We analytically and numerically investigate a signal light storing mechanism based on the controllable electromagnetically induced transparency(EIT)effect.We demonstrate that the isolation between the waveguide and th...We analytically and numerically investigate a signal light storing mechanism based on the controllable electromagnetically induced transparency(EIT)effect.We demonstrate that the isolation between the waveguide and the cavities cannot be achieved instantly as soon as the two cavities are tuned into resonance,no matter the index tuning rate is ultrafast or slow.We also investigate the temporal evolution features of the intracavity energy when the pulse during time is prolonged.We find many periodical oscillations of the trapped energy in both cavities,and they are entirely complementary.Our analysis shows that the adiabatic wavelength conversion in both cavities and a phase difference π between them play critical roles in this phenomenon.展开更多
The dynamic control of single-photon scattering in a pair of one-dimensional waveguides mediated by a time-modulated atom-cavity system is investigated.Two cases,where the waveguides are coupled symmetrically or asymm...The dynamic control of single-photon scattering in a pair of one-dimensional waveguides mediated by a time-modulated atom-cavity system is investigated.Two cases,where the waveguides are coupled symmetrically or asymmetrically to the atom-cavity system,are discussed in detail.The results show that such time-modulated atom-cavity configuration can behave as a dynamical tunable directional single-photon router.The photons with different frequencies can dynamically be routed from the incident waveguide into any ports of the other with a 100%probability via adjusting the modulated amplitude or phases of the time-modulated atom-cavity coupling strengths,associate with the help of the asymmetrical waveguide-cavity couplings.Furthermore,the influence of dissipation on the routing capability is investigated.It is shown that the present single-photon router is robust against the dissipative process of the system,especially the atomic dissipation.These results are expected to be applicable in quantum information processing and design quantum devices with dynamical modulation.展开更多
Modulation of light underpins a central part of modern optoelectronics.Con-ventional optical modulators based on refractive-index and absorption varia-tion in the presence of an electric field serve as the workhorse f...Modulation of light underpins a central part of modern optoelectronics.Con-ventional optical modulators based on refractive-index and absorption varia-tion in the presence of an electric field serve as the workhorse for diverse photonic technologies.However,these approaches based on electro-refraction or electro-absorption effect impose limitations on frequency converting and signal amplification.Lanthanide-activated phosphors offer a promising plat-form for nonlinear frequency conversion with an abundant spectrum.Here,we propose a novel approach to achieve frequency conversion and digital modula-tion of light signal by coupling lanthanide luminescence with an electrically responsive ferroelectric host.The technological benefits of such paradigm-shifting solution are highlighted by demonstrating a quasi-continuous and enhancement of the lanthanide luminescence.The ability to locally manipulate light emission can convert digital information signals into visible waveforms,and visualize electrical logic and arithmetic operations.The proof-of-concept device exhibits perspectives for developing light-compatible logic functions.These results pave the way to design more controllable lanthanide photonics with desired opto-electronic coupling.展开更多
Buckybowl structures as non-uniform electrostatic potential distributions of poly-cyclic aromatic materials show a unique photoelectric performance.In this work,OTC was utilized for dynamic modulation of triplet excit...Buckybowl structures as non-uniform electrostatic potential distributions of poly-cyclic aromatic materials show a unique photoelectric performance.In this work,OTC was utilized for dynamic modulation of triplet exciton transition processes.Five host molecules with different functional units were selected,thus providing dif-ferent intermolecular interactions in the host/guest systems.Therefore,the delayed emissions were regulated from 536 to 624 nm via the tuning of the triplet exciton transition processes of OTC in different hosts.Experimental data and theoretical calculations revealed that the varied triplet transition behaviors resulted from the competition between the intersystem crossing(ISC)process of OTC-monomer and the reverse intersystem crossing(RISC)process of OTC-aggregates.This work proves the superior structure of buckybowl-based luminophore for controlling triplet exciton transition processes and supplies a new perspective for persistent afterglow luminophore design.展开更多
