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Resonantly enhanced second-and third-harmonic generation in dielectric nonlinear metasurfaces 被引量:1
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作者 Ji Tong Wang Pavel Tonkaev +5 位作者 Kirill Koshelev Fangxing Lai Sergey Kruk Qinghai Song Yuri Kivshar Nicolae C.Panoiu 《Opto-Electronic Advances》 SCIE EI CAS CSCD 2024年第5期5-19,共15页
Nonlinear dielectric metasurfaces provide a promising approach to control and manipulate frequency conversion optical processes at the nanoscale,thus facilitating both advances in fundamental research and the developm... Nonlinear dielectric metasurfaces provide a promising approach to control and manipulate frequency conversion optical processes at the nanoscale,thus facilitating both advances in fundamental research and the development of new practical applications in photonics,lasing,and sensing.Here,we employ symmetry-broken metasurfaces made of centrosymmetric amorphous silicon for resonantly enhanced second-and third-order nonlinear optical response.Exploiting the rich physics of optical quasi-bound states in the continuum and guided mode resonances,we comprehensively study through rigorous numerical calculations the relative contribution of surface and bulk effects to second-harmonic generation(SHG)and the bulk contribution to third-harmonic generation(THG) from the meta-atoms.Next,we experimentally achieve optical resonances with high quality factors,which greatly boosts light-matter interaction,resulting in about 550 times SHG enhancement and nearly 5000-fold increase of THG.A good agreement between theoretical predictions and experimental measurements is observed.To gain deeper insights into the physics of the investigated nonlinear optical processes,we further numerically study the relation between nonlinear emission and the structural asymmetry of the metasurface and reveal that the generated harmonic signals arising from linear sharp resonances are highly dependent on the asymmetry of the meta-atoms.Our work suggests a fruitful strategy to enhance the harmonic generation and effectively control different orders of harmonics in all-dielectric metasurfaces,enabling the development of efficient active photonic nanodevices. 展开更多
关键词 second-harmonic generation third-harmonic generation bound state in the continuum guided mode resonance all-dielectric metasurfaces nonlinear optics
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Quantitative effect of kerogen type on the hydrocarbon generation potential of Paleogene lacustrine source rocks,Liaohe Western Depression,China 被引量:1
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作者 Sha-Sha Hui Xiong-Qi Pang +7 位作者 Fu-Jie Jiang Chen-Xi Wang Shu-Xing Mei Tao Hu Hong Pang Min Li Xiao-Long Zhou Kan-Yuan Shi 《Petroleum Science》 SCIE EI CAS CSCD 2024年第1期14-30,共17页
Kerogen types exert a decisive effect on the onset and capacity of hydrocarbon generation of source rocks.Lacustrine source rocks in the Liaohe Western Depression are characterized by thick deposition,high total organ... Kerogen types exert a decisive effect on the onset and capacity of hydrocarbon generation of source rocks.Lacustrine source rocks in the Liaohe Western Depression are characterized by thick deposition,high total organic carbon(TOC)content,various kerogen types,and a wide range of thermal maturity.Consequently,their hydrocarbon generation potential and resource estimation can be misinterpreted.In this study,geochemical tests,numerical analysis,hydrocarbon generation kinetics,and basin modeling were integrated to investigate the differential effects of kerogen types on the hydrocarbon generation potential of lacustrine source rocks.Optimized hydrocarbon generation and expulsion(HGE)models of different kerogen types were established quantitatively upon abundant Rock-Eval/TOC/vitrinite reflectance(R_(o))datasets.Three sets of good-excellent source rocks deposited in the fourth(Es4),third(Es3),and first(Es1)members of Paleogene Shahejie Formation,are predominantly types I-II_(1),II_(1)-II_(2),and II-III,respectively.The activation energy of types I-II_(2)kerogen is concentrated(180-230 kcal/mol),whereas that of type III kerogen is widely distributed(150-280 kcal/mol).The original hydrocarbon generation potentials of types I,II_(1),II_(2),and III kerogens are 790,510,270,and 85 mg/g TOC,respectively.The Ro values of the hydrocarbon generation threshold for type I-III source rocks gradually increase from 0.42%to 0.74%,and Ro values of the hydrocarbon expulsion threshold increase from 0.49%to 0.87%.Types I and II_(1)source rocks are characterized by earlier hydrocarbon generation,more rapid hydrocarbon expulsion,and narrower hydrocarbon generation windows than types II_(2)and III source rocks.The kerogen types also affect the HGE history and resource potential.Three types(conventional,tight,and shale oil/gas)and three levels(realistic,expected,and prospective)of hydrocarbon resources of different members in the Liaohe Western Depression are evaluated.Findings suggest that the Es3 member has considerable conventional and unconventional hydrocarbon resources.This study can quantitatively characterize the hydrocarbon generation potential of source rocks with different kerogen types,and facilitate a quick and accurate assessment of hydrocarbon resources,providing strategies for future oil and gas exploration. 展开更多
关键词 Kerogen type Hydrocarbon generation potential Lacustrine source rocks Liaohe western depression
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Prediction of corrosion rate for friction stir processed WE43 alloy by combining PSO-based virtual sample generation and machine learning 被引量:1
