Limited by the thermal environment, the entanglement of a massive object is extremely difficult to generate. Based on a coherent scattering mechanism, we propose a scheme to generate the entanglement of two optically ...Limited by the thermal environment, the entanglement of a massive object is extremely difficult to generate. Based on a coherent scattering mechanism, we propose a scheme to generate the entanglement of two optically levitated nanospheres through the Coulomb interaction. Two nanospheres are charged and coupled to each other through the Coulomb interaction.In this manner, the entanglement of two nanospheres is induced either under a weak/strong optomechanical coupling regime or under an ultra-strong optomechanical coupling regime. The charges, radius and distance of the two nanospheres are taken into consideration to enhance the Coulomb interaction, thereby achieving a higher degree of entanglement in the absence of ground-state cooling. The corresponding maximum entanglement can be attained as the dynamics of the system approaches the boundary between the steady and the unsteady regimes. This provides a useful resource for both quantum-enhanced sensing and quantum information processing, as well as a new platform for studying many-body physics.展开更多
We investigate the properties of the ponderomotive squeezing in an optomechanical system coupled to a charged nanomecbanical oscillator (NMO) nearby via Coulomb force. We find that the introduction of Coulomb intera...We investigate the properties of the ponderomotive squeezing in an optomechanical system coupled to a charged nanomecbanical oscillator (NMO) nearby via Coulomb force. We find that the introduction of Coulomb interaction allows the generation of squeezed output light from this system. Our numerical results show that the degree of squeezing can be tuned by the Coulomb coupling strength, the power of laser, and the frequencies of NMOs. Furthermore, the squeezing generated in our approach can be used to measure the Coulomb coupling strength.展开更多
We theoretically study the stationary entanglement of two charged nanomechanical oscillators coupling via Coulomb interaction in an optomechanical system with an additional Kerr medium.We show that the degree of entan...We theoretically study the stationary entanglement of two charged nanomechanical oscillators coupling via Coulomb interaction in an optomechanical system with an additional Kerr medium.We show that the degree of entanglement between two nanomechanical oscillators is suppressed by Kerr interaction due to photon blockade and enhanced by Coulomb coupling strength.We also show other parameters for adjusting and obtaining entanglement,such as the driving power and the frequencies of the two oscillators,and the entanglement is robust against temperature.Our study proves a way for adjusting stationary entanglement between two optomechanical oscillators by Coulomb interaction and Kerr medium.展开更多
We propose a scheme for entangling two nanomechanical oscillators by Coulomb interaction in an optomechanical system. We find that the steady-state entanglement of two charged nanomechanical oscillators can be obtaine...We propose a scheme for entangling two nanomechanical oscillators by Coulomb interaction in an optomechanical system. We find that the steady-state entanglement of two charged nanomechanical oscillators can be obtained when the coupling between them is stronger than a critical value which relies on the detuning. Remarkably, the degree of entanglement can be controlled by the Coulomb interaction and the frequencies of the two charged Oscillators.展开更多
The coulomb interaction among TCNQ- molecules in different stack structures was calculated by quantum chemistry CNDO method. The results of the calculation would be used to explain the change rule of the electricity p...The coulomb interaction among TCNQ- molecules in different stack structures was calculated by quantum chemistry CNDO method. The results of the calculation would be used to explain the change rule of the electricity property of the TCNQ complex very well.展开更多
We study electronic transport through a quantum dot (QD) with a precessing magnetic field. By using the Keldysh nonequilibrium Green function method, formulas of local density of states (LDOS) and conductance of Q...We study electronic transport through a quantum dot (QD) with a precessing magnetic field. By using the Keldysh nonequilibrium Green function method, formulas of local density of states (LDOS) and conductance of QD are derived self-consistently. It shows that the LDOS and conductance have obvious changes with the Coulomb blockade interaction. The intensity and angle of the magnetic field or temperatures, which reflect the mesoscopic structure of the QD are derived. The superiority of this device is that the QD can be controlled easily by the magnetic field, so it is valuable to apply in generating, manipulating and probing spin state.展开更多