Hollow metal-organic frameworks(MOFs)have attracted increasing attention in the field of catalysis in recent years due to their unique cavity structure with fast mass-diffusion rates and easily accessible active sites...Hollow metal-organic frameworks(MOFs)have attracted increasing attention in the field of catalysis in recent years due to their unique cavity structure with fast mass-diffusion rates and easily accessible active sites.Here,we report the use of dynamic modulators,which are formed by the in-situ imine condensation reaction of 4-aminobenzoic acid and 4-formylbenzoic acid,to regulate the growth of MOFs to synthesize well-defined hollow thioether functionalized UiO-67(denoted as H-UiO-67-S)single crystals.After supporting Pd nanoparticles,the designed catalysts Pd@H-UiO-67-S show excellent conversion(>99.9%),selectivity(>99.9%),and stability(10 cycles)in the selective hydrogenation of nitrobenzenes with other reducible groups.Density functional theory calculations and the experimental results reveal that Pd nanoparticles not only selectively adsorb the nitro-groups on nitrobenzene,but also restrict the adsorption of the aniline product,due to the interaction of thioether with Pd in the confined pores of H-UiO-67-S,finally result in a significant increase in selectivity of nitro-hydrogenation.展开更多
This paper presents a multi-HVDC emergency coordinated modulating strategy to enhance the transient stability of hybrid AC/DC power systems.First,the main factors that affect the unbalanced energy distribution during ...This paper presents a multi-HVDC emergency coordinated modulating strategy to enhance the transient stability of hybrid AC/DC power systems.First,the main factors that affect the unbalanced energy distribution during a fault are analyzed,and the dominant generators are determined online.Next,considering the influence on both generators in the sending and receiving ends,the assessment index that evaluates the effects of DC power support is established.On the basis of this,a dynamic DC power support strategy is put forward,and the DC support sequence table is promptly updated by the changing dominant generators.The AC/DC hybrid power system with multi-DC lines is built and used as a test system.The simulation results of different scenarios demonstrate that the proposed method could follow the dominant generator dynamically and adjust the DC participating in modulation to enhance the transient stability effectively and quickly.展开更多
Current methods for the detection of differential gene expression focus on finding individual genes that may be responsible for certain diseases or external irritants. However, for common genetic diseases, multiple ge...Current methods for the detection of differential gene expression focus on finding individual genes that may be responsible for certain diseases or external irritants. However, for common genetic diseases, multiple genes and their interactions should be understood and treated together during the exploration of disease causes and possible drug design. The present study focuses on analyzing the dynamic patterns of co-regulated modules during biological progression and determining those having remarkably varying activities, using the yeast cell cycle as a case study. We first constructed dynamic active protein-protein interaction networks by modeling the activity of proteins and assembling the dynamic co-regulation protein network at each time point. The dynamic active modules were detected using a method based on the Bayesian graphical model and then the modules with the most varied dispersion of clustering coefficients, which could be responsible for the dynamic mechanism of the cell cycle, were identified. Comparison of results from our functional module detection with the state-of-art functional module detection methods and validation of the ranking of activities of functional modules using GO annotations demonstrate the efficacy of our method for narrowing the scope of possible essential responding modules that could provide multiple targets for biologists to further experimentally validate.展开更多
This work demonstrates a two-step method to produce oxide-derived Cu nanowires on Cu mesh surface to offer a monolithic catalyst that outstandingly improves the hydrogen production from reforming formaldehyde and wate...This work demonstrates a two-step method to produce oxide-derived Cu nanowires on Cu mesh surface to offer a monolithic catalyst that outstandingly improves the hydrogen production from reforming formaldehyde and water under ambient conditions.Our results not only reveal that the special oxidederived nanostructure can significantly improve the formaldehyde reforming performance of Cu,but also display that the hydrogen production has a linear relationship with oxygen pressure.Specially,a maximum of 36 times increment in hydrogen generation rate is observed than that without oxygen during the reaction.Density functional theory calculations show that the formaldehyde molecule is adsorbed on Cu surface only when the adsorbed oxygen is in adjacency,and hydrogen release process is the ratedetermining step.This work highlights that the activity of deliberately synthesized catalyst can further be promoted by dynamic chemical modulation of surface states during working.展开更多