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作者 Annayath Maqbool Abdul Khalad Noor Zaman Khan 《Journal of Magnesium and Alloys》 SCIE EI CAS CSCD 2024年第4期1518-1528,共11页
The corrosion rate is a crucial factor that impacts the longevity of materials in different applications.After undergoing friction stir processing(FSP),the refined grain structure leads to a notable decrease in corros... The corrosion rate is a crucial factor that impacts the longevity of materials in different applications.After undergoing friction stir processing(FSP),the refined grain structure leads to a notable decrease in corrosion rate.However,a better understanding of the correlation between the FSP process parameters and the corrosion rate is still lacking.The current study used machine learning to establish the relationship between the corrosion rate and FSP process parameters(rotational speed,traverse speed,and shoulder diameter)for WE43 alloy.The Taguchi L27 design of experiments was used for the experimental analysis.In addition,synthetic data was generated using particle swarm optimization for virtual sample generation(VSG).The application of VSG has led to an increase in the prediction accuracy of machine learning models.A sensitivity analysis was performed using Shapley Additive Explanations to determine the key factors affecting the corrosion rate.The shoulder diameter had a significant impact in comparison to the traverse speed.A graphical user interface(GUI)has been created to predict the corrosion rate using the identified factors.This study focuses on the WE43 alloy,but its findings can also be used to predict the corrosion rate of other magnesium alloys. 展开更多
关键词 Corrosion rate Friction stir processing Virtual sample generation Particle swarm optimization Machine learning Graphical user interface
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Multi-objective optimization and evaluation of supercritical CO_(2) Brayton cycle for nuclear power generation 被引量:1
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作者 Guo-Peng Yu Yong-Feng Cheng +1 位作者 Na Zhang Ping-Jian Ming 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第2期183-209,共27页
The supercritical CO_(2) Brayton cycle is considered a promising energy conversion system for Generation IV reactors for its simple layout,compact structure,and high cycle efficiency.Mathematical models of four Brayto... The supercritical CO_(2) Brayton cycle is considered a promising energy conversion system for Generation IV reactors for its simple layout,compact structure,and high cycle efficiency.Mathematical models of four Brayton cycle layouts are developed in this study for different reactors to reduce the cost and increase the thermohydraulic performance of nuclear power generation to promote the commercialization of nuclear energy.Parametric analysis,multi-objective optimizations,and four decision-making methods are applied to obtain each Brayton scheme’s optimal thermohydraulic and economic indexes.Results show that for the same design thermal power scale of reactors,the higher the core’s exit temperature,the better the Brayton cycle’s thermo-economic performance.Among the four-cycle layouts,the recompression cycle(RC)has the best overall performance,followed by the simple recuperation cycle(SR)and the intercooling cycle(IC),and the worst is the reheating cycle(RH).However,RH has the lowest total cost of investment(C_(tot))of$1619.85 million,and IC has the lowest levelized cost of energy(LCOE)of 0.012$/(kWh).The nuclear Brayton cycle system’s overall performance has been improved due to optimization.The performance of the molten salt reactor combined with the intercooling cycle(MSR-IC)scheme has the greatest improvement,with the net output power(W_(net)),thermal efficiencyη_(t),and exergy efficiency(η_(e))improved by 8.58%,8.58%,and 11.21%,respectively.The performance of the lead-cooled fast reactor combined with the simple recuperation cycle scheme was optimized to increase C_(tot) by 27.78%.In comparison,the internal rate of return(IRR)increased by only 7.8%,which is not friendly to investors with limited funds.For the nuclear Brayton cycle,the molten salt reactor combined with the recompression cycle scheme should receive priority,and the gas-cooled fast reactor combined with the reheating cycle scheme should be considered carefully. 展开更多
关键词 Supercritical CO_(2)Brayton cycle Nuclear power generation Thermo-economic analysis Multi-objective optimization Decision-making methods
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In vivo label-free measurement of blood flow velocity symmetry based on dual line scanning third-harmonic generation microscopy excited at the 1700 nm window 被引量:1
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作者 Hui Cheng Jincheng Zhong +1 位作者 Ping Qiu Ke Wang 《Journal of Innovative Optical Health Sciences》 SCIE EI CSCD 2024年第1期61-68,共8页
Measurement of bloodflow velocity is key to understanding physiology and pathology in vivo.While most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the in... Measurement of bloodflow velocity is key to understanding physiology and pathology in vivo.While most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the instantaneous bloodflow velocity distribution.This is mainly due to the lack of measurement technology with high spatial and temporal resolution.Here,we tackle this problem with our recently developed dual-wavelength line-scan third-harmonic generation(THG)imaging technology.Simultaneous acquisition of dual-wavelength THG line-scanning signals enables measurement of bloodflow velocities at two radially symmetric positions in both venules and arterioles in mouse brain in vivo.Our results clearly show that the instantaneous bloodflow velocity is not symmetric under general conditions. 展开更多
