Properties of the chair doublet bands of the odd-odd Cs isotopes built on the πh11/2× vh11/2 configuration are investigated systematically within the supersymmetry scheme including many-body interactions and pos...Properties of the chair doublet bands of the odd-odd Cs isotopes built on the πh11/2× vh11/2 configuration are investigated systematically within the supersymmetry scheme including many-body interactions and possessing the SO(5)(or SU(5)) symmetry on the rotational symmetry. Quantitatively good results of the energy spectra, the energy staggering parameter as a function of the spin are obtained. The calculation shows that the stronger competition between the pairing and anti-pairing effects and the SU(3) symmetry broking more seriously exist in the stable chiral structure.展开更多
The communication in the physical layer between an interrogator and a tag of a passive Radio Frequency Identification (RFID) system operating between 860-960 MHz is defined by the Gen 2 protocol. The tag can be cons...The communication in the physical layer between an interrogator and a tag of a passive Radio Frequency Identification (RFID) system operating between 860-960 MHz is defined by the Gen 2 protocol. The tag can be considered a remote executing unit or a computer that executes instructions from the Gen 2 protocol. The selection of the parameter and command configuration within the protocol limitations is critical especially if the time available for the memory operations in a passive RFID system is limited. An effort is made to map the operation of the tag not in its states of operation as elaborately explained in the protocol but rather in its elementary format. The research reported in this article identifies all the parameters that affect the dynamic operation of the tag. The operation is further divided into singulation, read and write; identifying the significant parameters in each case. The choices of the different commands that can be adopted to perform identical operations on the tag are analyzed. The elements to consider in selecting the optimum command configuration are described. The impact of the different parameter and command configuration on the singulation, read and write time is calculated and recorded using a tested Gen 2 simulator program.展开更多
To validate the ability of full configuration interaction quantum Monte Carlo (FCIQMC) for studying the 2D Hubbard model near half-filling regime, the ground state energies of a 4×44×4 square lattice syste...To validate the ability of full configuration interaction quantum Monte Carlo (FCIQMC) for studying the 2D Hubbard model near half-filling regime, the ground state energies of a 4×44×4 square lattice system with various interaction strengths are calculated. It is found that the calculated results are in good agreement with those obtained by exact diagonalization (i.e., the exact values for a given basis set) when the population of psi particles (psips) is higher than the critical population required to correctly sample the ground state wave function. In addition, the variations of the average computational time per 20 Monte Carlo cycles with the coupling strength and the number of processors are also analyzed. The calculated results show that the computational efficiency of an FCIQMC calculation is mainly affected by the total population of psips and the communication between processors. These results can provide useful references for understanding the FCIQMC algorithm, studying the ground state properties of the 2D Hubbard model for the larger system size by the FCIQMC method and using a computational budget as effectively as possible.展开更多
A 3D nanostructured scaffold as the host for zinc enables effective inhibition of anodic dendrite growth.However,the increased electrode/electrolyte interface area provided by using 3D matrices exacerbates the passiva...A 3D nanostructured scaffold as the host for zinc enables effective inhibition of anodic dendrite growth.However,the increased electrode/electrolyte interface area provided by using 3D matrices exacerbates the passivation and localized corrosion of the Zn anode,ultimately bringing about the degradation of the electrochemical performance.Herein,a nanoscale coating of inorganic-organic hybrid(α-In_(2)Se_(3)-Nafion)onto a flexible carbon nanotubes(CNTs)framework(ISNF@CNTs)is designed as a Zn plating/stripping scaffold to ensure uniform Zn nucleation,thus achieving a dendrite-free and durable Zn anode.The intro-duced inorganic-organic interfacial layer is dense and sturdy,which hinders the direct exposure of deposited Zn to electrolytes and mitigates the side reactions.Meanwhile,the zincophilic nature of ISNF can largely reduce the nucleation energy barrier and promote the ion-diffusion transportation.Consequently,the ISNF@CNTs@Zn electrode exhibits a low-voltage hysteresis and a superior cycling life(over 1500 h),with dendrite-free Zn-plating behaviors in a typical symmetrical cell test.Additionally,the superior feature of ISNF@CNTs@Zn anode is further demonstrated by Zn-MnO_(2)cells in both coin and flexible quasi-solid-state configurations.This work puts forward an inspired remedy for advanced Zn-ion batteries.展开更多
