In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detect...In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detector following atmospheric transmission.To quantitatively analyze the effects of different satellite detection altitudes,burst heights,and transmission angles on the physical processes of X-ray transport and energy fluence,we developed an atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering correction.The proposed method is an improvement over the traditional analytical method that only computes direct-transmission X-rays.The traditional analytical method exhibits a maximum relative error of 67.79% compared with the Monte Carlo method.Our improved method reduces this error to within 10% under the same conditions,even reaching 1% in certain scenarios.Moreover,its computation time is 48,000 times faster than that of the Monte Carlo method.These results have important theoretical significance and engineering application value for designing satellite-borne nuclear detonation pulsed X-ray detectors,inverting nuclear detonation source terms,and assessing ionospheric effects.展开更多
A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-s...A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-stop curve of the pulse motor during the terminal guidance process is designed,along with its start-up logic.The effectiveness of the proposed guidance strategy is verified through simulation.展开更多
It remains challenging to effectively estimate the remaining capacity of the secondary lithium-ion batteries that have been widely adopted for consumer electronics,energy storage,and electric vehicles.Herein,by integr...It remains challenging to effectively estimate the remaining capacity of the secondary lithium-ion batteries that have been widely adopted for consumer electronics,energy storage,and electric vehicles.Herein,by integrating regular real-time current short pulse tests with data-driven Gaussian process regression algorithm,an efficient battery estimation has been successfully developed and validated for batteries with capacity ranging from 100%of the state of health(SOH)to below 50%,reaching an average accuracy as high as 95%.Interestingly,the proposed pulse test strategy for battery capacity measurement could reduce test time by more than 80%compared with regular long charge/discharge tests.The short-term features of the current pulse test were selected for an optimal training process.Data at different voltage stages and state of charge(SOC)are collected and explored to find the most suitable estimation model.In particular,we explore the validity of five different machine-learning methods for estimating capacity driven by pulse features,whereas Gaussian process regression with Matern kernel performs the best,providing guidance for future exploration.The new strategy of combining short pulse tests with machine-learning algorithms could further open window for efficiently forecasting lithium-ion battery remaining capacity.展开更多
In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved ...In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved in two steps. The detailed analysis of computational results of a PDE with a single detonation tube and a PDE with five detonation tubes are given in this paper. Complex wave systems are observed inside and outside a PDE. For a PDE with 5 detonation tubes, there is a big bow shock produced from a number of little shocks near the open ends of tubes. A lot of vortexes interact with shocks and a large expansion wave propagates forward and backward with respect to the PDE in a semi-oval shape.展开更多
In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the sol...In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the soliton selffrequency shift is remarkable and the photonic crystal fibre (PCF) parameters vary with the frequency considerably. The precision of numerical simulation by using ASSFM is higher than that by using split-step Fourier method in the process of laser pulse propagation in PCFs due to the fact that the variation of fibre parameters with the peak frequency in the pulse spectrum can be taken into account fully.展开更多
The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an i...The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an initially big spiral can successfully transfer to several small spirals by applying a pulse array method. The impacts of several important factors, such as array density, controlling intensity and pulsing time, are investigated. This control approach may be useful for the control of 2D spatiotemporal patterns and has potential applications in the control of some realistic systems, such as meteorological and cardiac systems.展开更多
