This paper investigates equation (1) in twocases:(i)P=0, (ii)P satisfies|P (i,x,y,z,w)<(A+|y|+|z|+|w|)q(t).whereq(t) is a nonnegative function of t. For case (i) the asymptotic stability in the large of the trivial...This paper investigates equation (1) in twocases:(i)P=0, (ii)P satisfies|P (i,x,y,z,w)<(A+|y|+|z|+|w|)q(t).whereq(t) is a nonnegative function of t. For case (i) the asymptotic stability in the large of the trivial solution x=0 is investigated and for case (ii) the boundedness result is obtained for solutions of equation (1). These results improve and include several well-known results.展开更多
It is found that the field of the combined mode of the probe wave and the phase conjugate wave in the process of non-degenerate four-wave mixing exhibits higher-order squeezing to all even orders. The higher-order squ...It is found that the field of the combined mode of the probe wave and the phase conjugate wave in the process of non-degenerate four-wave mixing exhibits higher-order squeezing to all even orders. The higher-order squeezed parameter and squeezed limit due to the modulation frequency are investigated. The smaller the modulation frequency is, the stronger the degree of higher-order squeezing becomes. Furthermore, the hlgher-order uncertainty relations in the process of non-degenerate four-wave mixing are presented for the first time. The product of higher-order noise moments is related to even order number N and the length L of the medium.展开更多
A novel soluble π-conjugated polymer, poly [(3-acetylpyrrole-2, 5-diyl) p-(N, N-dimethylamino) azobenzylidene] (PAPDMAABE), was synthesized by condensation of 3-acetylpyrrole with 4-aldehyde-4'-dimethylaminoaz...A novel soluble π-conjugated polymer, poly [(3-acetylpyrrole-2, 5-diyl) p-(N, N-dimethylamino) azobenzylidene] (PAPDMAABE), was synthesized by condensation of 3-acetylpyrrole with 4-aldehyde-4'-dimethylaminoazobenzene (ADMAA). The chemical structure of PAPDMAABE was characterized by Fourier transform infrared spectroscopy (FTIR), ^1H-NMR, and UV-Vis-NIR spectra. Transmission electron microscope (TEM) analysis for PAPDMAABE indicates that part of PAPDMAABE is in crystal state, due to the short-range order of the polymer. Thermogravimetric analysis (TGA) curve shows that the polymer has good thermal stability and its decomposition temperature is 248℃. The optical band gap of PAPDMAABE obtained from the optical absorption spectrum is about 1.73 eV. The resonant third-order nonlinear optical property of PAPDMAABE at 532 nm was studied using degenerate four-wave mixing (DFWM) technique. The resonant third-order nonlinear optical susceptibility of the polymer is about 7.48×10^-8 esu.展开更多
We introduce a new kind of four-mode continuous variable entangled state in Fock space. The completeness relation and the partly nonorthonormal property of such a state are proven. The scheme to generate this state is...We introduce a new kind of four-mode continuous variable entangled state in Fock space. The completeness relation and the partly nonorthonormal property of such a state are proven. The scheme to generate this state is presented by combining a symmetrical beamsplitter, a parametric down-conversion and a polarizer. After making a single-mode quadrature amplitude measurement, the remaining three modes are kept in entanglement. And its applications are also discussed.展开更多
Based on the second-order moments, this paper derives an analytical expression of the M^2 factor of four-petal Gaussian beam. The results show that the M^2 factor is only determined by the beam order n. The correspond...Based on the second-order moments, this paper derives an analytical expression of the M^2 factor of four-petal Gaussian beam. The results show that the M^2 factor is only determined by the beam order n. The corresponding numerical calculations are also given. As the beam order increases, the augment of M^2 factor is disciplinary. As the expression of M^2 factor is expressed in series form and becomes more complicated, a new concise formula of M^2 factor is also presented by using curve fitting of numerical calculations. When 3 ≤ n ≤ 200, the maximum error rate of fitting formula will not exceed 2.6% and the average error rate is 0.28%. This research is helpful to the applications of four-petal Gaussian beam.展开更多
The fully oxidized state of polyaniline (PANI), pernigraniline (PN), was synthesized by oxidation of the emeraldine base form of PAM dissolved in NMP solvent with m-chloroperoxybenzoic acid. The resulted PN was charac...The fully oxidized state of polyaniline (PANI), pernigraniline (PN), was synthesized by oxidation of the emeraldine base form of PAM dissolved in NMP solvent with m-chloroperoxybenzoic acid. The resulted PN was characterized by FTIR and UV-Visible spectra. The third-order nonlinear optical properties of PN in concentrated sulfuric acid (PN/H2SO4) were measured by a degenerated four wave mixing (DFWM) method. The results obtained suggest that the soliton-pair intermediate state associated with the degenerated state does not play a major role in the third order nonlinear optical properties of PANI.展开更多
A novel soluble π-conjugated polymer, poly[(3-octanoylpyrrole-2,5-diyl)-p-nitrobenzylidene] (POPNBE), was synthesized by a five-step reaction. As a result of introducing a long acyl to pyrrole at 3-position, the poly...A novel soluble π-conjugated polymer, poly[(3-octanoylpyrrole-2,5-diyl)-p-nitrobenzylidene] (POPNBE), was synthesized by a five-step reaction. As a result of introducing a long acyl to pyrrole at 3-position, the polymer can be easily solved in polar solvents and be processed into films. The chemical structures of the intermediates and POPNBE were characterized by FTIR, 1H NMR, and UV-Vis-NIR spectrometries. The absorption band in the range of 400-600 nm in the UV-Vis-NIR spectrum is due to the π-π * band gap transition. The optical band gap of POPNBE obtained from the optical absorption is about 1.72 eV. The resonant third-order nonlinear optical property of POPNBE at 532 nm was studied by using the degenerate four-wave mixing(DFWM) technique. The resonant third-order nonlinear optical susceptibility of POPNBE is about 3.42×10 -8 esu.展开更多
文摘This paper investigates equation (1) in twocases:(i)P=0, (ii)P satisfies|P (i,x,y,z,w)<(A+|y|+|z|+|w|)q(t).whereq(t) is a nonnegative function of t. For case (i) the asymptotic stability in the large of the trivial solution x=0 is investigated and for case (ii) the boundedness result is obtained for solutions of equation (1). These results improve and include several well-known results.