Constructing step-scheme(S-scheme)heterojunctions has become a popular strategy for efficient pho-tocatalytic H_(2)O_(2) generation.Herein,we in situ grew BiOBr nanosheets(NSs)on a Schiff-base covalent organic framewo...Constructing step-scheme(S-scheme)heterojunctions has become a popular strategy for efficient pho-tocatalytic H_(2)O_(2) generation.Herein,we in situ grew BiOBr nanosheets(NSs)on a Schiff-base covalent organic framework(COF)with largeπ-conjugated structures to prepare S-scheme BiOBr/COF photocat-alysts for H_(2)O_(2) synthesis.The highest photocatalytic H_(2)O_(2) production performance of the composite sample constituting the S-scheme heterojunction is 3749μmol g−1 h−1,which was 1.85 and 27 times the rates of COF and BiOBr,respectively.The construction of S-scheme heterojunction contributed to ef-ficient carrier transfer and separation in space and enhanced redox power.Moreover,the lying-down O_(2)-adsorption configuration on the COF surface favors the concerted two-electron O_(2) reduction process,which greatly reduced the reduction potential requirement for O_(2)-to-H_(2)O_(2) conversion.The synergy be-tween the S-scheme heterojunction and the unique O_(2)-COF interaction boosted photocatalytic H_(2)O_(2) pro-duction activity.展开更多
The effect of the two-nucleon excitation from p to sd shell is discussed on12 C and14C in the frame work of the nuclear shell model. The recently suggested shell-model Hamiltonian YSOX provides an suitable tool to inv...The effect of the two-nucleon excitation from p to sd shell is discussed on12 C and14C in the frame work of the nuclear shell model. The recently suggested shell-model Hamiltonian YSOX provides an suitable tool to investigate the 2hω excitation in psd region. Because the strength of the< pp|V |sdsd > interaction, which represents the interaction between the 0 and 2hω configurations, is considered in the construction of the Hamiltonian YSOX. The level of12 C is almost independent on the < pp|V |sdsd > interaction, but excitation energies of certain states in14 C are strongly affected by it.Further investigation shows that the percentage of 2hω configuration in these states is quite different from that of the ground state. The non-linear effects of the < pp|V |sdsd > interaction on the configurations and transition rates are also discussed.展开更多
基金Supported by the National Natural Science Foundation of China under Grant No.10475026the Natural Science Foundation of Zhejiang Province under Grant No.KY607518
文摘Properties of the chair doublet bands of the odd-odd Cs isotopes built on the πh11/2× vh11/2 configuration are investigated systematically within the supersymmetry scheme including many-body interactions and possessing the SO(5)(or SU(5)) symmetry on the rotational symmetry. Quantitatively good results of the energy spectra, the energy staggering parameter as a function of the spin are obtained. The calculation shows that the stronger competition between the pairing and anti-pairing effects and the SU(3) symmetry broking more seriously exist in the stable chiral structure.
文摘The communication in the physical layer between an interrogator and a tag of a passive Radio Frequency Identification (RFID) system operating between 860-960 MHz is defined by the Gen 2 protocol. The tag can be considered a remote executing unit or a computer that executes instructions from the Gen 2 protocol. The selection of the parameter and command configuration within the protocol limitations is critical especially if the time available for the memory operations in a passive RFID system is limited. An effort is made to map the operation of the tag not in its states of operation as elaborately explained in the protocol but rather in its elementary format. The research reported in this article identifies all the parameters that affect the dynamic operation of the tag. The operation is further divided into singulation, read and write; identifying the significant parameters in each case. The choices of the different commands that can be adopted to perform identical operations on the tag are analyzed. The elements to consider in selecting the optimum command configuration are described. The impact of the different parameter and command configuration on the singulation, read and write time is calculated and recorded using a tested Gen 2 simulator program.
基金Supported by the Natural Science Foundation for Colleges and Universities of Jiangsu Province under Grant No 16KJB140008the National Natural Science Foundation of China under Grant Nos 11447204 and 11647164+1 种基金the Natural Science Foundation of Jiangsu Province under Grant No BK20151079the Scientific Research Foundation of Nanjing Xiaozhuang University under Grant No 2015NXY34
文摘To validate the ability of full configuration interaction quantum Monte Carlo (FCIQMC) for studying the 2D Hubbard model near half-filling regime, the ground state energies of a 4×44×4 square lattice system with various interaction strengths are calculated. It is found that the calculated results are in good agreement with those obtained by exact diagonalization (i.e., the exact values for a given basis set) when the population of psi particles (psips) is higher than the critical population required to correctly sample the ground state wave function. In addition, the variations of the average computational time per 20 Monte Carlo cycles with the coupling strength and the number of processors are also analyzed. The calculated results show that the computational efficiency of an FCIQMC calculation is mainly affected by the total population of psips and the communication between processors. These results can provide useful references for understanding the FCIQMC algorithm, studying the ground state properties of the 2D Hubbard model for the larger system size by the FCIQMC method and using a computational budget as effectively as possible.
