期刊文献+
共找到145篇文章
< 1 2 8 >
每页显示 20 50 100
Disinfection Byproducts and Their Precursors in Drinking Water Sources:Origins,Influencing Factors,and Environmental Insights
1
作者 Rong Xiao Yang Deng +1 位作者 Zuxin Xu Wenhai Chu 《Engineering》 SCIE EI CAS CSCD 2024年第5期36-50,共15页
Tracing the contamination origins in water sources and identifying the impacts of natural and human processes are essential for ecological safety and public health.However,current analysis approaches are not ideal,as ... Tracing the contamination origins in water sources and identifying the impacts of natural and human processes are essential for ecological safety and public health.However,current analysis approaches are not ideal,as they tend to be laborious,time-consuming,or technically difficult.Disinfection byproducts(DBPs)are a family of well-known secondary pollutants formed by the reactions of chemical disinfectants with DBP precursors during water disinfection treatment.Since DBP precursors have various origins(e.g.,natural,domestic,industrial,and agricultural sources),and since the formation of DBPs from different precursors in the presence of specific disinfectants is distinctive,we argue that DBPs and DBP precursors can serve as alternative indicators to assess the contamination in water sources and identify pollution origins.After providing a retrospective of the origins of DBPs and DBP precursors,as well as the specific formation patterns of DBPs from different precursors,this article presents an overview of the impacts of various natural and anthropogenic factors on DBPs and DBP precursors in drinking water sources.In practice,the DBPs(i.e.,their concentration and speciation)originally present in source water and the DBP precursors determined using DBP formation potential tests—in which water samples are dosed with a stoichiometric excess of specific disinfectants in order to maximize DBP formation under certain reaction conditions—can be considered as alternative metrics.When jointly used with other water quality parameters(e.g.,dissolved organic carbon,dissolved organic nitrogen,fluorescence,and molecular weight distribution)and specific contaminants of emerging concern(e.g.,certain pharmaceuticals and personal care products),DBPs and DBP precursors in drinking water sources can provide a more comprehensive picture of water pollution for better managing water resources and ensuring human health. 展开更多
关键词 disinfection byproducts disinfection byproduct precursors Drinking water sources Contamination indicator Natural factors Human factors
下载PDF
Progress in Analytical Methods of Halogenated Disinfection By-Products
2
作者 Jing Wu 《Proceedings of Business and Economic Studies》 2024年第2期95-99,共5页
Ensuring the health and safety of drinking water is crucial for both nations and their citizens.Since the 20th century,the disinfection of drinking water,effectively controlling pathogens in water sources,has become o... Ensuring the health and safety of drinking water is crucial for both nations and their citizens.Since the 20th century,the disinfection of drinking water,effectively controlling pathogens in water sources,has become one of the significant advances in public health.However,the disinfectants used in the process,such as chlorine and chlorine dioxide,react with natural organic matter in the water to produce disinfection by-products(DBPs).Most of these DBPs contain chlorine,and if the source water contains bromine or iodine,brominated or iodinated DBPs,collectively referred to as Halogenated disinfection byproducts(X-DBPs),are formed.Numerous studies have found that X-DBPs pose potential risks to human health and the environment,leading to widespread concern.Mass spectrometry has become an important means of discovering new types of X-DBPs.This paper focuses on the study of methods for analyzing X-DBPs in drinking water using mass spectrometry. 展开更多
关键词 Halogenated disinfection by-products Drinking water High-resolution mass spectrometry
下载PDF
Characterization of dissolved organic matter fractions and its relationship with the disinfection by-product formation 被引量:13
3
作者 ZHANG Hua QU Jiuhui +1 位作者 LIU Huijuan WEI Dongbin 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2009年第1期54-61,共8页
Dissolved organic matter (DOM) has been identified as precursor for disinfection by-products (DBPs) formation during chlorination. Recently, it has been demonstrated that the characteristics of DOM influence the D... Dissolved organic matter (DOM) has been identified as precursor for disinfection by-products (DBPs) formation during chlorination. Recently, it has been demonstrated that the characteristics of DOM influence the DBPs formation mechanism. A study was, therefore, initiated to investigate the effects of DOM fractions on DBPs formation mechanism. In the chlorination process, organic acids are dominant precursors of total thihalomethanes (TTHM) because of the vc-o and unsaturated structures. Furthermore, the TTHM formation of organic acids was affected by pH more greatly. Based on the fluorescence spectroscopy analysis, DOM fractions contained several fluorescence substances. During chlorination, humic acid-like substances were found to exhibit high chlorine reactivity and hydrophobic organics decomposed to smaller molecules faster than hydrophilic organics even at lower chlorine dosages. Unlike hydrophobic fractions, hydrophilic organics showed no toxicity following chlorination, suggesting that the toxic structures in hydrophihc organics showed high chlorine reactivity during chlorination. 展开更多
