the HHG process.The cutoff of the harmonics can be extended remarkably,and the harmonic spectrum becomes smooth and has fewer modulations.We investigate the time-frequency profile of the time-dependent dipole,which shows that the short quantum path is enhanced and the long quantum path disappears in spatially inhomogeneous fields.The semi-classical three-step model is also applied to illustrate the physical mechanism of HHG.The influence of driving field carrier-envelop phase(CEP) on HHG is also discussed.By superposing a series of properly selected harmonics,an isolated attosecond pulse(IAP) with duration 53 as can be obtained by a 15-fs,1600-nm laser pulse with the parameter ε = 0.0013(e is the parameter that determines the order of inhomogeneity of the laser field).展开更多
The effects of two types of magnetic fields,namely harmonic magnetic field(HMF)and pulse magnetic field(PMF)on magnetic flux density,Lorentz force,temperature field,and microstructure of high purity Cu were studied by...The effects of two types of magnetic fields,namely harmonic magnetic field(HMF)and pulse magnetic field(PMF)on magnetic flux density,Lorentz force,temperature field,and microstructure of high purity Cu were studied by numerical simulation and experiment during electromagnetic direct chill casting.The magnetic field is induced by a magnetic generation system including an electromagnetic control system and a cylindrical crystallizer of 300 mm in diameter equipped with excitation coils.A comprehensive mathematical model for high purity Cu electromagnetic casting was established in finite element method.The distributions of magnetic flux density and Lorentz force generated by the two magnetic fields were acquired by simulation and experimental measurement.The microstructure of billets produced by HMF and PMF casting was compared.Results show that the magnetic flux density and penetrability of PMF are significantly higher than those of HMF,due to its faster variation in transient current and higher peak value of magnetic flux density.In addition,PMF drives a stronger Lorentz force and deeper penetration depth than HMF does,because HMF creates higher eddy current and reverse electromagnetic field which weakens the original electromagnetic field.The microstructure of a billet by HMF is composed of columnar structure regions and central fine grain regions.By contrast,the billet by PMF has a uniform microstructure which is characterized by ultra-refined and uniform grains because PMF drives a strong dual convection,which increases the uniformity of the temperature field,enhances the impact of the liquid flow on the edge of the liquid pool and reduces the curvature radius of liquid pool.Eventually,PMF shows a good prospect for industrialization.展开更多
The polarization properties of high-order harmonic generation(HHG) in the two-color circularly polarized laser fields are investigated by numerically solving the two-dimensional time-dependent Schr?dinger equation. By...The polarization properties of high-order harmonic generation(HHG) in the two-color circularly polarized laser fields are investigated by numerically solving the two-dimensional time-dependent Schr?dinger equation. By adding a wavelength of 1600-nm right-circular-polarized field to an 800-nm left-circular-polarized field, HHG is simulated from a real model of neon atom with p orbital, but not from a hydrogen-like atom model with s orbital. The orders of 3n + 1 can be selected while the orders of 3n + 2 are suppressed by adjusting the intensities of the two pulses. The physical mechanism is analyzed by time-frequency analysis and semiclassical model.展开更多
We theoretically investigate the high-order harmonic generation(HHG) of helium atom driven by bichromatic counterrotating circularly polarized laser fields. By changing the intensity ratio of the two driving laser fie...We theoretically investigate the high-order harmonic generation(HHG) of helium atom driven by bichromatic counterrotating circularly polarized laser fields. By changing the intensity ratio of the two driving laser fields, the spectral chirality of the HHG can be controlled. As the intensity ratio increases, the spectral chirality will change from positive-to negativevalue around a large intensity ratio of the two driving fields when the total laser intensity keeps unchanged. However, the sign of the spectral chirality can be changed from positive to negative around a small intensity ratio of the two driving fields when the total laser intensity changes. At this time, we can effectively control the helicity of the harmonic spectrum and the polarization of the resulting attosecond pulses by adjusting the intensity ratio of the two driving laser fields. As the intensity ratio and the total intensity of the driving laser fields increase, the relative intensity of either the left-circularly or right-circularly polarized harmonic can be enhanced. The attosecond pulses can evolve from being elliptical to near linear correspondingly.展开更多
Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,t...Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,the temporal and spectral features of the HHG were shown to carry profound insight into frequency-comb emission dynamics.Here we present an ab initio investigation of the temporal and spectral coherence of the frequency comb emitted in HHG of He atom driven by few-cycle pulse trains.We find that the emission of frequency combs features a destructive and constructive coherences caused by the phase interference of HHG,leading to suppression and enhancement of frequency-comb emission.The results reveal intriguing and substantially different nonlinear optical response behaviors for frequency-comb emission via HHG.The dynamical origin of frequency-comb emission is clarified by analyzing the phase coherence in HHG processes in detail.Our results provide fresh insight into the experimental realization of selective enhancement of frequency comb in the VUV–XUV regimes.展开更多
The effect of multiple rescattering processes on the harmonic emission from He atom in a spatially inhomogeneous field is discussed by solving the one-dimensional time-dependent Schrtdinger equation and the classical ...The effect of multiple rescattering processes on the harmonic emission from He atom in a spatially inhomogeneous field is discussed by solving the one-dimensional time-dependent Schrtdinger equation and the classical equation of motion. By establishing the physical model of the harmonic emission in the inhomogeneous field, we discuss the related characters of the multiple rescatterings process in the harmonic generation process. It shows that the second rescattering rather than the first rescattering tends to determine the harmonic cutoff energy when the inhomogeneous parameter is larger than 0.0055. Additionally, with the classica/simulation, the underlying physical mechanism of the continuum-continuum harmonics is also revealed. Moreover, this work may provide new physical insight into the harmonic generation in an inhomogeneous field, and is beneficial to further extract the harnaonic emission from molecular systems.展开更多
We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the ...We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the HHG with only one central Bohmian trajectory is in a good agreement with the ab initio time-dependent Schrodinger equation (TDSE) results. In contrast, with the increase of the amplitude of the second-color laser field, the HHG spectra from the single central Bohmian trajectory deviate from the TDSE results more and more significantly. By analyzing the Bohmian trajectories, we find that the significant deviation is due to the fact that the central Bohmian trajectory leaves the core quickly in the two-color laser field with the breaking of inversion symmetry. Interestingly, we find that another Bohmian trajectory with different initial position, which keeps oscillating around the core, could qualitatively well reproduce the TDSE results. Furthermore, we study the HHG spectrum in a two-color laser field with inversion symmetry and find that the HHG spectrum in TDSE can be still well simulated with the central Bohmian trajectory. These results indicate that, similar to the case of one color laser field, the HHG spectra in a two-color laser field can be also reproduced with a single Bohmian trajectory, although the initial position of the trajectory is dependent on the symmetry of the laser field. Our work thus demonstrates that Bohmian trajectory theory can be used as a promising tool in investigating the HHG process in a two-color laser field.展开更多
The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spec...The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spectra is dramatically extended and a continuous harmonic spectrum with the bandwidth of 113 eV is obtained. When a static field is added to the x direction, the quantum path control is realized and a supercontinuum spectrum can be obtained, which is beneficial to obtain a shorter attosecond pulse. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics in the combination of two-color circularly polarized laser fields and a static field, an isolated attosecond pulse with a duration of 30 as can be generated.展开更多
The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of ...The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of contributions to high-order harmonic generation(HHG) from different nuclei is realized by properly selecting the relative phase.When the relative phase is chosen to be φ= 0.4π,the contribution to HHG from one nucleus is much more than that from another.Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 e V to125 e V.The underlying physical mechanism is well explained by the time–frequency analysis and the semi-classical threestep model with a finite initial transverse velocity.By superposing several orders of harmonics,an isolated attosecond pulse with a duration of 80 as can be generated.展开更多
