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Three-dimensional isotropic microfabrication in glass using spatiotemporal focusing of high-repetition-rate femtosecond laser pulses 被引量:1
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作者 Yuanxin Tan Haotian Lv +10 位作者 Jian Xu Aodong Zhang Yunpeng Song Jianping Yu Wei Chen Yuexin Wan Zhaoxiang Liu Zhaohui Liu Jia Qi Yangjian Cai Ya Cheng 《Opto-Electronic Advances》 SCIE EI CAS CSCD 2023年第10期18-29,共12页
To improve the processing efficiency and extend the tuning range of 3D isotropic fabrication,we apply the simultaneous spatiotemporal focusing(SSTF)technique to a high-repetition-rate femtosecond(fs)fiber laser system... To improve the processing efficiency and extend the tuning range of 3D isotropic fabrication,we apply the simultaneous spatiotemporal focusing(SSTF)technique to a high-repetition-rate femtosecond(fs)fiber laser system.In the SSTF scheme,we propose a pulse compensation scheme for the fiber laser with a narrow spectral bandwidth by building an extra-cavity pulse stretcher.We further demonstrate truly 3D isotropic microfabrication in photosensitive glass with a tunable resolution ranging from 8μm to 22μm using the SSTF of fs laser pulses.Moreover,we systematically investigate the influences of pulse energy,writing speed,processing depth,and spherical aberration on the fabrication resolution.As a proof-of-concept demonstration,the SSTF scheme was further employed for the fs laser-assisted etching of complicated glass microfluidic structures with 3D uniform sizes.The developed technique can be extended to many applications such as advanced photonics,3D biomimetic printing,micro-electromechanical systems,and lab-on-a-chips. 展开更多
关键词 simultaneous spatiotemporal focusing technique pulse compensation pulse stretcher 3D isotropic fabrication chemical etching
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基于PULSE Labshop的双通道测量航空噪声方法研究
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作者 张青 蒋思毅 +1 位作者 闫国华 杨晓军 《科技与创新》 2024年第14期31-34,共4页
根据《航空器型号和适航合格审定噪声规定》(CCAR-36)中噪声测量规范,使用PULSE Labshop噪声振动测量仪进行双通道法测量航空噪声。针对PLUSE系统从硬件、软件2个方面进行了研究和分析,可为后续的多通道测量振动、噪声的各项测试提供基... 根据《航空器型号和适航合格审定噪声规定》(CCAR-36)中噪声测量规范,使用PULSE Labshop噪声振动测量仪进行双通道法测量航空噪声。针对PLUSE系统从硬件、软件2个方面进行了研究和分析,可为后续的多通道测量振动、噪声的各项测试提供基础性的理论帮助。同时,双通道法测量航空噪声实现了试验的冗余设计,一定程度上可提高试验的准确性。 展开更多
关键词 双通道法 航空噪声 pulse系统 适航规范
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On the generation of high-quality Nyquist pulses in mode-locked fiber lasers
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作者 任俞宣 葛锦蔓 +2 位作者 李小军 彭俊松 曾和平 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第3期424-427,共4页
Nyquist pulses have wide applications in many areas,from electronics to optics.Mode-locked lasers are ideal platforms to generate such pulses.However,how to generate high-quality Nyquist pulses in mode-locked lasers r... Nyquist pulses have wide applications in many areas,from electronics to optics.Mode-locked lasers are ideal platforms to generate such pulses.However,how to generate high-quality Nyquist pulses in mode-locked lasers remains elusive.We address this problem by managing different physical effects in mode-locked fiber lasers through extensive numerical simulations.We find that net dispersion,linear loss,gain and filter shaping can affect the quality of Nyquist pulses significantly.We also demonstrate that Nyquist pulses experience similariton shaping due to the nonlinear attractor effect in the gain medium.Our work may contribute to the design of Nyquist pulse sources and enrich the understanding of pulse shaping dynamics in mode-locked lasers. 展开更多
关键词 mode locking laser SOLITON FIBER pulse
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Intense Mid-Infrared Laser Pulse Generated via Flying-Mirror Red-Shifting in Near-Critical-Density Plasmas
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作者 鲁瑜 李东澳 +2 位作者 李倩妮 邵福球 余同普 《Chinese Physics Letters》 SCIE EI CAS CSCD 2024年第2期42-46,共5页