The diffusion behavior of polyelectrolytes in dilute salt-free solution is studied through a hybrid mesoscale simulation technique that combines the molecular dynamics method and the multiparticle collision dynamics a...The diffusion behavior of polyelectrolytes in dilute salt-free solution is studied through a hybrid mesoscale simulation technique that combines the molecular dynamics method and the multiparticle collision dynamics approach.To elucidate the effects of hydrodynamic interactions(HI),we compare results for hydrodynamic and random solvents.When HI are taken into account,we find that the chain diffusivity decreases initially and then increases gradually with the increasing strength of the Coulomb interaction.By contrast,when HI are switched off,the electrostatic-dependent diffusivity shows three distinct regions,and a plateau of approximately constant diffusivity manifests between two decreasing regions.The findings reveal that the dynamics of polyelectrolytes in dilute solution depend on the coupling effects of hydrodynamic and Coulomb interactions,and that these dynamics can be understood by considering the conformational changes of chains,the counterion condensation,and the dynamics of counterions.展开更多
In this report, the analytical expression of Coulombic interaction between a spherical nanoparticle and a tetragonal nanorod is derived. To evaluate the Coulombic interaction in the oriented attachment growth of tetra...In this report, the analytical expression of Coulombic interaction between a spherical nanoparticle and a tetragonal nanorod is derived. To evaluate the Coulombic interaction in the oriented attachment growth of tetragonal nanorods, we analyze the correlation between the Coulombic interaction and the important growth parameters, including: nanoparticle- nanorod separation, aspect ratio of the nanorods, and surface charge density. Our work opens up the opportunity to investi-gate interparticle interactions in the oriented attachment growth of tetragonal nanorods.展开更多
We investigate the low-energy structure (LES) in the above-threshold ionization spectrum at a mid-infrared laser wavelength with a semiclassical model. Using a softened Coulomb potential (CP) and changing the soft...We investigate the low-energy structure (LES) in the above-threshold ionization spectrum at a mid-infrared laser wavelength with a semiclassical model. Using a softened Coulomb potential (CP) and changing the softening parameter, we show that though the very low-energy structure (VLES) and high low-energy structure (HLES) are both due to the interaction between the ionic CP and the electron, the two structures have different physical mechanisms: the VLES can be attributed to the electron-ion Coulomb interaction at a rather small distance and the HLES is more likely to be ascribed to the electron-ion Coulomb interaction at a large distance.展开更多
It has been found that cold plasma is a facile and environmentally benign method for synthesizing supported metal catalysts, and great efforts have been devoted to enlarging its applications. However, little work has ...It has been found that cold plasma is a facile and environmentally benign method for synthesizing supported metal catalysts, and great efforts have been devoted to enlarging its applications. However, little work has been done to disclose the influence mechanism, which is significant for controllable synthesis. In this work, hydrogen cold plasma was adopted to synthesize a palladium catalyst supported on activated carbon (Pd/C-P) using HzPdC14 as a Pd precursor followed by calcination in hydrogen gas to remove the chlorine ions. The Pd/C-P catalyst was found to be made of larger Pd nanoparticles showing a decreased migration to the support outer surface than that prepared by the conventional thermal hydrogen reduction method (Pd/C-C). Meanwhile, the pore diameter of the activated carbon support is small (,-~4 nm). Therefore, Pd/C-P exhibits lower CO oxidation activity than Pd/C-C. It was proposed that the strong interaction between the activated carbon and PdC142-, and the enhanced metal-support interaction caused by hydrogen cold plasma reduction made it difficult for Pd nanoparticles to migrate to the support outer surface. The larger-sized Pd nanoparticles for Pd/C-P may be due to the Coulomb interaction resulting in the disturbance of the metal-support interaction. This work has important guiding significance for the controllable synthesis of supported metal catalysts by hydrogen cold plasma.展开更多