关键词 disinfection by-products CHLORINATION CHARACTERISTICS dissolved organic matter
下载PDF
Simultaneous Control of Microorganisms and Disinfection By-products by Sequential Chlorination 被引量:4
4
作者 CHAO CHEN XIAO-JIAN ZHANG +1 位作者 WEN-JIE HE HONG-DA HAN 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2007年第2期119-125,共7页
Objective To introduce a new sequential chlorination disinfection process in which short-term free chlorine and chloramine are sequentially added. Methods Pilot tests of this sequential chlorination were carried out i... Objective To introduce a new sequential chlorination disinfection process in which short-term free chlorine and chloramine are sequentially added. Methods Pilot tests of this sequential chlorination were carried out in a drinking water plant. Results The sequential chlorination disinfection process had the same or better efficiency on microbe (including virus) inactivation compared with the free chlorine disinfection process. There seemed to be some synergetic disinfection effect between free chlorine and monochloramine because they attacked different targets. The sequential chlorination disinfection process resulted in 35.7%-77.0% TTHM formation and 36.6%-54.8% THAA5 formation less than the free chlorination process. The poorer the water quality was, the more advantage the sequential chlorination disinfection had over the free chlorination. Conclusion This process takes advantages of free chlorine's quick inactivation of microorganisms and chloramine's low disinfection by-product (DBP) yield and long-term residual effect, allowing simultaneous control of microbes and DBPs in an effective and economic way. 展开更多
关键词 disinfection Free chlorine CHLORAMINE disinfection by-products MICROORGANISMS
下载PDF
Removal of disinfection by-products formation potential by biologically intensified process 被引量:2
5
作者 ANDong LIWei-guang +2 位作者 CUIFu-yi HEXin ZHANGJin-song 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2005年第2期315-318,共4页
The removal of disinfection by-products formation potential(DBPFP) in artificially intensified biological activated carbon(IBAC) process which is developed on the basis of traditional ozone granular activated carbon w... The removal of disinfection by-products formation potential(DBPFP) in artificially intensified biological activated carbon(IBAC) process which is developed on the basis of traditional ozone granular activated carbon was evaluated. By IBAC removals of 31% and 68% for THMFP and HAAFP were obtained respectively. Under identical conditions, the removals of the same substances were 4% and 32% respectively only by the granular activated carbon(GAC) process. Compared with GAC, the high removal rates of the two formed potential substances were due to the increasing of bioactivity of the media and the synergistic capabilities of biological degradation cooperating with activated carbon adsorption of organic compounds. A clear linear correlation(R 2=0.9562 and R 2=0.9007) between DOC HAAFP removal rate and Empty Bed Contact Time(EBCT) of IBAC process was observed, while that between THMFP removal rate and EBCT of GAC was R 2=0.9782. In addition certain linear correlations between THMFP, HAAFP and UV 254 (R 2=0.855 and R 2=0.7702) were found for the treated water. For IBAC process there are also more advantages such as long backwashing cycle time, low backwashing intensity and prolonging activated carbon lifetime and so on. 展开更多
关键词 intensified biological activated carbon(IBAC) disinfection by-products formation potential(DBPFP) empty bed contact time water treatment
下载PDF
Health Risk Assessment of Employees Exposed to Chlorination By-products of Recreational Water in Large Amusement Parks in Shanghai
6
作者 Weizhao Cao Yiming Zheng +4 位作者 Wenxuan Zhao Lisha Shi Yunhui Zhang Lijun Zhang Jian Chen 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2024年第8期865-875,共11页