High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs...High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs during the underwater high voltage pulse discharge process, which brings security risks to the stability of the pulse fracturing system. In order to solve this problem, an underwater pulse power discharge system was established, the circuit oscillation generation conditions were analyzed and the circuit oscillation suppression method was proposed. Firstly, the system structure was introduced and the charging model of the energy storage capacitor was established by the state space average method. Next, the electrode high-voltage breakdown model was established through COMSOL software, the electrode breakdown process was analyzed according to the electron density distribution image, and the plasma channel impedance was estimated based on the conductivity simulation results. Then the underwater pulse power discharge process and the circuit oscillation generation condition were analyzed, and the circuit oscillation suppression strategy of using the thyristor to replace the gas spark switch was proposed. Finally, laboratory experiments were carried out to verify the precision of the theoretical model and the suppression effect of circuit oscillation. The experimental results show that the voltage variation of the energy storage capacitor, the impedance change of the pulse power discharge process, and the equivalent circuit in each discharge stage were consistent with the theoretical model. The proposed oscillation suppression strategy cannot only prevent the damage caused by circuit oscillation but also reduce the damping oscillation time by77.1%, which can greatly improve the stability of the system. This research has potential application value in the field of underwater pulse power discharge for reservoir reconstruction.展开更多
A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite e...A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite element method (FEM) is used to solve Poisson's equation. In the proposed method, photoionization is considered by adopting an exact Helmholtz photoionization model. Furthermore, fully implicit discretization and variable time step are used to ensure the time-efficiency of the present method. Finally, the method is applied to a positive rod-plane corona problem. The numerical results are in agreement with the experimental results, and the validity of the proposed method is verified.展开更多
Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit co...Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit correction. The algorithm can be acquired by z transform method which is easier for derivation. However, the baseline drift of trapezoidal pulse appears because the noise superimposes on the input signal. In this paper,two new methods based on convergence analysis and noise suppression are proposed to remove the baseline drift resulting from trapezoidal pulse shaping. Simulations and experimental tests are carried out to verify the methods. The results demonstrate that the proposed methods can remove baseline drift in trapezoidal pulse shaping.展开更多
The study focused on the modification with platinum of dark defective titania obtained via pulsed laser ablation. Both the method of Pt introduction and the nature of the Pt precursor were varied. All samples exhibite...The study focused on the modification with platinum of dark defective titania obtained via pulsed laser ablation. Both the method of Pt introduction and the nature of the Pt precursor were varied. All samples exhibited similar phase compositions, specific surface areas, and Pt contents. High-resolution transmission electron microscopy coupled with pulsed CO adsorption revealed increased dispersity when photoreduction and the hydroxonitrate complex (Me _(4) N) _(2) [Pt _(2) (OH) _(2) (NO _(3) ) _(8) ] were used. The sample featured a high content of single-atom species and subnano-sized Pt clusters. The X-ray photoelectron spectroscopy results showed that the photoreduction method facilitated the appearance of a larger number of Pt ^(2+) states, which appeared owing to the strong metal-support interaction (SMSI) eff ect of the transfer of electron density from the electron-saturated defects on the TiO _(2) surface to Pt ^(4+) . In the hydrogen evolution reaction, samples with a significant fraction of the Pt ^(2+) ionic component, capable of generating short-lived Pt^(0) single-atom sites under irradiation due to the SMSI eff ect, exhibited the highest photocatalytic activity. The 0.5Pt(C)/TiO_(2) -Ph sample exhibited the highest hydrogen yield with a quantum efficiency of 0.53, retaining its activity even after 8 h of operation.展开更多
Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroac...Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroactivity of polyaniline were investigated. The results show that the electroactivity of polyaniline film strongly depends on the synthetic conditions, such as the ratio of “on time” to “off time”(ton/toff), frequency, monomer concentration, temperature and mean current density. Different electroactivities of polyaniline are caused by different morphologies of polyaniline. The nano-fibrous polyaniline has higher electroactivity than polyaniline with other morphologies. Under the following conditions: mean current density of pulse galvanostatic method 13mA·cm-2, ton/toff 1, frequency 200Hz, monomer concentration 0.3mol·L-1 and temperature 20℃, nano-fibrous polyaniline film with the highest electroactivity can be obtained.展开更多
