In this paper,self-designed multi-hollow needle electrodes are used as a high-voltage electrode in a packed bed dielectric barrier discharge reactor to facilitate fast gas flow through the active discharge area and ac...In this paper,self-designed multi-hollow needle electrodes are used as a high-voltage electrode in a packed bed dielectric barrier discharge reactor to facilitate fast gas flow through the active discharge area and achieve large-volume stable discharge.The dynamic characteristics of the plasma,the generated active species,and the energy transfer mechanisms in both positive discharge(PD)and negative discharge(ND)are investigated by using fast-exposure intensified charge coupled device(ICCD)images and time-resolved optical emission spectra.The experimental results show that the discharge intensity,number of discharge channels,and discharge volume are obviously enhanced when the multi-needle electrode is replaced by a multihollow needle electrode.During a single voltage pulse period,PD mainly develops in a streamer mode,which results in a stronger discharge current,luminous intensity,and E/N compared with the diffuse mode observed in ND.In PD,as the gap between dielectric beads changes from 0 to250μm,the discharge between the dielectric bead gap changes from a partial discharge to a standing filamentary micro-discharge,which allows the plasma to leave the local area and is conducive to the propagation of surface streamers.In ND,the discharge only appears as a diffusionlike mode between the gap of dielectric beads,regardless of whether there is a discharge gap.Moreover,the generation of excited states N_(2)^(+)(B^(2)∑_(u)^(+))and N2(C^(3)Π_(u))is mainly observed in PD,which is attributed to the higher E/N in PD than that in ND.However,the generation of the OH(A^(2)∑^(+))radical in ND is higher than in PD.It is not directly dominated by E/N,but mainly by the resonant energy transfer process between metastable N_(2)(A^(3)∑_(u)^(+))and OH(X^(2)Π).Furthermore,both PD and ND demonstrate obvious energy relaxation processes of electron-to-vibration and vibration-to-vibration,and no vibration-to-rotation energy relaxation process is observed.展开更多
On the unit sphere, the geometric problem of calculating the position of a point relative to three given points is considered. We know the length of three spherical segments that go out from the given points in the di...On the unit sphere, the geometric problem of calculating the position of a point relative to three given points is considered. We know the length of three spherical segments that go out from the given points in the direction of the unknown point. The requirement must be fulfilled: the distance from each point to an unknown point must be equal to the sum of the length of the segment outgoing from this point, and some increment, the same for all three segments. In the article, the conditions for the solvability of a geometric problem are established by the methods of spherical trigonometry and vector algebra. It is proved that when they are fulfilled, the problem is always solvable. The number of solutions is two, except in rare cases where there is only one solution. A solution method is presented. One of the practical applications is the problem of determining the time and location of a cloud-to-ground lightning discharge, which is directly reduced to this problem.展开更多
The operating performance of positive discharge blower is markedly influenced by the pulsation of the discharge flow, but difficult to be measured with experimental methods. The internal and discharge flow of positive...The operating performance of positive discharge blower is markedly influenced by the pulsation of the discharge flow, but difficult to be measured with experimental methods. The internal and discharge flow of positive discharge blower with involute type three-lobe are numerically investigated, both in air cooling and countercurrent cooling conditions by means of computational fluid dynamics (CFD). The unsteady compressible flow equations are solved using RNG x-ε turbulent model. The finite difference method and the second order upwind difference scheme are applied into discrete equations. In the numerical simulation, the dynamic mesh techniques are used to approach the rotating displacement of cell cubage and the alterability of inlet, outlet flow area. The non-uniform mesh is applied to the rotor-stator coupled area. The reliability of the numerical method is verified by simulating the inner flow and comparing with the semi-empirical theory. The flow flux curves and the distributing of velocity vector showed obvious vortex motion in all the discharge process, both in air cooling and countercurrent cooling conditions. These vortexes with different positions, intension and numbers at different rotating angles have remarkable influences on the discharge flux. For air cooling, the vortex produced a second pulsation with big-amplitude in a cycle, and led to the early appearance of maximum of backflow. For countercurrent cooling, the frequency of pulsation increased due to the pre-inflow, but the backflow at the outlet is prevented, also the pulsation strength has greatly decreased.展开更多
