In the face of global warming and increasing impervious surfaces,quantifying the change of climate potential productivity(CPP)is of great significance for the food production planning.Targeting the Dongting Lake Basin...In the face of global warming and increasing impervious surfaces,quantifying the change of climate potential productivity(CPP)is of great significance for the food production planning.Targeting the Dongting Lake Basin,which is a key area for food production in China,this paper uses meteorological data,as well as Climate Change Initiative Land Cover,and Shuttle Radar Topography Mission digital elevation model to investigate the CPP and its changes from 2000 to 2020.The suitability of land for cultivation(SLC),and the land use/land cover change(LUCC)are also considered.The results showed that the CPP varied from 9,825 to 20,895 kg ha^(-1).Even though the newly added impervious surfaces indirectly resulted in the decrease of CPP by of 9.81×10~8 kg,overall,the CPP increased at an average rate of 83.7 kg ha^(-1)a^(-1).Global warming is the strongest driver behind CPP increase,and CPP has played an important role in the conversions between cultivated land and other land types.The structure of land types tends to be optimized against this challenge.展开更多
Background: Nitrogen(N) deposition affects soil greenhouse gas(GHG) emissions, while biochar application reduces GHG emissions in agricultural soils. However, it remains unclear whether biochar amendment can alleviate...Background: Nitrogen(N) deposition affects soil greenhouse gas(GHG) emissions, while biochar application reduces GHG emissions in agricultural soils. However, it remains unclear whether biochar amendment can alleviate the promoting effects of N input on GHG emissions in forest soils. Here, we quantify the separate and combined effects of biochar amendment(0, 20, and 40 t·ha) and N addition(0, 30, 60, and 90 kg N·ha·yr) on soil GHG fluxes in a long-term field experiment at a Moso bamboo(Phyllostachys edulis) plantation.Results: Low and moderate N inputs(≤60 kg N·ha·yr) significantly increase mean annual soil carbon dioxide(CO) and nitrous oxide(NO) emissions by 17.0%–25.4% and 29.8%–31.2%, respectively, while decreasing methane(CH) uptake by 12.4%–15.9%, leading to increases in the global warming potential(GWP) of soil CHand NO fluxes by 32.4%–44.0%. Moreover, N addition reduces soil organic carbon(C;SOC) storage by 0.2%–6.5%. Compared to the control treatment, biochar amendment increases mean annual soil CO2emissions, CHuptake, and SOC storage by 18.4%–25.4%, 7.6%–15.8%, and 7.1%–13.4%, respectively, while decreasing NO emissions by 17.6%–19.2%, leading to a GWP decrease of 18.4%–21.4%. Biochar amendments significantly enhance the promoting effects of N addition on soil COemissions, while substantially offsetting the promotion of N2O emissions, inhibition of CHuptake, and decreased SOC storage, resulting in a GWP decrease of 9.1%–30.3%.Additionally, soil COand CHfluxes are significantly and positively correlated with soil microbial biomass C(MBC) and pH. Meanwhile, NO emissions have a significant and positive correlation with soil MBC and a negative correlation with pH.Conclusions: Biochar amendment can increase SOC storage and offset the enhanced GWP mediated by elevated N deposition and is, thus, a potential strategy for increasing soil C sinks and decreasing GWPs of soil CHand NO under increasing atmospheric N deposition in Moso bamboo plantations.展开更多
Potential natural vegetation(PNV)is a valuable reference for ecosystem renovation and has garnered increasing attention worldwide.However,there is limited knowledge on the spatio-temporal distributions,transitional pr...Potential natural vegetation(PNV)is a valuable reference for ecosystem renovation and has garnered increasing attention worldwide.However,there is limited knowledge on the spatio-temporal distributions,transitional processes,and underlying mechanisms of global natural vegetation,particularly in the case of ongoing climate warming.In this study,we visualize the spatio-temporal pattern and inter-transition procedure of global PNV,analyse the shifting distances and directions of global PNV under the influence of climatic disturbance,and explore the mechanisms of global PNV in response to temperature and precipitation fluctuations.To achieve this,we utilize meteorological data,mainly temperature and precipitation,from six phases:the Last Inter-Glacial(LIG),the Last Glacial Maximum(LGM),the Mid Holocene(MH),the Present Day(PD),2030(20212040)and 