Density functional theory calculations corrected by on-site Coulomb interactions were carried out o study the structures of polar CeO2 (100) surfaces as well as activities during catalytic CO oxidation. The stabilit...Density functional theory calculations corrected by on-site Coulomb interactions were carried out o study the structures of polar CeO2 (100) surfaces as well as activities during catalytic CO oxidation. The stabilities of various CeO2 (100) termination structures are discussed, and calculated energetics are presented. The most stable Ce〇2 (100) surface was obtained by removing half the outermost full layer of oxygen and the surface stability was found to decrease as the exposed oxygen concentration was increased. Assessing the reaction pathways leading to different final products during CO oxidation over the most stable CeO2 (100) surface, we determined that the formation of carbonate species competed with CO2 desorption. However, during CO oxidation on the less stable CeO2 (100) surfaces having more exposed oxygen, the CO is evidently able to react with surface oxygen, leading to CO2 formation and desorption. The calculation results and electronic analyses reported herein also indicate that the characteristic Ce 4/ orbitals are directly involved in deter-mining the surface stabilities and reactivities.展开更多
The spectral line intensities and line shifts of Lyman and Balmer series for transitions up to n=5 of hydrogen-like ion are studied in plasmas with densities and temperatures in the ranges n_(c)~10^(18)-10^(21)cm^(-3)...The spectral line intensities and line shifts of Lyman and Balmer series for transitions up to n=5 of hydrogen-like ion are studied in plasmas with densities and temperatures in the ranges n_(c)~10^(18)-10^(21)cm^(-3),T_(e)=0.3e1.2 eV respectively.The screened potential used to describe the interaction between charged particles includes the electron exchange-correlation and finite-temperature gradient effects and is valid for both weakly and strongly coupled plasmas.The dependencies of alpha,beta and gamma line shifts of Lyman and Balmer series on plasma density(for fixed temperature)and temperature(for fixed density)are investigated.The results for the H_(a)line shifts are compared with the available high-density experimental data.展开更多
We perform a variational Monte Carlo study of the nematic state in iron-pnictide superconductors within a realistic five-orbital model. Our numerical results show that the nematic state, formed by introducing an aniso...We perform a variational Monte Carlo study of the nematic state in iron-pnictide superconductors within a realistic five-orbital model. Our numerical results show that the nematic state, formed by introducing an anisotropic hopping order into the projected wave function, is not stable unless the off-site Coulomb interaction V exceeds a critical value. This demonstrates that V plays a key role in forming the nematic state in iron-pnictide superconductors. In the nematic state,the orbital order and the anisotropic spin correlations are consistent with the experimental observations. We argue that the experimentally observed anisotropic magnetic couplings and structural transition are associated with the nematic state and can be understood in a unified framework.展开更多
We study the effect of structure asymmetry on the energy spectrum and the far-infrared spectrum (FIR) of a lateral coupled quantum dot. The calculated spectrum shows that the parity break of coupled quantum dot resu...We study the effect of structure asymmetry on the energy spectrum and the far-infrared spectrum (FIR) of a lateral coupled quantum dot. The calculated spectrum shows that the parity break of coupled quantum dot results in more coherent superpositions in the low-lying states and exhibits unique anti-crossing in the two-electron FIR spectrum modulated by a magnetic field. We also find that the Coulomb correlation effect can make the FIR spectrum of coupled quantum dot without strict parity deviate greatly from Kohn theorem, which is just contrary to the symmetric case. Our results therefore suggest that FIR spectrum may be used to determine the symmetry of coupled quantum dot and to evaluate the degree of Coulomb interaction.展开更多
Calculation results of the Monte Carlo method of the average energy of the electrostatic interaction between the quarks are presented to the neutron and proton. The proposed model of the distribution of quarks in prot...Calculation results of the Monte Carlo method of the average energy of the electrostatic interaction between the quarks are presented to the neutron and proton. The proposed model of the distribution of quarks in protons and neutrons is possible to assess the area which included a strong (gluon) interaction. Given the fact that the probability of finding a quark in the field with strong interaction is less than one, there is a good agreement between the experimental and calculated values of the mass difference between the neutron and the proton.展开更多