Relativistic femtosecond mid-infrared pulses can be generated efficiently by laser interaction with near-criticaldensity plasmas.It is found theoretically and numerically that the radiation pressure of a circularly po... Relativistic femtosecond mid-infrared pulses can be generated efficiently by laser interaction with near-criticaldensity plasmas.It is found theoretically and numerically that the radiation pressure of a circularly polarized laser pulse first compresses the plasma electrons to form a dense flying mirror with a relativistic high speed.The pulse reflected by the mirror is red-shifted to the mid-infrared range.Full three-dimensional simulations demonstrate that the central wavelength of the mid-infrared pulse is tunable from 3µm to 14µm,and the laser energy conversion efficiency can reach as high as 13%.With a 0.5–10 PW incident laser pulse,the generated mid-infrared pulse reaches a peak power of 10–180 TW,which is interesting for various applications in ultrafast and high-field sciences. 展开更多
关键词 MIRROR Infrared pulse
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Electromagnetic pulses produced by a picosecond laser interacting with solid targets
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作者 牛爱慧 康宁 +5 位作者 许国潇 谢佳节 滕建 刘会亚 孙明营 李廷帅 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第5期430-436,共7页
A high-power laser ablating solid targets induces giant electromagnetic pulses(EMPs),which are intimately pertinent to laser parameters,such as energy and pulse width.In this study,we reveal the features of EMPs gener... A high-power laser ablating solid targets induces giant electromagnetic pulses(EMPs),which are intimately pertinent to laser parameters,such as energy and pulse width.In this study,we reveal the features of EMPs generated from a picosecond(ps)laser irradiating solid targets at the SG-Ⅱpicosecond petawatt(PSPW)laser facility.The laser energy and pulse,as well as target material and thickness,show determinative effects on the EMPs’amplitude.More intense EMPs are detected behind targets compared to those at the other three positions,and the EMP amplitude decreases from 90.09 kV/m to 17.8 kV/m with the gold target thickness increasing from 10μm to 20μm,which is suppressed when the laser pulse width is enlarged.The results are expected to provide more insight into EMPs produced by ps lasers coupling with targets and lay the foundation for an effective EMP shielding design in high-power laser infrastructures. 展开更多
关键词 LASER electromagnetic pulse TARGET PROTON
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Pulse rate estimation based on facial videos:an evaluation and optimization of the classical methods using both self-constructed and public datasets
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作者 Chao-Yong Wu Jian-Xin Chen +3 位作者 Yu Chen Ai-Ping Chen Lu Zhou Xu Wang 《Traditional Medicine Research》 2024年第1期14-22,共9页
Pulse rate is one of the important characteristics of traditional Chinese medicine pulse diagnosis,and it is of great significance for determining the nature of cold and heat in diseases.The prediction of pulse rate b... Pulse rate is one of the important characteristics of traditional Chinese medicine pulse diagnosis,and it is of great significance for determining the nature of cold and heat in diseases.The prediction of pulse rate based on facial video is an exciting research field for getting palpation information by observation diagnosis.However,most studies focus on optimizing the algorithm based on a small sample of participants without systematically investigating multiple influencing factors.A total of 209 participants and 2,435 facial videos,based on our self-constructed Multi-Scene Sign Dataset and the public datasets,were used to perform a multi-level and multi-factor comprehensive comparison.The effects of different datasets,blood volume pulse signal extraction algorithms,region of interests,time windows,color spaces,pulse rate calculation methods,and video recording scenes were analyzed.Furthermore,we proposed a blood volume pulse signal quality optimization strategy based on the inverse Fourier transform and an improvement strategy for pulse rate estimation based on signal-to-noise ratio threshold sliding.We found that the effects of video estimation of pulse rate in the Multi-Scene Sign Dataset and Pulse Rate Detection Dataset were better than in other datasets.Compared with Fast independent component analysis and Single Channel algorithms,chrominance-based method and plane-orthogonal-to-skin algorithms have a more vital anti-interference ability and higher robustness.The performances of the five-organs fusion area and the full-face area were better than that of single sub-regions,and the fewer motion artifacts and better lighting can improve the precision of pulse rate estimation. 展开更多