2090(2081–2100),and employ a widely-accepted comprehensive and sequential classification sy–stem(CSCS)for global PNV classification.We find that the spatial patterns of five PNV groups(forest,shrubland,savanna,grassland and tundra)generally align with their respective ecotopes,although their distributions have shifted due to fluctuating temperature and precipitation.Notably,we observe an unexpected transition between tundra and savanna despite their geographical distance.The shifts in distance and direction of five PNV groups are mainly driven by temperature and precipitation,although there is heterogeneity among these shifts for each group.Indeed,the heterogeneity observed among different global PNV groups suggests that they may possess varying capacities to adjust to and withstand the impacts of changing climate.The spatio-temporal distributions,mutual transitions and shift tendencies of global PNV and its underlying mechanism in face of changing climate,as revealed in this study,can significantly contribute to the development of strategies for mitigating warming and promoting re-vegetation in degraded regions worldwide.展开更多
Tropical cyclone heat potential （TCHP） in the ocean can affect tropical cyclone intensity and intensification. In this paper, TCHP change under global warming is presented based on 35 models from CMIP5 （Coupled Mod...Tropical cyclone heat potential （TCHP） in the ocean can affect tropical cyclone intensity and intensification. In this paper, TCHP change under global warming is presented based on 35 models from CMIP5 （Coupled Model Intercomparison Project, Phase 5）. As the upper ocean warms up, the TCHP of the global ocean is projected to increase by 140.6% in the 21st century under the RCP4.5 （＋4.5 W m 2 Representative Concentration Pathway） scenario, The increase is particularly significant in the western Pacific, northwestern Indian and western tropical Atlantic oceans. The increase of TCHP results from the ocean temperature warming above the depth of the 26~C isotherm （D26）, the deepening of D26, and the horizontal area expansion of SST above 26~C. Their contributions are 69.4%, 22.5% and 8.1%, respectively. Further, a suite of numerical experiments with an Ocean General Circulation Model （OGCM） is conducted to investigate the relative importance of wind stress and buoyancy forcing to the TCHP change under global warming. Results show that sea surface warming is the dominant forcing for the TCHP change, while wind stress and sea surface salinity change are secondary.展开更多
Perfluorocarbon gas is widely used in the semiconductor industry.However,perfluorocarbon has a negative effect on the global environment owing to its high global warming potential(GWP) value.An alternative solution is...Perfluorocarbon gas is widely used in the semiconductor industry.However,perfluorocarbon has a negative effect on the global environment owing to its high global warming potential(GWP) value.An alternative solution is essential.Therefore,we evaluated the possibility of replacing conventional perfluorocarbon etching gases such as CHF_3 with C_6F_(12)O,which has a low GWP and is in a liquid state at room temperature.In this study,silicon oxynitride(SiON) films were plasma-etched using inductively coupled CF4+C_6F_(12)O+O_2 mixed plasmas.Subsequently,the etching characteristics of the film,such as etching rate,etching profile,selectivity over Si,and photoresist,were investigated.A double Langmuir probe was used and optical emission spectroscopy was performed for plasma diagnostics.In addition,a contact angle goniometer and x-ray photoelectron spectroscope were used to confirm the change in the surface properties of the etched SiON film surface.Consequently,the etching characteristics of the C_6F_(12)O mixed plasma exhibited a lower etching rate,higher SiON/Si selectivity,lower plasma damage,and more vertical etched profiles than the conventional CHF_3 mixed plasma.In addition,the C_6F_(12)O gas can be recovered in the liquid state,thereby decreasing global warming.These results confirmed that the C_6F_(12)O precursor can sufficiently replace the conventional etching gas.展开更多