Flow against pipeline leakage and the pipe network sudden burst pipe to pipeline leakage flow for the application objects, an energy-efficient real-time scheduling scheme is designed extensively used in pipeline leak ...Flow against pipeline leakage and the pipe network sudden burst pipe to pipeline leakage flow for the application objects, an energy-efficient real-time scheduling scheme is designed extensively used in pipeline leak monitoring. The proposed scheme can adaptively adjust the network rate in real-time and reduce the cell loss rate, so that it can efficiently avoid the traffic congestion. The recent evolution of wireless sensor networks has yielded a demand to improve energy-efficient scheduling algorithms and energy-efficient medium access protocols. This paper proposes an energy-efficient real-time scheduling scheme that reduces power consumption and network errors on pipeline flux leak monitoring networks. The proposed scheme is based on a dynamic modulation scaling scheme which can scale the number of bits per symbol and a switching scheme which can swap the polling schedule between channels. Built on top of EDF scheduling policy, the proposed scheme enhances the power performance without violating the constraints of real-time streams. The simulation results show that the proposed scheme enhances fault-tolerance and reduces power consumption. Furthermore, that Network congestion avoidance strategy with an energy-efficient real-time scheduling scheme can efficiently improve the bandwidth utilization, TCP friendliness and reduce the packet drop rate in pipeline flux leak monitoring networks.展开更多
.Constructions of synthetic lattices in modulated ring resonators attract growing attention to interesting physics beyond the geometric dimensionality,where complicated connectivities between resonant frequency modes ....Constructions of synthetic lattices in modulated ring resonators attract growing attention to interesting physics beyond the geometric dimensionality,where complicated connectivities between resonant frequency modes are explored in many theoretical proposals.We implement experimental demonstration of generating a stub lattice along the frequency axis of light,in two coupled ring resonators of different lengths,with the longer one dynamically modulated.Such a synthetic photonic structure intrinsically exhibits the physics of flat band.We show that the time-resolved band structure read-out from the drop-port output of the excited ring is the intensity projection of the band structure onto a specific resonant mode in the synthetic momentum space,where gapped flat band,mode localization effect,and flat-to-nonflat band transition are observed in experiments and verified by simulations.This work provides evidence for constructing a synthetic stub lattice using two different rings,which,hence,makes a solid step toward experimentally constructing complicated lattices in multiple rings associated with synthetic frequency dimensions.展开更多
High temperature latent thermal storage is one of the critical techniques for a solar dynamic power system. This paper presents results from heat transfer analysis of a phase change salt containment canister A three-d...High temperature latent thermal storage is one of the critical techniques for a solar dynamic power system. This paper presents results from heat transfer analysis of a phase change salt containment canister A three-dimensional analysis program is developed to model heat transfer in a PCM canister. Analysis include effects of asymmetric circumference heat flux, conduction in canister walls, liquid PCM and solid PCM, void volume change and void location, and conduction and radiation across PCM vapor void. The PCM phase change process is modeled using the enthalpy method and the simulation results are compared with those of other two- dimensional investigations. It’s shown that there are large difference with two-dimensional analysis, therefore the three-dimensional model is necessary for system design of high temperature latent thermal storage.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.11774098)the Guangdong Natural Science Foundation(Grant Nos.2022A1515011950 and 2023A1515010781)the Science and Technology Program of Guangzhou(Grant No.202002030500)。
文摘We analytically and numerically investigate a signal light storing mechanism based on the controllable electromagnetically induced transparency(EIT)effect.We demonstrate that the isolation between the waveguide and the cavities cannot be achieved instantly as soon as the two cavities are tuned into resonance,no matter the index tuning rate is ultrafast or slow.We also investigate the temporal evolution features of the intracavity energy when the pulse during time is prolonged.We find many periodical oscillations of the trapped energy in both cavities,and they are entirely complementary.Our analysis shows that the adiabatic wavelength conversion in both cavities and a phase difference π between them play critical roles in this phenomenon.
