Number concentration and size distribution from gasoline ears are investigated at transient modes on the chassis dynamometers, which are measured using electrical low pressure impactor (ELPI) for the ECE15 and EUDC ...Number concentration and size distribution from gasoline ears are investigated at transient modes on the chassis dynamometers, which are measured using electrical low pressure impactor (ELPI) for the ECE15 and EUDC cycles. Results indicate that, during cold start, particle number emission is higher than that under hot start. It is found that the number of particles increases with the vehicle speeds. Furthermore, particles with diameter smaller than 200 nm constitute the predominant part of total emission in the entire cycle. In addition, the tentative information about composition of emitted particles is also discussed.展开更多
While Unleaded gasoline has the advantage of eliminating lead from automobile exhaust, its potential to reduce the exhaust gas and particles, merits further examination. In the present studies,the concentrations of hy...While Unleaded gasoline has the advantage of eliminating lead from automobile exhaust, its potential to reduce the exhaust gas and particles, merits further examination. In the present studies,the concentrations of hydrocarbons (HC) and earbon monoxides (CO) in emissions were analyzed on Santana engine Dynamometer under a standard test cycle, and total exhaust particles were collected from engines using leaded and unleaded gasoline. It was found that unleaded gasoline reduced the emissions of CO and HC, and decreased the quantity of vehicle exhaust particulate matters by 60%.With the unlead gasoline, only 23 kinds of organic substances, adsorbed in the particles, were identified by gas chromatography/mass spectrometer (GC/MS) while 32 components were detected using the leaded gasoline. The results of in vitro Salmonella/ microsomal test and micronucleus induction assay in CHL cells indicated that both types of gasoline increased the number of histidine-independent colonies and the frequencies of micronucleus induction; no significant differellce was found in their mutagenicity.展开更多
The working principle of a kind of compositive emission control system is inquired into, which includes exhaust heater, secondary air supplement, exhaust gas recirculation (EGR), thermal reactor and catalytic conver...The working principle of a kind of compositive emission control system is inquired into, which includes exhaust heater, secondary air supplement, exhaust gas recirculation (EGR), thermal reactor and catalytic converter, etc. The purification effect of CO, HC and NOx emission of the gasoline spark ignite (S.I.) engine is studied. The entire vehicle driving cycle tests based on the national emission standard and a series of the gasoline engine-testing bench tests including full load characteristic experiment, load characteristic experiment and idle speed experiment are done. The results show that the system has a very good emission control effect to CO, HC and NOx of gasoline engine. The construction of the system is very simple and can be mounted on the exhaust pipe conveniently without any alteration of the vehicle-use gasoline engine.展开更多
Fuel taxes are still a primary funding source for the development and maintenance of transportation infrastructure. Such a tax is collected as a flat fee from the importer or producer of the taxable fuel product. Fuel...Fuel taxes are still a primary funding source for the development and maintenance of transportation infrastructure. Such a tax is collected as a flat fee from the importer or producer of the taxable fuel product. Fuel-efficiency improvements and the adoption of zero-emission vehicles result in a continuous decrease in gasoline tax revenues. This paper proposes a novel distance-based alternative method to replace current gasoline tax collection systems in Japan by providing a software architecture platform. In this platform, we utilize driving information gathered via communication mechanisms installed in connected automated vehicles to develop a system that collects gasoline tax based on reserving spatio-temporal grids. Spatio-temporal sections are created by dividing space and time into equal grids and a designated tax charge is assigned. Connected automated vehicles reserve a planned travel route in advance and travel based on reservation information. The performance evaluation results indicate that the proposed system adequately reserves the requested grids and accurately collects gasoline taxes based on a spatio-temporal grid with minimum communication time and no data package loss. The proposed method is based on micro travel distance charges, which generates gasoline tax revenue by 5.7 percent for model year 2022 and 21.8 percent for model year 2030 as compared to the current flat-fee system.展开更多