The mixed alkali effect was investigated in the glass system 0.75B2O3-0.25[xNa2O-(1 -x)K20] through thermodynamic properties. The calorimetric measurements were performed in HF solution calorimetry at 298 K. The mix...The mixed alkali effect was investigated in the glass system 0.75B2O3-0.25[xNa2O-(1 -x)K20] through thermodynamic properties. The calorimetric measurements were performed in HF solution calorimetry at 298 K. The mixing enthalpy values show non-linear behaviour upon substitution of one alkali ion by another. This thermodynamic non-ideality is caused by the slight variations of distance between metallic cations, the macromolecular structure being unchanged. It can be explained, at least qualitatively, using electrolyte theory based on the Coulombic interactions of charged species originally developed by Debye and Hückel.展开更多
Nanodrugs capable of aggregating in the tumor microenvironment(TME)have demonstrated great efficiency in improving the therapeutic outcome.Among vari-ous approaches,the strategy utilizing electrostatic interaction as a...Nanodrugs capable of aggregating in the tumor microenvironment(TME)have demonstrated great efficiency in improving the therapeutic outcome.Among vari-ous approaches,the strategy utilizing electrostatic interaction as a driving force to achieve intratumor aggregation of nanodrugs has attracted great attention.However,the great difference between the two nanodrugs with varied physicochemical prop-erties makes their synchronous transport in blood circulation and equal-opportunity tumor uptake impossible,which significantly detracts from the beneficial effects of nanodrug aggregation inside tumors.We herein propose a new strategy to construct a pair of extremely similar nanodrugs,referred to as“twins-like nanodrugs(TLNs)”,which have identical physicochemical properties including the same morphology,size,and electroneutrality to render them the same blood circulation time and tumor entrance.The 1:1 mixture of TLNs(TLNs-Mix)intravenously injected into a mouse model efficiently accumulates in tumor sites and then transfers to oppositely charged nanodrugs for electrostatic interaction-driven coalescence via responding to matrix metalloproteinase-2(MMP-2)enriched in tumor.In addition to enhanced tumor retention,the thus-formed micron-sized aggregates show high echo intensity essen-tial for ultrasound imaging as well as ultrasound-triggered penetrative drug delivery.Owing to their distinctive features,the TLNs-Mix carrying sonosensitizer,immune adjuvant,and ultrasound contrast agent exert potent sonodynamic immunotherapy against hypovascular hepatoma,demonstrating their great potential in treating solid malignancies.展开更多
Scanning tunneling microscopy study revealed a van der Waals C60, solid film with 13% room-temperature lattice expansion on the GaAs(001) 2×4 surface. The mechanism involves fundamental Coulomb interaction due to...Scanning tunneling microscopy study revealed a van der Waals C60, solid film with 13% room-temperature lattice expansion on the GaAs(001) 2×4 surface. The mechanism involves fundamental Coulomb interaction due to charge transfer from the GaAs substrate. Theoretical calculation determines the charge transfer to be 1.76 electrons per C60 molecule. Oriented at its (110) crystallo-graphic axis this film also distinguishes itself from those formed on all other semiconductor and metal substrates where only the low-energy (111) hexagonal packing of C60 molecules was developed. It is shown that this is due to the one-dimensional confinement effect of the anisotropic substrate, which may have the prospect of controlling crystal growth.展开更多
We theoretically investigate the multistable behavior of a hybrid optomechanical system, in which a charged mechanical resonator is coupled via Coulomb interaction to an optomechanical cavity containing an optical par...We theoretically investigate the multistable behavior of a hybrid optomechanical system, in which a charged mechanical resonator is coupled via Coulomb interaction to an optomechanical cavity containing an optical parametric amplifier (OPA). It is shown that the multistable behavior of the mean intracavity photon number can be controlled flexibly by adjusting the nonlinear gain parameter of the OPA, the phase of the field pumping the OPA, the power and frequency of the field driving the cavity, and the Coulomb coupling strength between the two charged mechanical resonators. In particular, the increase of the nonlinear gain parameter can result in a transition from bistability to tristability. Moreover, the effect of the Coulomb coupling strength on the bistable behavior of the steady-state positions of the two mechanical resonators is discussed.展开更多
Through mean-field calculations,we demonstrate that,in a large Z nucleus binding multiple muons,these heavy leptons localize within a few dozen femtometers of the nucleus.The mutual Coulomb interactions between the mu...Through mean-field calculations,we demonstrate that,in a large Z nucleus binding multiple muons,these heavy leptons localize within a few dozen femtometers of the nucleus.The mutual Coulomb interactions between the muons and protons can lead to a substantial decrease in proton chemical potential,surpassing 1 MeV.These findings imply that,in principle,the proton-dripline can be expanded on the nuclear chart,suggesting the possible production of nuclei with Z around 120.展开更多
