Archimedean photonic crystal has become a research area of great interest due to its various unique properties. Here, we experimentally demonstrate the realization of reconfigurable(4, 6^(2))and(4, 8^(2)) Archimedean ...Archimedean photonic crystal has become a research area of great interest due to its various unique properties. Here, we experimentally demonstrate the realization of reconfigurable(4, 6^(2))and(4, 8^(2)) Archimedean plasma photonic crystals(APPCs) by use of dielectric barrier discharges in air. Dynamical control on both the macrostructures including the lattice symmetry and the crystal orientation, and the microstructures including the fine structures of scattering elements has been achieved. The formation mechanisms of APPCs are studied by time-resolved measurements together with numerical simulations. Large omnidirectional band gaps of APPCs have been obtained. The tunable topology of APPCs may offer new opportunities for fabricating multi-functional and highly-integrated microwave devices.展开更多
Improving energy efficiency in plasma NO removal is a critical issue.When the surface dielectric barrier discharge(SDBD)device is considered as a combination of multiple plasma actuators,the induced plasma aerodynamic...Improving energy efficiency in plasma NO removal is a critical issue.When the surface dielectric barrier discharge(SDBD)device is considered as a combination of multiple plasma actuators,the induced plasma aerodynamic effect cannot be ignored,which can affect the mass transfer,then affect the chemical reactions.Five SDBD devices with different electrode arrangements are studied for NO conversion.They correspond to different flow patterns.We find that the energy efficiency in an SDBD device with a common structure(Type 1)is 28%lower than that in SDBD devices with a special arrangement(Types 2–5).Two reasons may explain the results.First,fewer active species are produced in Type 1 because the development of discharge is hindered by the mutually exclusive electric field forces caused by the symmetrically distributed charged particles.Second,the plasma wind induced by the plasma actuator can enhance the mass and heat transfer.The mixing of reactants and products is better in Types 2–5 than Type 1 due to higher turbulence kinetic energy.展开更多
The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)conten...The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)content on the PDBD morphology, and revealed the possible underlying mechanism of the U-shaped formation. First, the morphological evolution under different conditions was recorded. A unique U-shaped region appears in the middle edge region when the gap is larger than 2 mm, while the entire discharge region remains columnar under a 2 mm gap in He PDBD. The width of the discharge and the U-shaped region increase with the increase in voltage, and decrease with the increase of the gap and O_(2)content. To explain this phenomenon,a two-dimensional symmetric model was developed to simulate the spatiotemporal evolution of different species and calculate the electric thrust. The discharge morphology evolution directly corresponds to the excited-state atomic reduction process. The electric thrust on the charged particles mainly determines the reaction region and strongly influences the U-shaped formation.When the gap is less than 2 mm, the electric thrust is homogeneous throughout the entire region,resulting in a columnar shape. However, when the gap is larger than 2 mm or O_(2)is added, the electric thrust in the edge region becomes greater than that in the middle, leading to the U-shaped formation. Furthermore, in He PDBD, the charged particles generating electric thrust are mainly electrons and helium ions, while in He/O_(2)PDBD those that generate electric thrust at the outer edge of the electrode surface are mainly various oxygen-containing ions.展开更多
The destruction of gaseous styrene was studied using a low-temperature plasma induced by tubular multilayer dielectric barrier discharge(DBD).The results indicate that the applied voltage,gas flow rate,inlet styrene...The destruction of gaseous styrene was studied using a low-temperature plasma induced by tubular multilayer dielectric barrier discharge(DBD).The results indicate that the applied voltage,gas flow rate,inlet styrene concentration and reactor configuration play important roles in styrene removal efficiency (ηstyrene) and energy yield(EY).Values of ηstyrene and EY reached 96%and 15567 mg/kWh when the applied voltage,gas flow rate,inlet styrene concentration and layers of quartz tubes were set at 10.8 kV,5.0 m/s,229 mg/m^3 and 5 layers,respectively.A qualitative analysis of the byproducts and a detailed discussion of the reaction mechanism are also presented.The results could facilitate industrial applications of the new DBD reactor for waste gas treatment.展开更多
An experimental system was established to explore the plasma flow control effect for helicopter rotors in hover mode.With the plasma actuator applied at the leading edge of the rotor blades,alternating current dielect...An experimental system was established to explore the plasma flow control effect for helicopter rotors in hover mode.With the plasma actuator applied at the leading edge of the rotor blades,alternating current dielectric barrier discharge(AC-DBD) plasma actuation was generated by a sinusoidal AC high-voltage generator.By direct force measurement,the influence of actuation parameters on the aerodynamic performance of the rotor was investigated at a tip Reynolds number of 1.7 × 105.AC-DBD actuation can delay the blade stall to more than 3° with a 20%increase of about in the thrust coefficient at the post-stall pitch.At a constant motor power driving the rotor,AC-DBD actuation could reduce the rotor’s torque at the stalled pitch and increase the rotational speed of the rotor.Also,AC-DBD actuation could maintain a relatively high hover efficiency of the rotor at large collective pitches.In a wide range of actuation parameters,AC-DBD plasma actuation could improve the rotor’s aerodynamic performance at large blade pitches.High-speed photography of the tuft motion on the blade’s upper surface showed that AC-DBD plasma actuation could promote the reattachment of the blade’s separation flow.展开更多