基金Project supported by China Postdoctoral Science Foundation (Grant No.2023M732028)the Fund from Zhejiang Province Key Laboratory of Quantum Technology and Device (Grant No.20230201)+3 种基金the Fundamental Research Funds for the Provincial Universities of Zhejiang Province,China (Grant No.GK199900299012-015)the Natural Science Foundation of Zhejiang Province,China (Grant No.LY21A040003)the National Natural Science Foundation of China (Grant Nos.12164022,12174288,and 12274326)the Natural Science Foundation of Jiangxi Province,China (Grant No.20232BAB201044)。
文摘The dynamic control of single-photon scattering in a pair of one-dimensional waveguides mediated by a time-modulated atom-cavity system is investigated.Two cases,where the waveguides are coupled symmetrically or asymmetrically to the atom-cavity system,are discussed in detail.The results show that such time-modulated atom-cavity configuration can behave as a dynamical tunable directional single-photon router.The photons with different frequencies can dynamically be routed from the incident waveguide into any ports of the other with a 100%probability via adjusting the modulated amplitude or phases of the time-modulated atom-cavity coupling strengths,associate with the help of the asymmetrical waveguide-cavity couplings.Furthermore,the influence of dissipation on the routing capability is investigated.It is shown that the present single-photon router is robust against the dissipative process of the system,especially the atomic dissipation.These results are expected to be applicable in quantum information processing and design quantum devices with dynamical modulation.
基金the financial support from the National Natural Science Foundation of China(No.52233014,12074044,11874230,12274243)the Research Grants Council of Hong Kong(PolyU SRFS2122-5S02)+1 种基金the Fund of State Key Laboratory of Information Photonics and Optical Communications(IPOC2021ZT05,IPOC2022A02)the Fundamental Research Funds for the Central Universities(BUPT).
文摘Modulation of light underpins a central part of modern optoelectronics.Con-ventional optical modulators based on refractive-index and absorption varia-tion in the presence of an electric field serve as the workhorse for diverse photonic technologies.However,these approaches based on electro-refraction or electro-absorption effect impose limitations on frequency converting and signal amplification.Lanthanide-activated phosphors offer a promising plat-form for nonlinear frequency conversion with an abundant spectrum.Here,we propose a novel approach to achieve frequency conversion and digital modula-tion of light signal by coupling lanthanide luminescence with an electrically responsive ferroelectric host.The technological benefits of such paradigm-shifting solution are highlighted by demonstrating a quasi-continuous and enhancement of the lanthanide luminescence.The ability to locally manipulate light emission can convert digital information signals into visible waveforms,and visualize electrical logic and arithmetic operations.The proof-of-concept device exhibits perspectives for developing light-compatible logic functions.These results pave the way to design more controllable lanthanide photonics with desired opto-electronic coupling.
基金National Natural Scientific Foundation of China,Grant/Award Numbers:21975021,21975020,21875019,21871119,22105019,22175023Beijing National Laboratory for Molecular Sciences,Grant/Award Number:BNLMS192007BIT Research and Innovation Promoting Project,Grant/Award Number:2022YCXZ035。
文摘Buckybowl structures as non-uniform electrostatic potential distributions of poly-cyclic aromatic materials show a unique photoelectric performance.In this work,OTC was utilized for dynamic modulation of triplet exciton transition processes.Five host molecules with different functional units were selected,thus providing dif-ferent intermolecular interactions in the host/guest systems.Therefore,the delayed emissions were regulated from 536 to 624 nm via the tuning of the triplet exciton transition processes of OTC in different hosts.Experimental data and theoretical calculations revealed that the varied triplet transition behaviors resulted from the competition between the intersystem crossing(ISC)process of OTC-monomer and the reverse intersystem crossing(RISC)process of OTC-aggregates.This work proves the superior structure of buckybowl-based luminophore for controlling triplet exciton transition processes and supplies a new perspective for persistent afterglow luminophore design.
