Quantification of regulated and emerging disinfection byproducts (DBPs) in swimming pool water,as well as the assessment of their lifetime health risk are limited in China.In this study,the occurrence of regulated DBP...Quantification of regulated and emerging disinfection byproducts (DBPs) in swimming pool water,as well as the assessment of their lifetime health risk are limited in China.In this study,the occurrence of regulated DBPs (e.g.,trihalomethanes,haloacetic acids) and emerging DBPs (e.g.,haloacetonitriles,haloacetaldehydes) in indoor swimming pool water and the corresponding source water at a city in Eastern China were determined.The concentrations of DBPs in swimming pool water were 1-2 orders of magnitude higher than that in source water.Lifetime cancer and non-cancer risks of DBPs stemming from swimming pool water were also estimated.Inhalation and dermal exposure were the most significant exposure routes related to swimming pool DBP cancer and non-cancer risks.For the first time,buccal and aural exposure were considered,and were proven to be important routes of DBP exposure (accounting for 17.9%-38.9%of total risk).The cancer risks of DBPs for all swimmers were higher than 10^(-6)of lifetime exposure risk recommended by United States Environmental Protection Agency,and the competitive adult swimmers experienced the highest cancer risk (7.82×10^(-5)).These findings provide important information and perspectives for future efforts to lower the health risks associated with exposure to DBPs in swimming pool water.展开更多
基金supported by the National Natural Science Foundation of China (Nos.52170009,52091542)the National Key Research and Development Program of China (No.2021YFC_(3)200702)+3 种基金the Program of Shanghai Academic Research Leader,China (No.21XD1424000)the International Cooperation Project of Shanghai Science and Technology Commission (No.20230714100)the Key Research and Development Program of Guangdong Province (No.2020B1111350001)the Tongji University Youth 100 Program。
文摘Quantification of regulated and emerging disinfection byproducts (DBPs) in swimming pool water,as well as the assessment of their lifetime health risk are limited in China.In this study,the occurrence of regulated DBPs (e.g.,trihalomethanes,haloacetic acids) and emerging DBPs (e.g.,haloacetonitriles,haloacetaldehydes) in indoor swimming pool water and the corresponding source water at a city in Eastern China were determined.The concentrations of DBPs in swimming pool water were 1-2 orders of magnitude higher than that in source water.Lifetime cancer and non-cancer risks of DBPs stemming from swimming pool water were also estimated.Inhalation and dermal exposure were the most significant exposure routes related to swimming pool DBP cancer and non-cancer risks.For the first time,buccal and aural exposure were considered,and were proven to be important routes of DBP exposure (accounting for 17.9%-38.9%of total risk).The cancer risks of DBPs for all swimmers were higher than 10^(-6)of lifetime exposure risk recommended by United States Environmental Protection Agency,and the competitive adult swimmers experienced the highest cancer risk (7.82×10^(-5)).These findings provide important information and perspectives for future efforts to lower the health risks associated with exposure to DBPs in swimming pool water.