In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigen...In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigenvalues and eigensolutions respectively.By the symplectic method,the solution of the local buckling of shells can be employed to the expansion series of symplectic eigensolutions in this system.As a result,relationships between critical buckling loads and other factors,such as length of pulse load,thickness of shells and circumferential orders,have been achieved.At the same time,symmetric and unsymmetric buckling modes have been discuss.Moreover,numerical results show that modes of post-buckling of shells can be Bamboo node-type,bending type,concave type and so on.Research in this paper provides analytical supports for ultimate load prediction and buckling failure assessment of cylindrical long shells under local axial pulse loads.展开更多
Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoerciviti...Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoercivities of the MnBi/Bi film are 1.5 T and 2.35 T at room temperature and at 373K, respectively, showing a positive temperature coefficient. Microstructural investigations show that the textured MnBi film results from the orientated growth induced by the textured Bi under-layer.展开更多
This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the...This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the three-pulse photon echo's amplitude and efficiency is analyzed with the Maxwell-Bloch equations solved by finite-difference timedomain method.We demonstrate that the amplitude of three-pulse echo will increase with the increasing of thickness and the optimum thickness to generate three-pulse photon echo is 0.3 cm for Tm^(3+):YAG when the attenuation of the input pulse is taken into account.Meanwhile,we find the expression 0.09 exp(α'L),which is previously employed to describe the relationship between echo's efficiency and thickness,should be modified as 1.3 · 0.09 exp(2.4 ·α'L) with the propagation of echo considered.展开更多
We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to...We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to simultaneously measure the weak temporal phase and temporal profile of pulses, which are almost transform- limited. A detailed analysis shows that this iterative method has valuable potential applications in the charac- terization of pulses with weak temporal phase.展开更多
Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for ca...Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for calculating the transmission loss. Firstly, the transmission loss of the single-cavity element was simulated without any airflow, and the effects of different structural parameters on the acoustic performance were investigated comprehensively. Secondly, the static transmission loss of the perforated intake pipe was obtained by the rectangular-pulse method, which is proved to be accurate enough compared with the result by finite element method. Thirdly, under the different conditions of the mean airflow and the operating temperature, the specific transmission loss was acquired respectively. In general, the peaks of the transmission loss are shifted to the lower frequency range because of the reverse airflow, but the amplitudes are irregularly changed. Besides, when the operating temperature increases, the peaks are shifted to the higher frequencies. Finally, with the designed perforated pipe installed to the intake system, the road tests were proceeded to evaluate the actual acoustic performance, and the result indicates that the intake sound pressure level is greatly attenuated. Typically in the range of 600–1500 Hz, the insertion loss of the intake noise at the decelerating moment is almost 20 d B(A), and the overall noise is reduced more than 14.2 d B(A). In conclusion, the perforated intake pipe has been proved excellent in improving the acoustic performance of intake system and could provide the guidance for the automotive engineering application.展开更多
The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and no...The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and notch tensile strength. All these characteristics are considered together in the selection of process parameters by modified taguchi method to analyse the effect of each welding process parameter on tensile properties. Experimental results are furnished to illustrate the approach.展开更多
An accurate energy calibration of a 5"× 2" BC501A liquid scintillator-based neutron detector by means of photon sources and the unfolding of pulse height spectra are described. The photon responses were measure...An accurate energy calibration of a 5"× 2" BC501A liquid scintillator-based neutron detector by means of photon sources and the unfolding of pulse height spectra are described. The photon responses were measured with 22Na, 137Cs and 54Mn photon sources and simulated using the GRESP code, which was developed at the Physiknlisch Technische Bundesanstalt in Germany. Pulse height spectra produced by three different photon sources were employed to investigate the effects of the unfolding techniques. It was found that the four unfolding codes of the HEPRO and UMG3.3 packages, including GRAVEL, UNFANA, MIEKE and MAXED, performed well with the test spectra and produced generally consistent results. They could therefore be used to obtain neutron energy spectra in toknmak experiments.展开更多
