Human activities lead to the accumulation of a large amount of nitrogen and phosphorus in sediments in rivers.Simultaneously,nitrogen and phosphorus can be affected by environment and re-enter the upper water body,cau...Human activities lead to the accumulation of a large amount of nitrogen and phosphorus in sediments in rivers.Simultaneously,nitrogen and phosphorus can be affected by environment and re-enter the upper water body,causing secondary pollution of the river water.In this study,laboratory simulation experiments were conducted initially to investigate the release of nitrogen and phosphorus from river sediments in Urumqi City and the surrounding areas in Xinjiang Uygur Autonomous Region of China and determine the factors that influence their release.The results of this study showed significant short-term differences in nitrogen and phosphorus release characteristics from sediments at different sampling points.The proposed secondary kinetics model(i.e.,pseudo-second-order kinetics model)better fitted the release process of sediment nitrogen and phosphorus.The release of nitrogen and phosphorus from sediments is a complex process driven by multiple factors,therefore,we tested the influence of three factors(pH,temperature,and disturbance intensity)on the release of nitrogen and phosphorus from sediments in this study.The most amount of nitrate nitrogen(NO_(3)^(–)-N)was released under neutral conditions,while the most significant release of ammonia nitrogen(NH_(4)^(+)-N)occurred under acidic and alkaline conditions.The release of nitrite nitrogen(NO_(2)^(-)-N)was less affected by pH.The dissolved total phosphorus(DTP)released significantly in the alkaline water environment,while the release of dissolved organic phosphorus(DOP)was more significant in acidic water.The release amount of soluble reactive phosphorus(SRP)increased with an increase in pH.The sediments released nitrogen and phosphorus at higher temperatures,particularly NH_(4)^(+)-N,NO_(3)^(–)-N,and SRP.The highest amount of DOP was released at 15.0℃.An increase in disturbance intensity exacerbated the release of nitrogen and phosphorus from sediments.NH_(4)^(+)-N,DTP,and SRP levels increased linearly with the intensity of disturbance,while NO_(3)^(–)-N and NO_(2)^(–)-N were more stable.This study provides valuable information for protecting and restoring the water environment in arid areas and has significant practical reference value.展开更多
With the development of economy,the impact of human activities on ecological environment is increasing,and environmental protection work is important.Trace elements(Co,Ni,Cu,Pb,Zn,Cd,Cr,and Sc)in surface fi ne-grained...With the development of economy,the impact of human activities on ecological environment is increasing,and environmental protection work is important.Trace elements(Co,Ni,Cu,Pb,Zn,Cd,Cr,and Sc)in surface fi ne-grained sediment samples from the Jiaozhou Bay catchment were selected to evaluate their 2015 environmental background values and the environmental quality.Using statistical analysis,the environmental background values(ranges)of Sc,Co,Ni,Cu,Pb,Zn,Cd,and Cr were calculated,being 13.1(10.8-15.4),12.4(8.6-16.2),32.0(22.9-41.2),29.6(13.5-64.9),24.1(13.0-44.6),77.6(38.5-156.5),0.07(0.02-0.20),and 82.5(66.5-104.0)mg/kg,respectively.The enrichment factor,contamination factor,and pollution load index were used to evaluate the pollution status of the Jiaozhou Bay catchment.The environmental background values of most elements are higher than those of the upper continental crust and lower than those of global shale.At present,the pollution in the eastern Jiaozhou Bay is much higher than that in the western part.The results shall be helpful for future management for trace element pollution monitoring in the Jiaozhou Bay catchment.展开更多
The continuously collected cores from the Permo-Carboniferous coal-bearing strata of the eastern Ordos Basin are essential for studying the hydrocarbon potential in this region.This study adopted sedimentological and ...The continuously collected cores from the Permo-Carboniferous coal-bearing strata of the eastern Ordos Basin are essential for studying the hydrocarbon potential in this region.This study adopted sedimentological and geochemical methods to analyze the sedimentary environment,material composition,and geochemical characteristics of the coal-bearing strata.The differences in depositional and paleoclimatic conditions were compared;and the factors influencing the organic matter content of fine-grained sediments were explored.The depositional environment of the Benxi and Jinci formations was lagoon to tidal flat with weakly reduced waters with low salinity and dry-hot paleoclimatic conditions;while that of the Taiyuan Formation was a carbonate platform and shallow water delta front,where the water was highly reductive.The xerothermic climate alternated with the warm and humid climate.The period of maximum transgression in the Permo-Carboniferous has the highest water salinity.The Shanxi Formation was deposited in a shallow water delta front with a brackish and fresh water environment and alternative weak reductiveness.And the paleoclimate condition is dry-hot.The TOC content in fine-grained samples was averaging 1.52%.The main controlling mechanism of organic matter in this area was the input conditions according to the analysis on input and preservation of organic matter.展开更多
This research study explored the levels of base status metals in soil sediments and particulate matter in the wellington industrial estate location;the main objectives were to: 1) determine sodium and potassium, 2) de...This research study explored the levels of base status metals in soil sediments and particulate matter in the wellington industrial estate location;the main objectives were to: 1) determine sodium and potassium, 2) determine calcium and magnesium, 3) determine available iron. The following hypotheses were put forward;H<sub>0</sub><sub>a</sub>: there is no significant difference in the concentration levels between Ca and Mg in the study area, H<sub>1</sub><sub>a</sub>: there is significant difference in the concentration levels between Ca and Mg in the study area, H<sub>0</sub><sub>b</sub>: there is no significant difference in the concentration levels between Na and K in the study area, H<sub>1</sub><sub>b</sub>: there is significant difference in the concentration levels between Na and K in the study area. Six locations were used to collect samples with the aid of scoop and gravel free auger (at varying depths of 0 - 5 cm and 5 - 10 cm) which are Wellington Industrial Estate Area 1 (WIEL 1), (WIEL 2), (WIEL 3), (WIEL 4), (WIEL 5), (WIEL 6);the samples were given laboratory treatment. Flame photometer, EDTA, and Spectrophotometer were used in the determinations of sodium and potassium, calcium and magnesium, and available iron respectively. The results indicated that levels of potassium were in medium range (moderately high);sodium levels were generally low when compared to Brook’s classification table. Levels of calcium were generally low and those of magnesium were moderate based on Brook’s table of classification. Levels of available iron which fall within the range of Quijano-Guerta (2003) were high;this implies such levels can lead to toxicity. In all locations, there was decrease in the levels of each metal in the samples with (5 - 10 cm) depth.展开更多