基金supported by the National Natural Science Foundation of China(Grant No.61771278)the Beijing Institute of Technology Research Fund Program for Young Scholars。
文摘Limited by the thermal environment, the entanglement of a massive object is extremely difficult to generate. Based on a coherent scattering mechanism, we propose a scheme to generate the entanglement of two optically levitated nanospheres through the Coulomb interaction. Two nanospheres are charged and coupled to each other through the Coulomb interaction.In this manner, the entanglement of two nanospheres is induced either under a weak/strong optomechanical coupling regime or under an ultra-strong optomechanical coupling regime. The charges, radius and distance of the two nanospheres are taken into consideration to enhance the Coulomb interaction, thereby achieving a higher degree of entanglement in the absence of ground-state cooling. The corresponding maximum entanglement can be attained as the dynamics of the system approaches the boundary between the steady and the unsteady regimes. This provides a useful resource for both quantum-enhanced sensing and quantum information processing, as well as a new platform for studying many-body physics.
文摘We investigate the properties of the ponderomotive squeezing in an optomechanical system coupled to a charged nanomecbanical oscillator (NMO) nearby via Coulomb force. We find that the introduction of Coulomb interaction allows the generation of squeezed output light from this system. Our numerical results show that the degree of squeezing can be tuned by the Coulomb coupling strength, the power of laser, and the frequencies of NMOs. Furthermore, the squeezing generated in our approach can be used to measure the Coulomb coupling strength.
基金Project supported by the National Natural Science Foundation of China(Grant No.11704051)。
文摘We theoretically study the stationary entanglement of two charged nanomechanical oscillators coupling via Coulomb interaction in an optomechanical system with an additional Kerr medium.We show that the degree of entanglement between two nanomechanical oscillators is suppressed by Kerr interaction due to photon blockade and enhanced by Coulomb coupling strength.We also show other parameters for adjusting and obtaining entanglement,such as the driving power and the frequencies of the two oscillators,and the entanglement is robust against temperature.Our study proves a way for adjusting stationary entanglement between two optomechanical oscillators by Coulomb interaction and Kerr medium.
基金supported by the Major Research Plan of the National Natural Science Foundation of China(Grant No.91121023)the National Natural Science Foundation of China(Grant Nos.61378012,60978009,and 11574092)+2 种基金the Specialized Research Fund for the Doctoral Program of Higher Education of China(Grant No.20124407110009)the National Basic Research Program of China(Grant Nos.2011CBA00200 and 2013CB921804)the Program for Changjiang Scholar and Innovative Research Team in University,China(Grant No.IRT1243)
文摘We propose a scheme for entangling two nanomechanical oscillators by Coulomb interaction in an optomechanical system. We find that the steady-state entanglement of two charged nanomechanical oscillators can be obtained when the coupling between them is stronger than a critical value which relies on the detuning. Remarkably, the degree of entanglement can be controlled by the Coulomb interaction and the frequencies of the two charged Oscillators.
文摘The coulomb interaction among TCNQ- molecules in different stack structures was calculated by quantum chemistry CNDO method. The results of the calculation would be used to explain the change rule of the electricity property of the TCNQ complex very well.
基金The project supported by National Natural Science Foundation of China under Grant No. 60671042 and the Fundamental Research Foundation for Key Projects of Shanghai Science and Technology Committee under Grant No. 06JC14032 tCorresponding author,
文摘We study electronic transport through a quantum dot (QD) with a precessing magnetic field. By using the Keldysh nonequilibrium Green function method, formulas of local density of states (LDOS) and conductance of QD are derived self-consistently. It shows that the LDOS and conductance have obvious changes with the Coulomb blockade interaction. The intensity and angle of the magnetic field or temperatures, which reflect the mesoscopic structure of the QD are derived. The superiority of this device is that the QD can be controlled easily by the magnetic field, so it is valuable to apply in generating, manipulating and probing spin state.