We report five types of patterns with square symmetry,including three novel types obtained by inserting a specially designed grid photonic crystal(PC)into a dielectric barrier discharge system.They are studied using a...We report five types of patterns with square symmetry,including three novel types obtained by inserting a specially designed grid photonic crystal(PC)into a dielectric barrier discharge system.They are studied using an intensified charge-coupled device camera and photomultiplier tubes.The three novel types of patterns are a square pattern with one structure,a square superlattice pattern with four sublattices and a(1/4)K_(grid)(K_(grid)is the basic wave vector of the grid),and another square pattern with a complex inversion discharge sequence.From the application viewpoint,the five types of patterns can be used as plasma photonic crystals(PPCs).Their band diagrams under a transverse-magnetic wave simulated by the finite element method show that there are a large number of band gaps.Compared with the original PC with only a unidirectional band gap,the five types of PPCs have tunable and omnidirectional band gaps,which is very important in controlling the propagation of electromagnetic waves in the mm-wave region.The experimental results enrich the pattern types in the dielectric barrier discharge system and provide a method for obtaining PPCs with symmetry controllability and bandgap tunability.展开更多
Sulfamethoxazole(SMX)is an antibiotic and widely present in aquatic environments,so it presents a serious threat to human health and sustainable development.A dielectric barrier discharge(DBD)plasma jet was utilized t...Sulfamethoxazole(SMX)is an antibiotic and widely present in aquatic environments,so it presents a serious threat to human health and sustainable development.A dielectric barrier discharge(DBD)plasma jet was utilized to degrade aqueous SMX,and the effects of various operating parameters(working gas,discharge power,etc)on SMX degradation performance were studied.The experimental results showed that the DBD plasma jet can obtain a relatively high degradation efficiency for SMX when the discharge power is high with an oxygen atmosphere,the initial concentration of SMX is low,and the aqueous solution is under acidic conditions.The reactive species produced in the liquid phase were detected,and OH radicals and O3were found to play a significant role in the degradation of SMX.Moreover,the process of SMX degradation could be better fitted by the quasi-first-order reaction kinetic equation.The analysis of the SMX degradation process indicated that SMX was gradually decomposed and 4-amino benzene sulfonic acid,benzene sulfonamide,4-nitro SMX,and phenylsulfinyl acid were detected,and thus three possible degradation pathways were finally proposed.The mineralization degree of SMX reached 90.04%after plasma treatment for 20 min,and the toxicity of the solution fluctuated with the discharge time but eventually decreased.展开更多
The paper presents comparative kinetic characteristics of the decomposition of 2,4-dichlorophenol in a dielectric barrier discharge and a combined plasma-catalytic process. Vermiculite containing 5% zirconium was used...The paper presents comparative kinetic characteristics of the decomposition of 2,4-dichlorophenol in a dielectric barrier discharge and a combined plasma-catalytic process. Vermiculite containing 5% zirconium was used as a catalyst. The destruction processes of 2,4-DCP proceed efficiently, the degree of decomposition increases in the combined plasma-catalytic process by a factor of 1.33 and reaches 80%. The experimental results were processed according to the first-order kinetic law (R<sup>2</sup> > 0.97), according to which the effective constants (0.36 ± 0.04) and (0.51 ± 0.03) s<sup>-1</sup> and the decomposition rates of 2,4-DCP (106 and 123 μmol/l·s) when treating model solutions without a catalyst and with vermiculite + Zr 5%, respectively, and the energy costs are 0.012 and 0.017 molecules/100eV. The main decomposition products present in the solution have been determined to be carboxylic acids, aldehydes, the contribution of which does not exceed 2%, as well as chloride ions, and in the gas phase they are carbon dioxide and molecular chlorine (the share of which does not exceed 1.5% of total chlorine content in the system).展开更多
The surface dielectric barrier discharge (SDBD) plasma actuator has shown great promise as an aerodynamic flow control device. In this paper, the encapsulated electrode width of a SDBD actuator is changed to study t...The surface dielectric barrier discharge (SDBD) plasma actuator has shown great promise as an aerodynamic flow control device. In this paper, the encapsulated electrode width of a SDBD actuator is changed to study the airflow acceleration behavior. The effects of encapsulated electrode width on the actuator performance are experimentally investigated by measuring the dielectric layer surface potential, time-averaged ionic wind velocity and thrust force. Experimental results show that the airflow velocity and thrust force increase with the encapsulated electrode width. The results can be attributed to the distinct plasma distribution at different encapsulated electrode widths.展开更多
The electronic excitation temperature of a surface dielectric barrier discharge (DBD) at atmospheric pressure has been experimentally investigated by optical emission spectroscopic measurements combined with numeric...The electronic excitation temperature of a surface dielectric barrier discharge (DBD) at atmospheric pressure has been experimentally investigated by optical emission spectroscopic measurements combined with numerical simulation. Experiments have been carried out to deter- mine the spatial distribution of electric field by using FEM software and the electronic excitation temperature in discharge by calculating ratio of two relative intensities of atomic spectral lines. In this work, we choose seven Ar atomic emission lines at 415.86 nm [(3s^23p^5)5p →(3s^23p^5)4s] and 706.7 nm, 714.7 nm, 738.4 nm, 751.5 nm, 794.8 nm and 800.6 nm [(3s^23p^5)4p → (3s^23p^5)4s] to estimate the excitation temperature under a Boltzmann approximation. The average electron energy is evaluated in each discharge by using line ratio of 337.1 nm (N2(C^3Пu →B3Пg)) to 391.4 nm (N2^+(B2 ∑u^+→ ∑g^+)). Furthermore, variations of the electronic excitation tempera- ture are presented versus dielectric thickness and dielectric materials. The discharge is stable and uniform along the axial direction, and the electronic excitation temperature at the edge of the copper electrode is the largest. The corresponding average electron energy is in the range of 1.6- 5.1 eV and the electric field is in 1.7-3.2 MV/m, when the distance from copper electrode varies from 0 cm to 6 cm. Moreover, the electronic excitation temperature with a higher permittivity leads to a higher dissipated electrical power.展开更多