关键词 1700 nm-Window third-harmonic generation imaging blood flow velocity
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Influence of Magmatic Intrusion on Abnormal Hydrocarbon Generation and Expulsion of Source Rock:A Case Study of the Dongying Sag,Bohai Bay Basin
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作者 LI Chuanming ZENG Jianhui +2 位作者 WANG Maoyun LONG Hui LIU Shuning 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2024年第5期1322-1337,共16页
How gabbro affects the generation and expulsion of hydrocarbons in muddy surrounding rocks is clarified by analyzing thin section,major and trace elements,total organic carbon(TOC),pyrolysis,extracts and vitrinite ref... How gabbro affects the generation and expulsion of hydrocarbons in muddy surrounding rocks is clarified by analyzing thin section,major and trace elements,total organic carbon(TOC),pyrolysis,extracts and vitrinite reflectance data from source rocks in the Chunxi area the Dongying Sag,Bohai Bay Basin,eastern China.The results show that a magma intrusion brings copious heat to the source rocks,which promotes abnormal maturation of organic matter(OM)and rapid hydrocarbon generation.The CH_(4)and H_(2)produced by gabbro alteration play a role in hydrocarbon generation of source rocks.The hydrothermal process during magma intrusion provides many different minerals to the source rock,resulting in carbonate-rich surrounding mudstone.The carbonate and clay minerals produced by volcanic mineral alteration jointly catalyze the hydrocarbon generation of the source rock.The high-temperature baking of the intrusion results in hydrothermal pressurization and hydrocarbon generation pressurization,causing many fractures in the surrounding rock.The generated oil and gas are discharged through the fractures under diffusion and pressure.Mantle-derived CO_(2)is also conducive to the expulsion of hydrocarbons because of its strong enrichment capacity for hydrocarbons. 展开更多
关键词 igneous rock hydrocarbon generation source rock high temperature CATALYSIS EOCENE Dongying Sag
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Harnessing overlapped temperature-salinity gradient in solar-driven interfacial seawater evaporation for efficient steam and electricity generation
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作者 Peida Li Dongtong He +2 位作者 Jingchang Sun Jieshan Qiu Zhiyu Wang 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第8期694-700,I0015,共8页
Solar-driven interfacial water evaporation(SIWE)offers a superb way to leverage concentrated solar heat to minimize energy dissipation during seawater desalination.It also engenders overlapped temperaturesalinity grad... Solar-driven interfacial water evaporation(SIWE)offers a superb way to leverage concentrated solar heat to minimize energy dissipation during seawater desalination.It also engenders overlapped temperaturesalinity gradient(TSG)between water-air interface and adjacent seawater,affording opportunities of harnessing electricity.However,the efficiency of conventional SIWE technologies is limited by significant challenges,including salt passivation to hinder evaporation and difficulties in exploiting overlapped TSG simultaneously.Herein,we report self-sustaining hybrid SIWE for not only sustainable seawater desalination but also efficient electricity generation from TSG.It enables spontaneous circulation of salt flux upon seawater evaporation,inducing a self-cleaning evaporative interface without salt passivation for stable steam generation.Meanwhile,this design enables spatial separation and simultaneous utilization of overlapped TSG to enhance electricity generation.These benefits render a remarkable efficiency of90.8%in solar energy utilization,manifesting in co-generation of solar steam at a fast rate of 2.01 kg m^(-2)-h^(-1)and electricity power of 1.91 W m^(-2)with high voltage.Directly interfacing the hybrid SIWE with seawater electrolyzer constructs a system for water-electricity-hydrogen co-generation without external electricity supply.It produces hydrogen at a rapid rate of 1.29 L h^(-1)m^(-2)and freshwater with 22 times lower Na+concentration than the World Health Organization(WHO)threshold. 展开更多
关键词 Solar-driven interfacial water evaporation Steam generation Electricity generation Seawater
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Hydrocarbon Generation Potential and Organic Matter Enrichment Mechanism of the Cambrian Marine Shale in the Tadong Low Uplift,Tarim Basin
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作者 MIAO Huan WANG Yanbin +5 位作者 JIANG Zhenxue ZHAO Shihu SHANG Peng GONG Xun TAO Chuanqi ZHANG Yu 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2024年第5期1301-1321,共21页