Based on grain size analysis for the offshore surface sediments of the Dalian Bay, the assemblages and distribution characteristics of grain size were acquired, and their sources and sedimentary environments as well a...Based on grain size analysis for the offshore surface sediments of the Dalian Bay, the assemblages and distribution characteristics of grain size were acquired, and their sources and sedimentary environments as well as the dominant factors were also discussed preliminarily. The results indicate that the silt has the highest content of 52% in average, followed by sand of 34%. Clay is enriched in the central plateau subregion with the average content of 14%. They are distributed with the strap-shape from east to west, which is consistent with the distribution pattern of minerals there. The coastal shallow-water slope in the north of the study area is characterized by the enrichment of coarser deposition, indicating strong hydrodynamic conditions and nearby source. With water depth increasing southward, silt and clay fraction, mainly enriched on a subaquatic platform with better sorting, are considered to be transported far away. To the further south of the study area with the deepest water off another subaquatic slop, coarse fraction is the highest, implying strong hydrodynamic conditions induced by tide currents which pass in and out the Bohai Sea and Yellow Sea Warm Current that enters the Bohai Sea.展开更多
Phosphorus is a key element and plays an important role in global biogeochemical cycles. The evolution of sedimentary environment is also influenced by phosphorus concentrations and fractions as well as phosphate sorp...Phosphorus is a key element and plays an important role in global biogeochemical cycles. The evolution of sedimentary environment is also influenced by phosphorus concentrations and fractions as well as phosphate sorption characteristics of the marine sediments. The geochemical characteristics of phosphorus and their environmental records were presented in Jiaozhou Bay sediments. Profiles of different forms of phosphorus were measured as well as the roles and vertical distributions of phosphorus forms in response to sedimentary environment changes were investigated. The results showed that inorganic phosphorus （IP） was the major fraction of total phosphorus （TP）; phosphorus which is bound to calcium, iron and occluded phosphorus, as well as the exchangeable phosphorus were the main forms of IP, especially calcium - phosphorus, including detrital carbonate-bound phosphorus （Det- P） and authigenic apatite-bound phosphorus （ACa- P）, are the uppermost constituent of IP in Jiaozhou Bay sediments. Moreover, the lead-210 chronology technology was employed to estimate how much phosphorus was buried ultimately in sediments. And the research showed that the impacts of human activities have increased remarkably in recent years especially between the 1980s and 2000. According to research, the development of Jiaozhou Bay environment in the past hundred years can be divided into three stages ： （ 1 ） before the 1980s characterized by the relatively low sedimentation rate, weak land-derived phosphorus inputs and low anthropogenic impacts; （2） from the 1980s to around 2000, accelerating in the 1990s, during which high sedimentation rates, high phosphorus abundance and burial fluxes due to the severe human activities impacted on the whole environmental system ; （ 3 ） after 2000, the period of the improvement of environment, the whole system has been improved including the decreasing sedimentation rates, concentration and the burial fluxes of phosphorus.展开更多
The Jiaozhou Bay is characterized by heavy eutrophication that is associated with intensive anthropogenic activities. Four core sediments from the Jiaozhou Bay are analyzed using bulk technologies, including sedimenta...The Jiaozhou Bay is characterized by heavy eutrophication that is associated with intensive anthropogenic activities. Four core sediments from the Jiaozhou Bay are analyzed using bulk technologies, including sedimentary total organic carbon（TOC）, total nitrogen（TN）, the stable carbon（δ13C） and nitrogen（δ15 N） isotopic composition to obtain the comprehensive understanding of the source and composition of sedimentary organic matter and further shed light on the environmental changes of the Jiaozhou Bay on a centennial time scale.Results suggest that the TOC and TN concentrations increase in the upper core, having indicated a probable eutrophication process since the 1920 s in the inner bay and the 2000 s in the bay mouth. The TOC and TN concentrations outside the bay have also changed since 1916 owing to the variation of terrigenous input.Considering TOC/TN ratio, δ13 C and δ15 N, it can be concluded there is a mixture of terrigenous and marine organic matter sources in the study area. A simple two end-member（terrigenous and marine） mixing model usingδ13 C indicats that 45%–79% of TOC in the Jiaozhou Bay is from the marine source. The environmental changes of the Jiaozhou Bay are recorded by geochemical proxies, which are influenced by the intensive anthropogenic activities（e.g., extensive use of fertilizers, and discharge of sewage） and climate changes（e.g., rainfall）.展开更多
Based on analysis of parameters of cores taken from Gaoyou Lake, including magnetic susceptibility, grain-size characteristics and sedimentary rate, environmental changes during the modern period were examined with th...Based on analysis of parameters of cores taken from Gaoyou Lake, including magnetic susceptibility, grain-size characteristics and sedimentary rate, environmental changes during the modern period were examined with the assistance of historical records and Gaoyou Lake water level materials. It is concluded that during the modern period a higher value of magnetic susceptibility and a lower sediment grain size coincided with a wet climate, while a lower value of magnetic susceptibility and a higher grain size were related with a dry climate. The results indicate that the climate in the 123 years period from 1880 to 2003AD can be divided into four stages： two low water level stages （1880-1915AD, 1948-1981AD） and two high water level stages （1915-1948AD, 1981-2003AD）. It appears that the regional climate generally underwent a dry-wet-dry-wet pattern in 30-year cycles. At present, it is at the end of a wet period, so the regional climate is expected to become dry in the near future. This conclusion corresponds with the climate records in the historical literature of the Gaoyou area, and it also matches with the climatic changes in North Jiangsu area.展开更多