A model was established based on Maxwell's equations and Navier-Stokes' equations to numerically simulate the electromagnetic field and flow field in a rectangular mold with sectional aspect ratio of 5:1. The ...A model was established based on Maxwell's equations and Navier-Stokes' equations to numerically simulate the electromagnetic field and flow field in a rectangular mold with sectional aspect ratio of 5:1. The FEM (Finite Element Method) and APDL (ANSYS Parametric Design Language) were employed for the model to execute the modeling, meshing, load applying and solving. The Ti-Al alloy melt was selected to illustrate and validate the effects of the harmonic field frequency on the distribution of the physical fields in the mold. The simulated results demonstrate that with an increasing frequency the electric current forms an ellipsoid cavity where it becomes much weaker, and that the melt flows more intensely with low frequency (less than 5 kHz) than with high frequency (more than 5 kHz). The melt is pinched from the central part in the mold to bipolar parts in which it forms two vortexes in each side. The maximum value of fluid velocity exists near the bipolar zone.展开更多
We investigate the plasmonic-field-enhanced high-order harmonic generation(HHG) of H atom driven by few-cycle laser pulses, by solving the time-dependent Schr?dinger equation(TDSE). Compared with the homogeneous ...We investigate the plasmonic-field-enhanced high-order harmonic generation(HHG) of H atom driven by few-cycle laser pulses, by solving the time-dependent Schr?dinger equation(TDSE). Compared with the homogeneous field, HHG spectra generated by inhomogeneous field exhibit two-plateau structure. We analyze the origin of the two plateaus by using the semiclassical trajectory method. Our results from both classical and TDSE simulations show that the cutoffs of the two plateaus are dramatically affected by the carrier-envelope phase(CEP) of laser pulse in the inhomogeneous field, even for a little longer pulse. Thus, we can determine the CEP of driving laser based on the cutoff position of HHG generated in the inhomogeneous field.展开更多
We theoretically investigate the two-center interference in high-order harmonics generated from the H2-+ in a combination of a mid-infrared laser and a terahertz field by numerically solving the time-dependent Schr &...We theoretically investigate the two-center interference in high-order harmonics generated from the H2-+ in a combination of a mid-infrared laser and a terahertz field by numerically solving the time-dependent Schr ¨odinger equation(TDSE).The interference minima in high-order harmonic generation(HHG) are effectively suppressed when a THz field is added.The contribution to HHG from the two separate nuclei is used to demonstrate the locating order of the harmonic minima.Furthermore, we also investigate the emission time of harmonics. The results show that the intensity of the short path around 60^th order after adding a THz field is stronger than that in the mid-infrared laser field, which further illustrates the suppression of the interference minima in HHG.展开更多
The harmonic force field and the vibrational spectrum of nitramide were calculated by using the ab initio gradient program TEXAS at the Hartree-Fock level with a 4-21G basis set. The directly computed theoretical harm...The harmonic force field and the vibrational spectrum of nitramide were calculated by using the ab initio gradient program TEXAS at the Hartree-Fock level with a 4-21G basis set. The directly computed theoretical harmonic force field was scaled by using empirical scale factors which are transferred from other molecules and provided an a priori prediction of fundamental frequencies and intensities. The average deviations between predicted vibrational frequencies of nitramide and experimental IR spectrum in an argon matrix are 63 cm-1 for symmetric vibrations and 41 cm-1 for antisymmetric modes. A new set of scale factors was optimized in this paper. These scale factors reduced the average deviations to 2. 3 cm-1 for symmetric modes and 0. 8 cm-1 for antisymmetric ones. The vibrational spectra of three isotopic derivatives of nitramide were predicted by using the force field resulted from the optimized set of scale factors, which are in good agreement with their experimental data in an argon matrix.展开更多
基金Science and Technology Project of SGCC,Grant/Award Number:5108-202218280A-2-355-XG。
文摘This study focuses on the degradation behaviour of metallised film capacitors,which are the essential components for the stability of converter valves in flexible ultra-high voltage direct current(HVDC)transmission systems.Through systematic experimentation,we investigated the failure mechanisms of MFCs under HVDC fields with superimposed harmonics,considering both equipment and material perspectives.The experiments subjected capacitors to 500 h of ageing under two conditions:a DC/AC-superimposed field with a constant DC component of 290 kV/mm and an AC ripple rate varying from 12%to 28%,and a control group aged solely under a DC field.Our findings indicate that capacitors aged under the DC/AC-superimposed field exhibited shorter lifespans and more significant capacitance loss than those aged under only the DC field.This difference in performance is primarily attributed to the distinct electrode loss behaviours observed under each ageing condition,which are key factors in the capacitors'capacitance decay.Moreover,the biaxially oriented polypropylene films in the DC-aged samples showed more severe deterioration,characterised by more noticeable molecular chain scission and reduced breakdown strength,compared to those aged under the DC/AC superimposed field.This difference is partly due to the moderate temperature increase caused by harmonics,which benefits the aggregation structure,and partly to the reduced molecular structure damage from the AC field.