Ground-level ozone contamination has been globally an urban air quality issue,particularly for China,which has recently made significant progress in purifying its sky.Unregulated exhaust emissions from motor vehicles,...Ground-level ozone contamination has been globally an urban air quality issue,particularly for China,which has recently made significant progress in purifying its sky.Unregulated exhaust emissions from motor vehicles,predominantly carbonyls and volatile organic compounds(VOCs),are among the leading contributors to ozone formation.In this chassislevel study,the unregulated emissions from five China-5 certified gasoline/CNG bi-fuel taxis,along with their ozone forming potential(OFP),were evaluated.It is found that carbonyls and VOCs were mainly emitted during the starting phase no matter the engine was cold or hot.Compared to gasoline,CNG fueling reduced VOCs emissions on a large scale,especially in the starting phase,but had elevated carbonyls.On a fleet average,CNG fueling derived 15%and 46%less OFP than gasoline in cold-and hot-start tests,respectively.VOCs contributed to over 90%of the total OFP of the exhaust.In terms of alleviating ground-level ozone contamination,CNG is a feasible alternative to gasoline on light-duty vehicles.展开更多
Black carbon(BC)is considered the second largest anthropogenic climate forcer,but the radiative effects of BC are highly correlated with its combustion sources.On-road vehicles are an important source of anthropogenic...Black carbon(BC)is considered the second largest anthropogenic climate forcer,but the radiative effects of BC are highly correlated with its combustion sources.On-road vehicles are an important source of anthropogenic BC.However,there are major uncertainties in the estimates of the BC emissions from on-road light-duty passenger vehicles(LDPVs),and results obtained with the portable emissions measurement system(PEMS)method are particularly lacking.We developed a PEMS platform and evaluated the on-road BC emissions from ten in-use LDPVs.We demonstrated that the BC emission factors(EFs)of gasoline direction injection(GDI)engine vehicles range from 1.10 to 1.56 mg.km^(-1),which are higher than the EFs of port fuel injection(PFI)engine vehicles(0.10–0.17 mg.km^(-1))by a factor of 11.The BC emissions during the cold-start phase contributed 2%–33%to the total emissions.A strong correlation(R^(2)=0.70)was observed between the relative BC EFs and average vehicle speed,indicating that traffic congestion alleviation could effectively mitigate BC emissions.Moreover,BC and particle number(PN)emissions were linearly correlated(R^(2)=0.90),and compared to PFI engine vehicles,the instantaneous PN-to-BC emission rates of GDI engine vehicles were less sensitive to vehicle specific power-to-velocity(VSPV)increase in all speed ranges.展开更多
At the beginning of the tests on application of ethanol gasoline in 2001, Chinese govern- ment promulgated a national standard, GB 18351-2001 “Ethanol Gasoline for Motor Vehicles”. The standard specifies three kinds...At the beginning of the tests on application of ethanol gasoline in 2001, Chinese govern- ment promulgated a national standard, GB 18351-2001 “Ethanol Gasoline for Motor Vehicles”. The standard specifies three kinds of ethanol gasoline, namely E10 (90 RON), E10 (93 RON) and E10 (95 RON). There were ethanol gasoline grades (90 RON and 93 RON) and conventional unleaded gaso- line(97 RON) available in the areas where tests were carried out. Vehicle owners were worried about the harmful action of ethanol to their vehicles because of lack of knowledge regarding ethanol fuel, and they only refueled their cars with conventional 97 RON unleaded gasoline. This idea might cause unnecessary costs to customers and could bring about difficulty to the tests as well. Besides, some other technical questions emerged during the experimental application of ethanol gasoline, such as water content, ethanol content in gasoline, etc. Based on the experiences accumulated during the application tests, the national standard GB 18351-2001 “Ethanol Gasoline for Motor Vehicles” was revised. The revised edition is designated as GB 18351-2004.展开更多