Influence of plasma actuators as a flow separation control device was investigated experimentally. Hump model was used to demonstrate the effect of plasma actuators on external flow separation, while for internal flow...Influence of plasma actuators as a flow separation control device was investigated experimentally. Hump model was used to demonstrate the effect of plasma actuators on external flow separation, while for internal flow separation a set of compressor cascade was adopted. In order to investigate the modification of the flow structure by the plasma actuator, the flow field was examined non-intrusively by particle image velocimetry measurements in the hump model experiment and by a hot film probe in the compressor cascade experiment. The results showed that the plasma actuator could be effective in controlling the flow separation both over the hump and in the compressor cascade when the incoming velocity was low. As the incoming velocity increased, the plasma actuator was less effective. It is urgent to enhance the intensity of the plasma actuator for its better application. Methods to increase the intensity of plasma actuator were also studied.展开更多
The article improves the process of dielectric barrier discharge(DBD)activated anode bonding.The treated surface was characterized by the hydrophilic surface test.The results showed that the hydrophilic angle was sign...The article improves the process of dielectric barrier discharge(DBD)activated anode bonding.The treated surface was characterized by the hydrophilic surface test.The results showed that the hydrophilic angle was significantly reduced under nano-gap conditions and the optimal discharge voltage was 2 kV.Then,the anodic bonding and dielectric barrier discharge activated bonding were performed in comparison experiments,and the bonding strength was characterized by tensile failure test.The results showed that the bonding strength was higher under the nano-gap dielectric barrier discharge.This process completed 110°C ultra-low temperature anodic bonding and the bonding strength reached 2 MPa.Finally,the mechanism of promoting bonding after activation is also discussed.展开更多
The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a par...The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a parallel DC electrode into the standard DBD design. This design improves the body force and induced jet velocity while allowing flexible control of the induced jet angle, overcoming the limitations of discharge extension and uncontrollable direction in traditional DBD plasma actuators. An integrated plasma power supply has been designed specifically for TES-DBD plasma actuators, streamlining the power supply management. The methodology involves designing the circuit topology for the TES-DBD power supply, followed by simulating and validating its operating principles using Multisim software. The operational performance of the power supply is evaluated through a comprehensive analysis of its electrical,thermal, and aerodynamic properties specific to TES-DBD plasma actuation.展开更多
To optimize the design of plasma injectors,the influence of different external electrodes on plasma-assisted flame stabilization was assessed by using a nonequilibrium plasma injector flame control setup.The electrica...To optimize the design of plasma injectors,the influence of different external electrodes on plasma-assisted flame stabilization was assessed by using a nonequilibrium plasma injector flame control setup.The electrical characteristics of the injector,flame structure parameters,flame intensity,discharge power,and cost-to-effectiveness ratio under different external electrodes(four mesh electrodes and one copper foil electrode)were analyzed using electrical and optical methods.The results show that reducing the mesh size of the external electrode leads to a decrease in breakdown voltage.Compared with a ceramic dielectric barrier-based injector,an injector with a quartz dielectric barrier produces a higher breakdown voltage under the same conditions.For the same actuation voltage,the discharge current increases as the mesh size of the external electrode decreases,and combustion is enhanced by the discharge plasma;therefore,it is better to adopt a smaller mesh hole size to realize good flame stabilization under a lower actuation voltage.However,under the studied working conditions,reducing the mesh hole size of the external electrode increases the cost-to-effectiveness ratio of plasma injector-based flame stabilization.Thus,considering the cost-to-effectiveness ratio and the weight of the injector,an external electrode with a larger mesh hole size should be chosen,which contradicts the above rule.展开更多
In order to better analyze the characteristics of particle distribution and its influencing factors in the ionized space during the process of coaxial dielectric barrier discharge,a self-designed two-dimensional axisy...In order to better analyze the characteristics of particle distribution and its influencing factors in the ionized space during the process of coaxial dielectric barrier discharge,a self-designed two-dimensional axisymmetric structure exciter was used to carry out optical diagnosis,with the electron temperature calculated through Gaussian fitting.A plasma model was applied to conduct research on the discharge process through numerical simulation,with the changes in electron density and electron temperature were analyzed by using different discharge parameters.The research results show that with an increase in discharge voltage,pressure inside the reactor and relative permittivity,the discharge process is promoted.In addition,a rise in current density leads to an increase in the number of charged particles on the surface of the medium during the discharge process,while a rise in discharge intensity causes an increase in the electron density.Electron temperature decreases due to the increased loss of collision energy between particles.These results were confirmed by comparing experimental data with simulation results.展开更多