By means of SEDEX, ASPILA and XRF, depth-dependent changes of different phosphorus forms in sediment cores from specific areas of the offshore Changjiang Estuary (Yangtze Estuary) in 1998 were analyzed. Results show t...By means of SEDEX, ASPILA and XRF, depth-dependent changes of different phosphorus forms in sediment cores from specific areas of the offshore Changjiang Estuary (Yangtze Estuary) in 1998 were analyzed. Results show that contents of total phosphorus (TP), organic-phosphorus (OP) and iron-phosphorus (Fe-P) decreased down-core, while those of absorbed-phosphorus (Ad-P) and calcium-phosphorus (Ca-P) increased. The distribution tendency of detritus-phosphorus (De-P) is not obvious. Results also show that TP, Fe-P and OP contents at Meso station of the Changjiang Estuary and Hangzhou Bay are higher than that of the other stations. This suggests that the pollutants carried by the Changjiang and the Qiantang rivers from inland have affected the natural environment in offshore area. TP, Fe-P and OP contents of each station become higher from bottom to top, indicating the amount of the terrestrial pollutants carried by the two rivers has been enhanced since the last 30-50 years. Ad-P, Ca-P, Fe-P and OP are all active phosphorus in sediments, and their re-cycling in sediment is closely related to each other.展开更多
Based on the analyses of environmental proxy data in lake sediments and instrumental records of Xinjiang in northwest China, the Holocene climate and hydrological variability and its environmental responses were studi...Based on the analyses of environmental proxy data in lake sediments and instrumental records of Xinjiang in northwest China, the Holocene climate and hydrological variability and its environmental responses were studied in different time scales and regions. The results showed that the Holocene climate variability had obvious differences between the north and south of Xinjiang. In northern Xinjiang, the Holocene climate was dry in the early period, humid in the middle period, and then changed to dry in the late period. However, the climate transition times were not consistent in different regions. In southern Xin- jiang, although there were many different types of climate change patterns inferred from different catch- ments, the warm and wet climate was recorded in most lake sediments in the middle Holocene. According to comparisons of some millennium scale records in lake sediments, the climate was warm and dry in the past 100 years. It can be concluded the climate showed a trend of aridity in Holocene. Especially in recent 50 years, the lake area has been shrinking rapidly because of the population growth and social economic development, which brings some environmental problems. Lake level and area changes were sensitively affected by the climate variation in geological history of Xinjiang and the lake level will continue to shrink because of the drought climate and strengthened human activities.展开更多
After nearly 20 years of construction,we have successfully solved a series of hydrologic sedimentaryand environment problems encountered during the construction of the big deep water harbour inLianyungang which can no...After nearly 20 years of construction,we have successfully solved a series of hydrologic sedimentaryand environment problems encountered during the construction of the big deep water harbour inLianyungang which can now accommodate ships of 50000 tonnage.With the economic development,the channel of 50000 tonnage will be built soon, and of 100000 tonnage is under planning. Theconstruction of the international container shipping hub at the harbour is being accelerated in anticipationof the opening of the second Eurasian land bridge.The future development of the harbour will givegreat impetus to the local economy of Lianyungang City and make it an international city.展开更多
Numerous lakes in western China are excellent sites for understanding environmental change.However,what dominates rare earth element(REE) variations are still under debate in the lake environmental research.In this st...Numerous lakes in western China are excellent sites for understanding environmental change.However,what dominates rare earth element(REE) variations are still under debate in the lake environmental research.In this study,we selected 28 surface sediment samples from 17 lakes(i.e.largescale lakes,small water bodies,etc.) in the QinghaiTibet Plateau and Xinjiang area.These samples were analyzed to reveal the behavior of the REEs and major elements.These REE patterns are characterized by light rare earth element(LREE) enrichment,weak Ce anomaly(0.84-0.98,0.94 on average) and negative Eu anomaly(0.53-1.00,0.67 on average).The homogeneous REE patterns may reflect similar REE of the source lithologys.However,the REE abundances showed some significant differences.In this study,water chemistry data analyses inferred that the highly REE values appear possibly in the saltwater lake,and also related to carbonate mineral,whereas p H played a minor role in REE concentrations.In large-scale lakes(e.g.Lake Bosten and Lake Ulungur),the results showed that the relatively larger REE values are in the margins of lakes.Moreover,lower REE contents are towards the central region.Comprehensive study suggested that five major factors control the REE contents:(1) The REE tends to increase with the increase of the weathering intensity.(2) Likewise,heavy mineral(i.e.rutile,anatase,zircon,etc.) are probably primary in these sediments because they are highly enriched in the REE.(3) The contribution of Fe-Mn oxides is significant in sediments because their concentrations highly correlate with the REE.(4) The carbonate mineral(mainly calcite) played a significant role on the REE values in the lakes because the REEs are incorporated into the carbonate minerals generating the low REE concentrations.(5) Major element analysis,mineral analysis,and grain-size data analysis showed that the REE distribution is chiefly influenced by finer grain-size component of lake sediments due to the decreasing proportion of quartz and feldspar than coarser one.Moreover,the clay minerals in finer grain-size sediments can highly absorb the REE.展开更多
The distribution of diatoms from surface sediments of the West Philippine Basin was analyzed, with 68 species and varieties of diatoms from 26 genera identified. Diatom abundance varied spatially, with the absolute ab...The distribution of diatoms from surface sediments of the West Philippine Basin was analyzed, with 68 species and varieties of diatoms from 26 genera identified. Diatom abundance varied spatially, with the absolute abundance of diatoms ranging from 0 to 3.4× 104 frustules/g. The seven tropical pelagic diatoms were Alveus marinus, Azpeitia africana, Azpeitia nodulifera, Hemidiscus cuneiformis, Hernidiscus cuneiformis var. ventricosus, Roperia tesselata and Rhizosolenia bergonii. The relative abundance of these species was greater than 20%, and their distribution pattern in the sediments was overlaid by the flow of the Kuroshio Current. Ethmodiscus rex was present at 159 stations, formed the most abundant and dominant species in the diatomaceous ooze, and thus referred to as Ethmodiscus ooze. Ethmodiscus rex was also a major contributor to primary production in the region. A principal component analysis was employed to explain the relationship between samples and variations in diatom species from the WPB. Four diatom assemblages were distinguished, representing different oceanographic conditions; their spatial distributions were closely related with the North Equatorial Current and Kuroshio Current patterns in the region. These diatom assemblages can therefore be useful in deciphering late Quaternary palaeoceanographic reconstructions of the West Philippine Basin.展开更多