基金supported by the National Basic Research Program of China(2012CB821500 and 2010CB631102)the National Natural Science Foundation of China(21274153)+1 种基金the support of the National Natural Science Foundation of China(21120102037)Computing Center of Jilin Province for essential support
文摘The diffusion behavior of polyelectrolytes in dilute salt-free solution is studied through a hybrid mesoscale simulation technique that combines the molecular dynamics method and the multiparticle collision dynamics approach.To elucidate the effects of hydrodynamic interactions(HI),we compare results for hydrodynamic and random solvents.When HI are taken into account,we find that the chain diffusivity decreases initially and then increases gradually with the increasing strength of the Coulomb interaction.By contrast,when HI are switched off,the electrostatic-dependent diffusivity shows three distinct regions,and a plateau of approximately constant diffusivity manifests between two decreasing regions.The findings reveal that the dynamics of polyelectrolytes in dilute solution depend on the coupling effects of hydrodynamic and Coulomb interactions,and that these dynamics can be understood by considering the conformational changes of chains,the counterion condensation,and the dynamics of counterions.
基金Project supported by the National Youth Natural Science Foundation,China(Grant No.61106099)
文摘In this report, the analytical expression of Coulombic interaction between a spherical nanoparticle and a tetragonal nanorod is derived. To evaluate the Coulombic interaction in the oriented attachment growth of tetragonal nanorods, we analyze the correlation between the Coulombic interaction and the important growth parameters, including: nanoparticle- nanorod separation, aspect ratio of the nanorods, and surface charge density. Our work opens up the opportunity to investi-gate interparticle interactions in the oriented attachment growth of tetragonal nanorods.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.10925420,11074026,11174330,and 11274050)the National Basic Research Program of China (Grant Nos.2011CB808102 and 2013CB922201)
文摘We investigate the low-energy structure (LES) in the above-threshold ionization spectrum at a mid-infrared laser wavelength with a semiclassical model. Using a softened Coulomb potential (CP) and changing the softening parameter, we show that though the very low-energy structure (VLES) and high low-energy structure (HLES) are both due to the interaction between the ionic CP and the electron, the two structures have different physical mechanisms: the VLES can be attributed to the electron-ion Coulomb interaction at a rather small distance and the HLES is more likely to be ascribed to the electron-ion Coulomb interaction at a large distance.
基金supported by National Natural Science Foundation of China (Grant Nos. 11505019, 21673026)Dalian Youth Science and Technology Project (Grant No. 2015R089)
文摘It has been found that cold plasma is a facile and environmentally benign method for synthesizing supported metal catalysts, and great efforts have been devoted to enlarging its applications. However, little work has been done to disclose the influence mechanism, which is significant for controllable synthesis. In this work, hydrogen cold plasma was adopted to synthesize a palladium catalyst supported on activated carbon (Pd/C-P) using HzPdC14 as a Pd precursor followed by calcination in hydrogen gas to remove the chlorine ions. The Pd/C-P catalyst was found to be made of larger Pd nanoparticles showing a decreased migration to the support outer surface than that prepared by the conventional thermal hydrogen reduction method (Pd/C-C). Meanwhile, the pore diameter of the activated carbon support is small (,-~4 nm). Therefore, Pd/C-P exhibits lower CO oxidation activity than Pd/C-C. It was proposed that the strong interaction between the activated carbon and PdC142-, and the enhanced metal-support interaction caused by hydrogen cold plasma reduction made it difficult for Pd nanoparticles to migrate to the support outer surface. The larger-sized Pd nanoparticles for Pd/C-P may be due to the Coulomb interaction resulting in the disturbance of the metal-support interaction. This work has important guiding significance for the controllable synthesis of supported metal catalysts by hydrogen cold plasma.