Cambrian shales in China and elsewhere contain abundant oil and gas resources.However,due to its deep burial and limited outcrop,there has been relatively little research conducted on it.The Cambrian shale of the Tado... Cambrian shales in China and elsewhere contain abundant oil and gas resources.However,due to its deep burial and limited outcrop,there has been relatively little research conducted on it.The Cambrian shale of the Tadong low uplift in the Tarim Basin of western China,specifically the Xidashan-Xishanbulake Formation(Fm.)and overlying Moheershan Fm.provide a case study through the use of organic petrology,mineralogy,organic and elemental geochemistry,with the aim of analyzing and exploring the hydrocarbon generation potential(PG)and organic matter(OM)enrichment mechanisms within these shale formations.The results indicate that:(1)the Cambrian shale of the Tadong low uplift exhibits relatively dispersed OM that consists of vitrinite-like macerals and solid bitumen.These formations have a higher content of quartz and are primarily composed of silica-based lithology;(2)shale samples from the Xidashan-Xishanbulake and Moheershan formations demonstrate high total organic carbon(TOC)and low pyrolytic hydrocarbon content(S_(2))content.The OM is predominantly typeⅠand typeⅡkerogens,indicating a high level of maturation in the wet gas period.These shales have undergone extensive hydrocarbon generation,showing characteristics of relatively poor PG;(3)the sedimentary environments of the Xidashan-Xishanbulake and Moheershan formations in the Tadong low uplift are similar.They were deposited in warm and humid climatic conditions,in oxygen-deficient environments,with stable terrigenous inputs,high paleoproductivity,high paleosalinity,weak water-holding capacity,and no significant hydrothermal activity;and(4)the relationship between TOC and the paleoproductivity parameter(P/Ti)is most significant in the Lower Cambrian Xidashan-Xishanbulake Fm.,whereas correlation with other indicators is not evident.This suggests a productivity-driven OM enrichment model,where input of landderived material was relatively small during the Middle Cambrian,and the ancient water exhibited lower salinity.A comprehensive pattern was formed under the combined control of paleoproductivity and preservation conditions.This study provides valuable guidance for oil and gas exploration in the Tarim Basin. 展开更多
关键词 Conventional resources hydrocarbon generation potential geochemistry sedimentary environment enrichment mechanism organic matter CAMBRIAN Tadong low uplift
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Impact of volcanism on the formation and hydrocarbon generation of organic-rich shale in the Jiyang Depression, Bohai Bay Basin, China
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作者 Jia-Hong Gao Xin-Ping Liang +5 位作者 Zhi-Jun Jin Quan-You Liu Chang-Rong Li Xiao-Wei Huang Ju-Ye Shi Peng Li 《Petroleum Science》 SCIE EI CAS CSCD 2024年第3期1539-1551,共13页
Globally,most organic-rich shales are deposited with volcanic ash layers.Volcanic ash,a source for many sedimentary basins,can affect the sedimentary water environment,alter the primary productivity,and preserve the o... Globally,most organic-rich shales are deposited with volcanic ash layers.Volcanic ash,a source for many sedimentary basins,can affect the sedimentary water environment,alter the primary productivity,and preserve the organic matter(OM)through physical,chemical,and biological reactions.With an increasing number of breakthroughs in shale oil exploration in the Bohai Bay Basin in recent years,less attention has been paid to the crucial role of volcanic impact especially its influence on the OM enrichment and hydrocarbon formation.Here,we studied the petrology,mineralogy,and geochemical characteristics of the organic-rich shale in the upper submember of the fourth member(Es_(4)^(1))and the lower submember of the third member(Es_(3)^(3))of the Shahejie Formation,aiming to better understand the volcanic impact on organic-rich shale formation.Our results show that total organic carbon is higher in the upper shale intervals rich in volcanic ash with enriched light rare earth elements and moderate Eu anomalies.This indicates that volcanism promoted OM formation before or after the eruption.The positive correlation between Eu/Eu*and Post-Archean Australian Shale indicates hydrothermal activity before the volcanic eruption.The plane graph of the hydrocarbon-generating intensity(S1+S2)suggests that the heat released by volcanism promoted hydrocarbon generation.Meanwhile,the nutrients carried by volcanic ash promoted biological blooms during Es_(4)^(1 )and Es_(3)^(3) deposition,yielding a high primary productivity.Biological blooms consume large amounts of oxygen and form anoxic environments conducive to the burial and preservation of OM.Therefore,this study helps to further understand the organic-inorganic interactions caused by typical geological events and provides a guide for the next step of shale oil exploration and development in other lacustrine basins in China. 展开更多
关键词 Volcanic ash Hydrocarbon generation Organic-rich shale Shahejie Formation Jiyang Depression
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Efficient C-N coupling in electrocatalytic urea generation on copper carbonate hydroxide electrocatalysts
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作者 Yinuo Wang Yian Wang +11 位作者 Qinglan Zhao Hongming Xu Shangqian Zhu Fei Yang Ernest P.Delmo Xiaoyi Qiu Chi Song Juhee Jang Tiehuai Li Ping Gao MDanny Gu Minhua Shao 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第6期289-298,I0008,共11页