We analyzed grain size composition to provide information on the types and distributions as well as depositional varieties of marine surface sediments from the area surrounding the Antarctic Peninsula. The samples ret...We analyzed grain size composition to provide information on the types and distributions as well as depositional varieties of marine surface sediments from the area surrounding the Antarctic Peninsula. The samples retrieved from the study area contain gravel, sand, silt and clay. As suggested by bathymetry and morphology, the study area is characterized by neritic, hemipelagic and pelagic deposits. The glacial-marine sediments can be divided into two types, residual paratill and compound paratill, which are primarily transported by glaciers and as ice-rafted debris. Ocean current effects on deposition are more obvious, and the deposit types are distributed consistently with terrain variations.展开更多
We studied diatom distribution from 62 samples from the uppermost 1 cm of sedimem in the South China Sea （SCS）, using grabs or box corers in three cruises between 2001-2007. Fifty six genera, 256 species and their v...We studied diatom distribution from 62 samples from the uppermost 1 cm of sedimem in the South China Sea （SCS）, using grabs or box corers in three cruises between 2001-2007. Fifty six genera, 256 species and their varieties were identified. Dominating species included Coscinodiscus africanus, Coscinodiscus nodulifer, Cyclotella stylorum, Hemidiscus cuneiformis, Melosira sulcata, Nitzschia marina, Roperia tesselata, Thalassionema nitzschioides, Thalassiosira excentrica, and Thalassiothrix longissima. Most surface sediments in the SCS were rich ill diatoms, except for a few coarse samples. Average diatom abundance in the study area was 104 607 valve/g. In terms of the abundance, ecology, and spatial distribution, seven diatom zones （Zones 1-7） were recognized. Zone 1 （northern continental shelf） is affected by warm currents, SCS northern branch of the Kuroshio, and northern coastal currents; Zone 2 （northwestern continental shelf） is affected by intense coastal currents; Zone 3 （Xisha Islands sea area） is a bathyal environment with transitional water masses; Zone 4 （sea basin） is a bathyal-to-deep sea with stable and uniform central water masses in a semi-enclosed marginal sea; Zone 5 （Nansba Islands marine area） is a pelagic environment with relatively high surface temperature; Zone 6 （northern Sunda Shelf） is a tropical shelf environment; and Zone 7 （northern Kalimantan Island shelf area） is affected by warm waters from the Indian Ocean and coastal waters. The data indicate that these diatom zones are closely related to topography, hydrodynamics, temperature, nutrients and especially the salinity. Better understanding of the relationship between diatom distribution and the oceanographic factors would help in the reconstruction of the SCS in the past.展开更多
A 107cm piston-core (SHC-2) was drilled at the site with water depth of 5m in South Hongshan Lake, northwest Tibet in 1998. Based upon the 0.72cm/a of modern sedimentary rate that was tested by 210Pb method and also c...A 107cm piston-core (SHC-2) was drilled at the site with water depth of 5m in South Hongshan Lake, northwest Tibet in 1998. Based upon the 0.72cm/a of modern sedimentary rate that was tested by 210Pb method and also calibrated by 137Cs method as well as the 1cm interval sample cutting level, a lake sedimentary record of 150-yr old and with a resolution of 1.4 yrs was obtained. Ratio of geochemistry contents (TOC, TN, CaCO3) and concentrations of trace elements such as B, Sr, Ba, Ca, Mg, K, Na, Al, Ti, Cu, Zn, Fe, Mn, Ni, Cr, V, Pb, etc were analyzed. The values of TOC, TN, C/N, CaCO3, Sr/Ba and Fe/Mn had clear environmental significance and well reflected the environmental changes. Geochemical multi-proxies of lacustrine sediments from SHC-2 core showed that the environmental changes in this area during the past 150 years could be reconstructed as follows: Stage 1 (1850s-1880s) was a cold period; Stage 2 (1880s-1920s) was a warm period. But the variation of lake water volume was stable in the two periods. Stage 3 (1920s-1950s) was a fluctuant and transitional period in temperature, but there were a short cold period in the 1920s and a warm period in the 1930s. Stage 4 (1950s-) showed a warming tendency, though there existed a cold period from the mid 1970s to the end of the 1980s. In the view of general trend in the past 150 years, South Hongshan Lake was shrinking gradually. It showed that, from the comparison with the Guliya ice core and meteorological records of adjacent weather stations, there is difference in the variations of temperature and precipitation among different regions and altitudes in Tibetan Plateau. It is necessary to search multi-scale and high-resolution records for environmental reconstruction and comparison.展开更多
As one of the lakes on the Yunnan-Guizhou plateau, Lake Chenghai, which is a typical closed lake with the precipitation accounting for one-third or more of the annual water input, has a high total salinity (almost lik...As one of the lakes on the Yunnan-Guizhou plateau, Lake Chenghai, which is a typical closed lake with the precipitation accounting for one-third or more of the annual water input, has a high total salinity (almost like a saline lake).The inorganic C,O isotopic composition of lake sediments bears much sensitive information about environmental change in the catchment, while their correlations revealed the hydrological conditions under which the lake was closed. Their compositional variations are controlled by temperature, precipitation, photosynthesis, dissolving equilibrium of the carbonate system and hydrological condition. According to our research on inorganic C, O isotopic composition of Lake Chenghai sediments, we investigated the environmental change of this catchment several decades ago. The results showed that Lake Chenghai has kept good hydrological closing conditions in the past several decades, as indicated by the good correlation of inorganic C, O isotopic composition of sediments; and that the environmental change in this catchment shows a tendency of periodical evolution on a 10\+\{-11\}-years scale, although the signal noise is relatively high at the bottom of the sediment core. And we also can extend C, O isotopes, a sensitive environmental indicator, to nearly saline lake environments with a high degree of mineralization.展开更多
基金the Xinjiang Science and Technology Support Project Plan(2022E02026)the Xinjiang Agricultural University Graduate Research and Innovation Programme(XJAUGRI2023049).
