This study investigated the potential role of soil colloids and dissolved organic matter （DOM） in transporting Cd through in situ undisturbed paddy soil monoliths. Brilliant Blue was used as a tracer to assess the e...This study investigated the potential role of soil colloids and dissolved organic matter （DOM） in transporting Cd through in situ undisturbed paddy soil monoliths. Brilliant Blue was used as a tracer to assess the effect of preferential flow on Cd down migration. Experimental results showed that deep penetration of Cd and Brilliant Blue into the soil profile took place due to the preferential flow through macropores, mainly earthworm channels, with much of chemicals thus bypassing the soil matrix. Dye tracer and Cd distribution within the soil matrix was fairly restricted to several centimeters. Colloid restrained the migration of both dye and Cd in the matrix and preferential flow area. DOM facilitated the transport of Cd and Brilliant Blue in matrix and macropores by about 10 cm over that of the control. Pearson＇s is correlation analysis revealed strong associations between Brilliant Blue concentrations, exchangeable Cd and total Cd concentrations in three studied plots indicating that they had taken the same preferential flow pathway.展开更多
The nature of subsurface flow depends largely on hydraulic conductivity of the vadoze zone, permeability of the underlying bedrock, existence of soil layers differing in hydraulic properties and macropore content, soi...The nature of subsurface flow depends largely on hydraulic conductivity of the vadoze zone, permeability of the underlying bedrock, existence of soil layers differing in hydraulic properties and macropore content, soil depth, and slope angle.Quantification of flow pathways on forested hillslopes is essential to understand hydrological dynamics and solute transport patterns.Acrisols, with their argic Bt horizons, are challenging in this respect.To further elucidate flow pathways of water and short-term variability of soil moisture patterns in Acrisols, a field study was conducted on a forested hillslope in a sub-catchment of the Tie Shan Ping(TSP)watershed, 25 km northeast of Chongqing City, China.This catchment is covered by a mixed secondary forest dominated by Masson pine(Pinus massoniana).Soil saturated hydraulic conductivity(K sat) was significantly reduced at the interface between the AB and Bt horizons(2.6 × 10^(-5) vs.1.2 × 10^(-6) m s^(-1)), which led to that the flow volume generated in the Bt horizon was of little quantitative importance compared to that in the AB horizon.There was a marked decrease in porosity between the OA and AB horizons, with a further decrease deeper in the mineral subsoil.Especially, the content of soil pores > 300 μm was higher in the AB horizon(14.3%)than in the Bt horizon(6.5%).This explained the difference in soil K sat values.This study showed that Bt horizon had limited water transport capability, forcing part of the infiltrated rainwater as interflow through the OA and AB horizons.Thus, the topsoil responded quickly to rainfall events, causing frequent cycles of saturation and aeration of soil pores.展开更多
基金supported by the National Natural Science Foundation of China (No.40571073)
文摘This study investigated the potential role of soil colloids and dissolved organic matter （DOM） in transporting Cd through in situ undisturbed paddy soil monoliths. Brilliant Blue was used as a tracer to assess the effect of preferential flow on Cd down migration. Experimental results showed that deep penetration of Cd and Brilliant Blue into the soil profile took place due to the preferential flow through macropores, mainly earthworm channels, with much of chemicals thus bypassing the soil matrix. Dye tracer and Cd distribution within the soil matrix was fairly restricted to several centimeters. Colloid restrained the migration of both dye and Cd in the matrix and preferential flow area. DOM facilitated the transport of Cd and Brilliant Blue in matrix and macropores by about 10 cm over that of the control. Pearson＇s is correlation analysis revealed strong associations between Brilliant Blue concentrations, exchangeable Cd and total Cd concentrations in three studied plots indicating that they had taken the same preferential flow pathway.
基金supported by the Norwegian Research Council(Nos.193725/S30 and 209696/E10)Chinese Academy of Science(CAS)(No.209696/E10)
文摘The nature of subsurface flow depends largely on hydraulic conductivity of the vadoze zone, permeability of the underlying bedrock, existence of soil layers differing in hydraulic properties and macropore content, soil depth, and slope angle.Quantification of flow pathways on forested hillslopes is essential to understand hydrological dynamics and solute transport patterns.Acrisols, with their argic Bt horizons, are challenging in this respect.To further elucidate flow pathways of water and short-term variability of soil moisture patterns in Acrisols, a field study was conducted on a forested hillslope in a sub-catchment of the Tie Shan Ping(TSP)watershed, 25 km northeast of Chongqing City, China.This catchment is covered by a mixed secondary forest dominated by Masson pine(Pinus massoniana).Soil saturated hydraulic conductivity(K sat) was significantly reduced at the interface between the AB and Bt horizons(2.6 × 10^(-5) vs.1.2 × 10^(-6) m s^(-1)), which led to that the flow volume generated in the Bt horizon was of little quantitative importance compared to that in the AB horizon.There was a marked decrease in porosity between the OA and AB horizons, with a further decrease deeper in the mineral subsoil.Especially, the content of soil pores > 300 μm was higher in the AB horizon(14.3%)than in the Bt horizon(6.5%).This explained the difference in soil K sat values.This study showed that Bt horizon had limited water transport capability, forcing part of the infiltrated rainwater as interflow through the OA and AB horizons.Thus, the topsoil responded quickly to rainfall events, causing frequent cycles of saturation and aeration of soil pores.