基金The authors acknowledge financial support from the National Natural Science Foundation of China(Nos.21905195,M.T.Z.and 22103055,J.G.)Natural Science Foundation of Tianjin City(No.20JCYBJC00800,M.T.Z.)+1 种基金Science and Technology Plans of Tianjin(No.21ZYJDJC00050,J.G.)PEIYANG Young Scholars Program of Tianjin University(No.2020XRX-0023,M.T.Z.).
文摘Hollow metal-organic frameworks(MOFs)have attracted increasing attention in the field of catalysis in recent years due to their unique cavity structure with fast mass-diffusion rates and easily accessible active sites.Here,we report the use of dynamic modulators,which are formed by the in-situ imine condensation reaction of 4-aminobenzoic acid and 4-formylbenzoic acid,to regulate the growth of MOFs to synthesize well-defined hollow thioether functionalized UiO-67(denoted as H-UiO-67-S)single crystals.After supporting Pd nanoparticles,the designed catalysts Pd@H-UiO-67-S show excellent conversion(>99.9%),selectivity(>99.9%),and stability(10 cycles)in the selective hydrogenation of nitrobenzenes with other reducible groups.Density functional theory calculations and the experimental results reveal that Pd nanoparticles not only selectively adsorb the nitro-groups on nitrobenzene,but also restrict the adsorption of the aniline product,due to the interaction of thioether with Pd in the confined pores of H-UiO-67-S,finally result in a significant increase in selectivity of nitro-hydrogenation.
基金This work was supported in part by the National Natural Science Foundation of China(51637005)the Science and Technology Project of SGCC(SGBJDK00KJJS1900088).
文摘This paper presents a multi-HVDC emergency coordinated modulating strategy to enhance the transient stability of hybrid AC/DC power systems.First,the main factors that affect the unbalanced energy distribution during a fault are analyzed,and the dominant generators are determined online.Next,considering the influence on both generators in the sending and receiving ends,the assessment index that evaluates the effects of DC power support is established.On the basis of this,a dynamic DC power support strategy is put forward,and the DC support sequence table is promptly updated by the changing dominant generators.The AC/DC hybrid power system with multi-DC lines is built and used as a test system.The simulation results of different scenarios demonstrate that the proposed method could follow the dominant generator dynamically and adjust the DC participating in modulation to enhance the transient stability effectively and quickly.
基金supported by the National Natural Science Foundation of China (No.30970780)Ph.D.Programs Foundation of Ministry of Education of China (No.20091103110005)
文摘Current methods for the detection of differential gene expression focus on finding individual genes that may be responsible for certain diseases or external irritants. However, for common genetic diseases, multiple genes and their interactions should be understood and treated together during the exploration of disease causes and possible drug design. The present study focuses on analyzing the dynamic patterns of co-regulated modules during biological progression and determining those having remarkably varying activities, using the yeast cell cycle as a case study. We first constructed dynamic active protein-protein interaction networks by modeling the activity of proteins and assembling the dynamic co-regulation protein network at each time point. The dynamic active modules were detected using a method based on the Bayesian graphical model and then the modules with the most varied dispersion of clustering coefficients, which could be responsible for the dynamic mechanism of the cell cycle, were identified. Comparison of results from our functional module detection with the state-of-art functional module detection methods and validation of the ranking of activities of functional modules using GO annotations demonstrate the efficacy of our method for narrowing the scope of possible essential responding modules that could provide multiple targets for biologists to further experimentally validate.