文摘Human activities lead to the accumulation of a large amount of nitrogen and phosphorus in sediments in rivers.Simultaneously,nitrogen and phosphorus can be affected by environment and re-enter the upper water body,causing secondary pollution of the river water.In this study,laboratory simulation experiments were conducted initially to investigate the release of nitrogen and phosphorus from river sediments in Urumqi City and the surrounding areas in Xinjiang Uygur Autonomous Region of China and determine the factors that influence their release.The results of this study showed significant short-term differences in nitrogen and phosphorus release characteristics from sediments at different sampling points.The proposed secondary kinetics model(i.e.,pseudo-second-order kinetics model)better fitted the release process of sediment nitrogen and phosphorus.The release of nitrogen and phosphorus from sediments is a complex process driven by multiple factors,therefore,we tested the influence of three factors(pH,temperature,and disturbance intensity)on the release of nitrogen and phosphorus from sediments in this study.The most amount of nitrate nitrogen(NO_(3)^(–)-N)was released under neutral conditions,while the most significant release of ammonia nitrogen(NH_(4)^(+)-N)occurred under acidic and alkaline conditions.The release of nitrite nitrogen(NO_(2)^(-)-N)was less affected by pH.The dissolved total phosphorus(DTP)released significantly in the alkaline water environment,while the release of dissolved organic phosphorus(DOP)was more significant in acidic water.The release amount of soluble reactive phosphorus(SRP)increased with an increase in pH.The sediments released nitrogen and phosphorus at higher temperatures,particularly NH_(4)^(+)-N,NO_(3)^(–)-N,and SRP.The highest amount of DOP was released at 15.0℃.An increase in disturbance intensity exacerbated the release of nitrogen and phosphorus from sediments.NH_(4)^(+)-N,DTP,and SRP levels increased linearly with the intensity of disturbance,while NO_(3)^(–)-N and NO_(2)^(–)-N were more stable.This study provides valuable information for protecting and restoring the water environment in arid areas and has significant practical reference value.
基金Supported by the Shandong Provincial Natural Science Foundation of China(No.ZR2020MD061)the Construction of Public Scientifi c Research Platform for Hydrobiology and Biotechnology,a Central-Government-Led Local Science and Technology Development Foundation(No.ZY2021HN04)the Independent Project of Hainan Provincial Key Laboratory of Marine Geological Resources and Environment(Nos.ZZ[2020]2019256-01,2019256[2020]HNHSKC-01)。
文摘With the development of economy,the impact of human activities on ecological environment is increasing,and environmental protection work is important.Trace elements(Co,Ni,Cu,Pb,Zn,Cd,Cr,and Sc)in surface fi ne-grained sediment samples from the Jiaozhou Bay catchment were selected to evaluate their 2015 environmental background values and the environmental quality.Using statistical analysis,the environmental background values(ranges)of Sc,Co,Ni,Cu,Pb,Zn,Cd,and Cr were calculated,being 13.1(10.8-15.4),12.4(8.6-16.2),32.0(22.9-41.2),29.6(13.5-64.9),24.1(13.0-44.6),77.6(38.5-156.5),0.07(0.02-0.20),and 82.5(66.5-104.0)mg/kg,respectively.The enrichment factor,contamination factor,and pollution load index were used to evaluate the pollution status of the Jiaozhou Bay catchment.The environmental background values of most elements are higher than those of the upper continental crust and lower than those of global shale.At present,the pollution in the eastern Jiaozhou Bay is much higher than that in the western part.The results shall be helpful for future management for trace element pollution monitoring in the Jiaozhou Bay catchment.
基金founded by the National Natural Science Foundation of China(Grant No.41772130)the Postgraduate Research&Practice Innovation Program of Jiangsu Province(Grant No.KYCX22_2602)+1 种基金the Graduate Innovation Program of China University of Mining and Technology(Grant No.2022WLKXJ035)the Fundamental Research Program of Shanxi Province(Grant No.202103021223283)。
文摘The continuously collected cores from the Permo-Carboniferous coal-bearing strata of the eastern Ordos Basin are essential for studying the hydrocarbon potential in this region.This study adopted sedimentological and geochemical methods to analyze the sedimentary environment,material composition,and geochemical characteristics of the coal-bearing strata.The differences in depositional and paleoclimatic conditions were compared;and the factors influencing the organic matter content of fine-grained sediments were explored.The depositional environment of the Benxi and Jinci formations was lagoon to tidal flat with weakly reduced waters with low salinity and dry-hot paleoclimatic conditions;while that of the Taiyuan Formation was a carbonate platform and shallow water delta front,where the water was highly reductive.The xerothermic climate alternated with the warm and humid climate.The period of maximum transgression in the Permo-Carboniferous has the highest water salinity.The Shanxi Formation was deposited in a shallow water delta front with a brackish and fresh water environment and alternative weak reductiveness.And the paleoclimate condition is dry-hot.The TOC content in fine-grained samples was averaging 1.52%.The main controlling mechanism of organic matter in this area was the input conditions according to the analysis on input and preservation of organic matter.
文摘This research study explored the levels of base status metals in soil sediments and particulate matter in the wellington industrial estate location;the main objectives were to: 1) determine sodium and potassium, 2) determine calcium and magnesium, 3) determine available iron. The following hypotheses were put forward;H<sub>0</sub><sub>a</sub>: there is no significant difference in the concentration levels between Ca and Mg in the study area, H<sub>1</sub><sub>a</sub>: there is significant difference in the concentration levels between Ca and Mg in the study area, H<sub>0</sub><sub>b</sub>: there is no significant difference in the concentration levels between Na and K in the study area, H<sub>1</sub><sub>b</sub>: there is significant difference in the concentration levels between Na and K in the study area. Six locations were used to collect samples with the aid of scoop and gravel free auger (at varying depths of 0 - 5 cm and 5 - 10 cm) which are Wellington Industrial Estate Area 1 (WIEL 1), (WIEL 2), (WIEL 3), (WIEL 4), (WIEL 5), (WIEL 6);the samples were given laboratory treatment. Flame photometer, EDTA, and Spectrophotometer were used in the determinations of sodium and potassium, calcium and magnesium, and available iron respectively. The results indicated that levels of potassium were in medium range (moderately high);sodium levels were generally low when compared to Brook’s classification table. Levels of calcium were generally low and those of magnesium were moderate based on Brook’s table of classification. Levels of available iron which fall within the range of Quijano-Guerta (2003) were high;this implies such levels can lead to toxicity. In all locations, there was decrease in the levels of each metal in the samples with (5 - 10 cm) depth.
