We report our numerical simulation on the dynamic interference photoelectron spectra for a one-dimensional （1D） He model exposed to intense ultrashort extreme ultraviolet （XUV） laser pulses. The results demonstrat...We report our numerical simulation on the dynamic interference photoelectron spectra for a one-dimensional （1D） He model exposed to intense ultrashort extreme ultraviolet （XUV） laser pulses. The results demonstrate an unambiguous interference feature in the photoelectron spectra, and the interference is unveiled to originate from the dynamic Stark effect. The interference photoelectron spectra are prompted for intense sub-femtosecond XUV laser pulses in double ionization. The stationary phase picture is corroborated qualitatively in the two-electron system. The ability of probing the dynamic Stark effect by the photoelectron spectra in a pragmatic experiment of single-photon double ionization of He may shed light on further investigation on multi-electron atoms and molecules.展开更多
The structure and the electron-transfer of cytochrome c binding on the anionic lipid vesicles were analyzed by electrochemical and various spectroscopic methods. It was found that upon binding to anionic lipid membran...The structure and the electron-transfer of cytochrome c binding on the anionic lipid vesicles were analyzed by electrochemical and various spectroscopic methods. It was found that upon binding to anionic lipid membrane, the formal potential of. cytochrome c shifted 30 mV negatively indicating an eager redox interaction than that in its native state. This is due to the local alteration of the coordination and the heme crevice. The structural Perturbation in which a molten globule-like state is formed during binding to anionic lipid vesicles is more important. This study may help to understand the mechanism of the electron-transfer reactions of cytochrome c at the mitochondrial membrane.展开更多
基金Supported by the National Natural Science Foundation of China under Grant Nos 61178028,11674243 and 11674242the National Basic Research Program of China under Grant No 2015CB755403
文摘We report our numerical simulation on the dynamic interference photoelectron spectra for a one-dimensional （1D） He model exposed to intense ultrashort extreme ultraviolet （XUV） laser pulses. The results demonstrate an unambiguous interference feature in the photoelectron spectra, and the interference is unveiled to originate from the dynamic Stark effect. The interference photoelectron spectra are prompted for intense sub-femtosecond XUV laser pulses in double ionization. The stationary phase picture is corroborated qualitatively in the two-electron system. The ability of probing the dynamic Stark effect by the photoelectron spectra in a pragmatic experiment of single-photon double ionization of He may shed light on further investigation on multi-electron atoms and molecules.
基金ProjectsupportedbytheNationalNaturalScienceFoundationofChina (No .2 983 5 12 0 )
文摘The structure and the electron-transfer of cytochrome c binding on the anionic lipid vesicles were analyzed by electrochemical and various spectroscopic methods. It was found that upon binding to anionic lipid membrane, the formal potential of. cytochrome c shifted 30 mV negatively indicating an eager redox interaction than that in its native state. This is due to the local alteration of the coordination and the heme crevice. The structural Perturbation in which a molten globule-like state is formed during binding to anionic lipid vesicles is more important. This study may help to understand the mechanism of the electron-transfer reactions of cytochrome c at the mitochondrial membrane.