Objective Chlorination is often used to disinfect recreational water in large amusement parks;however,the health hazards of chlorination disinfection by-products(DBPs)to occupational populations are unknown.This study... Objective Chlorination is often used to disinfect recreational water in large amusement parks;however,the health hazards of chlorination disinfection by-products(DBPs)to occupational populations are unknown.This study aimed to assess the exposure status of chlorinated DBPs in recreational water and the health risks to employees of large amusement parks.Methods Exposure parameters of employees of three large amusement parks in Shanghai were investigated using a questionnaire.Seven typical chlorinated DBPs in recreational water and spray samples were quantified by gas chromatography,and the health risks to amusement park employees exposed to chlorinated DBPs were evaluated according to the WHO's risk assessment framework.Results Trichloroacetic acid,dibromochloromethane,bromodichloromethane,and dichloroacetic acid were detected predominantly in recreational water.The carcinogenic and non-carcinogenic risks of the five DBPs did not exceed the risk thresholds.In addition,the carcinogenic and non-carcinogenic risks of mixed exposure to DBPs were within the acceptable risk limits.Conclusion Typical DBPs were widely detected in recreational water collected from three large amusement parks in Shanghai;however,the health risks of DBPs and their mixtures were within acceptable limits. 展开更多
关键词 Risk assessment WATER Environmental health Occupational exposure Chlorinated disinfection by-product
下载PDF
Removal characteristics of disinfection by-products formation potential by bioaugmentation activated carbon process
7
作者 王广智 李伟光 +2 位作者 黄丽坤 郜玉楠 张多英 《Journal of Harbin Institute of Technology(New Series)》 EI CAS 2010年第3期323-327,共5页
The high-active bacteria were screened from 8 dominant bacteria obtained from the natural water body,and then the bioaugmentation activated carbon was formed by hydraulic immobilization of the high-active bacteria. Pl... The high-active bacteria were screened from 8 dominant bacteria obtained from the natural water body,and then the bioaugmentation activated carbon was formed by hydraulic immobilization of the high-active bacteria. Plant-scale studies on removal characteristics of disinfection by-products formation potentials (DBPFP) by bioaugmentation activated carbon process were conducted for micro-polluted raw water treatment. The results show that the bioaugmentation activated carbon process has adopted better purification efficiency to THMFP and HAAFP than traditional biological activated carbon process,and that average removal efficiencies of THMFP and HAAFP can reach 35% and 39.7% during the test period,increasing by more than 10% compared with traditional biological activated carbon process. The removal efficiencies of THMFP and HAAFP are stable because of the biodegradation of the high-active bacteria and the adsorption of active carbon. The biodegradability of CHCl3 formation potential is better as compared with that of CHCl2Br and CHClBr2 formation potentials among THMFP,and high removal efficiency of CHCl3formation potential is obtained by bioaugmentation degradation of the high-active bacteria. The biodegradability of HAAFP is better in comparison with that of THMFP,and the chemical properties of HAAFP are propitious to adsorption of activated carbon. Thus,HAAFP is on predominance during the competitive removal process with THMFP. 展开更多
关键词 BIOAUGMENTATION activated carbon disinfection by-products formation potential high-active bacteria
下载PDF
Less pressure contributes to gravity-driven membrane ultrafiltration with greater performance:Enhanced driving efficiency and reduced disinfection by-products formation potential
8
作者 Xiaoting Wu Yufei Li +3 位作者 Zhaoyang Su Long Tian Muhammad Saboor Siddique Wenzheng Yu 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2024年第3期407-419,共13页
Gravity-driven membrane(GDM)systems have been well developed previously;however,impacts of driving(i.e.,transmembrane)pressure on their performance received little attention,which may infuence GDM performance.In this ... Gravity-driven membrane(GDM)systems have been well developed previously;however,impacts of driving(i.e.,transmembrane)pressure on their performance received little attention,which may infuence GDM performance.In this study,we evaluated 4 GDM systems via altering the transmembrane pressure from 50 mbar to 150 mbar with 2 groups,treating surface water in Beijing,China.Results showed that less driving pressure was more favorable.Specifically,compared to groups(150 mbar),groups under a pressure of 50 mbar were found to have greater normalized permeability and lower total resistance.During the whole operation period,the quality of effuents was gradually improved.For example,the removal efficiency of UV254was significantly improved;particularly,under low driving pressure,the removal efficiency of UV254in PES GDM system increased by 11.91%,as compared to the corresponding system under high driving pressure.This observation was consistent with the reduction on disinfection by-products(DBPs)formation potential;groups under 50 mbar achieved better DBPs potential control,indicating the advantages of lower driving pressure.Biofilms were analyzed and responsible for these differences,and distinct distributions of bacteria communities of two GDM systems under 50 and 150 mbar may be responsible for various humic-like substances removal efficiency.Overall,GDM systems under less pressure should be considered and expected to provide suggestions on the design of GDM systems in real applications. 展开更多