The influence of the ultra-short pulse wavelength on the populations in the three electronic states of CsI molecule is investigated using the time-dependent wave packet method. The calculated results show that the pop...The influence of the ultra-short pulse wavelength on the populations in the three electronic states of CsI molecule is investigated using the time-dependent wave packet method. The calculated results show that the populations in the two excited states approach to the maxima at the wavelengths of 369 nm and 297 nm, respectively. The photodissociation reaction channels of the CsI molecule can be chosen by controlling the pump pulse wavelength.展开更多
We present a new model of an electron gun for generating subrelativistic femtosecond (fs) electron pulses. The basic idea is to utilize a dc acceleration stage combined with a time focusing region, the time focusing...We present a new model of an electron gun for generating subrelativistic femtosecond (fs) electron pulses. The basic idea is to utilize a dc acceleration stage combined with a time focusing region, the time focusing electrode generates an electron energy chirp for bunching at the target. Without considering the space charge effects, simulations of the electron gun were carried out under the conditions of different dc voltages and various slopes of the voltage added on the time focusing electrode. Tracing and simulating large numbers of photoelectrons through Monte-Carlo and finite difference methods, the electron pulses with 1 ps can be compressed to 55 fs, which will allow significant advances in the field of ultrafast diagnosis.展开更多
文摘In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detector following atmospheric transmission.To quantitatively analyze the effects of different satellite detection altitudes,burst heights,and transmission angles on the physical processes of X-ray transport and energy fluence,we developed an atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering correction.The proposed method is an improvement over the traditional analytical method that only computes direct-transmission X-rays.The traditional analytical method exhibits a maximum relative error of 67.79% compared with the Monte Carlo method.Our improved method reduces this error to within 10% under the same conditions,even reaching 1% in certain scenarios.Moreover,its computation time is 48,000 times faster than that of the Monte Carlo method.These results have important theoretical significance and engineering application value for designing satellite-borne nuclear detonation pulsed X-ray detectors,inverting nuclear detonation source terms,and assessing ionospheric effects.
基金The National Natural Science Foundation of China(Project No.52102436)The Natural Science Foundation of Shanghai(Project No.23ZR1462700)+3 种基金The National Key Laboratory Open Fund for Strength and Structural Integrity(Project No.ASSIKFJJ202304006)The Shanghai Aerospace Science and Technology Innovation Fund(Project No.SAST2022-031)The National Key Laboratory of Space Intelligent Control(Project No.2023-JCJQ-LB-006-14)The Shanghai Key Laboratory of Spacecraft Mechanism(Project No.YY-F805202210025)。
文摘A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-stop curve of the pulse motor during the terminal guidance process is designed,along with its start-up logic.The effectiveness of the proposed guidance strategy is verified through simulation.
基金support from Shenzhen Municipal Development and Reform Commission(Grant Number:SDRC[2016]172)Shenzhen Science and Technology Program(Grant No.KQTD20170810150821146)Interdisciplinary Research and Innovation Fund of Tsinghua Shenzhen International Graduate School,and Shanghai Shun Feng Machinery Co.,Ltd.
文摘It remains challenging to effectively estimate the remaining capacity of the secondary lithium-ion batteries that have been widely adopted for consumer electronics,energy storage,and electric vehicles.Herein,by integrating regular real-time current short pulse tests with data-driven Gaussian process regression algorithm,an efficient battery estimation has been successfully developed and validated for batteries with capacity ranging from 100%of the state of health(SOH)to below 50%,reaching an average accuracy as high as 95%.Interestingly,the proposed pulse test strategy for battery capacity measurement could reduce test time by more than 80%compared with regular long charge/discharge tests.The short-term features of the current pulse test were selected for an optimal training process.Data at different voltage stages and state of charge(SOC)are collected and explored to find the most suitable estimation model.In particular,we explore the validity of five different machine-learning methods for estimating capacity driven by pulse features,whereas Gaussian process regression with Matern kernel performs the best,providing guidance for future exploration.The new strategy of combining short pulse tests with machine-learning algorithms could further open window for efficiently forecasting lithium-ion battery remaining capacity.
