The dynamical theory of spectroscopy with femtosecond pulse excitation is applied to a direct dissociation process.In the ultrashort pulse case,the fluorescence-like emission peak occurs in Raman scattering as the inc...The dynamical theory of spectroscopy with femtosecond pulse excitation is applied to a direct dissociation process.In the ultrashort pulse case,the fluorescence-like emission peak occurs in Raman scattering as the incident frequency is tuned near resonance.All properties of the spectroscopy can be explained by the correlation function.展开更多
文摘The dynamical theory of spectroscopy with femtosecond pulse excitation is applied to a direct dissociation process.In the ultrashort pulse case,the fluorescence-like emission peak occurs in Raman scattering as the incident frequency is tuned near resonance.All properties of the spectroscopy can be explained by the correlation function.
