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Resonant Andreev reflection in a normal-metal/quantum-dot/superconductor system with coupled Majorana bound states
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作者 王素新 李玉现 刘建军 《Chinese Physics B》 SCIE EI CAS CSCD 2016年第3期351-356,共6页
Andreev reflection (AR) in a normal-metal/quantum-dot/superconductor (N-QD-S) system with coupled Majorana bound states (MBSs) is investigated theoretically. We find that in the N--QD-S system, the AR can be enh... Andreev reflection (AR) in a normal-metal/quantum-dot/superconductor (N-QD-S) system with coupled Majorana bound states (MBSs) is investigated theoretically. We find that in the N--QD-S system, the AR can be enhanced when coupling to the MBSs is incorporated. Fano line-shapes can be observed in the AR conductance spectrum when there is an appropriate QD-MBS coupling or MBS-MBS coupling. The AR conductance is always e2/2h at the zero Fermi energy point when only QD--MBSs coupling is considered. In addition, the resonant AR occurs when the MBS-MBS coupling roughly equals to the QD energy level. We also find that an AR antiresonance appears when the QD energy level approximately equals to the sum of the QD-MBS coupling and the MBS-MBS coupling. These features may serve as characteristic signatures for the probe of MBSs. 展开更多
关键词 Majorana bound states andreev reflection Fano effect quantum dot
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Electronic transport through a periodic array of quantum-dot rings
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作者 薛海斌 张瀚尹 +2 位作者 聂一行 李志坚 梁九卿 《Chinese Physics B》 SCIE EI CAS CSCD 2010年第4期381-387,共7页
Using the tight-binding approximation and the transfer matrix method, this paper studies the electronic transport properties through a periodic array of quantum-dot (QD) rings threaded by a magnetic flux. It demonst... Using the tight-binding approximation and the transfer matrix method, this paper studies the electronic transport properties through a periodic array of quantum-dot (QD) rings threaded by a magnetic flux. It demonstrates that the even^odd parity of the QD number in a single ring and the number of the QD rings in the array play a crucial role in the electron transmission. For a single QD ring, the resonance and antiresonance transmission depend not only on the applied magnetic flux but also on the difference between the number of QDs on the two arms of the ring. For an array of QD rings, the transmission properties are related not only to the even-odd parity of the number No of QDs in the single ring but also to the even-odd parity of the ring number N in the array. When the incident electron energy is aligned with the site energy, for the array of N rings with No = odd the antiresonance transmission cannot occur but the resonance transmission may occur and the transmission spectrum has N resonance peaks (N - 1 resonance peaks) in a period for N = odd (for N = even). For the array of N rings with No = even the transmission properties depend on the flux threading the ring and the QD number on one arm of the ring. These results may be helpful in designing QD devices. 展开更多
