Internal collision double ionization of molecules driven by co-rotating two-color circularly polarized laser pulses

The double ionization process of molecules driven by co-rotating two-color circularly polarized fields is investigated with a three-dimensional classical ensemble model. Numerical results indicate that a considerable part of the sequential double ionization(DI) events of molecules occur through internal collision double ionization(ICD), and the ICD recollision mechanism is significantly different from that in non-sequential double ionization(NSDI). By analyzing the results of internuclear distances R = 5 a.u. and 2 a.u., these two recollision mechanisms are studied in depth. It is found that the dynamic behaviors of the recollision mechanisms of NSDI and ICD are similar. For NSDI, the motion range of electrons after the ionization is relatively large, and the electrons will return to the core after a period of time. In the ICD process,electrons will rotate around the parent ion before ionization, and the distance of the electron motion is relatively small. After a period of time, the electrons will come back to the core and collide with another electron. Furthermore, the molecular internuclear distance has a significant effect on the electron dynamic behavior of the two ionization mechanisms. This study will help to understand the multi-electron ionization process of complex systems.

Steering the energy sharing of electrons in nonsequential double ionization with orthogonally polarized two-color field

Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.

Effect of elliptical polarizations on nonsequential double ionization in two-color elliptically polarized laser fields

Using the classical ensemble model, we investigate the nonsequential double ionization（NSDI） of Ar and Mg in the two-color elliptically polarized laser pulse for different elliptical polarizations. Numerical results show that for Ar atoms the NSDI yield increases as the ellipticity increases, which is different from the case of Mg atoms. Moreover, the correlated behavior in the correlated electron momentum along the x direction and ion momentum distributions of Ar atoms are influenced by the ellipticity. By statistical analysis of different times, we can conclude that the ellipticity may be responsible for the NSDI processes. The correlated momenta distributions along the x direction at the recollision time are demonstrated and the results show that the travelling time and ellipticity can affect the emitted directions of both electrons.

Electron correlations in nonsequential double ionization of argon atoms by elliptically polarized laser pulses

Using a classical ensemble model, we investigate the correlation behaviour of electrons originating from nonsequential double ionization （NSDI） of argon atoms by the elliptically polarized laser pulses. Because of the ellipticity, not only the first electron to return but also the later return of tunneled electrons contribute significantly to NSDI. We mainly discuss two kinds of events of NSDI originating from the first and the second return separately. For the NSDI resulting from the recollision of the first return, the correlated electron momentum spectrum along the long axis of the laser polarization plane reveals an obvious V-like shape, located at the first and third quadrant. However, for the NSDI resulting from the recollision of the second return, the momenta of two electrons are distributed in the four quadrants uniformly. By analysing the trajectories of these two kinds, we find that the recollision energy and the laser phase at recollision are different for the first and second returning trajectories, which are responsible for the difference in the correlated behavior of the final electron momentum.

The effect of electron initial longitudinal velocity on the non-sequential double ionization process in an elliptically polarized laser field

The effect of initial longitudinal velocity of the tunnelled electron on the non-sequential double ionization （NSDI） process in an elliptically polarized laser field is studied by a semiclassical model. We find that the non-zero initial longitudinal velocity has a suppressing effect on single-return collision （SRC） events in the double ionization process, more specifically, it results in an obvious reduction in the center part of the correlation momentum distributions in the direction of the major polarization axis （z axis） and makes the distribution of single-return collision in the minor polarization axis （x axis） become narrower.

Relative phase effect of nonsequential double ionization in Ar by two-color elliptically polarized laser field

We investigated the nonsequential double ionization(NSDI)in Ar by two-color elliptically polarized laser field with a three-dimensional(3D)classical ensemble method.We study the relative phase effect of NSDI and distinguish two particular recollision channels in NSDI,which are recollision–impact ionization(RII)and recollision-induced excitation with subsequent ionization(RESI),according to the delay-time between the recollision and the final double ionization.The numerical results indicate that the ion momentum distribution is changed and the triangle structure is more obvious with the decrease of the relative phase.We also demonstrate that the RESI process always dominates in the whole double ionization process and the ratio of RESI and RII channels can be influenced by the relative phase.