Dielectric barrier discharge(DBD) plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for ...Dielectric barrier discharge(DBD) plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for the first time. X‐ray diffraction, N2 adsorption, ultraviolet–visible spectroscopy, scanning electron microscopy, transmission electron microscopy, X‐ray photoelectron spectrosco‐py, electrochemical impedance spectroscopy, electron paramagnetic resonance, O2 tempera‐ture‐programmed desorption, and photoluminescence were used to characterize the obtained cat‐alysts. The photocatalytic H2O2 production ability of the as‐prepared catalyst was investigated. The results show that plasma treatment influences the morphology, structure, and optical properties of the as‐prepared catalyst. Nitrogen vacancies are active centers, which can adsorb reactant oxygen molecules, trap photoelectrons, and promote the transfer of photoelectrons from the catalyst to the adsorbed oxygen molecules for the subsequent reduction reaction. This work provides a new strat‐egy for synthesizing g‐C3N4‐based catalysts.展开更多
A superimposed wire-plate dielectric barrier discharge reactor was used to remove toluene in this study. The effects of oxygen content, gas flow rate, gas initial concentration and with/without catalyst on toluene dec...A superimposed wire-plate dielectric barrier discharge reactor was used to remove toluene in this study. The effects of oxygen content, gas flow rate, gas initial concentration and with/without catalyst on toluene decomposition were investigated. It was found that an optimal toluene removal was achieved when the oxygen content was about 5%. Under this condition, the highest toluene removal efficiency of 80.8% was achieved when the gas concentration was 80 mg/m^3. The toluene removal efficiency decreased with the increase of the gas flow rate and the initial concentration of toluene. In addition, the ozone concentration decreased with the increase of the initial concentration of toluene. It suggested that combining DBD (dielectric barrier discharge) with Co3O4/Al2O3/foam nickel catalyst in-situ could improve the toluene removal efficiency and suppress ozone formation. Products analysis showed that the main products were CO and CO2 when oxygen was more than 5%.展开更多
The humidity effects on the benzene decomposition process were investigated by the dielectric barrier discharge(DBD) plasma reactor.The results showed that the water vapor played an important role in the benzene oxi...The humidity effects on the benzene decomposition process were investigated by the dielectric barrier discharge(DBD) plasma reactor.The results showed that the water vapor played an important role in the benzene oxidation process.It was found that there was an optimum humidity value for the benzene removal efficiency,and at around 60% relative humidity(RH),the optimum benzene removal efficiency was achieved.At a SIE of 378 J/L,the removal efficiency was 66% at 0% RH,while the removal efficiency reached 75.3% at 60% RH and dropped to 69% at 80% RH.Furthermore,the addition of water inhibited the formation of ozone and NO2 remarkably.Both of the concentrations of ozone and NO2 decreased with increasing of the RH at the same specific input energy.At a SIE of 256 J/L,the concentrations of ozone and NO2 were 5.4 mg/L and 1791 ppm under dry conditions,whereas they were only 3.4 mg/L and 1119 ppm at 63.5%RH,respectively.Finally,the outlet gas after benzene degradation was qualitatively analyzed by FT-IR and GC-MS to determine possible intermediate byproducts.The results suggested that the byproducts in decomposition of benzene primarily consisted of phenol and substitutions of phenol.Based on these byproducts a benzene degradation mechanism was proposed.展开更多
Experimental investigation was conducted to convert dimethyl ether (DME) in the presence of steam using dielectric barrier discharge (DBD) at atmospheric pressure and 373 K. The flow rate of DME was 20 ml/min. The int...Experimental investigation was conducted to convert dimethyl ether (DME) in the presence of steam using dielectric barrier discharge (DBD) at atmospheric pressure and 373 K. The flow rate of DME was 20 ml/min. The introduction of steam resulted in an increase in the DME conversion and the selectivity of oxygenates. Plasma steam-enhanced dimethyl ether (DME) conversion led to a direct synthesis of DMMT and DMET, with a high selectivity of 5.78% and 17.99%, respectively. The addition of steam promoted the formation of 'plasma aerosol' that was favored for the formation of liquid oxygenates. The reaction pathway of plasma DME conversion was proposed.展开更多
Plasma flow control(PFC) is a promising active flow control method with its unique advantages including the absence of moving components, fast response, easy implementation, and stable operation. The effectiveness o...Plasma flow control(PFC) is a promising active flow control method with its unique advantages including the absence of moving components, fast response, easy implementation, and stable operation. The effectiveness of plasma flow control by microsecond dielectric barrier discharge(μs-DBD), and by nanosecond dielectric barrier discharge(NS-DBD) are compared through the wind tunnel tests, showing a similar performance between μs-DBD and NS-DBD. Furthermore, theμs-DBD is implemented on an unmanned aerial vehicle(UAV), which is a scaled model of a newly developed amphibious plane. The wingspan of the model is 2.87 m, and the airspeed is no less than 30 m/s. The flight data, static pressure data,and Tufts images are recorded and analyzed in detail. Results of the flight test show that the μs-DBD works well on board without affecting the normal operation of the UAV model. When the actuators are turned on, the stall angle and maximum lift coefficient can be improved by 1.3° and 10.4%, and the static pressure at the leading edge of the wing can be reduced effectively in a proper range of angle of attack, which shows the ability of μs-DBD to act as plasma slats. The rolling moment produced by left-side μs-DBD actuation is greater than that produced by the maximum deflection of ailerons,which indicates the potential of μs-DBD to act as plasma ailerons. The results verify the feasibility and efficacy of μs-DBD plasma flow control in a real flight and lay the foundation for the full-sized airplane application.展开更多
基金supported by National Natural Science Foundation of China(Nos.12275065 and 11975089)Natural Science Foundation of Hebei Province(Nos.A2021201010 and A2021201003)+4 种基金Interdisciplinary Research Program of Natural Science of Hebei University(No.DXK202108)Hebei Provincial Central Government Guiding Local Science and Technology Development Funds(No.236Z1501G)Scientific Research and Innovation Team Foundation of Hebei University(No.IT2023B03)The Excellent Youth Research Innovation Team of Hebei University(No.QNTD202402)Regional Key Projects of National Natural Science Foundation of China(No.U23A20678).