A nuclear microprobe with high spatial resolution and high analytical sensitivity was applied to analyze trace elements, especially lead, in vehicle exhaust of Shanghai city. The result shows that the chemical composi...A nuclear microprobe with high spatial resolution and high analytical sensitivity was applied to analyze trace elements, especially lead, in vehicle exhaust of Shanghai city. The result shows that the chemical composition and its corresponding x-ray relative intensity are different among different vehicle exhausts. There are many kinds of metal elements in particles of vehicle exhaust, most arc harmful to people, such as Ti, Cr, Mn, Ph. etc. We found that the lead concentration was 6820 μg/g and the bromine concentration was 5300 μg/g iii the exhaust from Santana using leaded gasoline (SULG), which is higher than any other kinds of vehicle exhausts. We have also detected the minimum lead in the particles of unleaded gasoline and its content varies from one to another. Its mean concentration was 450 μg/g and the highest reached 6210 μg/g. The unleaded gasoline’s Pb existed in the whole particle while the leaded gasoline’s enriched in the surface of the particle and was more harmful to the human beings.展开更多
Considerable efforts have been devoted to characterising the chemical components of vehicle exhaust.However,these components may not accurately reflect the contribution of vehicle exhaust to atmospheric reactivity bec...Considerable efforts have been devoted to characterising the chemical components of vehicle exhaust.However,these components may not accurately reflect the contribution of vehicle exhaust to atmospheric reactivity because of the presence of species not accounted for(“missing species”)given the limitations of analytical instruments.In this study,we improved the laser photolysis–laser-induced fluorescence(LP-LIF)technique and applied it to directly measure the total OH reactivity(TOR)in exhaust gas from light-duty gasoline vehicles in China.The TOR for China Ⅰ to Ⅵ-a vehicles was 15.6,16.3,8.4,2.6,1.5,and 1.6×10^(4) sec^(-1),respectively,reflecting a notable drop as emission standards were upgraded.The TOR was comparable between cold and warm starts.The missing OH reactivity(MOR)values for China Ⅰ to Ⅳ vehicles were close to zero with a cold start but were much higher with a warm start.The variations in oxygenated volatile organic compounds(OVOCs)under different emission standards and for the two start conditions were similar to those of the MOR,indicating that OVOCs and the missing species may have similar production processes.Online measurement revealed that the duration of the stable driving stage was the primary factor leading to the production of OVOCs and missing species.Our findings underscore the importance of direct measurement of TOR from vehicle exhaust and highlight the necessity of adding OVOCs and other organic reactive gases in future upgrades of emission standards,such that the vehicular contribution to atmospheric reactivity can be more effectively controlled.展开更多
文摘Number concentration and size distribution from gasoline ears are investigated at transient modes on the chassis dynamometers, which are measured using electrical low pressure impactor (ELPI) for the ECE15 and EUDC cycles. Results indicate that, during cold start, particle number emission is higher than that under hot start. It is found that the number of particles increases with the vehicle speeds. Furthermore, particles with diameter smaller than 200 nm constitute the predominant part of total emission in the entire cycle. In addition, the tentative information about composition of emitted particles is also discussed.
文摘While Unleaded gasoline has the advantage of eliminating lead from automobile exhaust, its potential to reduce the exhaust gas and particles, merits further examination. In the present studies,the concentrations of hydrocarbons (HC) and earbon monoxides (CO) in emissions were analyzed on Santana engine Dynamometer under a standard test cycle, and total exhaust particles were collected from engines using leaded and unleaded gasoline. It was found that unleaded gasoline reduced the emissions of CO and HC, and decreased the quantity of vehicle exhaust particulate matters by 60%.With the unlead gasoline, only 23 kinds of organic substances, adsorbed in the particles, were identified by gas chromatography/mass spectrometer (GC/MS) while 32 components were detected using the leaded gasoline. The results of in vitro Salmonella/ microsomal test and micronucleus induction assay in CHL cells indicated that both types of gasoline increased the number of histidine-independent colonies and the frequencies of micronucleus induction; no significant differellce was found in their mutagenicity.
基金This project is supported by Provincial Natural Science Foundation of Guangdong, China and Provincial Environmental Protection Science Foundation of Guangdong, China(No.320-D38000).