Effect of Solvent Polarity on Excited-State Double Proton Transfer Process of 1,5-Dihydroxyanthraquinone

The excited-state double proton transfer(ESDPT)properties of 1,5-dihydroxyanthraquinone(1,5-DHAQ)in various solvents were investigated using femtosecond transient absorption spectroscopy and the DFT/TDDFT method.The steady-state fluorescence spectra in toluene,tetrahydrofuran(THF)and acetonitrile(ACN)solvents presented that the solvent polarity has an effect on the position of the ESDPT fluorescence emission peak for the 1,5-DHAQ system.Transient absorption spectra show that the increasing polarity of the solvent accelerates the rate of excited state dynamics.Calculated potential energy curves analysis further verified the experimental results.The ESDPT barrier decreases gradually with the increase of solvent polarity from toluene,THF to ACN solvent.It is convinced that the increase of solvent polarity can promote the occurrence of the ESDPT dynamic processes for the 1,5-DHAQ system.This work clarifies the mechanism of the influence of solvent polarity on the ESDPT process of 1,5-DHAQ,which provides novel ideas for design and synthesis of new hydroxyanthraquinone derivatives.

The Pionic Deuterium and the Pion Tetrahedron Vacuum Polarization

A double-well potential model is proposed for the pionic deuterium that enables to calculate the energy split, the potential barrier height and estimate the pion tetrahedron edge length. We propose that pion tetrahedrons, πTd = ud~dũ, play a central role in the Yukawa interaction by enabling quark exchange reactions between protons and neutrons by tunneling through a potential barrier. A vacuum polarization Feynman diagram is proposed for the πTd having chains of fermion loops for the two valence quarks and anti-quarks connected by gluons. With a higher order vacuum polarization diagram, the d and u quark loops are interleaved and the chiral symmetry is broken dynamically. The proposed πTd vacuum polarization integral does not diverge in both the IR and UV limits and vanishes in the limit of an infinite pion tetrahedron condensate. We propose a new Delbruck scattering Feynman diagram that includes d and u quark and anti-quark interleaved loops. We further propose that conversion of gravitons to photons may occur via quark and anti-quark loops that describe the pion tetrahedrons dynamics in the vacuum and may also transfer gravitational waves.

Double ferromagnetic metal/semiconductor schottky barrier confined quasi-ballistic transport channel as spin polarizer

Spin polarizer is one of the most important devices for the newly developing field of spintronics,which may revolute the popular information techniques.Here we present a phenomenal model for a novel spin polarizer,which utilizes two back to back ferromagnetic metal/semiconductor Schottky barriers to define a semiconductor transport channel whose length is less than the spin decoherence length of the host semiconductor.Along this channel,conducting electrons move diffusively in momentum space while they keep ballistic motion in spin space.Across the channel,electrons suffer a spin dependent tunneling,which establishes spin polarization along the channel.

Spin-polarized current in double quantum dots

We analyze the transport through asymmetric double quantum dots with an inhomogeneous Zeeman splitting in the presence of crossed dc and ac magnetic fields. A strong spin-polarized current can be obtained by changing the dc magnetic field. It is mainly due to the resonant tunnelling. But for the ferromagnetic right electrode, the electron spin resonance also plays an important role in transport. We show that the double quantum dots with three-level mixing under crossed dc and ac magnetic fields can act not only as a bipolar spin filter but also as a spin inverter under suitable conditions.