Urea generation through electrochemical CO_(2) and NO_(3)~-co-reduction reaction(CO_(2)NO_(3)RR)is still limited by either the low selectivity or yield rate of urea.Herein,we report copper carbonate hydroxide(Cu_2(OH)... Urea generation through electrochemical CO_(2) and NO_(3)~-co-reduction reaction(CO_(2)NO_(3)RR)is still limited by either the low selectivity or yield rate of urea.Herein,we report copper carbonate hydroxide(Cu_2(OH)_2CO_(3))as an efficient CO_(2)NO_(3)RR electrocatalyst with an impressive urea Faradaic efficiency of45.2%±2.1%and a high yield rate of 1564.5±145.2μg h~(-1)mg_(cat)~(-1).More importantly,H_(2) evolution is fully inhibited on this electrocatalyst over a wide potential range between-0.3 and-0.8 V versus reversible hydrogen electrode.Our thermodynamic simulation reveals that the first C-N coupling follows a unique pathway on Cu_2(OH)_2CO_(3) by combining the two intermediates,~*COOH and~*NHO.This work demonstrates that high selectivity and yield rate of urea can be simultaneously achieved on simple Cu-based electrocatalysts in CO_(2)NO_(3)RR,and provide guidance for rational design of more advanced catalysts. 展开更多
关键词 Copper carbonate hydroxide Co-reduction Urea generation C-N coupling DFT calculation
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Differences and identification on multi-time hydrocarbon generation of carboniferous-permian coaly source rocks in the Huanghua Depression,Bohai Bay Basin
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作者 Jin-Jun Xu Xian-Gang Cheng +5 位作者 Shu-Nan Peng Jun-Cai Jiang Qi-Long Wu Da Lou Fu-Qi Cheng La-Mei Lin 《Petroleum Science》 SCIE EI CAS CSCD 2024年第2期765-776,共12页
Coal is a solid combustible mineral,and coal-bearing strata have important hydrocarbon generation potential and contribute to more than 12%of the global hydrocarbon resources.However,the deposition and hydrocarbon evo... Coal is a solid combustible mineral,and coal-bearing strata have important hydrocarbon generation potential and contribute to more than 12%of the global hydrocarbon resources.However,the deposition and hydrocarbon evolution process of ancient coal-bearing strata is characterized by multiple geological times,leading to obvious distinctions in their hydrocarbon generation potential,geological processes,and production,which affect the evaluation and exploration of hydrocarbon resources derived from coaly source rocks worldwide.This study aimed to identify the differences on oil-generated parent macerals and the production of oil generated from different coaly source rocks and through different oil generation processes.Integrating with the analysis of previous tectonic burial history and hydrocarbon generation history,high-temperature and high-pressure thermal simulation experiments,organic geochemistry,and organic petrology were performed on the Carboniferous-Permian(C-P)coaly source rocks in the Huanghua Depression,Bohai Bay Basin.The oil-generated parent macerals of coal's secondary oil generation process(SOGP)were mainly hydrogen-rich collotelinite,collodetrinite,sporinite,and cutinite,while the oil-generated parent macerals of tertiary oil generation process(TOGP)were the remaining small amount of hydrogen-rich collotelinite,sporinite,and cutinite,as well as dispersed soluble organic matter and unexhausted residual hydrocarbons.Compared with coal,the oil-generated parent macerals of coaly shale SOGP were mostly sporinite and cutinite.And part of hydrogen-poor vitrinite,lacking hydrocarbon-rich macerals,and macerals of the TOGP,in addition to some remaining cutinite and a small amount of crude oil and bitumen from SOGP contributed to the oil yield.The results indicated that the changes in oil yield had a good junction between SOGP and TOGP,both coal and coaly shale had higher SOGP aborted oil yield than TOGP starting yield,and coaly shale TOGP peak oil yield was lower than SOGP peak oil yield.There were significant differences in saturated hydrocarbon and aromatic parameters in coal and coaly shale.Coal SOGP was characterized by a lower Ts/Tm and C31-homohopane22S/(22S+22R)and a higher Pr/n C17compared to coal TOGP,while the aromatic parameter methyl dibenzothiophene ratio(MDR)exhibited coaly shale TOGP was higher than coaly shale SOGP than coaly TOGP than coaly SOGP,and coal trimethylnaphthalene ratio(TNR)was lower than coaly shale TNR.Thus,we established oil generation processes and discriminative plates.In this way,we distinguished the differences between oil generation parent maceral,oil generation time,and oil production of coaly source rocks,and therefore,we provided important support for the evaluation,prediction,and exploration of oil resources from global ancient coaly source rocks. 展开更多
关键词 Thermal simulation Multi-time oil generation processes Coaly source rock CARBONIFEROUS-PERMIAN Huanghua Depression
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Natural high-porous diatomaceous-earth based self-floating aerogel for efficient solar steam power generation
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作者 Aitang Zhang Kai Wang +6 位作者 Md Julker Nine Mengyu Cao Hanwen Zong Zhiqiang Liu Hanwen Guo Jingquan Liu Dusan Losic 《Green Energy & Environment》 SCIE EI CAS CSCD 2024年第2期378-389,共12页
The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water resources.At present,many kinds of photothermal conversion materials have been developed and ... The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water resources.At present,many kinds of photothermal conversion materials have been developed and used as evaporators in seawater desalination.However,some evaporators need additional thermal insulation or water supply devices to achieve efficient photothermal conversion.In addition,their complex,time consuming and no scalable preparation process,high cost of raw materials and poor salt resistance hinder the practical application of these evaporator.Owing to its distinctive nanoporous structure,diatomite as fossilized single-cells algae diatoms is a promising natural silica-based material for seawater desalination.They are taken from sea and that makes true sense to use them in