关键词 quantum dots electronic transport antiresonance transmission resonance transmission
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Nonequilibrium Electron Transport Through a Quantum Dot from Kubo Formula
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作者 LǖRong ZHANGGuang-Ming 《Communications in Theoretical Physics》 SCIE CAS CSCD 2005年第4期749-752,共4页
Based on the Kubo formula for an electron tunneling junction, we revisit the nonequilibrium transport properties through a quantum dot. Since the Fermi level of the quantum dot is set by the conduction electrons of th... Based on the Kubo formula for an electron tunneling junction, we revisit the nonequilibrium transport properties through a quantum dot. Since the Fermi level of the quantum dot is set by the conduction electrons of the leads, we calculate the electron current from the left side by assuming the quantum dot coupled to the right lead as another side of the tunneling junction, and the other way round is used to calculate the current from the right side. By symmetrizing these two currents, an effective local density states on the dot can be obtained, and is discussed at high and low temperatures, respectively. 展开更多
关键词 不等电子传输 量子点 Kubo公式 KONDO效应 固体物理学
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Carrier transport in III–V quantum-dot structures for solar cells or photodetectors 被引量:1
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作者 王文奇 王禄 +9 位作者 江洋 马紫光 孙令 刘洁 孙庆灵 赵斌 王文新 刘伍明 贾海强 陈弘 《Chinese Physics B》 SCIE EI CAS CSCD 2016年第9期174-179,共6页
According to the well-established light-to-electricity conversion theory,resonant excited carriers in the quantum dots will relax to the ground states and cannot escape from the quantum dots to form photocurrent,which... According to the well-established light-to-electricity conversion theory,resonant excited carriers in the quantum dots will relax to the ground states and cannot escape from the quantum dots to form photocurrent,which have been observed in quantum dots without a p–n junction at an external bias.Here,we experimentally observed more than 88% of the resonantly excited photo carriers escaping from In As quantum dots embedded in a short-circuited p–n junction to form photocurrent.The phenomenon cannot be explained by thermionic emission,tunneling process,and intermediate-band theories.A new mechanism is suggested that the photo carriers escape directly from the quantum dots to form photocurrent rather than relax to the ground state of quantum dots induced by a p–n junction.The finding is important for understanding the low-dimensional semiconductor physics and applications in solar cells and photodiode detectors. 展开更多
关键词 quantum dots electronic transport p–n junctions photoluminescence
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Quantum transport through a multi-quantum-dot-pair chain side-coupled with Majorana bound states
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作者 江兆潭 仲成成 《Chinese Physics B》 SCIE EI CAS CSCD 2016年第6期474-482,共9页