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.92250306,11974137,and 12304302)the National Key Program for Science and Technology Research and Development of China(Grant No.2019YFA0307700)+1 种基金the Natural Science Foundation of Jilin Province,China(Grant Nos.YDZJ202101ZYTS157 and YDZJ202201ZYTS314)the Scientific Research Foundation of the Education Department of Jilin Province,China(Grant No.JJKH20230283KJ)。
文摘High-order harmonic generation(HHG) of Ar atom in an elliptically polarized intense laser field is experimentally investigated in this work.Interestingly,the anomalous ellipticity dependence on the laser ellipticity(ε) in the lower-order harmonics is observed,specifically in the 13rd-order,which displays a maximal harmonic intensity at ε ≈ 0.1,rather than at ε = 0 as expected.This contradicts the general trend of harmonic yield,which typically decreases with the increase of laser ellipticity.In this study,we attribute this phenomenon to the disruption of the symmetry of the wave function by the Coulomb effect,leading to the generation of a harmonic with high ellipticity.This finding provides valuable insights into the behavior of elliptically polarized harmonics and opens up a potential way for exploring new applications in ultrafast spectroscopy and light–matter interactions.
基金sponsored by the National Natural Science Foundation,Youth Foundation of China,Grant/Award Number:51607146Sichuan Natural Sciences Fund,Grant/Award Number:2023NSFSC0295。
文摘In generator design field,waveform total harmonic distortion(THD)and telephone harmonic factor(THF)are parameters commonly used to measure the impact of generator no-load voltage harmonics on the power communication quality.Tubular hydrogenerators are considered the optimal generator for exploiting low-head,high-flow hydro resources,and they have seen increasingly widespread application in China's power systems recent years.However,owing to the compact and constrained internal space of such generators,their internal magnetic-field harmonics are pronounced.Therefore,accurate calculation of their THD and THF is crucial during the analysis and design stages to ensure the quality of power communication.Especially in the electromagnetic field finite element modeling analysis of such generators,the type and order of the finite element meshes may have a significant impact on the THD and THF calculation results,which warrants in-depth research.To address this,this study takes a real 34 MW large tubular hydrogenerator as an example,and establishes its electromagnetic field finite element model under no-load conditions.Two types of meshes,five mesh densities,and two mesh orders are analyzed to reveal the effect of electromagnetic field finite element mesh types and orders on the calculation results of THD and THF for such generators.
基金This project was supported by the National Key Research and Development Program of China(Grant Nos.2022YFE134200 and 2019YFA0307700)the National Natural Science Foundation of China(Grant Nos.11604119,12104177,11904192,12074145,and 11704147)the Fundamental Research Funds for the Central Universities(Grant Nos.GK202207012 and QCYRCXM-2022-241).
文摘We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position in the harmonic emission by adjusting the absolute phase parameter within the frequency domain of the shaping pulse.This phenomenon holds potential significance for experimental setups necessitating precisely tuned single harmonics.Notably,we observe a modulated shift in the created harmonic photon energy,spanning an impressive range of 1.2 eV.This frequency peak shift is rooted in the asymmetry exhibited by the rising and falling edges of the laser pulse,directly influencing the position of the peak frequency emission.Our study quantifies the dependence of this tuning range and the asymmetry of the laser pulse,offering valuable insights into the underlying mechanisms driving this phenomenon.Furthermore,our investigation uncovers the emergence of semi-integer order harmonics as the phase parameter is altered.We attribute this discovery to the intricate interference between harmonics generated by the primary and secondary return cores.This observation introduces an innovative approach for generating semi-integer order harmonics,thus expanding our understanding of high-order harmonic generation.Ultimately,our work contributes to the broader comprehension of complex phenomena in laser-matter interactions and provides a foundation for harnessing these effects in various applications,particularly those involving precise spectral control and the generation of unique harmonic patterns.