基金The project supported by the National Natural Science Foundation of China(59906005)the Teaching Research Award Program for Outstanding Young Teachers in High Education Institutions of MOE,China
文摘In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved in two steps. The detailed analysis of computational results of a PDE with a single detonation tube and a PDE with five detonation tubes are given in this paper. Complex wave systems are observed inside and outside a PDE. For a PDE with 5 detonation tubes, there is a big bow shock produced from a number of little shocks near the open ends of tubes. A lot of vortexes interact with shocks and a large expansion wave propagates forward and backward with respect to the PDE in a semi-oval shape.
文摘In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the soliton selffrequency shift is remarkable and the photonic crystal fibre (PCF) parameters vary with the frequency considerably. The precision of numerical simulation by using ASSFM is higher than that by using split-step Fourier method in the process of laser pulse propagation in PCFs due to the fact that the variation of fibre parameters with the peak frequency in the pulse spectrum can be taken into account fully.
文摘The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an initially big spiral can successfully transfer to several small spirals by applying a pulse array method. The impacts of several important factors, such as array density, controlling intensity and pulsing time, are investigated. This control approach may be useful for the control of 2D spatiotemporal patterns and has potential applications in the control of some realistic systems, such as meteorological and cardiac systems.
基金financially supported by the National Science and Technology Major Project(No.2016ZX05034004)。
文摘High voltage fracturing technology was widely used in the field of reservoir reconstruction due to its advantages of being clean, pollution-free, and high-efficiency. However, high-frequency circuit oscillation occurs during the underwater high voltage pulse discharge process, which brings security risks to the stability of the pulse fracturing system. In order to solve this problem, an underwater pulse power discharge system was established, the circuit oscillation generation conditions were analyzed and the circuit oscillation suppression method was proposed. Firstly, the system structure was introduced and the charging model of the energy storage capacitor was established by the state space average method. Next, the electrode high-voltage breakdown model was established through COMSOL software, the electrode breakdown process was analyzed according to the electron density distribution image, and the plasma channel impedance was estimated based on the conductivity simulation results. Then the underwater pulse power discharge process and the circuit oscillation generation condition were analyzed, and the circuit oscillation suppression strategy of using the thyristor to replace the gas spark switch was proposed. Finally, laboratory experiments were carried out to verify the precision of the theoretical model and the suppression effect of circuit oscillation. The experimental results show that the voltage variation of the energy storage capacitor, the impedance change of the pulse power discharge process, and the equivalent circuit in each discharge stage were consistent with the theoretical model. The proposed oscillation suppression strategy cannot only prevent the damage caused by circuit oscillation but also reduce the damping oscillation time by77.1%, which can greatly improve the stability of the system. This research has potential application value in the field of underwater pulse power discharge for reservoir reconstruction.
基金Project supported by the National Basic Research Program of China(Grant No.2011CB209402)the National Natural Science Foundation of China(Grant No.51177041)the Fundamental Research Funds for the Central Universities,China(Grant No.12QX01)
文摘A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite element method (FEM) is used to solve Poisson's equation. In the proposed method, photoionization is considered by adopting an exact Helmholtz photoionization model. Furthermore, fully implicit discretization and variable time step are used to ensure the time-efficiency of the present method. Finally, the method is applied to a positive rod-plane corona problem. The numerical results are in agreement with the experimental results, and the validity of the proposed method is verified.
基金Supported by National High Technology Research and Development Program of China(863 Program)(No.2012AA061804-03)
文摘Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit correction. The algorithm can be acquired by z transform method which is easier for derivation. However, the baseline drift of trapezoidal pulse appears because the noise superimposes on the input signal. In this paper,two new methods based on convergence analysis and noise suppression are proposed to remove the baseline drift resulting from trapezoidal pulse shaping. Simulations and experimental tests are carried out to verify the methods. The results demonstrate that the proposed methods can remove baseline drift in trapezoidal pulse shaping.
