Pearl River Mouth Basin undergoes complex tectonic evolution processes and forms lacustrine,transitional and marine sediments.Drilling shows that there exist large petroleum reserves in the hydrocarbon-rich sags of Pe...Pearl River Mouth Basin undergoes complex tectonic evolution processes and forms lacustrine,transitional and marine sediments.Drilling shows that there exist large petroleum reserves in the hydrocarbon-rich sags of Pearl River Mouth Basin,South China Sea.To reduce the risk,the exploration,structural and sedimentary characteristics of the hydrocarbon-rich sags should be identified and described.Drilling,seismic,and microfossil data are integrated to interpret the structural and sedimentary evolution of the hydrocarbon-rich sags in Pearl River Mouth Basin.By analyzing the tectonic and sedimentary evolutionary characteristics,three conclusions may be drawn:1、The present regional tectonic characteristics of the PRMB are formed by mutual interactions of the Eurasian Plate,Pacific Plate,Philippine Plate and Indian Plate.During the Paleocene to early Eocene and late Eocene and early Oligocene,the PRMB is at the rifting stage.During the late Oligocene,the PRMB was at the rifting-depression transitional stage.After the Oligocene,the PRMB is at the depression stage.2、Tectonic conditions control the sedimentation process in the hydrocarbon-rich sags.During the lacustrine sedimentation stage,synsedimentary faults and intense faulting control the sedimentation.During the transitional sedimentation stage,weak fault activity influences the deposition process in the hydrocarbon-rich sags.During the marine sedimentation stage,weak fault activity and depression activity control the deposition process in the hydrocarbon-rich sags.3、Tectonic evolution affects the deposition process.The lacustrine,transitional and marine sedimentation corresponds to different tectonic conditions.The lacustrine sedimentation is formed under fault activity during the rifting stage.The transitional sedimentation is formed under weak fault activity during the late rifting stage.The marine sedimentation is formed under weak fault activity and depression activity during the rifting-depression and depression stages.4、The half graben is beneficial for the formation of lacustrine source rocks,which is responsible for the hydrocarbon-rich sag.Therefore the half graben mode contributes to the hydrocarbon-rich sags.展开更多
The method for pyrolysis of biomass to manufacture hydrocarbon-rich fuel remains challenging in terms of conversion of multifunctional biomass with high oxygen content and low thermal stability into a high-quality com...The method for pyrolysis of biomass to manufacture hydrocarbon-rich fuel remains challenging in terms of conversion of multifunctional biomass with high oxygen content and low thermal stability into a high-quality compound, featuring high content of hydrocarbons, low oxygen content, few functional groups, and high thermal stability. This study offers a promising prospect to derive hydrocarbon-rich oil through microwave-assisted fast catalytic pyrolysis by improving the effective hydrogen to carbon ratio(H/Ceff) of the raw materials. The proposed technique can promote the production of high-quality bio-oil through the molecular sieve catalyzed reduction of oxygenated compounds and mutagenic polyaromatic hydrocarbons. This work aims to review and summarize the research progress on microwave copyrolysis and microwave catalytic copyrolysis to demonstrate their benefits on enhancement of bio-oils derived from the biomass. This review focuses on the potential of optimizing the H/Ceff ratio, the microwave absorbent, and the HZSM-5 catalyst during the microwave copyrolysis to produce the valuable liquid fuel. This paper also proposes future directions for the use of this technique to obtain high yields of bio-oils.展开更多
基金the National Natural Science Foundation of China(No.41702135)the Yangtze Youth Fund(No.2015qq33),the 13th“Five-year”plan of the Ministry of Science and Technology of China(No.2016ZX05037-002)National Science and Technology Major Project(NO.2016ZX05015-006).
文摘Pearl River Mouth Basin undergoes complex tectonic evolution processes and forms lacustrine,transitional and marine sediments.Drilling shows that there exist large petroleum reserves in the hydrocarbon-rich sags of Pearl River Mouth Basin,South China Sea.To reduce the risk,the exploration,structural and sedimentary characteristics of the hydrocarbon-rich sags should be identified and described.Drilling,seismic,and microfossil data are integrated to interpret the structural and sedimentary evolution of the hydrocarbon-rich sags in Pearl River Mouth Basin.By analyzing the tectonic and sedimentary evolutionary characteristics,three conclusions may be drawn:1、The present regional tectonic characteristics of the PRMB are formed by mutual interactions of the Eurasian Plate,Pacific Plate,Philippine Plate and Indian Plate.During the Paleocene to early Eocene and late Eocene and early Oligocene,the PRMB is at the rifting stage.During the late Oligocene,the PRMB was at the rifting-depression transitional stage.After the Oligocene,the PRMB is at the depression stage.2、Tectonic conditions control the sedimentation process in the hydrocarbon-rich sags.During the lacustrine sedimentation stage,synsedimentary faults and intense faulting control the sedimentation.During the transitional sedimentation stage,weak fault activity influences the deposition process in the hydrocarbon-rich sags.During the marine sedimentation stage,weak fault activity and depression activity control the deposition process in the hydrocarbon-rich sags.3、Tectonic evolution affects the deposition process.The lacustrine,transitional and marine sedimentation corresponds to different tectonic conditions.The lacustrine sedimentation is formed under fault activity during the rifting stage.The transitional sedimentation is formed under weak fault activity during the late rifting stage.The marine sedimentation is formed under weak fault activity and depression activity during the rifting-depression and depression stages.4、The half graben is beneficial for the formation of lacustrine source rocks,which is responsible for the hydrocarbon-rich sag.Therefore the half graben mode contributes to the hydrocarbon-rich sags.
基金the financial support from the National Natural Science Foundation of China (No. 21766019, 21466022)the Key Research and Development Program of Jiangxi Province(20171BBF60023)+2 种基金the International Science&Technology Cooperation Project of China(2015DFA60170-4)the Science and Technology Research Project of Jiangxi Province Education Department(No.GJJ150213)the Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development Program (No. Y707sb1001)”
文摘The method for pyrolysis of biomass to manufacture hydrocarbon-rich fuel remains challenging in terms of conversion of multifunctional biomass with high oxygen content and low thermal stability into a high-quality compound, featuring high content of hydrocarbons, low oxygen content, few functional groups, and high thermal stability. This study offers a promising prospect to derive hydrocarbon-rich oil through microwave-assisted fast catalytic pyrolysis by improving the effective hydrogen to carbon ratio(H/Ceff) of the raw materials. The proposed technique can promote the production of high-quality bio-oil through the molecular sieve catalyzed reduction of oxygenated compounds and mutagenic polyaromatic hydrocarbons. This work aims to review and summarize the research progress on microwave copyrolysis and microwave catalytic copyrolysis to demonstrate their benefits on enhancement of bio-oils derived from the biomass. This review focuses on the potential of optimizing the H/Ceff ratio, the microwave absorbent, and the HZSM-5 catalyst during the microwave copyrolysis to produce the valuable liquid fuel. This paper also proposes future directions for the use of this technique to obtain high yields of bio-oils.