关键词 ULTRAFILTRATION Gravity driven operation Membrane fouling Biofilms disinfection by-products
原文传递
Waste Water Disinfection During SARS Epidemic for Microbiological and Toxicological Control 被引量:5
9
作者 CHAO CHEN XIAO-JIAN ZHANG YUN WANG LING-XIA ZHU JING LIU 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2006年第3期173-178,共6页
Objective To evaluate the disinfection of wastewater in China. Methods During the SARS epidemic occurred in Beijing, a study of different disinfection methods used in the main local wastewater plants including means o... Objective To evaluate the disinfection of wastewater in China. Methods During the SARS epidemic occurred in Beijing, a study of different disinfection methods used in the main local wastewater plants including means of chlorine, chlorine dioxide, ozone, and ultraviolet was carried out in our laboratory. The residual coliform, bacteria and trihalomethanes, haloacetic acids were determined after disinfection. Results Chlorine had fairly better efficiency on microorganism inactivation than chlorine dioxide with the same dosage. Formation of THMs and HAAs does not exceed the drinking water standard. UV irradiation had good efficiency on microorganism inactivation and good future of application in China. Organic material and ammonia nitrogen was found to be significant on inactivation and DBPs formation. Conclusion Chlorine disinfection seems to be the best available technology for coliform and bacteria inactivation. And it is of fairly low toxicological hazard due to the transformation of monochloramine. 展开更多
关键词 Wastewater disinfection Chlorine Chlorine dioxide Ozone Ultraviolet disinfection by-products
下载PDF
Disinfection of swimming pools with chlorine and derivatives: formation of organochlorinated and organobrominated compounds and exposure of pool personnel and swimmers 被引量:2
10
作者 Maria-Cristina Aprea Bruno Banchi +3 位作者 Liana Lunghini Massimo Pagliantini Antonio Peruzzi Gianfranco Sciarra 《Natural Science》 2010年第2期68-78,共11页
Chlorination of pool water leads to the forma-tion of many by-products, chloroform usually being the most abundant. The paper reports the results of a study evaluating exposure of bath-ers and pool employees to trihal... Chlorination of pool water leads to the forma-tion of many by-products, chloroform usually being the most abundant. The paper reports the results of a study evaluating exposure of bath-ers and pool employees to trihalomethanes (chloroform, bromodichloromethane, dibromo-chloromethane, bromoform) in four indoor swimming pools with chlorinated water. Chlo-roform concentrations in environmental air samples when the pool was in use (about 9 h), in the range 1-182 μg/m3, were greater near the pool than in the change rooms, passageways and offices. Chloroform concentrations in per-sonal air samples of pool employees were in the range 18-138 μg/m3. Urinary concentrations of chloroform averaged (geometric means) 0.123 and 0.165 μg/l and 0.404 and 0.342 μg/l prior and at the end of exposure during in water and out of water activities, respectively. The significant increase in urinary excretion of chloroform confirms that the source of the contaminant was pool water. Absorption of chloroform, estimated from airborne and water concentrations, was significantly correlated with delta chloroform (after/before exposure) and urinary concentra-tions of chloroform at the end of exposure. As chloroform is a toxic and possibly carcinogenic substance, these observations pose a problem principally for the general population of pool users. 展开更多
关键词 disinfection by-products Indoor SWIMMING POOL TRIHALOMETHANES Biological Monitoring EXPOSURE Urine
下载PDF
Identification of key precursors contributing to the formation of CX_(3)R-type disinfection by-products along the typical full-scale drinking water treatment processes 被引量:2
11
作者 Xu Yang Shunke Ding +4 位作者 Rong Xiao PinWang Zhenqi Du Ruihua Zhang Wenhai Chu 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2023年第6期81-92,共12页