文摘Archimedean photonic crystal has become a research area of great interest due to its various unique properties. Here, we experimentally demonstrate the realization of reconfigurable(4, 6^(2))and(4, 8^(2)) Archimedean plasma photonic crystals(APPCs) by use of dielectric barrier discharges in air. Dynamical control on both the macrostructures including the lattice symmetry and the crystal orientation, and the microstructures including the fine structures of scattering elements has been achieved. The formation mechanisms of APPCs are studied by time-resolved measurements together with numerical simulations. Large omnidirectional band gaps of APPCs have been obtained. The tunable topology of APPCs may offer new opportunities for fabricating multi-functional and highly-integrated microwave devices.
基金supported by the National Natural Science Foundation of China(60906053,61204069,61274118,61306144,61504079,and 11605112)Scientific and Innovative Action Plan of Shanghai(15DZ1160800 and 17XD1702400)China Postdoctoral Science Foundation(2016 M601595).
文摘Improving energy efficiency in plasma NO removal is a critical issue.When the surface dielectric barrier discharge(SDBD)device is considered as a combination of multiple plasma actuators,the induced plasma aerodynamic effect cannot be ignored,which can affect the mass transfer,then affect the chemical reactions.Five SDBD devices with different electrode arrangements are studied for NO conversion.They correspond to different flow patterns.We find that the energy efficiency in an SDBD device with a common structure(Type 1)is 28%lower than that in SDBD devices with a special arrangement(Types 2–5).Two reasons may explain the results.First,fewer active species are produced in Type 1 because the development of discharge is hindered by the mutually exclusive electric field forces caused by the symmetrically distributed charged particles.Second,the plasma wind induced by the plasma actuator can enhance the mass and heat transfer.The mixing of reactants and products is better in Types 2–5 than Type 1 due to higher turbulence kinetic energy.
基金financial support from the Interdisciplinary Fund of the Wuhan National High Magnetic Field Center (No. WHMFC202101)。
文摘The discharge morphology of pulsed dielectric barrier discharge(PDBD) plays important roles in its applications. Here, we systematically investigated the effects of the voltage amplitude,discharge gap, and O_(2)content on the PDBD morphology, and revealed the possible underlying mechanism of the U-shaped formation. First, the morphological evolution under different conditions was recorded. A unique U-shaped region appears in the middle edge region when the gap is larger than 2 mm, while the entire discharge region remains columnar under a 2 mm gap in He PDBD. The width of the discharge and the U-shaped region increase with the increase in voltage, and decrease with the increase of the gap and O_(2)content. To explain this phenomenon,a two-dimensional symmetric model was developed to simulate the spatiotemporal evolution of different species and calculate the electric thrust. The discharge morphology evolution directly corresponds to the excited-state atomic reduction process. The electric thrust on the charged particles mainly determines the reaction region and strongly influences the U-shaped formation.When the gap is less than 2 mm, the electric thrust is homogeneous throughout the entire region,resulting in a columnar shape. However, when the gap is larger than 2 mm or O_(2)is added, the electric thrust in the edge region becomes greater than that in the middle, leading to the U-shaped formation. Furthermore, in He PDBD, the charged particles generating electric thrust are mainly electrons and helium ions, while in He/O_(2)PDBD those that generate electric thrust at the outer edge of the electrode surface are mainly various oxygen-containing ions.
基金supported by Key Project of Science and Technology Commission of Shanghai Municipality(No.13231201903)National Key Technology R&D Program of China(No.2011BAJ07B04)
文摘The destruction of gaseous styrene was studied using a low-temperature plasma induced by tubular multilayer dielectric barrier discharge(DBD).The results indicate that the applied voltage,gas flow rate,inlet styrene concentration and reactor configuration play important roles in styrene removal efficiency (ηstyrene) and energy yield(EY).Values of ηstyrene and EY reached 96%and 15567 mg/kWh when the applied voltage,gas flow rate,inlet styrene concentration and layers of quartz tubes were set at 10.8 kV,5.0 m/s,229 mg/m^3 and 5 layers,respectively.A qualitative analysis of the byproducts and a detailed discussion of the reaction mechanism are also presented.The results could facilitate industrial applications of the new DBD reactor for waste gas treatment.
文摘An experimental system was established to explore the plasma flow control effect for helicopter rotors in hover mode.With the plasma actuator applied at the leading edge of the rotor blades,alternating current dielectric barrier discharge(AC-DBD) plasma actuation was generated by a sinusoidal AC high-voltage generator.By direct force measurement,the influence of actuation parameters on the aerodynamic performance of the rotor was investigated at a tip Reynolds number of 1.7 × 105.AC-DBD actuation can delay the blade stall to more than 3° with a 20%increase of about in the thrust coefficient at the post-stall pitch.At a constant motor power driving the rotor,AC-DBD actuation could reduce the rotor’s torque at the stalled pitch and increase the rotational speed of the rotor.Also,AC-DBD actuation could maintain a relatively high hover efficiency of the rotor at large collective pitches.In a wide range of actuation parameters,AC-DBD plasma actuation could improve the rotor’s aerodynamic performance at large blade pitches.High-speed photography of the tuft motion on the blade’s upper surface showed that AC-DBD plasma actuation could promote the reattachment of the blade’s separation flow.