Unanticipated sabotage of two underwater pipelines in the Baltic Sea(Nord Stream 1 and 2)happened on 26September 2022.Massive quantities of natural gas,primarily methane,were released into the atmosphere,which lasted ...Unanticipated sabotage of two underwater pipelines in the Baltic Sea(Nord Stream 1 and 2)happened on 26September 2022.Massive quantities of natural gas,primarily methane,were released into the atmosphere,which lasted for about one week.As a more powerful greenhouse gas than CO_(2),the potential climatic impact of methane is a global concern.Using multiple methods and datasets,a recent study reported a relatively accurate magnitude of the leaked methane at 0.22±0.03 million tons(Mt),which was lower than the initial estimate in the immediate aftermath of the event.Under an energy conservation framework used in IPCC AR6,we derived a negligible increase in global surface air temperature of 1.8×10^(-5)℃ in a 20-year time horizon caused by the methane leaks with an upper limit of 0.25 Mt.Although the resultant warming from this methane leak incident was minor,future carbon release from additional Earth system feedbacks,such as thawing permafrost,and its impact on the methane mitigation pathways of the Paris Agreement,warrants investigation.展开更多
为探求温室番茄节水减排优产的灌溉模式,以番茄(金鹏8号)为研究对象,设置I1和I2(对应作物-皿系数kcp为0.8和1.0)2个灌水水平,F1和F2(对应施氮量180 kg/hm^(2)和240 kg/hm^(2))2个施氮水平,A1、A2和CK(1倍和2倍文丘里加气量,不加气CK作...为探求温室番茄节水减排优产的灌溉模式,以番茄(金鹏8号)为研究对象,设置I1和I2(对应作物-皿系数kcp为0.8和1.0)2个灌水水平,F1和F2(对应施氮量180 kg/hm^(2)和240 kg/hm^(2))2个施氮水平,A1、A2和CK(1倍和2倍文丘里加气量,不加气CK作为对照处理)3个加气水平,采用3因素完全随机设计,共10个处理,每个处理重复3次,采用静态暗箱-气相色谱法对番茄全生育期温室气体排放进行监测分析,探究土壤CO_(2)、N_(2)O、CH_(4)排放与番茄产量的变化规律;分析灌水水平、施氮水平和加气水平对温室番茄产量和温室气体排放的影响,综合全球净增温潜势(Net global warming potential,NGWP)和温室气体排放强度(Greenhouse gas intensity,GHGI),提出以节水减排高产为目标的温室番茄水肥气一体化滴灌管理模式。结果表明:灌溉水平和施氮水平增大均会增加土壤CO_(2)、N_(2)O排放通量,I2处理较I1处理平均增加24.8%(P<0.05)与14.8%(P>0.05),F2处理比F1处理平均增加8.6%(P>0.05)与34.9%(P<0.05);加气灌溉对土壤CO_(2)、N_(2)O排放通量有显著影响,与CK处理相比,A1和A2处理分别平均增加5.5%、10.0%(P>0.05)和20.9%、62.9%(P<0.05)。番茄全生育期内土壤CH4排放通量呈现土壤为CH4的汇,灌水水平增大会增加土壤CH4排放通量,而施氮水平增加则会减小CH4排放通量,I2处理比I1处理平均增加27.8%(P<0.05),F2处理比F1处理平均减少25.5%(P<0.05);加气、施氮和灌水会显著增加番茄产量(P<0.05)。综合考虑经济因素和生态因素,A1F2I1处理效益最佳,即加气水平A1、施氮水平F2、灌水水平I1的组合策略可以兼顾节水优产减排要求,为西北地区温室番茄较优灌溉模式。展开更多
The significant increase in the demand for biomass waste treatment after garbage classification has led to housefly larvae treatment becoming an attractive treatment option.It can provide a source of protein while tre...The significant increase in the demand for biomass waste treatment after garbage classification has led to housefly larvae treatment becoming an attractive treatment option.It can provide a source of protein while treating biomass waste,which means that nutrients can be returned to the natural food chain.However,the performance of this technology in terms of its environmental impacts is still unclear,particularly with regards to global warming potential(GWP).This study used a life cycle assessment(LCA)approach to assess a housefly larvae treatment plant with a treatment capacity of 50 tons of biomass waste per day.The LCA results showed that the 95% confidence intervals for the GWP in summer and winter were determined to be 24.46-32.81 kg CO_(2) equivalent(CO_(2)-eq)/ton biomass waste and5.37-10.08 kg CO_(2)-eq/ton biomass waste,respectively.The greater GWP value in summer is due to the longer ventilation time and higher ventilation intensity in summer,which consumes more power.The main GWP contributions are from(1)electricity needs(accounting for 78.6% of emissions in summer and 70.2%in winter)and(2)product substitution by mature housefly larvae and compost(both summer and winter accounting for 96.8% of carbon reduction).展开更多
基金funded by the National Natural Science Foundation of China(Grant No.72174211)the Natural Science Foundation of Hunan Province(Grant No.2023JJ30693)。
文摘In the face of global warming and increasing impervious surfaces,quantifying the change of climate potential productivity(CPP)is of great significance for the food production planning.Targeting the Dongting Lake Basin,which is a key area for food production in China,this paper uses meteorological data,as well as Climate Change Initiative Land Cover,and Shuttle Radar Topography Mission digital elevation model to investigate the CPP and its changes from 2000 to 2020.The suitability of land for cultivation(SLC),and the land use/land cover change(LUCC)are also considered.The results showed that the CPP varied from 9,825 to 20,895 kg ha^(-1).Even though the newly added impervious surfaces indirectly resulted in the decrease of CPP by of 9.81×10~8 kg,overall,the CPP increased at an average rate of 83.7 kg ha^(-1)a^(-1).Global warming is the strongest driver behind CPP increase,and CPP has played an important role in the conversions between cultivated land and other land types.The structure of land types tends to be optimized against this challenge.