Identification and characterization of disinfection by-product(DBP)precursors could help optimize drinkingwater treatment processes and improve the quality of finishedwater.This study comprehensively investigated the ... Identification and characterization of disinfection by-product(DBP)precursors could help optimize drinkingwater treatment processes and improve the quality of finishedwater.This study comprehensively investigated the characteristics of dissolved organic matter(DOM),the hydrophilicity and molecule weight(MW)of DBP precursor and DBP-associated toxicity along the typical full-scale treatment processes.The results showed that dissolved organic carbon and dissolved organic nitrogen content,the fluorescence intensity and the SUVA254 value in raw water significantly decreased after the whole treatment processes.Conventional treatment processes were in favor of the removal of high-MW and hydrophobic DOM,which are important precursors of trihalomethane and haloacetic acid.Compared with conventional treatment processes,Ozone integrated with biological activated carbon(O3-BAC)processes enhanced the removal efficiencies of DOM with different MW and hydrophobic fractions,leading to a further decrease in almost all DBP formation potential and DBP-associated toxicity.However,almost 50%of the detected DBP precursors in raw water has not been removed after the coagulation-sedimentation-filtration integrated with O3-BAC advanced treatment processes.These remaining precursors were found to be mainly hydrophilic and low-MW(<1.0 kDa)organics.Moreover,they would largely contribute to the formation of haloacetaldehydes and haloacetonitriles,which dominated the calculated cytotoxicity.Since current drinking water treatment process could not effectively control the highly toxic DBPs,the removal of hydrophilic and low-MW organics in drinking water treatment plants should be focused on in the future. 展开更多
关键词 disinfection by-products Drinking water Characterization Key precursor HYDROPHILICITY MW distribution
原文传递
Alternate disinfection approaches or raise disinfectant dosages for sewage treatment plants to address the COVID-19 pandemic?From disinfection efficiency,DBP formation,and toxicity perspectives
12
作者 Xiaobin Liao Xinyue Liu +7 位作者 Yueyun He Xueping Tang Ruanjunjie Xia Yongjun Huang Wenhua Li Jing Zou Zhenming Zhou Mazhan Zhuang 《Frontiers of Environmental Science & Engineering》 SCIE EI CSCD 2024年第9期115-128,共14页
During the COVID-19 pandemic,most sewage treatment plants increased disinfectant dosages to inactivate pathogenic viruses and microorganisms more effectively.However,this approach also led to the production of more di... During the COVID-19 pandemic,most sewage treatment plants increased disinfectant dosages to inactivate pathogenic viruses and microorganisms more effectively.However,this approach also led to the production of more disinfection by-products(DBPs).To ensure both disinfection efficiency and a reduction in DBP formation,new disinfection protocols are required.In this study,the disinfection efficiency,DBP amounts,and toxicity changes resulting from ozone(O_(3)),ultraviolet(UV),chlorine(Cl_(2)),and their combined processes were examined.The results demonstrated that the O_(3)/UV/Cl_(2)combination achieved the highest disinfection efficiency.Chlorination produced the most DBPs,whereas UV treatment reduced the formation of trihalomethane(THM),halogenated ketones(HKs),haloacetic acids(HAA),dichloroacetonitrile(DCAN)and N-nitrosodimethylamine(NDMA)by 45.9%,52.6%,82.0%,67.95%,and 47%,respectively.O_(3)also significantly reduced their production by 99.1%,91.1%,99.5%,100%,and 35%.Intracellular organic matter(IOM)was identified as the primary DBP precursors,producing 2.94 times more DBPs than extracellular organic matter(EOM).The increased DBP formation during chlorination was attributed to IOM leakage and cell membrane damage,which was verified using scanning electron microscopy(SEM).The toxicities of DBPs were evaluated for six disinfection methods,revealing inconsistent results.The overall toxicities were assessed using zebrafish embryo experiments.Both evaluations indicated that chlorination alone was the least favorable method.In addition,the toxicities followed a sequence:Cl_(2)≈O_(3)/Cl_(2)>O_(3)>O_(3)/UV/Cl_(2)>UV>UV/Cl_(2).These findings can serve as a reference for sewage treatment plants in selecting appropriate disinfection methods to manage the COVID-19 epidemic from comprehensive perspective. 展开更多
关键词 Sewage bacteria disinfection by-products Toxicity OZONATION UV CHLORINATION
原文传递
Impact of ozonation on disinfection byproducts formation from phenylalanine during chlorination
13
作者 Sinong Huang Hongwei Liu +5 位作者 Kunming Wei Liang Zhang Xiaoyan Ma Qingsong Li Xueyan Li Andrea M.Dietrich 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2024年第10期199-211,共13页