文摘Based on grain size analysis for the offshore surface sediments of the Dalian Bay, the assemblages and distribution characteristics of grain size were acquired, and their sources and sedimentary environments as well as the dominant factors were also discussed preliminarily. The results indicate that the silt has the highest content of 52% in average, followed by sand of 34%. Clay is enriched in the central plateau subregion with the average content of 14%. They are distributed with the strap-shape from east to west, which is consistent with the distribution pattern of minerals there. The coastal shallow-water slope in the north of the study area is characterized by the enrichment of coarser deposition, indicating strong hydrodynamic conditions and nearby source. With water depth increasing southward, silt and clay fraction, mainly enriched on a subaquatic platform with better sorting, are considered to be transported far away. To the further south of the study area with the deepest water off another subaquatic slop, coarse fraction is the highest, implying strong hydrodynamic conditions induced by tide currents which pass in and out the Bohai Sea and Yellow Sea Warm Current that enters the Bohai Sea.
文摘Phosphorus is a key element and plays an important role in global biogeochemical cycles. The evolution of sedimentary environment is also influenced by phosphorus concentrations and fractions as well as phosphate sorption characteristics of the marine sediments. The geochemical characteristics of phosphorus and their environmental records were presented in Jiaozhou Bay sediments. Profiles of different forms of phosphorus were measured as well as the roles and vertical distributions of phosphorus forms in response to sedimentary environment changes were investigated. The results showed that inorganic phosphorus （IP） was the major fraction of total phosphorus （TP）; phosphorus which is bound to calcium, iron and occluded phosphorus, as well as the exchangeable phosphorus were the main forms of IP, especially calcium - phosphorus, including detrital carbonate-bound phosphorus （Det- P） and authigenic apatite-bound phosphorus （ACa- P）, are the uppermost constituent of IP in Jiaozhou Bay sediments. Moreover, the lead-210 chronology technology was employed to estimate how much phosphorus was buried ultimately in sediments. And the research showed that the impacts of human activities have increased remarkably in recent years especially between the 1980s and 2000. According to research, the development of Jiaozhou Bay environment in the past hundred years can be divided into three stages ： （ 1 ） before the 1980s characterized by the relatively low sedimentation rate, weak land-derived phosphorus inputs and low anthropogenic impacts; （2） from the 1980s to around 2000, accelerating in the 1990s, during which high sedimentation rates, high phosphorus abundance and burial fluxes due to the severe human activities impacted on the whole environmental system ; （ 3 ） after 2000, the period of the improvement of environment, the whole system has been improved including the decreasing sedimentation rates, concentration and the burial fluxes of phosphorus.
基金The Joint Fund between Natural Science Foundation of China and Shandong Province under contract No.U1606404the National Basic Research Program(973 Program)of China under contract Nos 2015CB452901 and 2015CB452902+1 种基金the National Key Research and Development Plan Sino-Australian Centre for Healthy Coasts under contract No.2016YFE0101500the Program for Aoshan Excellent Scholars of Qingdao National Laboratory for Marine Science and Technology of China under contract No.2015ASTP-OS13
文摘The Jiaozhou Bay is characterized by heavy eutrophication that is associated with intensive anthropogenic activities. Four core sediments from the Jiaozhou Bay are analyzed using bulk technologies, including sedimentary total organic carbon（TOC）, total nitrogen（TN）, the stable carbon（δ13C） and nitrogen（δ15 N） isotopic composition to obtain the comprehensive understanding of the source and composition of sedimentary organic matter and further shed light on the environmental changes of the Jiaozhou Bay on a centennial time scale.Results suggest that the TOC and TN concentrations increase in the upper core, having indicated a probable eutrophication process since the 1920 s in the inner bay and the 2000 s in the bay mouth. The TOC and TN concentrations outside the bay have also changed since 1916 owing to the variation of terrigenous input.Considering TOC/TN ratio, δ13 C and δ15 N, it can be concluded there is a mixture of terrigenous and marine organic matter sources in the study area. A simple two end-member（terrigenous and marine） mixing model usingδ13 C indicats that 45%–79% of TOC in the Jiaozhou Bay is from the marine source. The environmental changes of the Jiaozhou Bay are recorded by geochemical proxies, which are influenced by the intensive anthropogenic activities（e.g., extensive use of fertilizers, and discharge of sewage） and climate changes（e.g., rainfall）.
基金Foundation： National Natural Science Foundation of China, No.40271004Acknowledgements： We wish to thank Professor Wang Ying for her supervision during fieldwork and paper writing, Professor Bruce Mitchell, Associate Provost of University of Waterloo, for reviewing the paper, Shi Xiaodong and Luo Weiwei for making ^210pb dating measurements, and Ding Haiyan for participating in grain size and magnetic susceptibility measurements.
文摘Based on analysis of parameters of cores taken from Gaoyou Lake, including magnetic susceptibility, grain-size characteristics and sedimentary rate, environmental changes during the modern period were examined with the assistance of historical records and Gaoyou Lake water level materials. It is concluded that during the modern period a higher value of magnetic susceptibility and a lower sediment grain size coincided with a wet climate, while a lower value of magnetic susceptibility and a higher grain size were related with a dry climate. The results indicate that the climate in the 123 years period from 1880 to 2003AD can be divided into four stages： two low water level stages （1880-1915AD, 1948-1981AD） and two high water level stages （1915-1948AD, 1981-2003AD）. It appears that the regional climate generally underwent a dry-wet-dry-wet pattern in 30-year cycles. At present, it is at the end of a wet period, so the regional climate is expected to become dry in the near future. This conclusion corresponds with the climate records in the historical literature of the Gaoyou area, and it also matches with the climatic changes in North Jiangsu area.