关键词 pulse rate heart rate PHOTOPLETHYSMOGRAPHY observation and pulse diagnosis facial videos
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Efficient guiding and focusing of intense laser pulse using periodic thin slits
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作者 L.Xu T.W.Huang +6 位作者 K.Jiang C.N.Wu H.Peng P.C.hen R.Li H.B.Zhuo C.T.Zhou 《Matter and Radiation at Extremes》 SCIE EI CSCD 2024年第4期29-39,共11页
Slits have been widely used in laser-plasma interactions as plasma optical components for generating high-harmonic light and controlling laser-driven particle beams.Here,we propose and demonstrate that periodic thin s... Slits have been widely used in laser-plasma interactions as plasma optical components for generating high-harmonic light and controlling laser-driven particle beams.Here,we propose and demonstrate that periodic thin slits can be regarded as a new breed of optical elements for efficient focusing and guiding of intense laser pulse.The fundamental physics of intense laser interaction with thin slits is studied,and it is revealed that relativistic effects can lead to enhanced laser focusing far beyond the pure diffractive focusing regime.In addition,the interaction of an intense laser pulse with periodic thin slits makes it feasible to achieve multifold enhancement in both laser intensity and energy transfer efficiency compared with conventional waveguides.These results provide a novel method for manipulating ultra-intense laser pulses and should be of interest for many laser-based applications. 展开更多
关键词 laser pulse INTENSE
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A study of pulsed high voltage driven hollow-cathode electron beam sources through synchronous optical trigger
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作者 霍卫杰 贺伟国 +2 位作者 韩罗峰 朱康武 王锋 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第5期82-90,共9页
In this study,a pulsed,high voltage driven hollow-cathode electron beam sources through an optical trigger is designed with characteristics of simple structure,low cost,and easy triggering.To validate the new design,t... In this study,a pulsed,high voltage driven hollow-cathode electron beam sources through an optical trigger is designed with characteristics of simple structure,low cost,and easy triggering.To validate the new design,the characteristics of hollow-cathode discharge and electron beam characterization under pulsed high voltage drive are studied experimentally and discussed by discharge characteristics and analyses of waveform details,respectively.The validation experiments indicate that the pulsed high voltage supply significantly improves the frequency and stability of the discharge,which provides a new solution for the realization of a high-frequency,high-energy electron beam source.The peak current amplitude in the high-energy electron beam increases from 6.2 A to 79.6 A,which indicates the pulsed power mode significantly improves the electron beam performance.Besides,increasing the capacitance significantly affects the highcurrent,lower-energy electron beam more than the high-energy electron beam. 展开更多
关键词 hollow-cathode nanosecond pulsed electron beam sources optical trigger pulsed high voltage supply beam current distribution
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Spatial and temporal evolution of electromagnetic pulses from solid target irradiated with multi-hundred-terawatt laser pulse inside target chamber
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作者 何强友 邓志刚 +12 位作者 张智猛 夏亚东 张博 孟令彪 贺书凯 黄华 杨雷 刘红杰 范伟 林晨 周维民 李廷帅 颜学庆 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第2期62-69,共8页