基金sponsored by the National Natural Science Foundation of China,China(Grant Nos.31470529,32125027)Zhejiang A&F University Research and Development Fund,China(Nos.2022LFR006,2021LFR060).
文摘Background: Nitrogen(N) deposition affects soil greenhouse gas(GHG) emissions, while biochar application reduces GHG emissions in agricultural soils. However, it remains unclear whether biochar amendment can alleviate the promoting effects of N input on GHG emissions in forest soils. Here, we quantify the separate and combined effects of biochar amendment(0, 20, and 40 t·ha) and N addition(0, 30, 60, and 90 kg N·ha·yr) on soil GHG fluxes in a long-term field experiment at a Moso bamboo(Phyllostachys edulis) plantation.Results: Low and moderate N inputs(≤60 kg N·ha·yr) significantly increase mean annual soil carbon dioxide(CO) and nitrous oxide(NO) emissions by 17.0%–25.4% and 29.8%–31.2%, respectively, while decreasing methane(CH) uptake by 12.4%–15.9%, leading to increases in the global warming potential(GWP) of soil CHand NO fluxes by 32.4%–44.0%. Moreover, N addition reduces soil organic carbon(C;SOC) storage by 0.2%–6.5%. Compared to the control treatment, biochar amendment increases mean annual soil CO2emissions, CHuptake, and SOC storage by 18.4%–25.4%, 7.6%–15.8%, and 7.1%–13.4%, respectively, while decreasing NO emissions by 17.6%–19.2%, leading to a GWP decrease of 18.4%–21.4%. Biochar amendments significantly enhance the promoting effects of N addition on soil COemissions, while substantially offsetting the promotion of N2O emissions, inhibition of CHuptake, and decreased SOC storage, resulting in a GWP decrease of 9.1%–30.3%.Additionally, soil COand CHfluxes are significantly and positively correlated with soil microbial biomass C(MBC) and pH. Meanwhile, NO emissions have a significant and positive correlation with soil MBC and a negative correlation with pH.Conclusions: Biochar amendment can increase SOC storage and offset the enhanced GWP mediated by elevated N deposition and is, thus, a potential strategy for increasing soil C sinks and decreasing GWPs of soil CHand NO under increasing atmospheric N deposition in Moso bamboo plantations.