基金National Key Research and Development Program of China(No.2021YFE0114700)National Natural Science Foundation of China(Nos.52130701 and 51977096)。
文摘Electric field is an important parameter of plasma,which is related to electron temperature,electron density,excited species density,and so on.In this work,the electric field of an atmospheric pressure plasma jet is diagnosed by the electric field induced second harmonic(E-FISH)method,and the time-resolved electric field under different conditions is investigated.When positive pulse voltage is applied,the electric field has a peak of about 25 kV cm-1at the rising edge of the voltage pulse.A dark channel is left behind the plasma bullet and the electric field in the dark channel is about 5 kV cm-1.On the other hand,when negative pulse voltage is applied,the electric field has a peak of-16 kV cm-1when the negative voltage is increased to-8 kV.A relatively bright channel is left behind the plasma head and the electric field in this relatively bright channel is about-6 kV cm-1.When the pulse rising time increases from 60 to 200 ns,the peak electric field at both the rising edge and the falling edge of the voltage decreases significantly.When 0.5%of oxygen is added to the main working gas helium,the peak electric field at the rising edge is only about 15 kV cm-1.On the other hand,when 0.5%nitrogen is added,the peak electric field increases especially at the falling edge of the voltage pulse,where it increases reversely from-12 to-16 kV cm-1(the minus sign only represents the direction of electric field).
基金Project supported by the National Key Research and Development Program of China(Grant No.2019YFA0307700)the National Natural Science Foundation of China(Grant Nos.12074145,11627807,and 11975012)+2 种基金the Research Foundation for Basic Research of Jilin Province,China(Grant No.20220101003JC)the Fundamental Research Funds for the Central Universities of China(Grant No.30916011207)the Outstanding Youth Project of Taizhou University(Grant No.2019JQ002)。
文摘The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation process of highorder harmonic from the He atom under the action of orthogonal two-color combined pulse of fundamental frequency and higher intensity second harmonic fields is studied.In this paper,we propose to achieve quasi-chirp-free isolated attosecond pulses by superimposing a higher second-harmonic field on the orthogonal direction of the fundamental frequency field.It is found that the high-energy part of its harmonic emission exhibits small chirp characteristics,which can be used to synthesize isolated attosecond pulses.Through the analysis of the wave packets evolution and the classical motion trajectories of the electron,it is demonstrated that the quasi-chirp-free harmonic can be attributed to the simultaneous return of electrons ionized at different times to the parent particle.The influence of the relative phase of the two pulses on the harmonics is further analyzed,and it is observed that this phenomenon is sensitive to the relative phase,but it can still generate isolated attosecond pulses within a certain phase.
基金supported by the National Natural Science Foundation of China (Grant No.10974068)
文摘This paper theoretically investigates the high-order harmonic generation cutoff extension using intense few-cycle linearly chirped laser pulses. It shows that the cutoff of the harmonic can be extended remarkably by optimising the chirping parameters. The time-frequency characteristics of high-order harmonics with different chirping parameters are analysed by means of wavelet transform of the dipole acceleration. It also gives out the classical three-step model pictures of electron. By superposing a properly selected range of the harmonic spectrum, it obtains an isolated 65as pulse.