Giant electromagnetic pulses(EMPs) induced by high-power laser irradiating solid targets interfere with various experimental diagnoses and even damage equipment,so unveiling the evolution of EMPs inside the laser cham... Giant electromagnetic pulses(EMPs) induced by high-power laser irradiating solid targets interfere with various experimental diagnoses and even damage equipment,so unveiling the evolution of EMPs inside the laser chamber is crucial for designing effective EMP shielding.In this work,the transmission characteristics of EMPs as a function of distances from the target chamber center(TCC) are studied using B-dot probes.The mean EMP amplitude generated by picosecond laser-target interaction reaches 561 kV m^(-1),357 kV m^(-1),395 kV m^(-1),and 341 kV m^(-1)at 0.32 m,0.53 m,0.76 m,and 1 m from TCC,which decreases dramatically from 0.32 m to 0.53 m.However,it shows a fluctuation from 0.53 m to 1 m.The temporal features of EMPs indicate that time-domain EMP signals near the target chamber wall have a wider full width at half maximum compared to that close to TCC,mainly due to the echo oscillation of electromagnetic waves inside the target chamber based on simulation and experimentation.The conclusions of this study will provide a new approach to mitigate strong electromagnetic pulses by decreasing the echo oscillation of electromagnetic waves inside the target chamber during laser coupling with targets. 展开更多
关键词 TARGET electromagnetic pulses spatial distribution
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Electron vortices generation of photoelectron of H_(2)^(+) by counter-rotating circularly polarized attosecond pulses
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作者 杨浩婧 刘晓煜 +2 位作者 朱风筝 焦利光 刘爱华 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第1期362-367,共6页
Molecular-frame photoelectron momentum distributions(MF-PMDs) of an H_(2)^(+) molecule ion in the presence of a pair of counter-rotating circularly polarized attosecond extreme ultraviolet laser pulses is studied by n... Molecular-frame photoelectron momentum distributions(MF-PMDs) of an H_(2)^(+) molecule ion in the presence of a pair of counter-rotating circularly polarized attosecond extreme ultraviolet laser pulses is studied by numerically solving the two-dimensional time-dependent Schrodinger equation within the frozen-nuclei approximation. At small time delay, our simulations show that the electron vortex structure is sensitive to the time delay and relative phase between the counterrotating pulses when they are partially overlapped. By adjusting time delay and relative phase, we have the ability to manipulate the MF-PMDs and the appearance of spiral arms. We further show that the internuclear distance can affect the spiral vortices due to its different transition cross sections in the parallel and perpendicular geometries. The lowest-order perturbation theory is employed to interpret these phenomena qualitatively. It is concluded that the internuclear distancedependent transition cross sections and the confinement effect in diatomic molecules are responsible for the variation of vortex structures in the MF-PMDs. 展开更多
关键词 photoelectron momentum distribution attosecond pulse VORTEX
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Pulses in ground motions identified through surface partial matching and their impact on seismic rocking consequence
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作者 Tang Yuchuan Wang Jiankang Wu Gang 《Earthquake Engineering and Engineering Vibration》 SCIE EI CSCD 2024年第1期35-50,共16页
In seismology and earthquake engineering,it is fundamental to identify and characterize the pulse-like features in pulse-type ground motions.To capture the pulses that dominate structural responses,this study establis... In seismology and earthquake engineering,it is fundamental to identify and characterize the pulse-like features in pulse-type ground motions.To capture the pulses that dominate structural responses,this study establishes congruence and shift relationships between response spectrum surfaces.A similarity search between spectrum surfaces,supplemented with a similarity search in time series,has been applied to characterize the pulse-like features in pulse-type ground motions.The identified pulses are tested in predicting the rocking consequences of slender rectangular blocks under the original ground motions.Generally,the prediction is promising for the majority of the ground motions where the dominant pulse is correctly identified. 展开更多
关键词 velocity pulse ground motion surface similarity ROCKING OVERTURNING
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A Study to Observe Pulse Pressure Variation after Induction with Propofol for General Anesthesia