This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastew...This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastewater while the ground electrode was submerged in the wastewater. The electrical discharge starting at the tip of the high voltage electrode propagated toward the surface of the wastewater, producing various oxidative radicals and ozone. Oxygen was used as the working gas instead of air to prevent nitrogen oxides from forming. The simulated wastewater was made up with amaranth, which is a kind of azo dye. The results obtained showed that the chromaticity of the wastewater was almost completely removed within an hour. The ultraviolet/visible spectra of the wastewater treated by the electrical discharge revealed that the total hydrocarbon level also decreased significantly.展开更多
Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connect...Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connections between these pulses and the collective movement of charged species.The movement of species is divided into four parts with respect to time:the(1)initial growth of species,(2)formation and development of the streamer region and negative ion sheath,(3)dead time(the time interval between the pulses),and(4)rapid re-growth of species.The movement of the species in the four parts and the correspondence with the current pulse were analyzed.The numerical results indicated the following:the rapid rising of the species matched the rising edge of the pulses,the streamer region,and negative ion sheath appeared in the falling edge of the primary pulse,and the rapid re-growth of species matched the re-ignition of the pulses.The results were in qualitative agreement with deductions and experimental observations in the literature.展开更多
The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheri...The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheric N2 and O2 flows wetted with 10%H2O at 80 ℃ are used to investigate the relative concentrations of the produced radicals.The results indicate that the tendencies of the concentrations of radicals with discharge conditions are similar to each other due to their similar excitation processes by electron collision.The influence of oxygen flow mixed with the nitrogen flow on the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2S),N2+(B^2∑u^+ → X^2∑g+0-0),and N2(C^3Πu → B^3Πg 1-0) is presented.When the flow rate of oxygen addition is varied from 0-30 ml min^-1,the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2s),and N2^+(B^2∑u^+ →X^2∑g 0-0) increase and reach a maximum.Then,if the oxygen flow rate increases further,the emission intensities tend to decrease.However,the intensity of N2(C^3Πu → B^3Πg1-0) decreases monotonously with the increasing oxygen flow,which indicates that the electron density decreases with the increasing oxygen flow.By the tendencies of the relative intensities to N2(C^3Πu → B^3Πg 1-0),the concentrations of the total produced O,H,and N2^+ are shown to increase with the oxygen flow.Based on the reactions for the production of H and O without and with the addition of O2,the analytic solutions for H and O production are derived in accordance with the experimental results.展开更多
The electronic excitation temperature in a direct current positive streamer discharge based on ultra-thin sheet electrodes was measured by optical emission spectrometry in order to deposit materials for potential futu...The electronic excitation temperature in a direct current positive streamer discharge based on ultra-thin sheet electrodes was measured by optical emission spectrometry in order to deposit materials for potential future applications. It was remarkable that the electronic excitation temperature (Text) did not vary monotonically with the discharge current, but demonstrated a peak at a certain position. In a mixture of oxygen and argon (80% oxygen), the maximum Texc reached about 6300 K at an average current of 600 pA. Both the positive ions accumulation in the discharge region and the increase of the local temperature around the streamer channel caused by Joule heating are considered to be the main reasons for the variations of Texc.展开更多
The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investig...The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investigated in order to reveal their generation mechanism.In this paper,the line-to-plane electrodes are designed to measure and analyze the characteristics of corona current pulses from positive corona discharges.The influences of inter-electrode gap and line diameters on the detail characteristics of corona current pulses,such as pulse amplitude,rise time,duration time and repetition frequency,are carefully analyzed.The obtained results show that the pulse amplitude and the repetition frequency increase with the diameter of line electrode when the electric fields on the surface of line electrodes are same.With the increase of inter-electrode gap,the pulse amplitude and the repetition frequency first decrease and then turn to be stable,while the rise time first increases and finally turns to be stable.The distributions of electric field and space charges under the line electrodes are calculated,and the influences of inter-electrode gap and line electrode diameter on the experimental results are qualitatively explained.展开更多