基金supported by the National Natural Science Foundation of China(Grant Nos.11174108,11104108,and 11271158)
文摘We theoretically study the selection of the quantum path in high-order harmonics(HHG) and isolated attosecond pulse generation from a one-dimensional(1D) model of a H_2~+ molecule in few-cycle inhomogeneous laser fields.We show that the inhomogeneity of the laser fields play an important role in the HHG process.The cutoff of the harmonics can be extended remarkably,and the harmonic spectrum becomes smooth and has fewer modulations.We investigate the time-frequency profile of the time-dependent dipole,which shows that the short quantum path is enhanced and the long quantum path disappears in spatially inhomogeneous fields.The semi-classical three-step model is also applied to illustrate the physical mechanism of HHG.The influence of driving field carrier-envelop phase(CEP) on HHG is also discussed.By superposing a series of properly selected harmonics,an isolated attosecond pulse(IAP) with duration 53 as can be obtained by a 15-fs,1600-nm laser pulse with the parameter ε = 0.0013(e is the parameter that determines the order of inhomogeneity of the laser field).
基金financially supported by the National Key Research and Development Program of China(Grant No.2017YFB0305504)。
文摘The effects of two types of magnetic fields,namely harmonic magnetic field(HMF)and pulse magnetic field(PMF)on magnetic flux density,Lorentz force,temperature field,and microstructure of high purity Cu were studied by numerical simulation and experiment during electromagnetic direct chill casting.The magnetic field is induced by a magnetic generation system including an electromagnetic control system and a cylindrical crystallizer of 300 mm in diameter equipped with excitation coils.A comprehensive mathematical model for high purity Cu electromagnetic casting was established in finite element method.The distributions of magnetic flux density and Lorentz force generated by the two magnetic fields were acquired by simulation and experimental measurement.The microstructure of billets produced by HMF and PMF casting was compared.Results show that the magnetic flux density and penetrability of PMF are significantly higher than those of HMF,due to its faster variation in transient current and higher peak value of magnetic flux density.In addition,PMF drives a stronger Lorentz force and deeper penetration depth than HMF does,because HMF creates higher eddy current and reverse electromagnetic field which weakens the original electromagnetic field.The microstructure of a billet by HMF is composed of columnar structure regions and central fine grain regions.By contrast,the billet by PMF has a uniform microstructure which is characterized by ultra-refined and uniform grains because PMF drives a strong dual convection,which increases the uniformity of the temperature field,enhances the impact of the liquid flow on the edge of the liquid pool and reduces the curvature radius of liquid pool.Eventually,PMF shows a good prospect for industrialization.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11974229,11504221,and 11404204)the Scientific and Technological Innovation Program of Higher Education Institutions in Shanxi Province,China(Grant No.2019L0452)+1 种基金the Natural Science Foundation for Young Scientists of Shanxi Province,China(Grant No.2015021023)the Program for Top Young Academic Leaders of Higher Learning Institutions of Shanxi Province,China
文摘The polarization properties of high-order harmonic generation(HHG) in the two-color circularly polarized laser fields are investigated by numerically solving the two-dimensional time-dependent Schr?dinger equation. By adding a wavelength of 1600-nm right-circular-polarized field to an 800-nm left-circular-polarized field, HHG is simulated from a real model of neon atom with p orbital, but not from a hydrogen-like atom model with s orbital. The orders of 3n + 1 can be selected while the orders of 3n + 2 are suppressed by adjusting the intensities of the two pulses. The physical mechanism is analyzed by time-frequency analysis and semiclassical model.
基金Project supported by the National Natural Science Foundation of China(Grant No.61575077)the Natural Science Foundation of Jilin Province of China(Grant No.20180101225JC)+1 种基金the China Postdoctoral Science Foundation(Grants Nos.2018M641766 and 2019T120232)the Graduate Innovation Fund of Jilin University,China(Grant No.101832018C105)
文摘We theoretically investigate the high-order harmonic generation(HHG) of helium atom driven by bichromatic counterrotating circularly polarized laser fields. By changing the intensity ratio of the two driving laser fields, the spectral chirality of the HHG can be controlled. As the intensity ratio increases, the spectral chirality will change from positive-to negativevalue around a large intensity ratio of the two driving fields when the total laser intensity keeps unchanged. However, the sign of the spectral chirality can be changed from positive to negative around a small intensity ratio of the two driving fields when the total laser intensity changes. At this time, we can effectively control the helicity of the harmonic spectrum and the polarization of the resulting attosecond pulses by adjusting the intensity ratio of the two driving laser fields. As the intensity ratio and the total intensity of the driving laser fields increase, the relative intensity of either the left-circularly or right-circularly polarized harmonic can be enhanced. The attosecond pulses can evolve from being elliptical to near linear correspondingly.