基金supported by National Natural Science Foundation of China(No.12075075)the Natural Science Foundation of Hebei Province, China(Nos.2020201016 and A2018201154)。
文摘We report five types of patterns with square symmetry,including three novel types obtained by inserting a specially designed grid photonic crystal(PC)into a dielectric barrier discharge system.They are studied using an intensified charge-coupled device camera and photomultiplier tubes.The three novel types of patterns are a square pattern with one structure,a square superlattice pattern with four sublattices and a(1/4)K_(grid)(K_(grid)is the basic wave vector of the grid),and another square pattern with a complex inversion discharge sequence.From the application viewpoint,the five types of patterns can be used as plasma photonic crystals(PPCs).Their band diagrams under a transverse-magnetic wave simulated by the finite element method show that there are a large number of band gaps.Compared with the original PC with only a unidirectional band gap,the five types of PPCs have tunable and omnidirectional band gaps,which is very important in controlling the propagation of electromagnetic waves in the mm-wave region.The experimental results enrich the pattern types in the dielectric barrier discharge system and provide a method for obtaining PPCs with symmetry controllability and bandgap tunability.
基金supported jointly by National Natural Science Foundation of China(Nos.U20A20372,51807046,51777206)the Natural Science Foundation of Anhui Province(Nos.2108085MD136,1908085MA29)。
文摘Sulfamethoxazole(SMX)is an antibiotic and widely present in aquatic environments,so it presents a serious threat to human health and sustainable development.A dielectric barrier discharge(DBD)plasma jet was utilized to degrade aqueous SMX,and the effects of various operating parameters(working gas,discharge power,etc)on SMX degradation performance were studied.The experimental results showed that the DBD plasma jet can obtain a relatively high degradation efficiency for SMX when the discharge power is high with an oxygen atmosphere,the initial concentration of SMX is low,and the aqueous solution is under acidic conditions.The reactive species produced in the liquid phase were detected,and OH radicals and O3were found to play a significant role in the degradation of SMX.Moreover,the process of SMX degradation could be better fitted by the quasi-first-order reaction kinetic equation.The analysis of the SMX degradation process indicated that SMX was gradually decomposed and 4-amino benzene sulfonic acid,benzene sulfonamide,4-nitro SMX,and phenylsulfinyl acid were detected,and thus three possible degradation pathways were finally proposed.The mineralization degree of SMX reached 90.04%after plasma treatment for 20 min,and the toxicity of the solution fluctuated with the discharge time but eventually decreased.
文摘The paper presents comparative kinetic characteristics of the decomposition of 2,4-dichlorophenol in a dielectric barrier discharge and a combined plasma-catalytic process. Vermiculite containing 5% zirconium was used as a catalyst. The destruction processes of 2,4-DCP proceed efficiently, the degree of decomposition increases in the combined plasma-catalytic process by a factor of 1.33 and reaches 80%. The experimental results were processed according to the first-order kinetic law (R<sup>2</sup> > 0.97), according to which the effective constants (0.36 ± 0.04) and (0.51 ± 0.03) s<sup>-1</sup> and the decomposition rates of 2,4-DCP (106 and 123 μmol/l·s) when treating model solutions without a catalyst and with vermiculite + Zr 5%, respectively, and the energy costs are 0.012 and 0.017 molecules/100eV. The main decomposition products present in the solution have been determined to be carboxylic acids, aldehydes, the contribution of which does not exceed 2%, as well as chloride ions, and in the gas phase they are carbon dioxide and molecular chlorine (the share of which does not exceed 1.5% of total chlorine content in the system).
基金supported by National Natural Science Foundation of China(No.11175037)National Natural Science Foundation for Young Scientists of China(No.11305017)Special Fund for Theoretical Physics(No.11247239)
文摘The surface dielectric barrier discharge (SDBD) plasma actuator has shown great promise as an aerodynamic flow control device. In this paper, the encapsulated electrode width of a SDBD actuator is changed to study the airflow acceleration behavior. The effects of encapsulated electrode width on the actuator performance are experimentally investigated by measuring the dielectric layer surface potential, time-averaged ionic wind velocity and thrust force. Experimental results show that the airflow velocity and thrust force increase with the encapsulated electrode width. The results can be attributed to the distinct plasma distribution at different encapsulated electrode widths.
文摘The electronic excitation temperature of a surface dielectric barrier discharge (DBD) at atmospheric pressure has been experimentally investigated by optical emission spectroscopic measurements combined with numerical simulation. Experiments have been carried out to deter- mine the spatial distribution of electric field by using FEM software and the electronic excitation temperature in discharge by calculating ratio of two relative intensities of atomic spectral lines. In this work, we choose seven Ar atomic emission lines at 415.86 nm [(3s^23p^5)5p →(3s^23p^5)4s] and 706.7 nm, 714.7 nm, 738.4 nm, 751.5 nm, 794.8 nm and 800.6 nm [(3s^23p^5)4p → (3s^23p^5)4s] to estimate the excitation temperature under a Boltzmann approximation. The average electron energy is evaluated in each discharge by using line ratio of 337.1 nm (N2(C^3Пu →B3Пg)) to 391.4 nm (N2^+(B2 ∑u^+→ ∑g^+)). Furthermore, variations of the electronic excitation tempera- ture are presented versus dielectric thickness and dielectric materials. The discharge is stable and uniform along the axial direction, and the electronic excitation temperature at the edge of the copper electrode is the largest. The corresponding average electron energy is in the range of 1.6- 5.1 eV and the electric field is in 1.7-3.2 MV/m, when the distance from copper electrode varies from 0 cm to 6 cm. Moreover, the electronic excitation temperature with a higher permittivity leads to a higher dissipated electrical power.