文摘It is found that the field of the combined mode of the probe wave and the phase conjugate wave in the process of non-degenerate four-wave mixing exhibits higher-order squeezing to all even orders. The higher-order squeezed parameter and squeezed limit due to the modulation frequency are investigated. The smaller the modulation frequency is, the stronger the degree of higher-order squeezing becomes. Furthermore, the hlgher-order uncertainty relations in the process of non-degenerate four-wave mixing are presented for the first time. The product of higher-order noise moments is related to even order number N and the length L of the medium.
基金the National Natural Science Foundation of China for financial support of this work(No.60277002).
文摘A novel soluble π-conjugated polymer, poly [(3-acetylpyrrole-2, 5-diyl) p-(N, N-dimethylamino) azobenzylidene] (PAPDMAABE), was synthesized by condensation of 3-acetylpyrrole with 4-aldehyde-4'-dimethylaminoazobenzene (ADMAA). The chemical structure of PAPDMAABE was characterized by Fourier transform infrared spectroscopy (FTIR), ^1H-NMR, and UV-Vis-NIR spectra. Transmission electron microscope (TEM) analysis for PAPDMAABE indicates that part of PAPDMAABE is in crystal state, due to the short-range order of the polymer. Thermogravimetric analysis (TGA) curve shows that the polymer has good thermal stability and its decomposition temperature is 248℃. The optical band gap of PAPDMAABE obtained from the optical absorption spectrum is about 1.73 eV. The resonant third-order nonlinear optical property of PAPDMAABE at 532 nm was studied using degenerate four-wave mixing (DFWM) technique. The resonant third-order nonlinear optical susceptibility of the polymer is about 7.48×10^-8 esu.
基金supported by the Natural Science Foundation of Jiangxi Province,China (Grant No 2007GZW0171)the Foundation of Education Department of Jiangxi Province,China (Grant No [2007] 136)
文摘We introduce a new kind of four-mode continuous variable entangled state in Fock space. The completeness relation and the partly nonorthonormal property of such a state are proven. The scheme to generate this state is presented by combining a symmetrical beamsplitter, a parametric down-conversion and a polarizer. After making a single-mode quadrature amplitude measurement, the remaining three modes are kept in entanglement. And its applications are also discussed.
基金Project supported by the Scientific Research Fund of Zhejiang Provincial Education Department (Grant No 20060677)
文摘Based on the second-order moments, this paper derives an analytical expression of the M^2 factor of four-petal Gaussian beam. The results show that the M^2 factor is only determined by the beam order n. The corresponding numerical calculations are also given. As the beam order increases, the augment of M^2 factor is disciplinary. As the expression of M^2 factor is expressed in series form and becomes more complicated, a new concise formula of M^2 factor is also presented by using curve fitting of numerical calculations. When 3 ≤ n ≤ 200, the maximum error rate of fitting formula will not exceed 2.6% and the average error rate is 0.28%. This research is helpful to the applications of four-petal Gaussian beam.
基金This work was partly supported by NNSFC,Chinese Academy of Sciences and Director Foundation of the Institute of Chemistry,Academia Sinica
文摘The fully oxidized state of polyaniline (PANI), pernigraniline (PN), was synthesized by oxidation of the emeraldine base form of PAM dissolved in NMP solvent with m-chloroperoxybenzoic acid. The resulted PN was characterized by FTIR and UV-Visible spectra. The third-order nonlinear optical properties of PN in concentrated sulfuric acid (PN/H2SO4) were measured by a degenerated four wave mixing (DFWM) method. The results obtained suggest that the soliton-pair intermediate state associated with the degenerated state does not play a major role in the third order nonlinear optical properties of PANI.
文摘A novel soluble π-conjugated polymer, poly[(3-octanoylpyrrole-2,5-diyl)-p-nitrobenzylidene] (POPNBE), was synthesized by a five-step reaction. As a result of introducing a long acyl to pyrrole at 3-position, the polymer can be easily solved in polar solvents and be processed into films. The chemical structures of the intermediates and POPNBE were characterized by FTIR, 1H NMR, and UV-Vis-NIR spectrometries. The absorption band in the range of 400-600 nm in the UV-Vis-NIR spectrum is due to the π-π * band gap transition. The optical band gap of POPNBE obtained from the optical absorption is about 1.72 eV. The resonant third-order nonlinear optical property of POPNBE at 532 nm was studied by using the degenerate four-wave mixing(DFWM) technique. The resonant third-order nonlinear optical susceptibility of POPNBE is about 3.42×10 -8 esu.