基金the National Natural Science Foundation of China(Grant Nos.12074239 and 91850209)the Natural Science Foundation of Guangdong Province,China(Grant Nos.2020A1515010927 and 2020ST084)+1 种基金the Fund from the Department of Education of Guangdong Province,China(Grant Nos.2019KTSCX038 and 2020KCXTD012)the Fund from Shantou University(Grant No.NTF18030).
文摘Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,the temporal and spectral features of the HHG were shown to carry profound insight into frequency-comb emission dynamics.Here we present an ab initio investigation of the temporal and spectral coherence of the frequency comb emitted in HHG of He atom driven by few-cycle pulse trains.We find that the emission of frequency combs features a destructive and constructive coherences caused by the phase interference of HHG,leading to suppression and enhancement of frequency-comb emission.The results reveal intriguing and substantially different nonlinear optical response behaviors for frequency-comb emission via HHG.The dynamical origin of frequency-comb emission is clarified by analyzing the phase coherence in HHG processes in detail.Our results provide fresh insight into the experimental realization of selective enhancement of frequency comb in the VUV–XUV regimes.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11404204,11274215,and 11504221)the Natural Science Foundation for Young Scientists of Shanxi Province,China(Grant No.2015021023)+1 种基金Program for the Top Young Academic Leaders of Higher Learning Institutions of Shanxi Province,ChinaInnovation Project for Postgraduates of Shanxi Province,China(Grant No.2017BY085)
文摘The effect of multiple rescattering processes on the harmonic emission from He atom in a spatially inhomogeneous field is discussed by solving the one-dimensional time-dependent Schrtdinger equation and the classical equation of motion. By establishing the physical model of the harmonic emission in the inhomogeneous field, we discuss the related characters of the multiple rescatterings process in the harmonic generation process. It shows that the second rescattering rather than the first rescattering tends to determine the harmonic cutoff energy when the inhomogeneous parameter is larger than 0.0055. Additionally, with the classica/simulation, the underlying physical mechanism of the continuum-continuum harmonics is also revealed. Moreover, this work may provide new physical insight into the harmonic generation in an inhomogeneous field, and is beneficial to further extract the harnaonic emission from molecular systems.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11334009,11474321,and 11527807)
文摘We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the HHG with only one central Bohmian trajectory is in a good agreement with the ab initio time-dependent Schrodinger equation (TDSE) results. In contrast, with the increase of the amplitude of the second-color laser field, the HHG spectra from the single central Bohmian trajectory deviate from the TDSE results more and more significantly. By analyzing the Bohmian trajectories, we find that the significant deviation is due to the fact that the central Bohmian trajectory leaves the core quickly in the two-color laser field with the breaking of inversion symmetry. Interestingly, we find that another Bohmian trajectory with different initial position, which keeps oscillating around the core, could qualitatively well reproduce the TDSE results. Furthermore, we study the HHG spectrum in a two-color laser field with inversion symmetry and find that the HHG spectrum in TDSE can be still well simulated with the central Bohmian trajectory. These results indicate that, similar to the case of one color laser field, the HHG spectra in a two-color laser field can be also reproduced with a single Bohmian trajectory, although the initial position of the trajectory is dependent on the symmetry of the laser field. Our work thus demonstrates that Bohmian trajectory theory can be used as a promising tool in investigating the HHG process in a two-color laser field.