文摘The working principle of a kind of compositive emission control system is inquired into, which includes exhaust heater, secondary air supplement, exhaust gas recirculation (EGR), thermal reactor and catalytic converter, etc. The purification effect of CO, HC and NOx emission of the gasoline spark ignite (S.I.) engine is studied. The entire vehicle driving cycle tests based on the national emission standard and a series of the gasoline engine-testing bench tests including full load characteristic experiment, load characteristic experiment and idle speed experiment are done. The results show that the system has a very good emission control effect to CO, HC and NOx of gasoline engine. The construction of the system is very simple and can be mounted on the exhaust pipe conveniently without any alteration of the vehicle-use gasoline engine.
文摘Fuel taxes are still a primary funding source for the development and maintenance of transportation infrastructure. Such a tax is collected as a flat fee from the importer or producer of the taxable fuel product. Fuel-efficiency improvements and the adoption of zero-emission vehicles result in a continuous decrease in gasoline tax revenues. This paper proposes a novel distance-based alternative method to replace current gasoline tax collection systems in Japan by providing a software architecture platform. In this platform, we utilize driving information gathered via communication mechanisms installed in connected automated vehicles to develop a system that collects gasoline tax based on reserving spatio-temporal grids. Spatio-temporal sections are created by dividing space and time into equal grids and a designated tax charge is assigned. Connected automated vehicles reserve a planned travel route in advance and travel based on reservation information. The performance evaluation results indicate that the proposed system adequately reserves the requested grids and accurately collects gasoline taxes based on a spatio-temporal grid with minimum communication time and no data package loss. The proposed method is based on micro travel distance charges, which generates gasoline tax revenue by 5.7 percent for model year 2022 and 21.8 percent for model year 2030 as compared to the current flat-fee system.
基金received funding support from the National Natural Science Foundation of China (No.52272342)the National Engineering Laboratory for Mobile Source Emission Control Technology,China (No.NELMS2018A17).
文摘Ground-level ozone contamination has been globally an urban air quality issue,particularly for China,which has recently made significant progress in purifying its sky.Unregulated exhaust emissions from motor vehicles,predominantly carbonyls and volatile organic compounds(VOCs),are among the leading contributors to ozone formation.In this chassislevel study,the unregulated emissions from five China-5 certified gasoline/CNG bi-fuel taxis,along with their ozone forming potential(OFP),were evaluated.It is found that carbonyls and VOCs were mainly emitted during the starting phase no matter the engine was cold or hot.Compared to gasoline,CNG fueling reduced VOCs emissions on a large scale,especially in the starting phase,but had elevated carbonyls.On a fleet average,CNG fueling derived 15%and 46%less OFP than gasoline in cold-and hot-start tests,respectively.VOCs contributed to over 90%of the total OFP of the exhaust.In terms of alleviating ground-level ozone contamination,CNG is a feasible alternative to gasoline on light-duty vehicles.
基金supported by the National Natural Science Foundation of China(51708327 and 51978404)。
文摘Black carbon(BC)is considered the second largest anthropogenic climate forcer,but the radiative effects of BC are highly correlated with its combustion sources.On-road vehicles are an important source of anthropogenic BC.However,there are major uncertainties in the estimates of the BC emissions from on-road light-duty passenger vehicles(LDPVs),and results obtained with the portable emissions measurement system(PEMS)method are particularly lacking.We developed a PEMS platform and evaluated the on-road BC emissions from ten in-use LDPVs.We demonstrated that the BC emission factors(EFs)of gasoline direction injection(GDI)engine vehicles range from 1.10 to 1.56 mg.km^(-1),which are higher than the EFs of port fuel injection(PFI)engine vehicles(0.10–0.17 mg.km^(-1))by a factor of 11.The BC emissions during the cold-start phase contributed 2%–33%to the total emissions.A strong correlation(R^(2)=0.70)was observed between the relative BC EFs and average vehicle speed,indicating that traffic congestion alleviation could effectively mitigate BC emissions.Moreover,BC and particle number(PN)emissions were linearly correlated(R^(2)=0.90),and compared to PFI engine vehicles,the instantaneous PN-to-BC emission rates of GDI engine vehicles were less sensitive to vehicle specific power-to-velocity(VSPV)increase in all speed ranges.