基金funded by the National Natural Science Foundation of China(grants No.30960264,31160475 and 42071258)Open Research Fund of TPESER(grant No.TPESER202208)+2 种基金Special Fund for Basic Scientific Research of Central Colleges,Chang’an University,China(grant No.300102353501)Natural Science Foundation of Gansu Province,China(grant No.22JR5RA857)Higher Education Novel Foundation of Gansu Province,China(grant No.2021B-130)。
文摘Potential natural vegetation(PNV)is a valuable reference for ecosystem renovation and has garnered increasing attention worldwide.However,there is limited knowledge on the spatio-temporal distributions,transitional processes,and underlying mechanisms of global natural vegetation,particularly in the case of ongoing climate warming.In this study,we visualize the spatio-temporal pattern and inter-transition procedure of global PNV,analyse the shifting distances and directions of global PNV under the influence of climatic disturbance,and explore the mechanisms of global PNV in response to temperature and precipitation fluctuations.To achieve this,we utilize meteorological data,mainly temperature and precipitation,from six phases:the Last Inter-Glacial(LIG),the Last Glacial Maximum(LGM),the Mid Holocene(MH),the Present Day(PD),2030(20212040)and 2090(2081–2100),and employ a widely-accepted comprehensive and sequential classification sy–stem(CSCS)for global PNV classification.We find that the spatial patterns of five PNV groups(forest,shrubland,savanna,grassland and tundra)generally align with their respective ecotopes,although their distributions have shifted due to fluctuating temperature and precipitation.Notably,we observe an unexpected transition between tundra and savanna despite their geographical distance.The shifts in distance and direction of five PNV groups are mainly driven by temperature and precipitation,although there is heterogeneity among these shifts for each group.Indeed,the heterogeneity observed among different global PNV groups suggests that they may possess varying capacities to adjust to and withstand the impacts of changing climate.The spatio-temporal distributions,mutual transitions and shift tendencies of global PNV and its underlying mechanism in face of changing climate,as revealed in this study,can significantly contribute to the development of strategies for mitigating warming and promoting re-vegetation in degraded regions worldwide.
基金supported by the National Basic Research Program of China (Grant No. 2012CB 955601)the National Natural Science Foundation of China (Grant Nos. 41206021 and 41125019)the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDA11010103)
文摘Tropical cyclone heat potential （TCHP） in the ocean can affect tropical cyclone intensity and intensification. In this paper, TCHP change under global warming is presented based on 35 models from CMIP5 （Coupled Model Intercomparison Project, Phase 5）. As the upper ocean warms up, the TCHP of the global ocean is projected to increase by 140.6% in the 21st century under the RCP4.5 （＋4.5 W m 2 Representative Concentration Pathway） scenario, The increase is particularly significant in the western Pacific, northwestern Indian and western tropical Atlantic oceans. The increase of TCHP results from the ocean temperature warming above the depth of the 26~C isotherm （D26）, the deepening of D26, and the horizontal area expansion of SST above 26~C. Their contributions are 69.4%, 22.5% and 8.1%, respectively. Further, a suite of numerical experiments with an Ocean General Circulation Model （OGCM） is conducted to investigate the relative importance of wind stress and buoyancy forcing to the TCHP change under global warming. Results show that sea surface warming is the dominant forcing for the TCHP change, while wind stress and sea surface salinity change are secondary.
基金supported by the Korea Institute of Energy Technology Evaluation and Planning (KETEP)the Ministry of Trade, Industry & Energy (MOTIE) of the Republic of Korea (No. 20172010105910)。
文摘Perfluorocarbon gas is widely used in the semiconductor industry.However,perfluorocarbon has a negative effect on the global environment owing to its high global warming potential(GWP) value.An alternative solution is essential.Therefore,we evaluated the possibility of replacing conventional perfluorocarbon etching gases such as CHF_3 with C_6F_(12)O,which has a low GWP and is in a liquid state at room temperature.In this study,silicon oxynitride(SiON) films were plasma-etched using inductively coupled CF4+C_6F_(12)O+O_2 mixed plasmas.Subsequently,the etching characteristics of the film,such as etching rate,etching profile,selectivity over Si,and photoresist,were investigated.A double Langmuir probe was used and optical emission spectroscopy was performed for plasma diagnostics.In addition,a contact angle goniometer and x-ray photoelectron spectroscope were used to confirm the change in the surface properties of the etched SiON film surface.Consequently,the etching characteristics of the C_6F_(12)O mixed plasma exhibited a lower etching rate,higher SiON/Si selectivity,lower plasma damage,and more vertical etched profiles than the conventional CHF_3 mixed plasma.In addition,the C_6F_(12)O gas can be recovered in the liquid state,thereby decreasing global warming.These results confirmed that the C_6F_(12)O precursor can sufficiently replace the conventional etching gas.