基金supported by National Natural Science Foundations of China(Nos.51977023 and 52077026)the Fundamental Research Funds for the Central Universities(No.DUT23YG227)。
文摘In this paper,self-designed multi-hollow needle electrodes are used as a high-voltage electrode in a packed bed dielectric barrier discharge reactor to facilitate fast gas flow through the active discharge area and achieve large-volume stable discharge.The dynamic characteristics of the plasma,the generated active species,and the energy transfer mechanisms in both positive discharge(PD)and negative discharge(ND)are investigated by using fast-exposure intensified charge coupled device(ICCD)images and time-resolved optical emission spectra.The experimental results show that the discharge intensity,number of discharge channels,and discharge volume are obviously enhanced when the multi-needle electrode is replaced by a multihollow needle electrode.During a single voltage pulse period,PD mainly develops in a streamer mode,which results in a stronger discharge current,luminous intensity,and E/N compared with the diffuse mode observed in ND.In PD,as the gap between dielectric beads changes from 0 to250μm,the discharge between the dielectric bead gap changes from a partial discharge to a standing filamentary micro-discharge,which allows the plasma to leave the local area and is conducive to the propagation of surface streamers.In ND,the discharge only appears as a diffusionlike mode between the gap of dielectric beads,regardless of whether there is a discharge gap.Moreover,the generation of excited states N_(2)^(+)(B^(2)∑_(u)^(+))and N2(C^(3)Π_(u))is mainly observed in PD,which is attributed to the higher E/N in PD than that in ND.However,the generation of the OH(A^(2)∑^(+))radical in ND is higher than in PD.It is not directly dominated by E/N,but mainly by the resonant energy transfer process between metastable N_(2)(A^(3)∑_(u)^(+))and OH(X^(2)Π).Furthermore,both PD and ND demonstrate obvious energy relaxation processes of electron-to-vibration and vibration-to-vibration,and no vibration-to-rotation energy relaxation process is observed.
文摘On the unit sphere, the geometric problem of calculating the position of a point relative to three given points is considered. We know the length of three spherical segments that go out from the given points in the direction of the unknown point. The requirement must be fulfilled: the distance from each point to an unknown point must be equal to the sum of the length of the segment outgoing from this point, and some increment, the same for all three segments. In the article, the conditions for the solvability of a geometric problem are established by the methods of spherical trigonometry and vector algebra. It is proved that when they are fulfilled, the problem is always solvable. The number of solutions is two, except in rare cases where there is only one solution. A solution method is presented. One of the practical applications is the problem of determining the time and location of a cloud-to-ground lightning discharge, which is directly reduced to this problem.
基金supported by National Natural Science Foundation of China (Grant No. 10802058)
文摘The operating performance of positive discharge blower is markedly influenced by the pulsation of the discharge flow, but difficult to be measured with experimental methods. The internal and discharge flow of positive discharge blower with involute type three-lobe are numerically investigated, both in air cooling and countercurrent cooling conditions by means of computational fluid dynamics (CFD). The unsteady compressible flow equations are solved using RNG x-ε turbulent model. The finite difference method and the second order upwind difference scheme are applied into discrete equations. In the numerical simulation, the dynamic mesh techniques are used to approach the rotating displacement of cell cubage and the alterability of inlet, outlet flow area. The non-uniform mesh is applied to the rotor-stator coupled area. The reliability of the numerical method is verified by simulating the inner flow and comparing with the semi-empirical theory. The flow flux curves and the distributing of velocity vector showed obvious vortex motion in all the discharge process, both in air cooling and countercurrent cooling conditions. These vortexes with different positions, intension and numbers at different rotating angles have remarkable influences on the discharge flux. For air cooling, the vortex produced a second pulsation with big-amplitude in a cycle, and led to the early appearance of maximum of backflow. For countercurrent cooling, the frequency of pulsation increased due to the pre-inflow, but the backflow at the outlet is prevented, also the pulsation strength has greatly decreased.