基金Natural Science Foundation for Young Scientists of Henan Province,Grant/Award Number:202300410071Key Research Project of Henan Provincial Higher Education,Grant/Award Number:21A140007National Natural Science Foundation of China,Grant/Award Numbers:62174049,52003073,52102285。
文摘A 3D nanostructured scaffold as the host for zinc enables effective inhibition of anodic dendrite growth.However,the increased electrode/electrolyte interface area provided by using 3D matrices exacerbates the passivation and localized corrosion of the Zn anode,ultimately bringing about the degradation of the electrochemical performance.Herein,a nanoscale coating of inorganic-organic hybrid(α-In_(2)Se_(3)-Nafion)onto a flexible carbon nanotubes(CNTs)framework(ISNF@CNTs)is designed as a Zn plating/stripping scaffold to ensure uniform Zn nucleation,thus achieving a dendrite-free and durable Zn anode.The intro-duced inorganic-organic interfacial layer is dense and sturdy,which hinders the direct exposure of deposited Zn to electrolytes and mitigates the side reactions.Meanwhile,the zincophilic nature of ISNF can largely reduce the nucleation energy barrier and promote the ion-diffusion transportation.Consequently,the ISNF@CNTs@Zn electrode exhibits a low-voltage hysteresis and a superior cycling life(over 1500 h),with dendrite-free Zn-plating behaviors in a typical symmetrical cell test.Additionally,the superior feature of ISNF@CNTs@Zn anode is further demonstrated by Zn-MnO_(2)cells in both coin and flexible quasi-solid-state configurations.This work puts forward an inspired remedy for advanced Zn-ion batteries.
基金This work was supported by the National Natural Science Foundation of China(Nos.22278324,51932007,22238009,U1905215,52073223,52073034,and 22208332)the Postdoctoral Science Foundation of China(No.2022M712946)the Natural Science Foundation of Hubei Province of China(No.2022CFA001).
文摘Constructing step-scheme(S-scheme)heterojunctions has become a popular strategy for efficient pho-tocatalytic H_(2)O_(2) generation.Herein,we in situ grew BiOBr nanosheets(NSs)on a Schiff-base covalent organic framework(COF)with largeπ-conjugated structures to prepare S-scheme BiOBr/COF photocat-alysts for H_(2)O_(2) synthesis.The highest photocatalytic H_(2)O_(2) production performance of the composite sample constituting the S-scheme heterojunction is 3749μmol g−1 h−1,which was 1.85 and 27 times the rates of COF and BiOBr,respectively.The construction of S-scheme heterojunction contributed to ef-ficient carrier transfer and separation in space and enhanced redox power.Moreover,the lying-down O_(2)-adsorption configuration on the COF surface favors the concerted two-electron O_(2) reduction process,which greatly reduced the reduction potential requirement for O_(2)-to-H_(2)O_(2) conversion.The synergy be-tween the S-scheme heterojunction and the unique O_(2)-COF interaction boosted photocatalytic H_(2)O_(2) pro-duction activity.
基金National Natural Science Foundation of China(11305272)Specialized Research Fund for the Doctoral Program of Higher Education(20130171120014)+2 种基金Fundamental Research Funds for the Central Universities(14lgpy29)Guangdong Natural Science Foundation(2014A030313217)Pearl River S&T Nova Program of Guangzhou(201506010060)
文摘The effect of the two-nucleon excitation from p to sd shell is discussed on12 C and14C in the frame work of the nuclear shell model. The recently suggested shell-model Hamiltonian YSOX provides an suitable tool to investigate the 2hω excitation in psd region. Because the strength of the< pp|V |sdsd > interaction, which represents the interaction between the 0 and 2hω configurations, is considered in the construction of the Hamiltonian YSOX. The level of12 C is almost independent on the < pp|V |sdsd > interaction, but excitation energies of certain states in14 C are strongly affected by it.Further investigation shows that the percentage of 2hω configuration in these states is quite different from that of the ground state. The non-linear effects of the < pp|V |sdsd > interaction on the configurations and transition rates are also discussed.