As a strong oxidizing agent,ozone is used in some water treatment facilities for disinfection,taste and odor control,and removal of organic micropollutants.Phenylalanine(Phe)was used as the target amino acid to compre... As a strong oxidizing agent,ozone is used in some water treatment facilities for disinfection,taste and odor control,and removal of organic micropollutants.Phenylalanine(Phe)was used as the target amino acid to comprehensively investigate variability of disinfection byproducts(DBPs)formation during chlorine disinfection and residual chlorine conditions subsequent to ozonation.The results showed that subsequent to ozonation,the typical regulated and unregulated DBPs formation potential(DBPsFP),including trichloromethane(TCM),dichloroacetonitrile(DCAN),chloral hydrate(CH),dichloroacetic acid(DCAA),trichloroacetic acid(TCAA),and trichloroacetamide(TCAcAm)increased substantially,by 2.4,3.3,5.6,1.2,2.5,and 6.0 times,respectively,compared with only chlorination.Ozonation also significantly increased the DBPs yield under a 2 day simulated residual chlorine condition that mimicked the water distribution system.DBPs formations followed pseudo first order kinetics.The formation rates of DBPs in the first 6 hr were higher for TCM(0.214 hr^(−1)),DCAN(0.244 hr^(−1)),CH(0.105 hr^(−1)),TCAcAm(0.234 hr^(−1)),DCAA(0.375 hr^(−1))and TCAA(0.190 hr^(−1))than thereafter.The peak DBPsFP of TCM,DCAN,CH,TCAcAm,DCAA,and TCAA were obtained when that ozonation time was set at 5–15 min.Ozonation times>30 min increased the mineralization of Phe and decreased the formation of DBPs upon chlorination.Increasing bromine ion(Br^(−1))concentration increased production of bromine-DBPs and decreased chlorine-DBPs formation by 59.3%–92.2%.Higher ozone dosages and slight alkaline favored to reduce DBP formation and cytotoxicity.The ozonation conditions should be optimized for all application purposes including DBPs reduction. 展开更多
关键词 OZONE Amino acids CHLORINATION disinfection by-products
原文传递
Bacteria inactivation by sulfate radical:progress and non-negligible disinfection by-products 被引量:1
14
作者 Xin Zhou Xiaoya Ren +8 位作者 Yu Chen Haopeng Feng Jiangfang Yu Kang Peng Yuying Zhang Wenhao Chen Jing Tang Jiajia Wang Lin Tang 《Frontiers of Environmental Science & Engineering》 SCIE EI CSCD 2023年第3期23-36,共14页
Sulfate radicals have been increasingly used for the pathogen inactivation due to their strong redox ability and high selectivity for electron-rich species in the last decade.The application of sulfate radicals in wat... Sulfate radicals have been increasingly used for the pathogen inactivation due to their strong redox ability and high selectivity for electron-rich species in the last decade.The application of sulfate radicals in water disinfection has become a very promising technology.However,there is currently a lack of reviews of sulfate radicals inactivated pathogenic microorganisms.At the same time,less attention has been paid to disinfection by-products produced by the use of sulfate radicals to inactivate microorganisms.This paper begins with a brief overview of sulfate radicals’properties.Then,the progress in water disinfection by sulfate radicals is summarized.The mechanism and inactivation kinetics of inactivating microorganisms are briefly described.After that,the disinfection by-products produced by reactions of sulfate radicals with chlorine,bromine,iodide ions and organic halogens in water are also discussed.In response to these possible challenges,this article concludes with some specific solutions and future research directions. 展开更多
关键词 Sulfate radicals disinfection by-products Inactivation mechanisms Bacterial inactivation Water disinfection
原文传递
Genotoxicity Induced by Low Dose and Mixed Exposure to Haloacetaldehydes,an Emerging Class of Drinking Water Disinfection By-products
15
作者 YANG Lili MA Wuren +6 位作者 JIANG Zhiqiang CHEN Yu QIU Meiyue ZHOU Ying James C.CRABBE ZHENG Weiwei QU Weidong 《Chemical Research in Chinese Universities》 SCIE CAS CSCD 2023年第3期481-491,共11页
Haloacetaldehydes(HALs)are the third largest disinfection by-products(DBPs)class by mass in drinking water.Most of them alone in high doses are more cytotoxic and genotoxic than regulated DBPs.However,the toxic effect... Haloacetaldehydes(HALs)are the third largest disinfection by-products(DBPs)class by mass in drinking water.Most of them alone in high doses are more cytotoxic and genotoxic than regulated DBPs.However,the toxic effects of mixed exposure to HALs at environmentally relevant levels are still unknown.Given that genotoxicity is critical for risk assessment,we employed multiple genotoxic tests including the Salmonella typhimurium revertant mutation assay(Ames assay),the single cell gel electrophoresis(SCGE)assay,the cytoplasmic blocking micronucleus(CBMN)assay,and theγ-H2AX assay to investigate the genotoxicity of HALs based on the HALs concentrations and components detected in the finished drinking water of Shanghai,China.The results demonstrated the concentrations of HALs were low,ranging from 0.04µg/L to 4.47µg/L,and the total concentration was 10.85µg/L.Although the mutagenicity of HALs was negative even at 1000-fold concentrations in the real world,mixed exposure to 100 and 1000-fold concentrations HALs resulted in DNA and chromosomal damage in human hepotocyte(HepG2)cells.HALs significantly increased the levels of reactive oxygen species(ROS)andγ-H2AX and activated nuclear factor erythroid-derived factor 2-related factor 2(NRF2)pathway-related protein expressions in HepG2 cells.The antioxidant NAC could ameliorate NRF2 pathway-related protein expression and DNA damage caused by HALs,suggesting that the genotoxicity of mixed exposure to HALs involved cellular oxidative stress and NRF2 pathway activation. 展开更多