基金The cooperative project between Government of China and Japan
文摘By means of SEDEX, ASPILA and XRF, depth-dependent changes of different phosphorus forms in sediment cores from specific areas of the offshore Changjiang Estuary (Yangtze Estuary) in 1998 were analyzed. Results show that contents of total phosphorus (TP), organic-phosphorus (OP) and iron-phosphorus (Fe-P) decreased down-core, while those of absorbed-phosphorus (Ad-P) and calcium-phosphorus (Ca-P) increased. The distribution tendency of detritus-phosphorus (De-P) is not obvious. Results also show that TP, Fe-P and OP contents at Meso station of the Changjiang Estuary and Hangzhou Bay are higher than that of the other stations. This suggests that the pollutants carried by the Changjiang and the Qiantang rivers from inland have affected the natural environment in offshore area. TP, Fe-P and OP contents of each station become higher from bottom to top, indicating the amount of the terrestrial pollutants carried by the two rivers has been enhanced since the last 30-50 years. Ad-P, Ca-P, Fe-P and OP are all active phosphorus in sediments, and their re-cycling in sediment is closely related to each other.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (KZCX2-EW-308)the National Basic Research Program of China (2006FY110600)the National Natural Science Foundation of China (41071139 and 40971117)
文摘Based on the analyses of environmental proxy data in lake sediments and instrumental records of Xinjiang in northwest China, the Holocene climate and hydrological variability and its environmental responses were studied in different time scales and regions. The results showed that the Holocene climate variability had obvious differences between the north and south of Xinjiang. In northern Xinjiang, the Holocene climate was dry in the early period, humid in the middle period, and then changed to dry in the late period. However, the climate transition times were not consistent in different regions. In southern Xin- jiang, although there were many different types of climate change patterns inferred from different catch- ments, the warm and wet climate was recorded in most lake sediments in the middle Holocene. According to comparisons of some millennium scale records in lake sediments, the climate was warm and dry in the past 100 years. It can be concluded the climate showed a trend of aridity in Holocene. Especially in recent 50 years, the lake area has been shrinking rapidly because of the population growth and social economic development, which brings some environmental problems. Lake level and area changes were sensitively affected by the climate variation in geological history of Xinjiang and the lake level will continue to shrink because of the drought climate and strengthened human activities.
文摘After nearly 20 years of construction,we have successfully solved a series of hydrologic sedimentaryand environment problems encountered during the construction of the big deep water harbour inLianyungang which can now accommodate ships of 50000 tonnage.With the economic development,the channel of 50000 tonnage will be built soon, and of 100000 tonnage is under planning. Theconstruction of the international container shipping hub at the harbour is being accelerated in anticipationof the opening of the second Eurasian land bridge.The future development of the harbour will givegreat impetus to the local economy of Lianyungang City and make it an international city.
基金supported by a grant from Research Fund for the Doctoral Program of Higher Education of East China University of Technology (DHBK2019012)Key Laboratory for Digital Land and Resources of Jiangxi Province,East China University of Technology (DLLJ202018)。
文摘Numerous lakes in western China are excellent sites for understanding environmental change.However,what dominates rare earth element(REE) variations are still under debate in the lake environmental research.In this study,we selected 28 surface sediment samples from 17 lakes(i.e.largescale lakes,small water bodies,etc.) in the QinghaiTibet Plateau and Xinjiang area.These samples were analyzed to reveal the behavior of the REEs and major elements.These REE patterns are characterized by light rare earth element(LREE) enrichment,weak Ce anomaly(0.84-0.98,0.94 on average) and negative Eu anomaly(0.53-1.00,0.67 on average).The homogeneous REE patterns may reflect similar REE of the source lithologys.However,the REE abundances showed some significant differences.In this study,water chemistry data analyses inferred that the highly REE values appear possibly in the saltwater lake,and also related to carbonate mineral,whereas p H played a minor role in REE concentrations.In large-scale lakes(e.g.Lake Bosten and Lake Ulungur),the results showed that the relatively larger REE values are in the margins of lakes.Moreover,lower REE contents are towards the central region.Comprehensive study suggested that five major factors control the REE contents:(1) The REE tends to increase with the increase of the weathering intensity.(2) Likewise,heavy mineral(i.e.rutile,anatase,zircon,etc.) are probably primary in these sediments because they are highly enriched in the REE.(3) The contribution of Fe-Mn oxides is significant in sediments because their concentrations highly correlate with the REE.(4) The carbonate mineral(mainly calcite) played a significant role on the REE values in the lakes because the REEs are incorporated into the carbonate minerals generating the low REE concentrations.(5) Major element analysis,mineral analysis,and grain-size data analysis showed that the REE distribution is chiefly influenced by finer grain-size component of lake sediments due to the decreasing proportion of quartz and feldspar than coarser one.Moreover,the clay minerals in finer grain-size sediments can highly absorb the REE.
基金Supported by the National Natural Science Foundation of China(Nos.41306083,41106076)the Special Fund for Scientific Research Foundation of the Third Institute of Oceanography,State Oceanic Administration,China(Nos.2010002,2013032)
文摘The distribution of diatoms from surface sediments of the West Philippine Basin was analyzed, with 68 species and varieties of diatoms from 26 genera identified. Diatom abundance varied spatially, with the absolute abundance of diatoms ranging from 0 to 3.4× 104 frustules/g. The seven tropical pelagic diatoms were Alveus marinus, Azpeitia africana, Azpeitia nodulifera, Hemidiscus cuneiformis, Hernidiscus cuneiformis var. ventricosus, Roperia tesselata and Rhizosolenia bergonii. The relative abundance of these species was greater than 20%, and their distribution pattern in the sediments was overlaid by the flow of the Kuroshio Current. Ethmodiscus rex was present at 159 stations, formed the most abundant and dominant species in the diatomaceous ooze, and thus referred to as Ethmodiscus ooze. Ethmodiscus rex was also a major contributor to primary production in the region. A principal component analysis was employed to explain the relationship between samples and variations in diatom species from the WPB. Four diatom assemblages were distinguished, representing different oceanographic conditions; their spatial distributions were closely related with the North Equatorial Current and Kuroshio Current patterns in the region. These diatom assemblages can therefore be useful in deciphering late Quaternary palaeoceanographic reconstructions of the West Philippine Basin.