基金National Natural Science Foundation of China(Nos.50676094,50676095,50776086 and 50736007)Fundamental Researches of National Defense in Chinese Academy of Sciences(No.AB20070090)
文摘Influence of plasma actuators as a flow separation control device was investigated experimentally. Hump model was used to demonstrate the effect of plasma actuators on external flow separation, while for internal flow separation a set of compressor cascade was adopted. In order to investigate the modification of the flow structure by the plasma actuator, the flow field was examined non-intrusively by particle image velocimetry measurements in the hump model experiment and by a hot film probe in the compressor cascade experiment. The results showed that the plasma actuator could be effective in controlling the flow separation both over the hump and in the compressor cascade when the incoming velocity was low. As the incoming velocity increased, the plasma actuator was less effective. It is urgent to enhance the intensity of the plasma actuator for its better application. Methods to increase the intensity of plasma actuator were also studied.
基金Project(6140863020216JW30001)supported by the General Armaments Department Pre-research Fund,China。
文摘The article improves the process of dielectric barrier discharge(DBD)activated anode bonding.The treated surface was characterized by the hydrophilic surface test.The results showed that the hydrophilic angle was significantly reduced under nano-gap conditions and the optimal discharge voltage was 2 kV.Then,the anodic bonding and dielectric barrier discharge activated bonding were performed in comparison experiments,and the bonding strength was characterized by tensile failure test.The results showed that the bonding strength was higher under the nano-gap dielectric barrier discharge.This process completed 110°C ultra-low temperature anodic bonding and the bonding strength reached 2 MPa.Finally,the mechanism of promoting bonding after activation is also discussed.
基金supported by National Natural Science Foundation of China (Nos. 61971345 and 52107174)。
文摘The three-electrode sliding dielectric barrier discharge(TES-DBD) plasma actuator significantly enhances the ionization rate and momentum exchange between charged particles and neutral particles by incorporating a parallel DC electrode into the standard DBD design. This design improves the body force and induced jet velocity while allowing flexible control of the induced jet angle, overcoming the limitations of discharge extension and uncontrollable direction in traditional DBD plasma actuators. An integrated plasma power supply has been designed specifically for TES-DBD plasma actuators, streamlining the power supply management. The methodology involves designing the circuit topology for the TES-DBD power supply, followed by simulating and validating its operating principles using Multisim software. The operational performance of the power supply is evaluated through a comprehensive analysis of its electrical,thermal, and aerodynamic properties specific to TES-DBD plasma actuation.
基金supported by Beijing Natural Science Foundation(No.3222062)National Natural Science Foundation of China(No.12102482)。
文摘To optimize the design of plasma injectors,the influence of different external electrodes on plasma-assisted flame stabilization was assessed by using a nonequilibrium plasma injector flame control setup.The electrical characteristics of the injector,flame structure parameters,flame intensity,discharge power,and cost-to-effectiveness ratio under different external electrodes(four mesh electrodes and one copper foil electrode)were analyzed using electrical and optical methods.The results show that reducing the mesh size of the external electrode leads to a decrease in breakdown voltage.Compared with a ceramic dielectric barrier-based injector,an injector with a quartz dielectric barrier produces a higher breakdown voltage under the same conditions.For the same actuation voltage,the discharge current increases as the mesh size of the external electrode decreases,and combustion is enhanced by the discharge plasma;therefore,it is better to adopt a smaller mesh hole size to realize good flame stabilization under a lower actuation voltage.However,under the studied working conditions,reducing the mesh hole size of the external electrode increases the cost-to-effectiveness ratio of plasma injector-based flame stabilization.Thus,considering the cost-to-effectiveness ratio and the weight of the injector,an external electrode with a larger mesh hole size should be chosen,which contradicts the above rule.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.51509035 and 51409158)the Project of Shenyang Science and Technology Bureau (Grant No.RC200010)the National Natural Science Foundation of Liaoning Province of China (Grant No.2020-KF-13-03)。
文摘In order to better analyze the characteristics of particle distribution and its influencing factors in the ionized space during the process of coaxial dielectric barrier discharge,a self-designed two-dimensional axisymmetric structure exciter was used to carry out optical diagnosis,with the electron temperature calculated through Gaussian fitting.A plasma model was applied to conduct research on the discharge process through numerical simulation,with the changes in electron density and electron temperature were analyzed by using different discharge parameters.The research results show that with an increase in discharge voltage,pressure inside the reactor and relative permittivity,the discharge process is promoted.In addition,a rise in current density leads to an increase in the number of charged particles on the surface of the medium during the discharge process,while a rise in discharge intensity causes an increase in the electron density.Electron temperature decreases due to the increased loss of collision energy between particles.These results were confirmed by comparing experimental data with simulation results.