Ferroelectricity induced by the absorption of water molecules on double helix SnIP

We study the ferroelectricity in a one-dimensional(1D)system composed of a double helix SnIP with absorbing water molecules.Our ab initio calculations reveal two factors that are critical to the electrical polarization.The first one is the orientation of polarized water molecules staying in the R2 region of SnIP.The second one is the displacement of I atom which roots from subtle interaction with absorbed water molecules.A reasonable scenario of polarization flipping is proposed in this study.In the scenario,the water molecule is rolling-up with keeping the magnitude of its electrical dipole and changing its direction,meanwhile,the displacement of I atoms is also reversed.Highly tunable polarization can be achieved by applying strain,with 26.5%of polarization enhancement by applying tensile strain,with only 4%degradation is observed with 4%compressive strain.Finally,the direct band gap is also found to be correlated with strain.

Separating spins by dwell time of electrons across parallel double δ-magnetic-barrier nanostructure applied by bias

The dwell time and spin polarization(SP)of electrons tunneling through a parallel doubleδ-magnetic-barrier nanostructure in the presence of a bias voltage is studied theoretically in this work.This nanostructure can be constructed by patterning two asymmetric ferromagnetic stripes on the top and bottom of InAs/AlxIn1-xAs heterostructure,respectively.An evident SP effect remains after a bias voltage is applied to the nanostructure.Moreover,both magnitude and sign of spin-polarized dwell time can be manipulated by properly changing the bias voltage,which may result in an electrically-tunable temporal spin splitter for spintronics device applications.

Propagation properties of stochastic electromagnetic double-vortex beams in a turbulent atmosphere

Based on the extended Huygens-Fresnel principle, we study the propagation properties of stochastic electromagnetic double-vortex beams in a turbulent atmosphere. The result shows that the spreading of partially coherent double-vortex beams can be smaller than that of fully coherent ones. The degree of polarization of this kind of beam will experience change, which is dependent on the degree of polarization of the source plane, the atmospheric turbulence, topological charge, and the spatial coherence. The results may have applications in space optical communication.

Experimental Measurement of the Generalized Stokes Parameters of a Radially Polarized Random Electromagnetic Beam

Utilizing the Young’s double slits and Mach-Zehnder interferometer, we proposed an experimental method to measure the generalized Stokes parameters of a radially polarized random electromagnetic beam. After the partially coherent beam propagating through the Young’s double slits, the interference fringe is obtained by the help of a Mach-Zehnder interferometer consisting of apertures, quarter-wave plates and polarizers. The electric cross-spectral density matrix is detected by the coherence degree of interference fringe and the density of each single slit. The generalized Stokes parameters can be obtained from the electric cross-spectral density matrix. This experiment measures the generalized Stokes parameters of the random electromagnetic beam successfully. The results show that the spectral degree of coherence for copolarized cases (xx and yy) is similar with that for cross-polaried cases (xy and yx) for the radially polarized random electromagnetic beam. This method will help us determine the change of the polarization and coherence of the light in propagation by detecting the change of the generalized Stokes parameters.

双层电介质界面极化电流测量装置的设计与实现

界面夹层极化现象是高电压技术中的重要知识点。为了使学生更好地掌握双层电介质界面极化电流的测量,研制了一套界面极化电流测量装置——极化-去极化电流测量装置。基于极化-去极化电流测量原理,设计了无线传输数据的皮安表、可输出0~5 kV电压的程控直流高压电源以及分析显示数据的上位机控制程序,然后基于该测量装置设计了双层电介质界面极化电流测量实验。结果表明,该测量装置解决了双层电介质界面极化电流不易测量、学生理解难的问题。将实验教学与实际工程问题紧密连接,把微观的工程技术问题转变为宏观的实验现象,对于培养学生的科研思维及分析问题、解决问题能力有重要意义。

各向异性超表面宽带高效极化转换

为了实现水平方向和垂直方向入射电磁波的高效率、宽带反射型交叉极化转换,提出了一种各向异性超表面结构,使用数值模拟仿真方法以及有限元分析方法进行研究。结果表明,所设计双十字结构超表面的电磁响应谱产生了4个共振区,从而导致了极化转换带宽的扩展。响应频段覆盖了Ku波段的10.7~18.7 GHz,其极化转换率(polarization conversion ratio,PCR)大于0.94。此外,在入射波角度为0°~50°内,都能保持较高的极化转换性能。该极化转换器具有简单的几何形状和较宽的工作频带,可能在伪装隐身、雷达通信和天线等应用中具有潜在的价值。

一道二重积分的多种异向思维解法探讨

本文针对2022年全国硕士研究生入学考试试题中一道二重积分问题,探讨了运用Green公式、极坐标变换、对称性、挖补思想、区域可加性等多种计算方法,并给出了相应的分析过程及解答.