基金supported by the National Key Research and Development Program(Grant No.2017YFA0603503)the National Natural Science Foundation of China(Grant No.41605057)。
文摘Unanticipated sabotage of two underwater pipelines in the Baltic Sea(Nord Stream 1 and 2)happened on 26September 2022.Massive quantities of natural gas,primarily methane,were released into the atmosphere,which lasted for about one week.As a more powerful greenhouse gas than CO_(2),the potential climatic impact of methane is a global concern.Using multiple methods and datasets,a recent study reported a relatively accurate magnitude of the leaked methane at 0.22±0.03 million tons(Mt),which was lower than the initial estimate in the immediate aftermath of the event.Under an energy conservation framework used in IPCC AR6,we derived a negligible increase in global surface air temperature of 1.8×10^(-5)℃ in a 20-year time horizon caused by the methane leaks with an upper limit of 0.25 Mt.Although the resultant warming from this methane leak incident was minor,future carbon release from additional Earth system feedbacks,such as thawing permafrost,and its impact on the methane mitigation pathways of the Paris Agreement,warrants investigation.
文摘为探求温室番茄节水减排优产的灌溉模式,以番茄(金鹏8号)为研究对象,设置I1和I2(对应作物-皿系数kcp为0.8和1.0)2个灌水水平,F1和F2(对应施氮量180 kg/hm^(2)和240 kg/hm^(2))2个施氮水平,A1、A2和CK(1倍和2倍文丘里加气量,不加气CK作为对照处理)3个加气水平,采用3因素完全随机设计,共10个处理,每个处理重复3次,采用静态暗箱-气相色谱法对番茄全生育期温室气体排放进行监测分析,探究土壤CO_(2)、N_(2)O、CH_(4)排放与番茄产量的变化规律;分析灌水水平、施氮水平和加气水平对温室番茄产量和温室气体排放的影响,综合全球净增温潜势(Net global warming potential,NGWP)和温室气体排放强度(Greenhouse gas intensity,GHGI),提出以节水减排高产为目标的温室番茄水肥气一体化滴灌管理模式。结果表明:灌溉水平和施氮水平增大均会增加土壤CO_(2)、N_(2)O排放通量,I2处理较I1处理平均增加24.8%(P<0.05)与14.8%(P>0.05),F2处理比F1处理平均增加8.6%(P>0.05)与34.9%(P<0.05);加气灌溉对土壤CO_(2)、N_(2)O排放通量有显著影响,与CK处理相比,A1和A2处理分别平均增加5.5%、10.0%(P>0.05)和20.9%、62.9%(P<0.05)。番茄全生育期内土壤CH4排放通量呈现土壤为CH4的汇,灌水水平增大会增加土壤CH4排放通量,而施氮水平增加则会减小CH4排放通量,I2处理比I1处理平均增加27.8%(P<0.05),F2处理比F1处理平均减少25.5%(P<0.05);加气、施氮和灌水会显著增加番茄产量(P<0.05)。综合考虑经济因素和生态因素,A1F2I1处理效益最佳,即加气水平A1、施氮水平F2、灌水水平I1的组合策略可以兼顾节水优产减排要求,为西北地区温室番茄较优灌溉模式。
基金supported by the National Key Research and Development Program of China(No.2018YFD1100600)Shanghai Municipal Government State-Owned Assets Supervision and Administration Commission(No.2022028)。
文摘The significant increase in the demand for biomass waste treatment after garbage classification has led to housefly larvae treatment becoming an attractive treatment option.It can provide a source of protein while treating biomass waste,which means that nutrients can be returned to the natural food chain.However,the performance of this technology in terms of its environmental impacts is still unclear,particularly with regards to global warming potential(GWP).This study used a life cycle assessment(LCA)approach to assess a housefly larvae treatment plant with a treatment capacity of 50 tons of biomass waste per day.The LCA results showed that the 95% confidence intervals for the GWP in summer and winter were determined to be 24.46-32.81 kg CO_(2) equivalent(CO_(2)-eq)/ton biomass waste and5.37-10.08 kg CO_(2)-eq/ton biomass waste,respectively.The greater GWP value in summer is due to the longer ventilation time and higher ventilation intensity in summer,which consumes more power.The main GWP contributions are from(1)electricity needs(accounting for 78.6% of emissions in summer and 70.2%in winter)and(2)product substitution by mature housefly larvae and compost(both summer and winter accounting for 96.8% of carbon reduction).
