Exploration of High-Harmonic Generation from the CS2 Molecule by the Lewenstein Method in Two-Color Circularly Polarized Laser Field

The high harmonic generation(HHG) from the CS_2 molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS_2 molecule,which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover,an isolated 110 as pulse can be obtained by superposing the harmonics from 130 th to 180 th order.

Distinguishing high-harmonic generation from surface and bulk states in topological insulator Bi_(2)Se_(3)

We demonstrated a scheme to differentiate the high-harmonic generation[HHG)originating from the surface states and bulk states of the topological insulator Bi_(2)Se_(3).By adopting two-color mid-infrared laser fields on Bi_(2)Se_(3),we found that the nonlinear response sensitively depends on the relative phase of the driving fields.The even harmonics arise from the surface states with a clear signature,whose modulation period equals the cycle of the second-harmonic generation[SHG]field.We reveal that the weak SHG perturbs the nontrivial dipole phase of the electron-hole pair in surface states,and thus leads to the modulation of HHG.It provides a means to manipulate the ultrafast dynamics in surface states through adopting a weak perturbing laser field.

Even-order high-harmonic generation from solids in velocity gauge

We present a velocity-gauge model for the generation of even-order high harmonics, and reveal that the even-order harmonics originate from the multiple-step transitions among the energy bands in momentum space, while the odd-order harmonics are mainly from direct transitions. The lower valence band is found vital for the generation of even harmonics. Relative intensity of even-order harmonics versus the odd orders is calculated and shows a growing trend as the laser field amplitude increases.

Wave mixing and high-harmonic generation enhancement by a two-color field driven dielectric metasurface[Invited]

High-harmonic generation in metasurfaces,driven by strong laser fields,has been widely studied.Compared to plasma,all-dielectric nanoscale metasurfaces possess larger nonlinearity response and higher damage threshold.Additionally,it can strongly localize the driven field,greatly enhancing its peak amplitude.In this work,we adopt a Fano resonant micronano structure with transmission peaks at different wavelengths and explore its nonlinear response by both single and twocolor pump fields.Compared to the high-order harmonics induced by the first resonant wavelength,the intensity of the high-harmonic radiation results is enhanced by one order of magnitude,when the metasurface is driven by various resonant and non-resonant wavelength combinations of a two-color field.

High-Harmonic Generation and Correlated Electron Emission from Relativistic Plasma Mirrors at 1 kHz Repetition Rate

We report evidence for the first generation of XUV spectra from relativistic surface high-harmonic generation(SHHG)on plasma mirrors at a kilohertz repetition rate,emitted simultaneously with energetic electrons.SHHG spectra and electron angular distributions are measured as a function of the experimentally controlled plasma density gradient scale length Lg for three increasingly short and intense driving pulses:24 fs and a0=1:1,8 fs and a0=1:6,and finally 4 fs and a0≈2:1,where a0 is the peak vector potential normalized by mec/e with the elementary charge e,the electron rest mass me,and the vacuum light velocity c.For all driver pulses,we observe correlated relativistic SHHG and electron emission in the range Lg∈½λ/20,λ/4,with an optimum gradient scale length of Lg≈λ/10.This universal optimal Lg-range is rationalized by deriving a direct intensity-independent link between the scale length Lg and an effective similarity parameter for relativistic laser-plasma interactions.

Development of a control system for the fourth-harmonic cavity of the HLS storage ring

Harmonic RF cavities are commonly used in storage rings to lengthen the bunches and thus suppress the beam's instabilities and increase its Touschek lifetime. The voltage and phase of the electromagnetic fields in the harmonic cavity are of great importance for stretching the bunch. In the Hefei Light Source storage ring, a passive fourth-harmonic cavity is installed, and the cavity is monitored and controlled by an analog control module provided by its manufacturer. To vary and maintain the voltage of the harmonic cavity in a more effective way, a digital proportional, integral, and derivative feedback system based on the Experimental Physics and Industrial Control System is developed on top of the analog control module. This paper reports the details of the development of this voltage control system. Some test and operational results are also presented.

High harmonic generation driven by twocolor relativistic circularly polarized laser pulses at various frequency ratios

High harmonic generation(HHG)by two-color counter-rotating relativistic laser pulses with arbitrary frequency ratio is investigated through particle-in-cell simulations.It is shown that the dichromatic laser driver at various frequency ratios can effectively produce high-order harmonics with different spectral features.A general selection rule of this extended scheme can be obtained and the corresponding harmonic helicity can be identified through a simple analytical model based on a relativistic oscillating mirror.Thus,the results in this paper may offer new opportunities for arbitrary spectral control of generated harmonics,which is of significance for diverse potential applications in practice.

Attosecond probing and control of charge migration in carbon-chain molecule

In quantum mechanics,when an electron is quickly ripped off from a molecule,a superposition of new eigenstates of the cation creates an electron wave packet that governs the charge flow inside,which has been called charge migration(CM).Experimentally,extracting such dynamics at its natural(attosecond)timescale is quite difficult.We report the first such experiment in a linear carbon-chain molecule,butadiyne(C_(4)H_(2)),via high-harmonic spectroscopy(HHS).By employing advanced theoretical and computational tools,we showed that the wave packet and the CM of a single molecule are reconstructed from the harmonic spectra for each fixed-in-space angle of the molecule.For this onedimensional molecule,we calculate the center of charge <x>(t) to obtain v_(cm),to quantify the migration speed and how it depends on the orientation angle.The findings also uncover how the electron dynamics at the first few tens to hundreds of attoseconds depends on molecular structure.The method can be extended to other molecules where the HHS technique can be employed.

Lensless diffractive imaging with ultra-broadbandtable-top sources: from infrared to extreme-ultravioletwavelengths

Lensless imaging is an approach to microscopy in which a high-resolution image of an object is reconstructed from one or more measured diffraction patterns,providing a solution in situations where the use of imaging optics is not possible.However,current lensless imaging methods are typically limited by the need for a light source with a narrow,stable and accurately known spectrum.We have developed a general approach to lensless imaging without spectral bandwidth limitations or sample requirements.We use two time-delayed coherent light pulses and show that scanning the pulse-to-pulse time delay allows the reconstruction of diffraction-limited images for all the spectral components in the pulse.In addition,we introduce an iterative phase retrieval algorithm that uses these spectrally resolved Fresnel diffraction patterns to obtain high-resolution images of complex extended objects.We demonstrate this two-pulse imaging method with octave-spanning visible light sources,in both transmission and reflection geometries,and with broadband extreme-ultraviolet radiation from a high-harmonic generation source.Our approach enables effective use of low-flux ultra-broadband sources,such as table-top high-harmonic generation systems,for high-resolution imaging.