We investigate the quantum transport properties through a special kind of quantum dot(QD) system composed of a serially coupled multi-QD-pair(multi-QDP) chain and side-coupled Majorana bound states(MBSs) by usin... We investigate the quantum transport properties through a special kind of quantum dot(QD) system composed of a serially coupled multi-QD-pair(multi-QDP) chain and side-coupled Majorana bound states(MBSs) by using the Green functions method,where the conductance can be classified into two kinds:the electron tunneling(ET) conductance and the Andreev reflection(AR) one.First we find that for the nonzero MBS-QDP coupling a sharp AR-induced zero-bias conductance peak with the height of e^2/h is present(or absent) when the MBS is coupled to the far left(or the other) QDP.Moreover,the MBS-QDP coupling can suppress the ET conductance and strengthen the AR one,and further split into two sub-peaks each of the total conductance peaks of the isolated multi-QDPs,indicating that the MBS will make obvious influences on the competition between the ET and AR processes.Then we find that the tunneling rate ΓLis able to affect the conductances of leads L and R in different ways,demonstrating that there exists a ΓL-related competition between the AR and ET processes.Finally we consider the effect of the inter-MBS coupling on the conductances of the multi-QDP chains and it is shown that the inter-MBS coupling will split the zero-bias conductance peak with the height of e^2/h into two sub-peaks.As the inter-MBS coupling becomes stronger,the two sub-peaks are pushed away from each other and simultaneously become lower,which is opposite to that of the single QDP chain where the two sub-peaks with the height of about e^2/2h become higher.Also,the decay of the conductance sub-peaks with the increase of the MBS-QDP coupling becomes slower as the number of the QDPs becomes larger.This research should be an important extension in studying the transport properties in the kind of QD systems coupled with the side MBSs,which is helpful for understanding the nature of the MBSs,as well as the MBS-related QD transport properties. 展开更多
关键词 electron transport quantum dot andreev reflection
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Spin-Dependent Electron Properties of a Triple-Terminal Quantum Dot Structure
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作者 HAN Yu GONG Wei-Jiang WEI Guo-Zhu 《Communications in Theoretical Physics》 SCIE CAS CSCD 2009年第12期1117-1124,共8页
Electron transport properties of a triple-terminal Aharonov-Bohm interferometer are theoretically studied.By applying a Rashba spin-orbit coupling to a quantum dot locally, we find that remarkable spin polarization co... Electron transport properties of a triple-terminal Aharonov-Bohm interferometer are theoretically studied.By applying a Rashba spin-orbit coupling to a quantum dot locally, we find that remarkable spin polarization comesabout in the electron transport process with tuning the structure parameters, i.e., the magnetic flux or quantum dotlevels. When the quantum dot levels are aligned with the Fermi level, there only appear spin polarization in thisstructure by the presence of an appropriate magnetic flux. However, in absence of magnetic flux spin polarization andspin separation can be simultaneously realized with the adjustment of quantum dot levels, namely, an incident electronfrom one terminal can select a specific terminal to depart from the quantum dots according to its spin state. 