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作者 Kunal Tewari Vibhu Raghuvanshi +3 位作者 Deepak Mishra Nitin Pahuja Maj Jyotsna Om Bahadur Thapa 《World Journal of Cardiovascular Diseases》 CAS 2024年第5期343-350,共8页
Background and Aims: Pulse pressure variation (PPV) is a reliable and predictive dynamic parameter presently being utilized for fluid responsiveness. In the operating room, fluid administration based on PPV monitoring... Background and Aims: Pulse pressure variation (PPV) is a reliable and predictive dynamic parameter presently being utilized for fluid responsiveness. In the operating room, fluid administration based on PPV monitoring helps the physician in deciding whether to volume resuscitate or use interventions in patients undergoing surgery. Propofol is an intravenous induction agent which lowers blood pressure. There are multiple causes such as depression in cardiac output, and peripheral vasodilatation for hypotension. We undertook this study to observe the utility of PPV as a guide to fluid therapy after propofol induction. Primary outcome of our study was to monitor PPV as a marker of fluid responsiveness for the hypotension caused by propofol induction. Secondary outcome included the correlation of PPV with other hemodynamic parameters like heart rate (HR), systolic blood pressure (SBP), and diastolic blood pressure (DBP);after induction with propofol at regular interval of time. Methods: A total number of 90 patients were recruited. Either of the radial artery was then cannulated under local anaesthesia with 20G VygonLeadercath arterial cannula and invasive monitoring transduced. A baseline recording of heart rate (HR), systolic blood pressure (SBP), diastolic blood pressure (DBP) and PPV was then recorded. Patients were then induced with predetermined doses of propofol (2 mg/kg) and recordings of HR, SBP, DBP, and PPV were taken at 5, 10 and 15 minutes. Results: Intraoperatively, PPV was significantly higher at 5 minutes and significantly lower at 15 minutes after induction. It was observed that there were no statistically significant correlations between PPV and SBP or DBP. PPV was strongly and directly associated with HR. Conclusion: We were able to establish that PPV predicts fluid responsiveness in hypotension caused by propofol induction;and can be used to administer fluid therapy in managing such hypotension. However, PPV was not directly correlated with hypotension subsequent to propofol administration. 展开更多
关键词 pulse Pressure Variation (PPV) PROPOFOL Fluid Responsiveness
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A global model of intensity autocorrelation to determine laser pulse duration
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作者 彭雨菲 刘励强 +1 位作者 洪丽红 李志远 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第5期446-451,共6页
We present a new global model of collinear autocorrelation based on second harmonic generation nonlinearity.The model is rigorously derived from the nonlinear coupled wave equation specific to the autocorrelation meas... We present a new global model of collinear autocorrelation based on second harmonic generation nonlinearity.The model is rigorously derived from the nonlinear coupled wave equation specific to the autocorrelation measurement configuration,without requiring a specific form of the incident pulse function.A rigorous solution of the nonlinear coupled wave equation is obtained in the time domain and expressed in a general analytical form.The global model fully accounts for the nonlinear interaction and propagation effects within nonlinear crystals,which are not captured by the classical local model.To assess the performance of the global model compared to the classic local model,we investigate the autocorrelation signals obtained from both models for different incident pulse waveforms and different full-widthes at half-maximum(FWHMs).When the incident pulse waveform is Lorentzian with an FWHM of 200 fs,the global model predicts an autocorrelation signal FWHM of 399.9 fs,while the classic local model predicts an FWHM of 331.4 fs.The difference between the two models is 68.6 fs,corresponding to an error of 17.2%.Similarly,for a sech-type incident pulse with an FWHM of 200 fs,the global model predicts an autocorrelation signal FWHM of 343.9 fs,while the local model predicts an FWHM of 308.8 fs.The difference between the two models is 35.1 fs,with an error of 10.2%.We further examine the behavior of the models for Lorentzian pulses with FWHMs of 100 fs,200 fs and 500 fs.The differences between the global and local models are 17.1 fs,68.6 fs and 86.0 fs,respectively,with errors approximately around 17%.These comparative analyses clearly demonstrate the superior accuracy of the global model in intensity autocorrelation modeling. 展开更多