基金supported the National Natural Science Foundation of China(21421004,21573067)~~
文摘Density functional theory calculations corrected by on-site Coulomb interactions were carried out o study the structures of polar CeO2 (100) surfaces as well as activities during catalytic CO oxidation. The stabilities of various CeO2 (100) termination structures are discussed, and calculated energetics are presented. The most stable Ce〇2 (100) surface was obtained by removing half the outermost full layer of oxygen and the surface stability was found to decrease as the exposed oxygen concentration was increased. Assessing the reaction pathways leading to different final products during CO oxidation over the most stable CeO2 (100) surface, we determined that the formation of carbonate species competed with CO2 desorption. However, during CO oxidation on the less stable CeO2 (100) surfaces having more exposed oxygen, the CO is evidently able to react with surface oxygen, leading to CO2 formation and desorption. The calculation results and electronic analyses reported herein also indicate that the characteristic Ce 4/ orbitals are directly involved in deter-mining the surface stabilities and reactivities.
基金This work was supported by the National Key Research and Development Program of China(Grant No.2017YFA0402300)National Natural Science Foundation of China(Grants No.11474033,11474032 and 11534011)Science Challenge Project(Grant No.TZ2016001).
文摘The spectral line intensities and line shifts of Lyman and Balmer series for transitions up to n=5 of hydrogen-like ion are studied in plasmas with densities and temperatures in the ranges n_(c)~10^(18)-10^(21)cm^(-3),T_(e)=0.3e1.2 eV respectively.The screened potential used to describe the interaction between charged particles includes the electron exchange-correlation and finite-temperature gradient effects and is valid for both weakly and strongly coupled plasmas.The dependencies of alpha,beta and gamma line shifts of Lyman and Balmer series on plasma density(for fixed temperature)and temperature(for fixed density)are investigated.The results for the H_(a)line shifts are compared with the available high-density experimental data.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11274310,11474287,11174072,and 91221103)the Specialized Research Fund for the Doctoral Program of Higher Education of China(Grant No.20104208110001)
文摘We perform a variational Monte Carlo study of the nematic state in iron-pnictide superconductors within a realistic five-orbital model. Our numerical results show that the nematic state, formed by introducing an anisotropic hopping order into the projected wave function, is not stable unless the off-site Coulomb interaction V exceeds a critical value. This demonstrates that V plays a key role in forming the nematic state in iron-pnictide superconductors. In the nematic state,the orbital order and the anisotropic spin correlations are consistent with the experimental observations. We argue that the experimentally observed anisotropic magnetic couplings and structural transition are associated with the nematic state and can be understood in a unified framework.
基金supported by the National Natural Science Foundation of China (Grant No.11074025)the National Basic Research Program of China (Grant No.2011CB922200)a grant from the China Academy of Engineering Physics
文摘We study the effect of structure asymmetry on the energy spectrum and the far-infrared spectrum (FIR) of a lateral coupled quantum dot. The calculated spectrum shows that the parity break of coupled quantum dot results in more coherent superpositions in the low-lying states and exhibits unique anti-crossing in the two-electron FIR spectrum modulated by a magnetic field. We also find that the Coulomb correlation effect can make the FIR spectrum of coupled quantum dot without strict parity deviate greatly from Kohn theorem, which is just contrary to the symmetric case. Our results therefore suggest that FIR spectrum may be used to determine the symmetry of coupled quantum dot and to evaluate the degree of Coulomb interaction.
文摘Calculation results of the Monte Carlo method of the average energy of the electrostatic interaction between the quarks are presented to the neutron and proton. The proposed model of the distribution of quarks in protons and neutrons is possible to assess the area which included a strong (gluon) interaction. Given the fact that the probability of finding a quark in the field with strong interaction is less than one, there is a good agreement between the experimental and calculated values of the mass difference between the neutron and the proton.
文摘The mixed alkali effect was investigated in the glass system 0.75B2O3-0.25[xNa2O-(1 -x)K20] through thermodynamic properties. The calorimetric measurements were performed in HF solution calorimetry at 298 K. The mixing enthalpy values show non-linear behaviour upon substitution of one alkali ion by another. This thermodynamic non-ideality is caused by the slight variations of distance between metallic cations, the macromolecular structure being unchanged. It can be explained, at least qualitatively, using electrolyte theory based on the Coulombic interactions of charged species originally developed by Debye and Hückel.