基金supported by the National Natural Science Foundation of China(Grant Nos.61575077,11271158,and 11574117)
文摘The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spectra is dramatically extended and a continuous harmonic spectrum with the bandwidth of 113 eV is obtained. When a static field is added to the x direction, the quantum path control is realized and a supercontinuum spectrum can be obtained, which is beneficial to obtain a shorter attosecond pulse. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics in the combination of two-color circularly polarized laser fields and a static field, an isolated attosecond pulse with a duration of 30 as can be generated.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11271158,61575077,and 11574117)
文摘The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of contributions to high-order harmonic generation(HHG) from different nuclei is realized by properly selecting the relative phase.When the relative phase is chosen to be φ= 0.4π,the contribution to HHG from one nucleus is much more than that from another.Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 e V to125 e V.The underlying physical mechanism is well explained by the time–frequency analysis and the semi-classical threestep model with a finite initial transverse velocity.By superposing several orders of harmonics,an isolated attosecond pulse with a duration of 80 as can be generated.
基金supported by the Program for New Century Excellent Talents in Universities (GrantNo. NCET-08-0164) of China’s Ministry of Educationthe Foundation of National Key Laboratory for Precision Hot Processing of Metals, China
文摘A model was established based on Maxwell's equations and Navier-Stokes' equations to numerically simulate the electromagnetic field and flow field in a rectangular mold with sectional aspect ratio of 5:1. The FEM (Finite Element Method) and APDL (ANSYS Parametric Design Language) were employed for the model to execute the modeling, meshing, load applying and solving. The Ti-Al alloy melt was selected to illustrate and validate the effects of the harmonic field frequency on the distribution of the physical fields in the mold. The simulated results demonstrate that with an increasing frequency the electric current forms an ellipsoid cavity where it becomes much weaker, and that the melt flows more intensely with low frequency (less than 5 kHz) than with high frequency (more than 5 kHz). The melt is pinched from the central part in the mold to bipolar parts in which it forms two vortexes in each side. The maximum value of fluid velocity exists near the bipolar zone.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11264036,11364038,and 11465016)
文摘We investigate the plasmonic-field-enhanced high-order harmonic generation(HHG) of H atom driven by few-cycle laser pulses, by solving the time-dependent Schr?dinger equation(TDSE). Compared with the homogeneous field, HHG spectra generated by inhomogeneous field exhibit two-plateau structure. We analyze the origin of the two plateaus by using the semiclassical trajectory method. Our results from both classical and TDSE simulations show that the cutoffs of the two plateaus are dramatically affected by the carrier-envelope phase(CEP) of laser pulse in the inhomogeneous field, even for a little longer pulse. Thus, we can determine the CEP of driving laser based on the cutoff position of HHG generated in the inhomogeneous field.
基金supported by the National Natural Science Foundation of China(Grant Nos.61575077,11574117,and 11271158)the Graduate Innovation Fund of Jilin University,China(Grant No.2016153)
文摘We theoretically investigate the two-center interference in high-order harmonics generated from the H2-+ in a combination of a mid-infrared laser and a terahertz field by numerically solving the time-dependent Schr ¨odinger equation(TDSE).The interference minima in high-order harmonic generation(HHG) are effectively suppressed when a THz field is added.The contribution to HHG from the two separate nuclei is used to demonstrate the locating order of the harmonic minima.Furthermore, we also investigate the emission time of harmonics. The results show that the intensity of the short path around 60^th order after adding a THz field is stronger than that in the mid-infrared laser field, which further illustrates the suppression of the interference minima in HHG.
基金Supported by the National Natural Science Foundation of China
文摘The harmonic force field and the vibrational spectrum of nitramide were calculated by using the ab initio gradient program TEXAS at the Hartree-Fock level with a 4-21G basis set. The directly computed theoretical harmonic force field was scaled by using empirical scale factors which are transferred from other molecules and provided an a priori prediction of fundamental frequencies and intensities. The average deviations between predicted vibrational frequencies of nitramide and experimental IR spectrum in an argon matrix are 63 cm-1 for symmetric vibrations and 41 cm-1 for antisymmetric modes. A new set of scale factors was optimized in this paper. These scale factors reduced the average deviations to 2. 3 cm-1 for symmetric modes and 0. 8 cm-1 for antisymmetric ones. The vibrational spectra of three isotopic derivatives of nitramide were predicted by using the force field resulted from the optimized set of scale factors, which are in good agreement with their experimental data in an argon matrix.