文摘This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastewater while the ground electrode was submerged in the wastewater. The electrical discharge starting at the tip of the high voltage electrode propagated toward the surface of the wastewater, producing various oxidative radicals and ozone. Oxygen was used as the working gas instead of air to prevent nitrogen oxides from forming. The simulated wastewater was made up with amaranth, which is a kind of azo dye. The results obtained showed that the chromaticity of the wastewater was almost completely removed within an hour. The ultraviolet/visible spectra of the wastewater treated by the electrical discharge revealed that the total hydrocarbon level also decreased significantly.
基金supported by National Natural Science Foundation of China(No.51907145)。
文摘Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connections between these pulses and the collective movement of charged species.The movement of species is divided into four parts with respect to time:the(1)initial growth of species,(2)formation and development of the streamer region and negative ion sheath,(3)dead time(the time interval between the pulses),and(4)rapid re-growth of species.The movement of the species in the four parts and the correspondence with the current pulse were analyzed.The numerical results indicated the following:the rapid rising of the species matched the rising edge of the pulses,the streamer region,and negative ion sheath appeared in the falling edge of the primary pulse,and the rapid re-growth of species matched the re-ignition of the pulses.The results were in qualitative agreement with deductions and experimental observations in the literature.
基金supported by National Natural Science Foundation of China under Grant No.513377014
文摘The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheric N2 and O2 flows wetted with 10%H2O at 80 ℃ are used to investigate the relative concentrations of the produced radicals.The results indicate that the tendencies of the concentrations of radicals with discharge conditions are similar to each other due to their similar excitation processes by electron collision.The influence of oxygen flow mixed with the nitrogen flow on the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2S),N2+(B^2∑u^+ → X^2∑g+0-0),and N2(C^3Πu → B^3Πg 1-0) is presented.When the flow rate of oxygen addition is varied from 0-30 ml min^-1,the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2s),and N2^+(B^2∑u^+ →X^2∑g 0-0) increase and reach a maximum.Then,if the oxygen flow rate increases further,the emission intensities tend to decrease.However,the intensity of N2(C^3Πu → B^3Πg1-0) decreases monotonously with the increasing oxygen flow,which indicates that the electron density decreases with the increasing oxygen flow.By the tendencies of the relative intensities to N2(C^3Πu → B^3Πg 1-0),the concentrations of the total produced O,H,and N2^+ are shown to increase with the oxygen flow.Based on the reactions for the production of H and O without and with the addition of O2,the analytic solutions for H and O production are derived in accordance with the experimental results.
文摘The electronic excitation temperature in a direct current positive streamer discharge based on ultra-thin sheet electrodes was measured by optical emission spectrometry in order to deposit materials for potential future applications. It was remarkable that the electronic excitation temperature (Text) did not vary monotonically with the discharge current, but demonstrated a peak at a certain position. In a mixture of oxygen and argon (80% oxygen), the maximum Texc reached about 6300 K at an average current of 600 pA. Both the positive ions accumulation in the discharge region and the increase of the local temperature around the streamer channel caused by Joule heating are considered to be the main reasons for the variations of Texc.
基金supported by National Natural Science Foundation of China under Grant No.51707066by the Fundamental Research Funds for the Central Universities under Grant No.2017 MS004 and No.XCA17003-04
文摘The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investigated in order to reveal their generation mechanism.In this paper,the line-to-plane electrodes are designed to measure and analyze the characteristics of corona current pulses from positive corona discharges.The influences of inter-electrode gap and line diameters on the detail characteristics of corona current pulses,such as pulse amplitude,rise time,duration time and repetition frequency,are carefully analyzed.The obtained results show that the pulse amplitude and the repetition frequency increase with the diameter of line electrode when the electric fields on the surface of line electrodes are same.With the increase of inter-electrode gap,the pulse amplitude and the repetition frequency first decrease and then turn to be stable,while the rise time first increases and finally turns to be stable.The distributions of electric field and space charges under the line electrodes are calculated,and the influences of inter-electrode gap and line electrode diameter on the experimental results are qualitatively explained.