文摘At the beginning of the tests on application of ethanol gasoline in 2001, Chinese govern- ment promulgated a national standard, GB 18351-2001 “Ethanol Gasoline for Motor Vehicles”. The standard specifies three kinds of ethanol gasoline, namely E10 (90 RON), E10 (93 RON) and E10 (95 RON). There were ethanol gasoline grades (90 RON and 93 RON) and conventional unleaded gaso- line(97 RON) available in the areas where tests were carried out. Vehicle owners were worried about the harmful action of ethanol to their vehicles because of lack of knowledge regarding ethanol fuel, and they only refueled their cars with conventional 97 RON unleaded gasoline. This idea might cause unnecessary costs to customers and could bring about difficulty to the tests as well. Besides, some other technical questions emerged during the experimental application of ethanol gasoline, such as water content, ethanol content in gasoline, etc. Based on the experiences accumulated during the application tests, the national standard GB 18351-2001 “Ethanol Gasoline for Motor Vehicles” was revised. The revised edition is designated as GB 18351-2004.
基金Supported by the National Natural science Foundation of China (Major Project No. 19392100, andProject No. 19475061)
文摘A nuclear microprobe with high spatial resolution and high analytical sensitivity was applied to analyze trace elements, especially lead, in vehicle exhaust of Shanghai city. The result shows that the chemical composition and its corresponding x-ray relative intensity are different among different vehicle exhausts. There are many kinds of metal elements in particles of vehicle exhaust, most arc harmful to people, such as Ti, Cr, Mn, Ph. etc. We found that the lead concentration was 6820 μg/g and the bromine concentration was 5300 μg/g iii the exhaust from Santana using leaded gasoline (SULG), which is higher than any other kinds of vehicle exhausts. We have also detected the minimum lead in the particles of unleaded gasoline and its content varies from one to another. Its mean concentration was 450 μg/g and the highest reached 6210 μg/g. The unleaded gasoline’s Pb existed in the whole particle while the leaded gasoline’s enriched in the surface of the particle and was more harmful to the human beings.
基金supported by the National Natural Science Foundation of China(Nos.91644221 and 41627809)the National Key Research and Development Program of China(Nos.2016YFC0202201 and 2018YFC0213904)the Key-Area Research and Development Program of Guangdong Province(No.2019B110206001).
文摘Considerable efforts have been devoted to characterising the chemical components of vehicle exhaust.However,these components may not accurately reflect the contribution of vehicle exhaust to atmospheric reactivity because of the presence of species not accounted for(“missing species”)given the limitations of analytical instruments.In this study,we improved the laser photolysis–laser-induced fluorescence(LP-LIF)technique and applied it to directly measure the total OH reactivity(TOR)in exhaust gas from light-duty gasoline vehicles in China.The TOR for China Ⅰ to Ⅵ-a vehicles was 15.6,16.3,8.4,2.6,1.5,and 1.6×10^(4) sec^(-1),respectively,reflecting a notable drop as emission standards were upgraded.The TOR was comparable between cold and warm starts.The missing OH reactivity(MOR)values for China Ⅰ to Ⅳ vehicles were close to zero with a cold start but were much higher with a warm start.The variations in oxygenated volatile organic compounds(OVOCs)under different emission standards and for the two start conditions were similar to those of the MOR,indicating that OVOCs and the missing species may have similar production processes.Online measurement revealed that the duration of the stable driving stage was the primary factor leading to the production of OVOCs and missing species.Our findings underscore the importance of direct measurement of TOR from vehicle exhaust and highlight the necessity of adding OVOCs and other organic reactive gases in future upgrades of emission standards,such that the vehicular contribution to atmospheric reactivity can be more effectively controlled.