基于WMIAEKF的锂离子电池SOC与容量联合估算

精确的荷电状态(SOC)估算对可靠的电池管理系统来说十分关键。基于二阶等效电路模型,提出了一种加权多新息自适应扩展卡尔曼滤波(WMIAEKF)算法,该算法可以解决传统多新息算法中误差累积的问题,从而提高SOC估算精度。实验仿真结果表明,所提算法比传统的自适应扩展卡尔曼(AEKF)以及多新息自适应扩展卡尔曼(MIAEKF)精度要高,最大误差控制在1.15%以内。此外,基于该算法提出了一种改进的多时间尺度双卡尔曼滤波算法,其中,WMIAEKF用于SOC估算,AEKF用于容量估算,两者结合对电池的SOC和容量进行实时的联合估算。所提算法能够对电池SOC以及容量进行较精确的估计,在新欧洲行驶工况(NEDC)下,SOC估算误差始终控制在1.2%,并且在面对错误容量初始值时也能保持较好的鲁棒性。

极地钻探用铝合金双壁钻杆结构强度的有限元分析及试验研究

为了实现钻穿冰盖、直接获取冰下基岩样品的科研目标,本文设计了一种极地钻探用铝合金双壁钻杆,使钻杆可以满足极地上覆积雪层、冰层、冰岩夹层和冰下基岩等不同地层的空气反循环、水力反循环、绳索取心钻进相配合等钻进需求。依据铝合金双壁钻杆在极限拉伸、极限拉扭组合工况下的受力情况,开展了双壁钻杆的有限元分析,并对双壁钻杆外管与钢接头连接试样进行了拉伸试验与扭转试验。双壁钻杆有限元分析结果表明:在极限拉伸和极限拉扭组合工况下铝合金双壁钻杆中产生的最大应力分别为183.8 MPa与161.9 MPa,均小于铝合金材料的屈服强度489.99 MPa。双壁钻杆外管与钢接头连接试样强度试验结果也表明:拉伸试样破坏时的极限可承载拉力为399.5 kN,远大于提升1000 m双壁钻杆所需的拉力(208.11 kN);扭转试样破坏时的极限可承载扭矩为8264.7N·m,同样大于钻杆在正常钻进过程当中所承受的最大扭矩(1990.56 N·m)。上述结果表明,极地钻探用铝合金双壁钻杆设计方案可以满足极地钻探使用要求。

利用水波初至偏振方位反演海底地震仪位置及方位

OBS(Ocean Bottom Seismometer,海底地震仪)在布放到海底之后,其方位指向通常是随机的;由于海流等因素的影响,其实际位置通常也会偏离投放位置,因此需要对其位置及方位进行重定位定向。针对目前的定位和定向方法大多基于走时计算,本文首先讨论了利用海底地震仪的水波初至偏振方位进行海底地震仪水平位置及方位重定位定向的线性反演方法和非线性反演方法,给出了线性反演的近似公式,并分析了近似公式的误差;然后,通过大量理论模型试验对比了两种方法的误差及稳定性;最后,对我国南海某地的5台OBS实测数据进行了反演处理。理论模型试验结果表明,在一些特殊情况下,线性反演存在不收敛的情况,而非线性方法则具有较好的稳定性和较高的精度。非线性反演方法采用差分演化算法,对比了直接优化方位角残差目标函数和双差法,结果表明,对于理论模型和实际数据两种方法得到的结果几乎完全相同,但迭代收敛情况双差法明显好于前者,双差法经600余次迭代达到最优稳定状态,而前者在迭代1000多次之后才达到稳定最优状态。