the sea.Herein,we report the first example of synthesis robust three-dimensional(3D)natural-diatomite composite by assembling polyaniline nanoparticles covered diatomite into the polyvinyl alcohol pre-treated melamine foam frameworks and demonstrate its application as new evaporator for seawater desalination.The porous framework does not only improve the sunlight scattering efficiency,but also offer large network of channels for water transportation.The inherent mechanism behind salt desalination process involves the absorption of water molecules on the surface of the internal silica micro-nano pores,and evaporation under the heat induced by the polyaniline absorbed sunlight.Meanwhile,the metal ions are segregated by many available pores and channels to achieve the self-desalting effect.The developed evaporator possesses the superiority of multi-stage pore structure,strong hydrophilicity,low thermal conductivity,excellent light absorption,fast water transportation and salt-resistant crystallization as well as good durability.The evaporation rate without an additional device is found to be 1.689 kg m^(-2)h^(-1)under 1-Sun irradiation,and the energy conversion efficiency is as high as 95%.This work creates a platform and develops the prospect of employing green and sustainable natural-diatomite composite evaporator for practical applications of seawater desalination. 展开更多
关键词 DIATOMITE Micro/nanopores Polyaniline Three-dimensional composite Solar steam generation
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Amphipathic Janus Nanofibers Aerogel for Efficient Solar Steam Generation
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作者 Rui Wang Jinshuo Deng +6 位作者 Ping Wu Qianli Ma Xiangting Dong Wensheng Yu Guixia Liu Jinxian Wang Lei Liu 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第4期422-432,共11页
Solar steam generation is a promising water purification technology due to its low-cost and environmentally friendly applications in water purification and desalination.However,hydrophilic or hydrophobic materials alo... Solar steam generation is a promising water purification technology due to its low-cost and environmentally friendly applications in water purification and desalination.However,hydrophilic or hydrophobic materials alone are insufficient in achieving necessary characteristics for constructing highquality solar steam generators with good comprehensive properties.Herein,novel hydrophile/hydrophobe amphipathic Janus nanofibers aerogel is designed and used as a host material for preparing solar steam generators.The product consists of an internal cubic aerogel and an external layer of photothermal materials.The internal aerogel is composed of electrospun amphipathic Janus nanofibers.Owing to the unique composition and structure,the prepared solar steam generator integrates the features of high water evaporation rate(2.944 kg m^(-2)h^(-1)under 1 kW m^(-2)irradiation),selffloating,salt-resisting,and fast performance recovery after flipping.Moreover,the product also exhibits excellent properties on desalination and removal of organic pollutants.Compared with traditional hydrophilic aerogel host material,the amphipathic Janus nanofibers aerogel brings much higher water evaporation rate and salt resistance. 展开更多
关键词 AEROGELS electrospinning photothermal materials solar desalination solar steam generation
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MTTSNet:Military time-sensitive targets stealth network via real-time mask generation
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作者 Siyu Wang Xiaogang Yang +4 位作者 Ruitao Lu Zhengjie Zhu Fangjia Lian Qing-ge Li Jiwei Fan 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期601-612,共12页
The automatic stealth task of military time-sensitive targets plays a crucial role in maintaining national military security and mastering battlefield dynamics in military applications.We propose a novel Military Time... The automatic stealth task of military time-sensitive targets plays a crucial role in maintaining national military security and mastering battlefield dynamics in military applications.We propose a novel Military Time-sensitive Targets Stealth Network via Real-time Mask Generation(MTTSNet).According to our knowledge,this is the first technology to automatically remove military targets in real-time from videos.The critical steps of MTTSNet are as follows:First,we designed a real-time mask generation network based on the encoder-decoder framework,combined with the domain expansion structure,to effectively extract mask images.Specifically,the ASPP structure in the encoder could achieve advanced semantic feature fusion.The decoder stacked high-dimensional information with low-dimensional information to obtain an effective mask layer.Subsequently,the domain expansion module guided the adaptive expansion of mask images.Second,a context adversarial generation network based on gated convolution was constructed to achieve background restoration of mask positions in the original image.In addition,our method worked in an end-to-end manner.A particular semantic segmentation dataset for military time-sensitive targets has been constructed,called the Military Time-sensitive Target Masking Dataset(MTMD).The MTMD dataset experiment successfully demonstrated that this method could create a mask that completely occludes the target and that the target could be hidden in real time using this mask.We demonstrated the concealment performance of our proposed method by comparing it to a number of well-known and highly optimized baselines. 展开更多