展开更多
关键词 量子点结构 电子特性 自旋相关 终端 电子传输特性 自旋极化 耦合量子点 自旋轨道
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Fano effect of a parallel-coupled triple Rashba quantum dot system
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作者 贺泽龙 吕天全 +3 位作者 崔莲 薛惠杰 李林军 尹海涛 《Chinese Physics B》 SCIE EI CAS CSCD 2011年第11期456-463,共8页
Using the nonequilibrium Keldysh Green's function technique, the Fano effect of a parallel-coupled triple Rashba quantum dot system is investigated. The conductance as a function of electron energy is numerically cal... Using the nonequilibrium Keldysh Green's function technique, the Fano effect of a parallel-coupled triple Rashba quantum dot system is investigated. The conductance as a function of electron energy is numerically calculated. Compared with the case of a parallel-coupled double quantum dot system, two additional Fano resonance peaks occur in the conductance spectrum. By adjusting the structural parameters, the two Fano resonance peaks may change into the resoaance peaks. In addition, the influence of Rashba spin-orbit interaction on the conductance is studied. 展开更多
关键词 nonequilibrium Green's function Fano effect quantum dot electronic transport
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Fano effect of a laterally coupled vertical triple quantum dot system
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作者 贺泽龙 吕天全 张迪 《Chinese Physics B》 SCIE EI CAS CSCD 2013年第2期445-448,共4页
Using the nonequilibrium Green's function technique,electron transport through a laterally coupled vertical triple quantum dot is investigated.The conductance as a function of electron energy is numerically calculate... Using the nonequilibrium Green's function technique,electron transport through a laterally coupled vertical triple quantum dot is investigated.The conductance as a function of electron energy is numerically calculated.The evolution of the conductance strongly depends on the configuration of dot levels and interdot coupling strengths. 展开更多
关键词 nonequilibrium Green's function Fano effect quantum dot electron transport
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Full Counting Statistics of Superconductor-Quantum Dot-Superconductor Contacts in the Presence of Interactions
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作者 Henning Soller 《Open Journal of Applied Sciences》 2019年第5期386-393,共8页