基金supported by the Pilot Program of University of Liaoning Innovation and Education Reform~~
文摘Dielectric barrier discharge(DBD) plasma is considered to be a promising method to synthesize solid catalysts. In this work, DBD plasma was used to synthesize a nitrogen‐vacancy‐doped g‐C3N4 catalyst in situ for the first time. X‐ray diffraction, N2 adsorption, ultraviolet–visible spectroscopy, scanning electron microscopy, transmission electron microscopy, X‐ray photoelectron spectrosco‐py, electrochemical impedance spectroscopy, electron paramagnetic resonance, O2 tempera‐ture‐programmed desorption, and photoluminescence were used to characterize the obtained cat‐alysts. The photocatalytic H2O2 production ability of the as‐prepared catalyst was investigated. The results show that plasma treatment influences the morphology, structure, and optical properties of the as‐prepared catalyst. Nitrogen vacancies are active centers, which can adsorb reactant oxygen molecules, trap photoelectrons, and promote the transfer of photoelectrons from the catalyst to the adsorbed oxygen molecules for the subsequent reduction reaction. This work provides a new strat‐egy for synthesizing g‐C3N4‐based catalysts.
文摘A superimposed wire-plate dielectric barrier discharge reactor was used to remove toluene in this study. The effects of oxygen content, gas flow rate, gas initial concentration and with/without catalyst on toluene decomposition were investigated. It was found that an optimal toluene removal was achieved when the oxygen content was about 5%. Under this condition, the highest toluene removal efficiency of 80.8% was achieved when the gas concentration was 80 mg/m^3. The toluene removal efficiency decreased with the increase of the gas flow rate and the initial concentration of toluene. In addition, the ozone concentration decreased with the increase of the initial concentration of toluene. It suggested that combining DBD (dielectric barrier discharge) with Co3O4/Al2O3/foam nickel catalyst in-situ could improve the toluene removal efficiency and suppress ozone formation. Products analysis showed that the main products were CO and CO2 when oxygen was more than 5%.
基金supported by National Natural Science Foundation of China(Nos.11205007 and 11205029)
文摘The humidity effects on the benzene decomposition process were investigated by the dielectric barrier discharge(DBD) plasma reactor.The results showed that the water vapor played an important role in the benzene oxidation process.It was found that there was an optimum humidity value for the benzene removal efficiency,and at around 60% relative humidity(RH),the optimum benzene removal efficiency was achieved.At a SIE of 378 J/L,the removal efficiency was 66% at 0% RH,while the removal efficiency reached 75.3% at 60% RH and dropped to 69% at 80% RH.Furthermore,the addition of water inhibited the formation of ozone and NO2 remarkably.Both of the concentrations of ozone and NO2 decreased with increasing of the RH at the same specific input energy.At a SIE of 256 J/L,the concentrations of ozone and NO2 were 5.4 mg/L and 1791 ppm under dry conditions,whereas they were only 3.4 mg/L and 1119 ppm at 63.5%RH,respectively.Finally,the outlet gas after benzene degradation was qualitatively analyzed by FT-IR and GC-MS to determine possible intermediate byproducts.The results suggested that the byproducts in decomposition of benzene primarily consisted of phenol and substitutions of phenol.Based on these byproducts a benzene degradation mechanism was proposed.
基金The project supported by the National Natural Science Foundation of China (No. 20376060)
文摘Experimental investigation was conducted to convert dimethyl ether (DME) in the presence of steam using dielectric barrier discharge (DBD) at atmospheric pressure and 373 K. The flow rate of DME was 20 ml/min. The introduction of steam resulted in an increase in the DME conversion and the selectivity of oxygenates. Plasma steam-enhanced dimethyl ether (DME) conversion led to a direct synthesis of DMMT and DMET, with a high selectivity of 5.78% and 17.99%, respectively. The addition of steam promoted the formation of 'plasma aerosol' that was favored for the formation of liquid oxygenates. The reaction pathway of plasma DME conversion was proposed.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.51336011 and 51607188)the China Postdoctoral Science Foundation(Grant No.2014M562446)the PhD Research Startup Foundation of Xi’an University of Technology(Grant No.256081802)
文摘Plasma flow control(PFC) is a promising active flow control method with its unique advantages including the absence of moving components, fast response, easy implementation, and stable operation. The effectiveness of plasma flow control by microsecond dielectric barrier discharge(μs-DBD), and by nanosecond dielectric barrier discharge(NS-DBD) are compared through the wind tunnel tests, showing a similar performance between μs-DBD and NS-DBD. Furthermore, theμs-DBD is implemented on an unmanned aerial vehicle(UAV), which is a scaled model of a newly developed amphibious plane. The wingspan of the model is 2.87 m, and the airspeed is no less than 30 m/s. The flight data, static pressure data,and Tufts images are recorded and analyzed in detail. Results of the flight test show that the μs-DBD works well on board without affecting the normal operation of the UAV model. When the actuators are turned on, the stall angle and maximum lift coefficient can be improved by 1.3° and 10.4%, and the static pressure at the leading edge of the wing can be reduced effectively in a proper range of angle of attack, which shows the ability of μs-DBD to act as plasma slats. The rolling moment produced by left-side μs-DBD actuation is greater than that produced by the maximum deflection of ailerons,which indicates the potential of μs-DBD to act as plasma ailerons. The results verify the feasibility and efficacy of μs-DBD plasma flow control in a real flight and lay the foundation for the full-sized airplane application.