文摘The study focused on the modification with platinum of dark defective titania obtained via pulsed laser ablation. Both the method of Pt introduction and the nature of the Pt precursor were varied. All samples exhibited similar phase compositions, specific surface areas, and Pt contents. High-resolution transmission electron microscopy coupled with pulsed CO adsorption revealed increased dispersity when photoreduction and the hydroxonitrate complex (Me _(4) N) _(2) [Pt _(2) (OH) _(2) (NO _(3) ) _(8) ] were used. The sample featured a high content of single-atom species and subnano-sized Pt clusters. The X-ray photoelectron spectroscopy results showed that the photoreduction method facilitated the appearance of a larger number of Pt ^(2+) states, which appeared owing to the strong metal-support interaction (SMSI) eff ect of the transfer of electron density from the electron-saturated defects on the TiO _(2) surface to Pt ^(4+) . In the hydrogen evolution reaction, samples with a significant fraction of the Pt ^(2+) ionic component, capable of generating short-lived Pt^(0) single-atom sites under irradiation due to the SMSI eff ect, exhibited the highest photocatalytic activity. The 0.5Pt(C)/TiO_(2) -Ph sample exhibited the highest hydrogen yield with a quantum efficiency of 0.53, retaining its activity even after 8 h of operation.
基金Project(50473022) supported by the National Natural Science Foundation project supported by the State Key Laboratoryof Chemo/Biosensing and Chemometrics of China
文摘Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroactivity of polyaniline were investigated. The results show that the electroactivity of polyaniline film strongly depends on the synthetic conditions, such as the ratio of “on time” to “off time”(ton/toff), frequency, monomer concentration, temperature and mean current density. Different electroactivities of polyaniline are caused by different morphologies of polyaniline. The nano-fibrous polyaniline has higher electroactivity than polyaniline with other morphologies. Under the following conditions: mean current density of pulse galvanostatic method 13mA·cm-2, ton/toff 1, frequency 200Hz, monomer concentration 0.3mol·L-1 and temperature 20℃, nano-fibrous polyaniline film with the highest electroactivity can be obtained.
基金This research is funded by the grants from Dalian Project of Innovation Foundation of Science and Technology(No.2018J11CY005)Research Program of State Key Laboratory of Structural Analysis for Industrial Equipment(No.S18313).
文摘In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigenvalues and eigensolutions respectively.By the symplectic method,the solution of the local buckling of shells can be employed to the expansion series of symplectic eigensolutions in this system.As a result,relationships between critical buckling loads and other factors,such as length of pulse load,thickness of shells and circumferential orders,have been achieved.At the same time,symmetric and unsymmetric buckling modes have been discuss.Moreover,numerical results show that modes of post-buckling of shells can be Bamboo node-type,bending type,concave type and so on.Research in this paper provides analytical supports for ultimate load prediction and buckling failure assessment of cylindrical long shells under local axial pulse loads.
基金Supported by the National Natural Science Foundation of China under Grant Nos 51171001,51371009 and 50971003the Foundation of Key Laboratory of Neutron Physics of CAEP under Grant No 2014BB02
文摘Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoercivities of the MnBi/Bi film are 1.5 T and 2.35 T at room temperature and at 373K, respectively, showing a positive temperature coefficient. Microstructural investigations show that the textured MnBi film results from the orientated growth induced by the textured Bi under-layer.
基金Project supported by Tianjin Research Program Application Foundation and Advanced Technology,China(Grant No.15JCQNJC01100)
文摘This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the three-pulse photon echo's amplitude and efficiency is analyzed with the Maxwell-Bloch equations solved by finite-difference timedomain method.We demonstrate that the amplitude of three-pulse echo will increase with the increasing of thickness and the optimum thickness to generate three-pulse photon echo is 0.3 cm for Tm^(3+):YAG when the attenuation of the input pulse is taken into account.Meanwhile,we find the expression 0.09 exp(α'L),which is previously employed to describe the relationship between echo's efficiency and thickness,should be modified as 1.3 · 0.09 exp(2.4 ·α'L) with the propagation of echo considered.