In this paper, we discuss the full counting statistics of superconducting quantum dot contacts. We discuss the effects both of phonon and onsite electronic interaction focusing on the experimentally most relevant case... In this paper, we discuss the full counting statistics of superconducting quantum dot contacts. We discuss the effects both of phonon and onsite electronic interaction focusing on the experimentally most relevant case of strong onsite electronic interactions. We find that in general, the Josephson effect and multiple Andreev reflections in these systems are strongly suppressed due to the onsite interaction. However, in case resonant phonons are found, the effect of the onsite interaction can be overcome. 展开更多
关键词 SUPERCONDUCTOR Nanoelectronics Tunnel JUNCTION Full COUNTING Statistics quantum dot andreev reflection
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铁磁性电极条件下T形双量子点结构中马约拉纳束缚态的解耦现象
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作者 代雪峰 贡同 《物理学报》 SCIE EI CAS CSCD 北大核心 2024年第5期304-315,共12页
通过将马约拉纳束缚态侧耦合到主通道中的量子点,从理论上研究了T形双量子点体系的输运性质.结果表明,调整侧耦合量子点能级和量子点-马约拉纳束缚态耦合方式,可以在线性输运区观察到马约拉纳束缚态与T形双量子点解耦的现象.引入铁磁性... 通过将马约拉纳束缚态侧耦合到主通道中的量子点,从理论上研究了T形双量子点体系的输运性质.结果表明,调整侧耦合量子点能级和量子点-马约拉纳束缚态耦合方式,可以在线性输运区观察到马约拉纳束缚态与T形双量子点解耦的现象.引入铁磁性电极后,电导平台的出现或损坏明显依赖于体系中磁场与电极极化方向的差异,而马约拉纳束缚态的解耦现象仍然稳固.本工作有助于进一步诠释T形双量子点体系中马约拉纳束缚态的解耦现象,为深入认知以及探测马约拉纳束缚态提供理论支持. 展开更多
关键词 andreev反射 马约拉纳束缚态 量子点 解耦
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耦合Majorana束缚态T形双量子点中的Andreev反射
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作者 王素新 李玉现 +1 位作者 王宁 刘建军 《物理学报》 SCIE EI CAS CSCD 北大核心 2016年第13期233-239,共7页
研究了连接在正常金属电极和超导电极之间的耦合Majorana束缚态(MBSs)T形双量子点结构中的Andreev反射.研究发现,对于T形双量子点结构,当入射能量等于边耦合量子点能级时Andreev反射电导出现Fano振荡,连接MBSs之后,零费米能附近出现一... 研究了连接在正常金属电极和超导电极之间的耦合Majorana束缚态(MBSs)T形双量子点结构中的Andreev反射.研究发现,对于T形双量子点结构,当入射能量等于边耦合量子点能级时Andreev反射电导出现Fano振荡,连接MBSs之后,零费米能附近出现一对新的Fano型振荡峰.如果忽略两个MBSs之间的相互作用,零费米能点的Andreev反射电导为定值1/2G_0(G_0=2e^2/h),不受量子点能级、双量子点之间耦合强度以及量子点与MBSs之间的耦合强度的影响.此外,在没有耦合MBSs的T形双量子点结构中,调节双量子点间的耦合强度可以使零费米能附近的Andreev反射电导出现由共振带向反共振带的转变,而耦合MBSs之后,又可以使反共振消失转而出现新的共振峰. 展开更多
关键词 Majorana束缚态 双量子点 andreev反射 Fano效应
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BaSnO_(3)电子传输层在量子点太阳能电池中的应用
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作者 石宇星 江德华 +10 位作者 汪丽婧 李世杰 郭章旺 赵骏 何东祥 叶滨 曾涛 施玮 陈云霞 苏小丽 董罡 《陶瓷学报》 CAS 北大核心 2024年第3期492-500,共9页
电子传输层作为新型薄膜太阳电池重要组成部分承担光生电子的传输角色。研究通过简单共沉淀法合成尺寸分布较好的三元BaSnO_(3)(简称BSO)纳米晶,考察了不同热处理温度对BSO相形成影响规律,XRD测试结果表明:升高温度有利于降低纳米晶中... 电子传输层作为新型薄膜太阳电池重要组成部分承担光生电子的传输角色。研究通过简单共沉淀法合成尺寸分布较好的三元BaSnO_(3)(简称BSO)纳米晶,考察了不同热处理温度对BSO相形成影响规律,XRD测试结果表明:升高温度有利于降低纳米晶中碳酸钡等杂质含量,提高BSO纳米晶相纯度。将合成的BSO纳米晶首次作为电子传输层材料应用于PbS胶体量子点太阳能电池中,在1200℃(2 h)条件下合成的BSO纳米晶对应器件性能优于商业TiO2纳米晶对照组,这主要得益于BSO/PbS量子点界面电荷的高效萃取和低复合。对应同批次最佳器件的性能为:Jsc=25.199 mA·cm^(−2)、Voc=0.480 V、FF=0.534及PCE=6.454%,且表现出良好的工作稳定性。该工作证实BaSnO_(3)纳米材料可作为量子点太阳电池电子传输材料使用,为今后进一步提升同类型器件的性能提供参考。 展开更多
关键词 BaSnO_(3) 电子传输层 量子点 太阳能电池 效率
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层状铁磁体Fe0.26TaS2的Andreev反射谱
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作者 于晓洋 冯红磊 +4 位作者 辜刚旭 刘永河 李治林 徐同帅 李永庆 《物理学报》 SCIE EI CAS CSCD 北大核心 2019年第24期272-280,共9页
如何避免界面反应、可靠地提取材料的自旋极化率是自旋电子学的一个基本问题.本文选取了一种独特的铁磁性层状过渡族金属硫化物Fe0.26TaS2,研究了单晶材料的磁性、电子输运和Andreev反射谱.磁性和输运结果表明,低温下Fe0.26TaS2单晶存... 如何避免界面反应、可靠地提取材料的自旋极化率是自旋电子学的一个基本问题.本文选取了一种独特的铁磁性层状过渡族金属硫化物Fe0.26TaS2,研究了单晶材料的磁性、电子输运和Andreev反射谱.磁性和输运结果表明,低温下Fe0.26TaS2单晶存在强磁各向异性、双峰磁电阻和反常霍尔效应.通过干法转移方案制备的干净界面的Fe0.26TaS2超导异质结的Andreev反射谱,发现该材料的自旋极化率为47%±7%.本文展示的干法转移制备超导/磁性异质结的方法可广泛用于测量各种二维磁性材料的自旋极化率. 展开更多