关键词 Unregulated disinfection by-product Haloacetaldehyde Mixed exposure GENOTOXICITY
原文传递
Removal of organic matter and disinfection by-products precursors in a hybrid process combining ozonation with ceramic membrane ultrafiltration 被引量:8
16
作者 Xiaojiang FAN Yi TAO +3 位作者 Dequan WEI Xihui ZHANG Ying LEI Hiroshi NOGUCHI 《Frontiers of Environmental Science & Engineering》 SCIE EI CAS CSCD 2015年第1期112-120,共9页
The performance of an integrated process including coagulation, ozonation, ceramic ultrafiltration (UF) and biologic activated carbon (BAC) filtration was investigated for the removal of organic matter and disinfe... The performance of an integrated process including coagulation, ozonation, ceramic ultrafiltration (UF) and biologic activated carbon (BAC) filtration was investigated for the removal of organic matter and disinfection by-products (DBPs) precursors from micropolluted surface water. A pilot scale plant with the capacity of 120 m3 per day was set up and operated for the treatment of drinking water. Ceramic membranes were used with the filtration area of 50 m2 and a pore size of 60 nm. Dissolved organic matter was divided into five fractions including hydrophobic acid (HoA), base (HOB) and neutral (HoN), weakly hydrophobic acid (WHOA) and hydrophilic matter (HIM) by DAX-8 and XAD-4 resins. The experiment results showed that the removal of organic matter was significantly improved with ozonation in advance. In sum, the integrated process removed 73% of dissolved organic carbon (DOC), 87% of UV254, 77% of trihalomethane (THMs) precursors, 76% of haloacetic acid (HAAs) precursors, 83%of trichloracetic aldehyde (CH) precursor, 77% of dichloroaeetonitrile (DCAN) precursor, 51% of trichloroacetonitrile (TCAN) precursor, 96% of 1,1,1- trichloroacetone (TCP) precursor and 63% of trichloroni- tromethane (TCNM) precursor. Hydrophobic organic matter was converted into hydrophilic organic matter during ozonation/UF, while the organic matter with molecular weight of 1000-3000 Da was remarkably decreased and converted into lower molecular weight organic matter ranged from 200-500 Da. DOC had a close linear relationship with the formation potential of DBPs. 展开更多
关键词 ceramic ultrafiltration(UF) OZONATION organic matter HYDROPHILIC HYDROPHOBIC disinfection by-products
原文传递
Control of Bromate and THM Precursors Using Ozonation Combined System 被引量:1
17
作者 SHU-GUANG XIE DONG-WEN SHI +2 位作者 DONG-HUI WEN RUI WANG DAN-LI XI 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2007年第3期217-225,共9页
Objective To investigate the feasibility of reducing THM precursors and controlling bromate taste and odor in drinking water taken from the Yellow River by an ozonation combined system. Methods The appropriate ozone d... Objective To investigate the feasibility of reducing THM precursors and controlling bromate taste and odor in drinking water taken from the Yellow River by an ozonation combined system. Methods The appropriate ozone dosage was determined, and then the changes of TOC, UV254 and THM formation potential (THMFP) in the combined system were evaluated. Results One mg/L ozone could effectively remove taste and odor and meet the maximum allowable bromate level in drinking water. The pre-ozonation increased THMFP, but the conventional treatment system could effectively reduce the odor. The bio-ceramic filter could partly reduce CHC13FP, but sometimes might increase CHCl2BrFP and CHClBr2FP. The biological activated carbon (BAC) filter could effectively reduce CHC13FP and CHCl2BrFP, but increase CHClBr2FP. Compared with other filters, the fresh activated carbon (FAC) filter performed better in reducing THMFP and even reduced CHClBr2FP. Conclusion The combined system can effectively reduce taste, odor, CHC13FP, and CHCl2BrFP and also bring bromate under control. 展开更多
关键词 BROMATE OZONATION disinfection by-products Activated carbon
下载PDF
Toxicity effects of disinfection byproduct chloroacetic acid to Microcystis aeruginosa: Cytotoxicity and mechanisms 被引量:1
18
作者 Jing Ye Jiawei Ni +7 位作者 Fuxiang Tian Xiyan Ji Meifang Hou Yuanting Li Lei Yang Runxiang Wang Wenwu Xu Liang Meng 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2023年第7期229-239,共11页