关键词 intensity autocorrelation global model ultrashort pulses pulse-width measurement
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Stable photocurrent-voltage characteristics of perovskite single crystal detectors obtained by pulsed bias
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作者 刘新 陈之龙 +4 位作者 王虎 张雯清 董昊 王鹏祥 邵宇川 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第4期209-214,共6页
Photocurrent-voltage characterization is a crucial method for assessing key parameters in x-ray or y-ray semiconductor detectors,especially the carrier mobility lifetime product.However,the high biases during photocur... Photocurrent-voltage characterization is a crucial method for assessing key parameters in x-ray or y-ray semiconductor detectors,especially the carrier mobility lifetime product.However,the high biases during photocurrent measurements tend to cause severe ion migration,which can lead to the instability and inaccuracy of the test results.Given the mixed electronic-ionic charac teristics,it is imperative to devise novel methods capable of precisely measuring photocurrentvoltage characteristics under high bias conditions,free from interference caused by ion migration.In this paper,pulsed bias is employed to explore the photocurrent-voltage characteristics of MAPbBr_(3) single crystals.The method yields stable photocurrent-voltage characteristics at a pulsed bias of up to 30 V,proving to be effective in mitigating ion migration.Through fitting the modified Hecht equation,we determined the mobility lifetime products of 1.0×10^(2) cm^(2)·V^(-1)for hole and 2.78×10~(-3)cm^(2)·V^(-1)for electron.This approach offers a promising solution for accurately measuring the transport properties of carriers in perovskite. 展开更多
关键词 perovskites ion migration pulsed bias mobility lifetime product
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Generating attosecond pulses with controllable polarization from cyclic H_(3)^(2+) molecules by bichromatic circular fields
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作者 张思琪 张冰 +2 位作者 闫博 姜向前 孙秀冬 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第2期305-310,共6页
We investigate the polarization properties of harmonics from the cyclic H_(3)^(2+) molecular ions in tailored bichromatic counter-rotating circularly polarized(BCCP)fields by solving the time-dependent Schrödinge... We investigate the polarization properties of harmonics from the cyclic H_(3)^(2+) molecular ions in tailored bichromatic counter-rotating circularly polarized(BCCP)fields by solving the time-dependent Schrödinger equation.The allowed harmonics and their helicities are associated with the symmetry compatibility of the field-target systems,and large intensity difference between adjacent harmonics with opposite helicities appears in a wide spectral range when the BCCP field is at certain rotation angles.We try to explain the intensity difference by using a recombination model based on the quantum-orbit theory and by analyzing the ionization pathways.Moreover,to synthesize attosecond pulse trains with tunable polarization,the intensity difference is manipulated by introducing a seed XUV field,and by changing the relative amplitude ratio as well as the helicity of BCCP fields. 展开更多
关键词 high-order harmonic generation attosecond pulse multi-center interference
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Model prediction of inactivation of Aeromonas salmonicida grown on poultry in situ by intense pulsed light
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作者 Jingwen Wang Zhenzhen Ning +2 位作者 Yifan Chen Xinglian Xu Huhu Wang 《Food Science and Human Wellness》 SCIE CSCD 2024年第2期1011-1017,共7页