基金supported by the China Bao Wu Low Carbon Metallurgical Innovation Foundation(No.BWLCF202113)the Fundamental Research Funds for the Central Universities(Nos.N2202012,N180206004)the National Natural Science Foundation of China(No.51971059)。
文摘This work demonstrates a two-step method to produce oxide-derived Cu nanowires on Cu mesh surface to offer a monolithic catalyst that outstandingly improves the hydrogen production from reforming formaldehyde and water under ambient conditions.Our results not only reveal that the special oxidederived nanostructure can significantly improve the formaldehyde reforming performance of Cu,but also display that the hydrogen production has a linear relationship with oxygen pressure.Specially,a maximum of 36 times increment in hydrogen generation rate is observed than that without oxygen during the reaction.Density functional theory calculations show that the formaldehyde molecule is adsorbed on Cu surface only when the adsorbed oxygen is in adjacency,and hydrogen release process is the ratedetermining step.This work highlights that the activity of deliberately synthesized catalyst can further be promoted by dynamic chemical modulation of surface states during working.
基金Xinjiang Production and Construction Corps Industrial Technology Research Plans (Grant No. 2007GG15)the Tarim University Principal Youth Fund (Grant No. TDZKQN05002)
文摘Flow against pipeline leakage and the pipe network sudden burst pipe to pipeline leakage flow for the application objects, an energy-efficient real-time scheduling scheme is designed extensively used in pipeline leak monitoring. The proposed scheme can adaptively adjust the network rate in real-time and reduce the cell loss rate, so that it can efficiently avoid the traffic congestion. The recent evolution of wireless sensor networks has yielded a demand to improve energy-efficient scheduling algorithms and energy-efficient medium access protocols. This paper proposes an energy-efficient real-time scheduling scheme that reduces power consumption and network errors on pipeline flux leak monitoring networks. The proposed scheme is based on a dynamic modulation scaling scheme which can scale the number of bits per symbol and a switching scheme which can swap the polling schedule between channels. Built on top of EDF scheduling policy, the proposed scheme enhances the power performance without violating the constraints of real-time streams. The simulation results show that the proposed scheme enhances fault-tolerance and reduces power consumption. Furthermore, that Network congestion avoidance strategy with an energy-efficient real-time scheduling scheme can efficiently improve the bandwidth utilization, TCP friendliness and reduce the packet drop rate in pipeline flux leak monitoring networks.
基金National Natural Science Foundation of China(12104297,12122407,and 11974245)National Key R&D Program of China(2017YFA0303701)+3 种基金Shanghai Municipal Science and Technology Major Project(2019SHZDZX01)Natural Science Foundation of Shanghai(19ZR1475700)China Postdoctoral Science Foundation(2020M671090)L.Y.acknowledges support from the Program for Professor of Special Appointment(Eastern Scholar)at Shanghai Institutions of Higher Learning.X.C.also acknowledges the support from Shandong Quancheng Scholarship(00242019024).
文摘.Constructions of synthetic lattices in modulated ring resonators attract growing attention to interesting physics beyond the geometric dimensionality,where complicated connectivities between resonant frequency modes are explored in many theoretical proposals.We implement experimental demonstration of generating a stub lattice along the frequency axis of light,in two coupled ring resonators of different lengths,with the longer one dynamically modulated.Such a synthetic photonic structure intrinsically exhibits the physics of flat band.We show that the time-resolved band structure read-out from the drop-port output of the excited ring is the intensity projection of the band structure onto a specific resonant mode in the synthetic momentum space,where gapped flat band,mode localization effect,and flat-to-nonflat band transition are observed in experiments and verified by simulations.This work provides evidence for constructing a synthetic stub lattice using two different rings,which,hence,makes a solid step toward experimentally constructing complicated lattices in multiple rings associated with synthetic frequency dimensions.
文摘High temperature latent thermal storage is one of the critical techniques for a solar dynamic power system. This paper presents results from heat transfer analysis of a phase change salt containment canister A three-dimensional analysis program is developed to model heat transfer in a PCM canister. Analysis include effects of asymmetric circumference heat flux, conduction in canister walls, liquid PCM and solid PCM, void volume change and void location, and conduction and radiation across PCM vapor void. The PCM phase change process is modeled using the enthalpy method and the simulation results are compared with those of other two- dimensional investigations. It’s shown that there are large difference with two-dimensional analysis, therefore the three-dimensional model is necessary for system design of high temperature latent thermal storage.