基金Key Areas Research and Development Program of Guangzhou,Grant/Award Number:202007020006National Natural Science Foundation of China,Grant/Award Numbers:51933011,31971296,52173125,82102194Natural Science Foundation of the Guangdong Province,Grant/Award Numbers:2021A1515111006,2023A1515011822。
文摘Nanodrugs capable of aggregating in the tumor microenvironment(TME)have demonstrated great efficiency in improving the therapeutic outcome.Among vari-ous approaches,the strategy utilizing electrostatic interaction as a driving force to achieve intratumor aggregation of nanodrugs has attracted great attention.However,the great difference between the two nanodrugs with varied physicochemical prop-erties makes their synchronous transport in blood circulation and equal-opportunity tumor uptake impossible,which significantly detracts from the beneficial effects of nanodrug aggregation inside tumors.We herein propose a new strategy to construct a pair of extremely similar nanodrugs,referred to as“twins-like nanodrugs(TLNs)”,which have identical physicochemical properties including the same morphology,size,and electroneutrality to render them the same blood circulation time and tumor entrance.The 1:1 mixture of TLNs(TLNs-Mix)intravenously injected into a mouse model efficiently accumulates in tumor sites and then transfers to oppositely charged nanodrugs for electrostatic interaction-driven coalescence via responding to matrix metalloproteinase-2(MMP-2)enriched in tumor.In addition to enhanced tumor retention,the thus-formed micron-sized aggregates show high echo intensity essen-tial for ultrasound imaging as well as ultrasound-triggered penetrative drug delivery.Owing to their distinctive features,the TLNs-Mix carrying sonosensitizer,immune adjuvant,and ultrasound contrast agent exert potent sonodynamic immunotherapy against hypovascular hepatoma,demonstrating their great potential in treating solid malignancies.
文摘Scanning tunneling microscopy study revealed a van der Waals C60, solid film with 13% room-temperature lattice expansion on the GaAs(001) 2×4 surface. The mechanism involves fundamental Coulomb interaction due to charge transfer from the GaAs substrate. Theoretical calculation determines the charge transfer to be 1.76 electrons per C60 molecule. Oriented at its (110) crystallo-graphic axis this film also distinguishes itself from those formed on all other semiconductor and metal substrates where only the low-energy (111) hexagonal packing of C60 molecules was developed. It is shown that this is due to the one-dimensional confinement effect of the anisotropic substrate, which may have the prospect of controlling crystal growth.
基金supported by the National Natural Science Foundation of China(Grant No.11304110)the Natural Science Foundation of Jiangsu Province(Grant Nos.BK20130413 and BK20140450)the Natural Science Foundation of the Jiangsu Higher Education Institutions of China (Grant No.13KJB140002)
文摘We theoretically investigate the multistable behavior of a hybrid optomechanical system, in which a charged mechanical resonator is coupled via Coulomb interaction to an optomechanical cavity containing an optical parametric amplifier (OPA). It is shown that the multistable behavior of the mean intracavity photon number can be controlled flexibly by adjusting the nonlinear gain parameter of the OPA, the phase of the field pumping the OPA, the power and frequency of the field driving the cavity, and the Coulomb coupling strength between the two charged mechanical resonators. In particular, the increase of the nonlinear gain parameter can result in a transition from bistability to tristability. Moreover, the effect of the Coulomb coupling strength on the bistable behavior of the steady-state positions of the two mechanical resonators is discussed.
基金Supported by the Natural Science Foundation of China(11775099)。
文摘Through mean-field calculations,we demonstrate that,in a large Z nucleus binding multiple muons,these heavy leptons localize within a few dozen femtometers of the nucleus.The mutual Coulomb interactions between the muons and protons can lead to a substantial decrease in proton chemical potential,surpassing 1 MeV.These findings imply that,in principle,the proton-dripline can be expanded on the nuclear chart,suggesting the possible production of nuclei with Z around 120.