The aim of this study was to evaluate the factors influencing the inactivation effect of intense pulsed light(IPL)on Aeromonas salmonicida grown on chicken meat and skin,and to further develop prediction models of ina... The aim of this study was to evaluate the factors influencing the inactivation effect of intense pulsed light(IPL)on Aeromonas salmonicida grown on chicken meat and skin,and to further develop prediction models of inactivation.In this work,chicken meat and skin inoculated with meat-borne A.salmonicida isolates were subjected to IPL treatments under different conditions.The results showed that IPL had obvious bactericidal effect in the chicken skin and thickness groups when the treatment voltage and time were 7 V combined with 5 s.In addition,the lethality curves of A.salmonicida were fitted under IPL conditions of 3.5-7.5 V.The comparison of statistical parameters revealed that the Weibull model could best fit the mortality curves and could accurately predict the mortality dynamic of A.salmonicida grown on chicken skin.And further a secondary model between the scale factor b and the treatment voltage in Weibull model was established using linear equations,which determined that the secondary model could accurately predict the inactivation of A.salmonicida.This study provides a theoretical basis for future prediction models of Aeromonas,and also provides new ideas for sterilization approaches of meat-borne Aeromonas. 展开更多
关键词 Aeromonas salmonicida Intense pulsed light INACTIVATION Chicken meat MODEL
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Electrokinetic-mechanism of water and furfural oxidation on pulsed laser-interlaced Cu_(2)O and CoO on nickel foam 被引量:1
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作者 Yewon Oh Jayaraman Theerthagiri +3 位作者 M.L.Aruna Kumari Ahreum Min Cheol Joo Moon Myong Yong Choi 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第4期145-154,共10页
The electrocatalytic oxidation of biomass-derived furfural(FF)feedstocks into 2-furoic acid(FA)holds immense industrial potential in optics,cosmetics,polymers,and food.Herein,we fabricated Co O/Ni O/nickel foam(NF)and... The electrocatalytic oxidation of biomass-derived furfural(FF)feedstocks into 2-furoic acid(FA)holds immense industrial potential in optics,cosmetics,polymers,and food.Herein,we fabricated Co O/Ni O/nickel foam(NF)and Cu_(2)O/Ni O/NF electrodes via in situ pulsed laser irradiation in liquids(PLIL)for the bifunctional electrocatalysis of oxygen evolution reaction(OER)and furfural oxidation reaction(FOR),respectively.Simultaneous oxidation of NF surface to NiO and deposition of CoO and/or Cu_(2)O on NF during PLIL offer distinct advantages for enhancing both the OER and FOR.CoO/NiO/NF electrocatalyst provides a consistently low overpotential of~359 m V(OER)at 10 m A/cm^(2),achieving the maximum FA yield(~16.37 m M)with 61.5%selectivity,79.5%carbon balance,and a remarkable Faradaic efficiency of~90.1%during 2 h of FOR at 1.43 V(vs.reversible hydrogen electrode).Mechanistic pathway via in situ electrochemical-Raman spectroscopy on CoO/NiO/NF reveals the involvement of phase transition intermediates(NiOOH and CoOOH)as surface-active centers during electrochemical oxidation.The carbonyl carbon in FF is attacked by hydroxyl groups to form unstable hydrates that subsequently undergo further oxidation to yield FA products.This method holds promise for large-scale applications,enabling simultaneous production of renewable building materials and fuel. 展开更多
关键词 pulsed laser irradiation in liquids Water and furfural oxidation In situ Raman spectroscopy CoO/NiO/nickel foam Cu_(2)O/Nio/nickel foam 2-furoic acid
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Generation and regulation of electromagnetic pulses generated by femtosecond lasers interacting with multitargets
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作者 Ya-Dong Xia De-Feng Kong +14 位作者 Qiang-You He Zhen Guo Dong-Jun Zhang Tong Yang Hao Cheng Yu-Ze Li Yang Yan Xiao Liang Ping Zhu Xing-Long Xie Jian-Qiang Zhu Ting-Shuai Li Chen Lin Wen-Jun Ma Xue-Qing Yan 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第1期96-107,共12页
Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(... Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(2))femtosecond(fs)lasers with metal flat,plastic flat,and plastic nanowire-array(NWA)targets.Detailed analyses are conducted on the EMPs in terms of their spatial distribution,time and frequency domains,radiation energy,and protection.The results indicate that EMPs from metal targets exhibit larger amplitudes at varying angles than those generated by other types of targets and are enhanced significantly for NWA targets.Using a plastic target holder and increasing the laser focal spot can significantly decrease the radiation energy of the EMPs.Moreover,the composite shielding materials indicate an effective shielding effect against EMPs.The simulation results show that the NWA targets exert a collimating effect on thermal electrons,which directly affects the distribution of EMPs.This study provides guidance for regulating EMPs by controlling the laser focal spot,target parameters,and target rod material and is beneficial for electromagnetic-shielding design. 展开更多
关键词 Electromagnetic pulses Laser plasma interaction Electromagnetic shielding Electron distribution
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Performance of pulsed plasma thruster at low discharge energy
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作者 李鸿俊 林泽豪 +3 位作者 胡浩俊 吴文东 陈爱虹 杜德扬 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第4期122-132,共11页
As the size of satellites scales down, low-power and compact propulsion systems such as the pulsed plasma thruster(PPT) are needed for stabilizing these miniature satellites in orbit. Most PPT systems are operated at ... As the size of satellites scales down, low-power and compact propulsion systems such as the pulsed plasma thruster(PPT) are needed for stabilizing these miniature satellites in orbit. Most PPT systems are operated at 2 J or more of discharge energy. In this work, the performance of a PPT with a side-fed, tongue-flared electrode configuration operated within a lower discharge energy range of 0.5-2.5 J has been investigated. Ablation and charring of the polytetrafluoroethylene propellant surface were analyzed through field-effect scanning electron microscopy imaging and energy-dispersive X-ray spectroscopy. When the discharge energy fell below 2 J, inconsistencies occurred in the specific impulse and the thrust efficiency due to the measurement of the low mass bit. At energy ≥2 J, the performance parameters are compared with other PPT systems of similar configuration and discussed in depth. 展开更多
关键词 pulsed plasma thruster low discharge energy performance parameters
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Dielectric barrier discharge plasma-assisted catalytic ammonia synthesis:synergistic effect of Ni-MOF-74 catalyst and nanosecond pulsed plasma
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作者 徐晓芳 孙萌 +4 位作者 宋勤龙 吴璇 陈冲冲 陈强 张海宝 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第6期40-49,共10页
Ammonia is one of the most important chemical raw materials in both manufacture and life of human.Traditionally Haber-Bosch method for ammonia synthesis involves high temperature and high pressure conditions,leading t... Ammonia is one of the most important chemical raw materials in both manufacture and life of human.Traditionally Haber-Bosch method for ammonia synthesis involves high temperature and high pressure conditions,leading to significant energy consumption and environmental pollution.Non-thermal plasma(NTP) is a promising alternative approach to ammonia synthesis at low temperature and atmospheric pressure.In this study,the synergistic effect of nanosecond pulsed dielectric barrier discharge(np-DBD) and Ni-MOF-74 catalyst was investigated in ammonia synthesis by utilizing nitrogen and hydrogen as feedstock.The results demonstrated that the plasma catalytic-synthesis process parameters play a crucial role in the synthesis process of ammonia.The highest ammonia synthesis rate of 5145.16 μmol·g^(-1)·h^(-1)with an energy efficiency of 1.27 g·kWh^(-1)was observed in the presence of the Ni-MOF-74 catalyst,which was3.7 times higher than that without Ni-MOF-74 catalyst.The synergistic effect of Ni-MOF-74catalyst and nanosecond pulsed plasma was explored by in-situ plasma discharge diagnostics. 展开更多
关键词 AMMONIA SYNTHESIS low-temperature plasma nanosecond pulsed power source Ni-MOF-74
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