关键词 Deep learning Military application Targets stealth network Mask generation Generative adversarial network
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Enhanced picosecond terahertz wave generation based on cascade effects in a terahertz parametric generator
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作者 张敬喜 王与烨 +5 位作者 徐炳烽 陈锴 刘紫鲲 马鸿儒 徐德刚 姚建铨 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第8期271-275,共5页
Enhanced terahertz wave generation via a Stokes cascade process has been demonstrated using picosecond pulse pumped terahertz parametric generation at 1 kHz repetition rate.Clear cascade saturation of terahertz output... Enhanced terahertz wave generation via a Stokes cascade process has been demonstrated using picosecond pulse pumped terahertz parametric generation at 1 kHz repetition rate.Clear cascade saturation of terahertz output was observed,and the corresponding cascade-Stokes spectra were analyzed.The maximum terahertz wave average power was 22μW under a pump power of 30 W,whereas the maximum power conversion efficiency was 8×10^(-7)under a pump power of 21 W.The THz power fluctuation was measured to be about 1%in 20 min.This THz parametric source with a relatively stable output is suitable for a variety of practical applications. 展开更多
关键词 terahertz parametric generation stimulated polariton cascade effect CLN crystal
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Spin-controlled generation of a complete polarization set with randomly-interleaved plasmonic metasurfaces
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作者 Sören im Sande Yadong Deng +1 位作者 Sergey I.Bozhevolnyi Fei Ding 《Opto-Electronic Advances》 SCIE EI CAS CSCD 2024年第8期16-24,共9页
Optical metasurfaces,comprising subwavelength quasi-planar nanostructures,constitute a universal platform for manipulating the amplitude,phase,and polarization of light,thus paving a way for the next generation of hig... Optical metasurfaces,comprising subwavelength quasi-planar nanostructures,constitute a universal platform for manipulating the amplitude,phase,and polarization of light,thus paving a way for the next generation of highly integrated multifunctional optical devices.In this work,we introduce a reflective metasurface for the generation of a complete(angularly resolved)polarization set by randomly interleaving anisotropic plasmonic meta-atoms acting as nanoscale wave plates.In the proof-of-concept demonstration,we achieve multidirectional beam-steering into different polarization channels forming a complete set of polarization states,which can also be dynamically altered by switching the spin of incident light.The developed design concept represents a significant advancement in achieving flat polarization optics with advanced functionalities. 展开更多
关键词 plasmonic metasurface randomly interleaved multidirectional beam-steering spin-controlled all-polarization generation
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Blade Wrap Angle Impact on Centrifugal Pump Performance:Entropy Generation and Fluid-Structure Interaction Analysis
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作者 Hayder Kareem Sakran Mohd Sharizal Abdul Aziz Chu Yee Khor 《Computer Modeling in Engineering & Sciences》 SCIE EI 2024年第7期109-137,共29页
The centrifugal pump is a prevalent power equipment widely used in different engineering patterns,and the impeller blade wrap angle significantly impacts its performance.A numerical investigation was conducted to anal... The centrifugal pump is a prevalent power equipment widely used in different engineering patterns,and the impeller blade wrap angle significantly impacts its performance.A numerical investigation was conducted to analyze the influence of the blade wrap angle on flow characteristics and energy distribution of a centrifugal pump evaluated as a low specific speed with a value of 69.This study investigates six impellermodels that possess varying blade wrap angles(95°,105°,115°,125°,135°,and 145°)that were created while maintaining the same volute and other geometrical characteristics.The investigation of energy loss was conducted to evaluate the values of total and entropy generation rates(TEG,EGR).The fluid-structure interaction was considered numerically using the software tools ANSYS Fluent and ANSYSWorkbench.The elastic structural dynamic equation was used to estimate the structural response,while the shear stress transport k–ωturbulence model was utilized for the fluid domain modeling.The findings suggest that the blade wrap angle has a significant influence on the efficiency of the pump.The impeller featuring a blade wrap angle of 145°exhibits higher efficiency,with a notable increase of 3.76%relative to the original model.Variations in the blade wrap angle impact the energy loss,shaft power,and pump head.The model with a 145°angle exhibited a maximum equivalent stress of 14.8MPa and a total deformation of 0.084 mm.The results provide valuable insights into the intricate flow mechanism of the centrifugal pump,particularly when considering various blade wrap angles. 展开更多
关键词 Centrifugal pump blade wrap angle entropy generation theory fluid-structure interaction hydraulic performance
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Identifying multidisciplinary problems from scientific publications based on a text generation method
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作者 Ziyan Xu Hongqi Han +2 位作者 Linna Li Junsheng Zhang Zexu Zhou 《Journal of Data and Information Science》 CSCD 2024年第3期213-237,共25页