基金supported by the Chinese Polar Environment Comprehensive Investigation & Assessment Programs (Grant nos. CHINARE2012-01-02 and CHINARE2013-01-02)the National Natural Science Foundation of China (Grant no. 41206056)China Ocean Mineral Resource R&D Association (Grant no.DY12513R03)
文摘We analyzed grain size composition to provide information on the types and distributions as well as depositional varieties of marine surface sediments from the area surrounding the Antarctic Peninsula. The samples retrieved from the study area contain gravel, sand, silt and clay. As suggested by bathymetry and morphology, the study area is characterized by neritic, hemipelagic and pelagic deposits. The glacial-marine sediments can be divided into two types, residual paratill and compound paratill, which are primarily transported by glaciers and as ice-rafted debris. Ocean current effects on deposition are more obvious, and the deposit types are distributed consistently with terrain variations.
基金Supported by the National Natural Science Foundation of China(Nos.40676026,41076079,40831160519)the Basic Research Program of China(973Program)(No.2010CB428704)
文摘We studied diatom distribution from 62 samples from the uppermost 1 cm of sedimem in the South China Sea （SCS）, using grabs or box corers in three cruises between 2001-2007. Fifty six genera, 256 species and their varieties were identified. Dominating species included Coscinodiscus africanus, Coscinodiscus nodulifer, Cyclotella stylorum, Hemidiscus cuneiformis, Melosira sulcata, Nitzschia marina, Roperia tesselata, Thalassionema nitzschioides, Thalassiosira excentrica, and Thalassiothrix longissima. Most surface sediments in the SCS were rich ill diatoms, except for a few coarse samples. Average diatom abundance in the study area was 104 607 valve/g. In terms of the abundance, ecology, and spatial distribution, seven diatom zones （Zones 1-7） were recognized. Zone 1 （northern continental shelf） is affected by warm currents, SCS northern branch of the Kuroshio, and northern coastal currents; Zone 2 （northwestern continental shelf） is affected by intense coastal currents; Zone 3 （Xisha Islands sea area） is a bathyal environment with transitional water masses; Zone 4 （sea basin） is a bathyal-to-deep sea with stable and uniform central water masses in a semi-enclosed marginal sea; Zone 5 （Nansba Islands marine area） is a pelagic environment with relatively high surface temperature; Zone 6 （northern Sunda Shelf） is a tropical shelf environment; and Zone 7 （northern Kalimantan Island shelf area） is affected by warm waters from the Indian Ocean and coastal waters. The data indicate that these diatom zones are closely related to topography, hydrodynamics, temperature, nutrients and especially the salinity. Better understanding of the relationship between diatom distribution and the oceanographic factors would help in the reconstruction of the SCS in the past.
基金Under the auspices of the National (G19980408) and CAS(s Key Project for Basic Research on Tibetan Plateau (KZ951-A1-204, KZ95T-
文摘A 107cm piston-core (SHC-2) was drilled at the site with water depth of 5m in South Hongshan Lake, northwest Tibet in 1998. Based upon the 0.72cm/a of modern sedimentary rate that was tested by 210Pb method and also calibrated by 137Cs method as well as the 1cm interval sample cutting level, a lake sedimentary record of 150-yr old and with a resolution of 1.4 yrs was obtained. Ratio of geochemistry contents (TOC, TN, CaCO3) and concentrations of trace elements such as B, Sr, Ba, Ca, Mg, K, Na, Al, Ti, Cu, Zn, Fe, Mn, Ni, Cr, V, Pb, etc were analyzed. The values of TOC, TN, C/N, CaCO3, Sr/Ba and Fe/Mn had clear environmental significance and well reflected the environmental changes. Geochemical multi-proxies of lacustrine sediments from SHC-2 core showed that the environmental changes in this area during the past 150 years could be reconstructed as follows: Stage 1 (1850s-1880s) was a cold period; Stage 2 (1880s-1920s) was a warm period. But the variation of lake water volume was stable in the two periods. Stage 3 (1920s-1950s) was a fluctuant and transitional period in temperature, but there were a short cold period in the 1920s and a warm period in the 1930s. Stage 4 (1950s-) showed a warming tendency, though there existed a cold period from the mid 1970s to the end of the 1980s. In the view of general trend in the past 150 years, South Hongshan Lake was shrinking gradually. It showed that, from the comparison with the Guliya ice core and meteorological records of adjacent weather stations, there is difference in the variations of temperature and precipitation among different regions and altitudes in Tibetan Plateau. It is necessary to search multi-scale and high-resolution records for environmental reconstruction and comparison.
文摘As one of the lakes on the Yunnan-Guizhou plateau, Lake Chenghai, which is a typical closed lake with the precipitation accounting for one-third or more of the annual water input, has a high total salinity (almost like a saline lake).The inorganic C,O isotopic composition of lake sediments bears much sensitive information about environmental change in the catchment, while their correlations revealed the hydrological conditions under which the lake was closed. Their compositional variations are controlled by temperature, precipitation, photosynthesis, dissolving equilibrium of the carbonate system and hydrological condition. According to our research on inorganic C, O isotopic composition of Lake Chenghai sediments, we investigated the environmental change of this catchment several decades ago. The results showed that Lake Chenghai has kept good hydrological closing conditions in the past several decades, as indicated by the good correlation of inorganic C, O isotopic composition of sediments; and that the environmental change in this catchment shows a tendency of periodical evolution on a 10\+\{-11\}-years scale, although the signal noise is relatively high at the bottom of the sediment core. And we also can extend C, O isotopes, a sensitive environmental indicator, to nearly saline lake environments with a high degree of mineralization.