关键词 Fe0.26TaS2 层状铁磁体 磁性 输运 andreev反射谱 自旋极化率
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耦合三端子量子点系统中Andreev反射调控的热电输运
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作者 郝方原 王瑞强 《华南师范大学学报(自然科学版)》 CAS 北大核心 2014年第1期37-41,共5页
以耦合到超导电极、铁磁金属电极及正常金属电极的三端子量子点混杂系统为研究对象,系统研究了自旋极化电子的Andreev反射过程对热电流的影响.研究发现,Andreev反射过程及正常的隧穿过程2种机制的竞争不仅导致热电荷流大小和方向的改变... 以耦合到超导电极、铁磁金属电极及正常金属电极的三端子量子点混杂系统为研究对象,系统研究了自旋极化电子的Andreev反射过程对热电流的影响.研究发现,Andreev反射过程及正常的隧穿过程2种机制的竞争不仅导致热电荷流大小和方向的改变,而且导致热自旋流大小和方向的改变.可通过调控门电压及超导体与量子点耦合强度实现. 展开更多
关键词 Master方程 andreev反射 热电输运 藕合三端子量子点
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Transport Through a Precessing Spin Coupled to Noncollinearly Polarized Ferromagnetic Leads
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作者 王贤超 辛子华 冯丽雅 《Communications in Theoretical Physics》 SCIE CAS CSCD 2010年第2期351-354,共4页
量磁性的纺纱联合了到 noncollinearly 极化的铁磁性的领先(F-MS-F ) 的通过按岁差向前运行的电子运输在这篇论文被学习了。nonequilibrium 格林功能途径被用来面对外部偏爱计算状态(LDOS ) 和水流的本地密度。LDOS 和电子水流的人物被... 量磁性的纺纱联合了到 noncollinearly 极化的铁磁性的领先(F-MS-F ) 的通过按岁差向前运行的电子运输在这篇论文被学习了。nonequilibrium 格林功能途径被用来面对外部偏爱计算状态(LDOS ) 和水流的本地密度。LDOS 和电子水流的人物被获得。通道水流为不同按岁差向前运行的角度和领先的磁化的不同配置被调查。当按岁差向前运行的角度拿时,调查揭示那 </2 和否定偏爱被使用,不那样,反响的通道水流出现积极偏爱什么时候被使用,出现。当领先完全被极化,按岁差向前运行的天使拿 0 时,通道水流随着二领先的配置变化;并且当二领先是反平行的时,它成为零。 展开更多
关键词 铁磁耦合 自旋极化 运输 非平衡格林函数 铁磁性耦合 信息 课程 体育
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利用ZnCl_(2)原位钝化电子传输层提高量子点发光二极管性能 被引量:1
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作者 王北恒 高懿韦 +3 位作者 王艳林 曹松 余春燕 翟光美 《微纳电子技术》 CAS 北大核心 2023年第12期1928-1936,共9页
在量子点发光二极管(QLED)中,电子-空穴注入不平衡和量子点层/电子传输层间界面的荧光猝灭限制着QLED效率的提升。基于此,采用金属卤化物(ZnCl_(2))原位处理电子传输层方法来减少氧化锌(ZnO)电子传输层的氧空位,同时有效钝化其表面不饱... 在量子点发光二极管(QLED)中,电子-空穴注入不平衡和量子点层/电子传输层间界面的荧光猝灭限制着QLED效率的提升。基于此,采用金属卤化物(ZnCl_(2))原位处理电子传输层方法来减少氧化锌(ZnO)电子传输层的氧空位,同时有效钝化其表面不饱和键,因此在一定程度上实现抑制量子点/电子传输层界面的荧光猝灭和提高QLED中的电子-空穴注入平衡的目的,最终得到了高亮度、高效率的QLED。原位钝化处理后的ZnO基QLED的最大亮度、峰值电流效率、峰值功率效率和峰值外量子效率(EQE)分别从未处理QLED的176800 cd/m^(2)、9.86 cd/A、8.38 lm/W和7.42%提高到219200 cd/m^(2)、15.14 cd/A、12.66 lm/W和11.65%。结果表明,ZnCl_(2)原位钝化ZnO电子传输层对QLED性能的提升起到重要的作用。 展开更多
关键词 量子点发光二极管(QLED) ZNO 原位钝化 ZnCl_(2) 电子传输层
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HgTe量子点体系中的电子输运
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作者 桂勇 高阳 《淮南师范学院学报》 2023年第2期145-148,共4页
文章为探究HgTe量子点和传统半导体量子点的性能优劣,理论上研究HgTe量子点的电子性质,利用非平衡格林函数方法,研究了两个铁磁电极之间的HgTe量子点在小偏压下的电流输运性质,并将其与传统半导体量子点进行比较。研究发现,对于HgTe量... 文章为探究HgTe量子点和传统半导体量子点的性能优劣,理论上研究HgTe量子点的电子性质,利用非平衡格林函数方法,研究了两个铁磁电极之间的HgTe量子点在小偏压下的电流输运性质,并将其与传统半导体量子点进行比较。研究发现,对于HgTe量子点体态,其电子性质与输运性质与传统半导体量子点类似;对于HgTe量子点边缘态,量子点边缘处的电子可以延伸到量子点的中心,从而在小偏压下就会产生电流,导致HgTe量子点的输运性能优于传统半导体量子点。同时,输运电导会随着量子点的半径减小、温度增高而减小。 展开更多
关键词 拓扑绝缘体 量子点 电子输运
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Quantum Transport through a Triple Quantum Dot System in the Presence of Majorana Bound States
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作者 江兆潭 曹智远 仲成成 《Communications in Theoretical Physics》 SCIE CAS CSCD 2016年第5期622-628,共7页