Chlorine-based disinfectants are widely used for disinfection in wastewater treatment.The mechanism of the effects of chlorinated disinfection by-products on cyanobacteria was unclear.Herein,the physiological effects ... Chlorine-based disinfectants are widely used for disinfection in wastewater treatment.The mechanism of the effects of chlorinated disinfection by-products on cyanobacteria was unclear.Herein,the physiological effects of chloroacetic acid(CAA)on Microcystis aeruginosa(M.aeruginosa),including acute toxicity,oxidative stress,apoptosis,production of microcystin-LR(MC-LR),and the microcystin transportation-related gene mcyH transcript abundance have been investigated.CAA exposure resulted in a significant change in the cell ultrastructure,including thylakoid damage,disappearance of nucleoid,production of gas vacuoles,increase in starch granule,accumulation of lipid droplets,and disruption of cytoplasm membranes.Meanwhile,the apoptosis rate of M.aeruginosa increased with CAA concentration.The production of MC-LR was affected by CAA,and the transcript abundance of mcyH decreased.Our results suggested that CAA poses acute toxicity to M.aeruginosa,and it could cause oxidative damage,stimulate MC-LR production,and damage cell ultrastructure.This study may provide information about the minimum concentration of CAA in the water environment,which is safe for aquatic organisms,especially during the global coronavirus disease 2019 pandemic period. 展开更多
关键词 disinfection by-products MICROCYSTIN Oxidative damage Ultrastructure characteristics APOPTOSIS
原文传递
Research progress of disinfection and disinfection by-products in China 被引量:19
19
作者 Xuefeng Sun Miao Chen +1 位作者 Dongbin Wei Yuguo Du 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2019年第7期52-67,共16页
Disinfection is an indispensable water treatment process for killing harmful pathogens and protecting human health. However, the disinfection has caused significant public concern due to the formation of toxic disinfe... Disinfection is an indispensable water treatment process for killing harmful pathogens and protecting human health. However, the disinfection has caused significant public concern due to the formation of toxic disinfection by-products(DBPs). Lots of studies on disinfection and DBPs have been performed in the world since 1974. Although related studies in China started in1980 s, a great progress has been achieved during the last three decades. Therefore, this review summarized the main achievements on disinfection and DPBs studies in China, which included:(1) the occurrence of DBPs in water of China,(2) the identification and detection methods of DBPs,(3) the formation mechanisms of DBPs during disinfection process,(4) the toxicological effects and epidemiological surveys of DBPs,(5) the control and management countermeasures of DBPs in water disinfection, and(6) the challenges and chances of DBPs studies in future. It is expected that this review would provide useful information and reference for optimizing disinfection process, reducing DBPs formation and protecting human health. 展开更多
关键词 disinfection disinfection by-products IDENTIFICATION FORMATION MECHANISMS TOXICOLOGY Control
原文传递
Enhanced removal of organic matter and typical disinfection byproduct precursors in combined iron–carbon micro electrolysis-UBAF process for drinking water pre-treatment 被引量:4
20
作者 Yinghan Chen Tao Lin Wei Chen 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2019年第4期315-327,共13页
The organic matter and two types of disinfection byproduct(DBP) precursors in micropolluted source water were removed using an iron–carbon micro-electrolysis(ICME)combined with up-flow biological aerated filter(UBAF)... The organic matter and two types of disinfection byproduct(DBP) precursors in micropolluted source water were removed using an iron–carbon micro-electrolysis(ICME)combined with up-flow biological aerated filter(UBAF) process. Two pilot-scale experiments(ICME-UBAF and UBAF alone) were used to investigate the effect of the ICME system on the removal of organic matter and DBP precursors. The results showed that ICME pretreatment removed 15.6% of dissolved organic matter(DOM)and significantly improved the removal rate in the subsequent UBAF process. The ICME system removed 31% of trichloromethane(TCM) precursors and 20% of dichloroacetonitrile(DCAN) precursors. The results of measurements of the molecular weight distribution and hydrophilic fractions of DOM and DBP precursors showed that ICME pretreatment played a key role in breaking large-molecular-weight organic matter into low-molecular-weight components, and the hydrophobic fraction into hydrophilic compounds, which was favorable for subsequent biodegradation by UBAF.Three-dimensional fluorescence spectroscopy(3D-EEM) further indicated that the ICME system improved the removal of TCM and DCAN precursors. The biomass analysis indicated the presence of a larger and more diverse microbial community in the ICME-UBAF system than for the UBAF alone. The high-throughput sequencing results revealed that domination of the genera Sphingomonas, Brevundimonas and Sphingorhabdus contributed to the better removal of organic matter and two types of DBP precursors. Also, Nitrosomonas and Pseudomonas were beneficial for ammonia removal. 展开更多
关键词 DRINKING water pre-treatment MICRO-ELECTROLYSIS UP-FLOW biological aerated filter Organic matter disinfection by-product precursors
原文传递
上一页 1 2 8 下一页 到第
使用帮助 返回顶部