Purpose:A text generation based multidisciplinary problem identification method is proposed,which does not rely on a large amount of data annotation.Design/methodology/approach:The proposed method first identifies the... Purpose:A text generation based multidisciplinary problem identification method is proposed,which does not rely on a large amount of data annotation.Design/methodology/approach:The proposed method first identifies the research objective types and disciplinary labels of papers using a text classification technique;second,it generates abstractive titles for each paper based on abstract and research objective types using a generative pre-trained language model;third,it extracts problem phrases from generated titles according to regular expression rules;fourth,it creates problem relation networks and identifies the same problems by exploiting a weighted community detection algorithm;finally,it identifies multidisciplinary problems based on the disciplinary labels of papers.Findings:Experiments in the“Carbon Peaking and Carbon Neutrality”field show that the proposed method can effectively identify multidisciplinary research problems.The disciplinary distribution of the identified problems is consistent with our understanding of multidisciplinary collaboration in the field.Research limitations:It is necessary to use the proposed method in other multidisciplinary fields to validate its effectiveness.Practical implications:Multidisciplinary problem identification helps to gather multidisciplinary forces to solve complex real-world problems for the governments,fund valuable multidisciplinary problems for research management authorities,and borrow ideas from other disciplines for researchers.Originality/value:This approach proposes a novel multidisciplinary problem identification method based on text generation,which identifies multidisciplinary problems based on generative abstractive titles of papers without data annotation required by standard sequence labeling techniques. 展开更多
关键词 Problem identification MULTIDISCIPLINARY Text generation Text classification
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Insight into the dynamics of non-Newtonian Carreau fluid when viscous dissipation,entropy generation,convective heating and diffusion are significant
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作者 ZHOU Shuang-shuang Muhammad Ijaz Khan +1 位作者 Sami Ullah Khan Sumaira Qayyum 《Applied Mathematics(A Journal of Chinese Universities)》 SCIE CSCD 2024年第1期34-46,共13页
The investigation endorsed the convective flow of Carreau nanofluid over a stretched surface in presence of entropy generation optimization.The novel dynamic of viscous dissipation is utilized to analyze the thermal m... The investigation endorsed the convective flow of Carreau nanofluid over a stretched surface in presence of entropy generation optimization.The novel dynamic of viscous dissipation is utilized to analyze the thermal mechanism of magnetized flow.The convective boundary assumptions are directed in order to examine the heat and mass transportation of nanofluid.The thermal concept of thermophoresis and Brownian movements has been re-called with the help of Buongiorno model.The problem formulated in dimensionless form is solved by NDSolve MATHEMATICA.The graphical analysis for parameters governed by the problem is performed with physical applications.The affiliation of entropy generation and Bejan number for different parameters is inspected in detail.The numerical data for illustrating skin friction,heat and mass transfer rate is also reported.The motion of the fluid is highest for the viscosity ratio parameter.The temperature of the fluid rises via thermal Biot number.Entropy generation rises for greater Brinkman number and diffusion parameter. 展开更多
关键词 heat generation surface reaction CNTs based nano uid stretching/shrinking sheet thermal radiation
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A Probing Model of Secret Key Generation Based on Channel Autocorrelation Function
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作者 Xia Enjun Hu Binjie Shen Qiaoqiao 《China Communications》 SCIE CSCD 2024年第6期163-175,共13页
Secret key generation(SKG)is a promising solution to the problem of wireless communications security.As the first step of SKG,channel probing affects it significantly.Although there have been some probing schemes,ther... Secret key generation(SKG)is a promising solution to the problem of wireless communications security.As the first step of SKG,channel probing affects it significantly.Although there have been some probing schemes,there is a lack of research on the optimization of the probing process.This study investigates how to optimize correlated parameters to maximize the SKG rate(SKGR)in the time-division duplex(TDD)mode.First,we build a probing model which includes the effects of transmitting power,the probing period,and the dimension of sample vectors.Based on the model,the analytical expression of the SKGR is given.Next,we formulate an optimization problem for maximizing the SKGR and give an algorithm to solve it.We conclude the SKGR monotonically increases as the transmitting power increases.Relevant mathematical proofs are given in this study.From the simulation results,increasing appropriately the probing period and the dimension of the sample vector could increase the SKGR dramatically compared to a yardstick,which indicates the importance of optimizing the parameters related to the channel probing phase. 展开更多
关键词 channel autocorrelation function channel probing optimization problem physical layer security secret key generation
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