基金Supported by the National Natural Science Foundation of China under Grant No 61205103
文摘We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to simultaneously measure the weak temporal phase and temporal profile of pulses, which are almost transform- limited. A detailed analysis shows that this iterative method has valuable potential applications in the charac- terization of pulses with weak temporal phase.
基金Project(51705454)supported by the National Natural Science Foundation of China
文摘Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for calculating the transmission loss. Firstly, the transmission loss of the single-cavity element was simulated without any airflow, and the effects of different structural parameters on the acoustic performance were investigated comprehensively. Secondly, the static transmission loss of the perforated intake pipe was obtained by the rectangular-pulse method, which is proved to be accurate enough compared with the result by finite element method. Thirdly, under the different conditions of the mean airflow and the operating temperature, the specific transmission loss was acquired respectively. In general, the peaks of the transmission loss are shifted to the lower frequency range because of the reverse airflow, but the amplitudes are irregularly changed. Besides, when the operating temperature increases, the peaks are shifted to the higher frequencies. Finally, with the designed perforated pipe installed to the intake system, the road tests were proceeded to evaluate the actual acoustic performance, and the result indicates that the intake sound pressure level is greatly attenuated. Typically in the range of 600–1500 Hz, the insertion loss of the intake noise at the decelerating moment is almost 20 d B(A), and the overall noise is reduced more than 14.2 d B(A). In conclusion, the perforated intake pipe has been proved excellent in improving the acoustic performance of intake system and could provide the guidance for the automotive engineering application.
文摘The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and notch tensile strength. All these characteristics are considered together in the selection of process parameters by modified taguchi method to analyse the effect of each welding process parameter on tensile properties. Experimental results are furnished to illustrate the approach.
基金supported by the State Key Development Program for Basic Research of China (Nos. 2008CB717803, 2009GB107001,2007CB209903)the Research Fund for the Doctoral Program of Higher Education of China (No. 200610011023)National Natural Science Foundation of China (No. 10875002)
文摘An accurate energy calibration of a 5"× 2" BC501A liquid scintillator-based neutron detector by means of photon sources and the unfolding of pulse height spectra are described. The photon responses were measured with 22Na, 137Cs and 54Mn photon sources and simulated using the GRESP code, which was developed at the Physiknlisch Technische Bundesanstalt in Germany. Pulse height spectra produced by three different photon sources were employed to investigate the effects of the unfolding techniques. It was found that the four unfolding codes of the HEPRO and UMG3.3 packages, including GRAVEL, UNFANA, MIEKE and MAXED, performed well with the test spectra and produced generally consistent results. They could therefore be used to obtain neutron energy spectra in toknmak experiments.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 10674114 and 10604045)
文摘The influence of the ultra-short pulse wavelength on the populations in the three electronic states of CsI molecule is investigated using the time-dependent wave packet method. The calculated results show that the populations in the two excited states approach to the maxima at the wavelengths of 369 nm and 297 nm, respectively. The photodissociation reaction channels of the CsI molecule can be chosen by controlling the pump pulse wavelength.
基金supported the Young Scientists Fund of the National Natural Science Foundation of China(Grant No.60901036)the National Natural Science Foundation of China(Grant No.60777027)the Innovation Laboratory Fund of the Chinese Academy of Sciences(Grant No.CXJJ-10-S13)
文摘We present a new model of an electron gun for generating subrelativistic femtosecond (fs) electron pulses. The basic idea is to utilize a dc acceleration stage combined with a time focusing region, the time focusing electrode generates an electron energy chirp for bunching at the target. Without considering the space charge effects, simulations of the electron gun were carried out under the conditions of different dc voltages and various slopes of the voltage added on the time focusing electrode. Tracing and simulating large numbers of photoelectrons through Monte-Carlo and finite difference methods, the electron pulses with 1 ps can be compressed to 55 fs, which will allow significant advances in the field of ultrafast diagnosis.