We study the electron transport through a special quantum-dot(QD)structure composed of three QDs and two Majorana bound states(MBSs)using the nonequilibrium Green’s function technique.This QD-MBS ring structure inclu... We study the electron transport through a special quantum-dot(QD)structure composed of three QDs and two Majorana bound states(MBSs)using the nonequilibrium Green’s function technique.This QD-MBS ring structure includes two channels with the two coupled MBSs being Channel 1 and one QD being Channel 2,and three types of transport processes such as the electron transmission(ET),the Andreev reflection(AR),and the crossed Andreev reflection(CAR).By comparing the ET,AR,and CAR processes through Channels 1 and 2,we make a systematic study on the transport properties of the QD-MBS ring.It is shown that there appear two kinds of characteristic transport patterns for Channels 1 and 2,as well as the interplay between the two patterns.Of particular interest is that there exists an AR-assisted ET process in Channel 2,which is different from that in Channel 1.Thus a clear"X"pattern due to the ET and AR processes appears in the ET,AR,and CAR transmission coefficients.Moreover,we study how Channel 2 affects the three transport processes when Channel 1 is tuned in the ET and CAR regimes.It is shown that the transport properties of the ET,AR and CAR processes can be adjusted by tuning the energy level of the QD embedded in Channel 2.We believe this research should be a helpful reference for understanding the transport properties in the QD-MBS coupled systems. 展开更多
关键词 耦合系统 量子点 束缚态 量子传输 通道耦合 非平衡格林函数 电子传输 运输过程
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一种新型Si电子束蒸发器的研制及其应用研究 被引量:16
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作者 王科范 刘金锋 +4 位作者 邹崇文 徐彭寿 潘海滨 张西庚 王文君 《真空科学与技术学报》 EI CAS CSCD 北大核心 2005年第1期75-78,共4页
我们成功地设计出一种新型的Si电子束蒸发器 ,并将它应用于Ge/Si(111)量子点的生长。由于采用悬臂式设计 ,它完全克服了高压短路的问题。电子束蒸发器的性能试验表明 ,稳定输出功率可以控制输出稳定的Si束流。应用这种电子束蒸发器可以... 我们成功地设计出一种新型的Si电子束蒸发器 ,并将它应用于Ge/Si(111)量子点的生长。由于采用悬臂式设计 ,它完全克服了高压短路的问题。电子束蒸发器的性能试验表明 ,稳定输出功率可以控制输出稳定的Si束流。应用这种电子束蒸发器可以在 70 0℃ ,成功沉积出平整的单晶Si薄膜。进一步的试验表明 ,在这种缓冲层表面可以自组装生长出Ge量子点。 展开更多
关键词 电子束蒸发 量子点 缓冲层 SI(111) 输出功率 薄膜 束流 自组装 单晶 表面
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单晶二氧化钛纳米棒阵列的修饰及其在量子点敏化太阳电池中的应用(英文) 被引量:2
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作者 王时茂 董伟伟 +4 位作者 方晓东 邓赞红 邵景珍 胡林华 朱俊 《物理化学学报》 SCIE CAS CSCD 北大核心 2014年第5期873-880,共8页
使用TiCl4溶液对单晶TiO2纳米棒阵列(TNRs)进行修饰,通过在TiO2纳米棒表面合成TiO2纳米颗粒来提高TNRs的表面积,提高TNRs对量子点的吸附能力,并在此基础上研究了TiCl4修饰时间对基于单晶TNRs的CdS/CdSe量子点敏化太阳电池光伏性能的影响... 使用TiCl4溶液对单晶TiO2纳米棒阵列(TNRs)进行修饰,通过在TiO2纳米棒表面合成TiO2纳米颗粒来提高TNRs的表面积,提高TNRs对量子点的吸附能力,并在此基础上研究了TiCl4修饰时间对基于单晶TNRs的CdS/CdSe量子点敏化太阳电池光伏性能的影响,同时结合强度调制光电流谱(IMPS)研究了TiO2纳米棒阵列的电子传输性能.结果表明:TiCl4修饰可以大幅提高基于单晶TNRs的CdS/CdSe量子点敏化太阳电池的光伏性能,在TiCl4修饰时间为60 h时,其短路电流密度和光电转换效率分别由修饰前的(2.93±0.07)mA·cm-2和0.36%±0.02%提高至(8.19±0.12)mA·cm-2和1.17%±0.07%.同时,IMPS测试表明电子在单晶TiO2纳米棒阵列中的传输速率高于在TiO2纳米颗粒薄膜中的传输速率,证明了单晶TiO2纳米棒阵列在电子传输方面的优越性. 展开更多
关键词 量子点敏化太阳电池 光阳极 二氧化钛 纳米棒阵列 修饰 电子传输
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