The sustainability of the coking industry is supported by reasonable production profit and environmental quality requirements.The traditional measures substantially increased the related costs for enterprises to reach...The sustainability of the coking industry is supported by reasonable production profit and environmental quality requirements.The traditional measures substantially increased the related costs for enterprises to reach standards.This paper aims to develop a comprehensive cost combined environmental impact assessment method that is necessary for the analysis of wastewater treatment systems.Typical three coking wastewater treatment processes in China were evaluated.Results showed that eutrophication dominantly contributed to the overall environmental effect.Improving effluent quality could significantly reduce the total environmental impact.In terms of an economic perspective,the price of raw materials was the main factor that affected the operating cost of comprehensive treatment.Based on subsystem analysis,the pretreatment stage accounted for the majority of environmental and cost burdens,respectively reaching 64%-78%and 64%-86%.Optimizing the pretreatment process by enhancing the efficiency of high concentration raw material recovery and substituting toxic raw materials for extractant could reduce the environmental impact and economic cost by 43.8%and 57%,respectively,which was an effective way to improve the potential performance of coking wastewater treatment plants(WWTPs).展开更多
The environmental burdens of Chinese copper production have been identified and quantified in the context of typical technologies, materials supplies and environmental emissions by a life cycle approach. Primary and s...The environmental burdens of Chinese copper production have been identified and quantified in the context of typical technologies, materials supplies and environmental emissions by a life cycle approach. Primary and secondary copper production using copper ores and scraps, respectively, were analyzed in detail. The flash and bath smelting approaches and the recycling of copper scraps were selected as representative copper production processes. A quantitative analysis was also conducted to assess the influence of material transport distance in copper production. Life cycle assessment (LCA) results showed that resources depletion and human health contribute significantly to environmental burdens in Chinese copper production. In addition, the secondary copper production has dramatically lower environmental burdens than the primary production. There is no obvious distinction in overall environmental burdens in primary copper production by flash or bath smelting approach. However, resources depletion is lower and the damage to human health is higher for flash smelting approach. Ecosystem quality damage is slight for both approaches. Environ- mental burdens from the mining stage contribute most in all life cycle stages in primary copper production. In secondary copper production, the electrolytic refining stage dominates. Based on the life cycle assessment results, some suggestions for improving environmental performance were proposed to meet the sustainable development of Chinese copper industry.展开更多
China is the largest producer and consumer of HFC-134a(1,1,1,2-tetrafluoroethane)in the world.Coal-based route is mainly adopted to produce HFC-134a,which suffers from large waste and CO_(2) emissions.Natural gas is a...China is the largest producer and consumer of HFC-134a(1,1,1,2-tetrafluoroethane)in the world.Coal-based route is mainly adopted to produce HFC-134a,which suffers from large waste and CO_(2) emissions.Natural gas is a low-carbon and clean energy resource,and no research has been found on the environment and economy of producing HFC-134a from natural gas.In this study,CML 2001 method was used to carry out the life cycle assessment of natural gas(partial oxidation)-based and natural gas(plasma cracking)-based routes(abbreviated as gas(O)-based and gas(P)-based routes,respectively),and their environmental performances were compared with coal-based and oil-based routes.Meanwhile,considering that China is vigorously promoting the transformation of energy structure,and the application of electric heating equipment to replace fossil-based heating equipment in industrial field,which has a great impact on the environmental performance of the production processes,the authors conducted a scenario analysis.The results showed that the gas(O)-based route had the most favourable environmental benefits.However,the gas(P)-based route had the highest potential for reducing environmental burdens,and its environmental benefit was the most favourable in scenario 2050.Additionally,the economic performance of the gas(P)-based route was significantly better than that of gas(O)-based and coal-based routes.展开更多
The objective of this paper is to understand the benefits that one can achieve for large-scale supercritical CO_(2)(S-CO_(2))coal-fired power plants.The aspects of energy environment and economy of 1000 MW S-CO_(2)coa...The objective of this paper is to understand the benefits that one can achieve for large-scale supercritical CO_(2)(S-CO_(2))coal-fired power plants.The aspects of energy environment and economy of 1000 MW S-CO_(2)coal-fired power generation system and 1000 MW ultra-supercritical(USC)water-steam Rankine cycle coal-fired power generation system are analyzed and compared at the similar main vapor parameters,by adopting the neural network genetic algorithm and life cycle assessment(LCA)methodology.Multi-objective optimization of the 1000 MW S-CO_(2)coal-fired power generation system is further carried out.The power generation efficiency,environmental impact load,and investment recovery period are adopted as the objective functions.The main vapor parameters of temperature and pressure are set as the decision variables.The results are concluded as follows.First,the total energy consumption of the S-CO_(2)coal-fired power generation system is 10.48 MJ/k Wh and the energy payback ratio is 34.37%.The performance is superior to the USC coal-fired power generation system.Second,the resource depletion index of the S-CO_(2)coal-fired power generation system is 4.38μPRchina,90,which is lower than that of the USC coal-fired power generation system,and the resource consumption is less.Third,the environmental impact load of the S-CO_(2)coal-fired power generation system is 0.742 m PEchina,90,which is less than that of the USC coal-fired power generation system,0.783 m PEchina,90.Among all environmental impact types,human toxicity potential HTP and global warming potential GWP account for the most environmental impact.Finally,the investment cost of the S-CO_(2)coal-fired power generation system is generally less than that of the USC coal-fired power generation system because the cost of the S-CO_(2)turbine is only half of the cost of the steam turbine.The optimal turbine inlet temperature T_(5)becomes smaller,and the optimal turbine inlet pressure is unchanged at 622.082°C/30 MPa.展开更多
To address current challenges regarding sustainable development of wastewater treatment and provide scientific support in decision procedures towards sustainable solutions, new approaches, frameworks and methodologies...To address current challenges regarding sustainable development of wastewater treatment and provide scientific support in decision procedures towards sustainable solutions, new approaches, frameworks and methodologies about different possible solutions and their potential sustainability implications are needed. One way to facilitate sustainability assessment of wastewater is Life Cycle Assessment (LCA) methodology;however, it fails to map the full scope of wastewater impacts. This paper presents a framework to evaluate the performance of Wastewater Treatment Facilities (WWTF) taking into consideration various factors for insuring environmental sustainability. A total of nine indicators, seven environmental and two economic related to four wastewater treatment facilities, were assessed. Apart from evaluating the sustainability, this study also discussed the link of life cycle approach and social aspects of wastewater. The results show that for the environmental dimension using LCA provides information on different types of environmental activities and different impact categories. LCA can thus be used to quantify and compare the multiple types of impacts caused by one type of use or emission, as well as the various resource uses or emissions that contribute to one type of impacts. For the economic dimension, there is still a need for consistent and robust indicators and methods. The empirical results suggest that the environmental sustainability framework can be used in the first phase of the decision procedure that leads to a strategic choice for sustainable resource recovery from wastewater in developing countries. This motives researchers and decision-makers to consider the whole picture, and not just individual aspects, when considering different futures scenarios.展开更多
基金funding by the National Natural Science Foundation of China(No.51978643)Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDA21021102)+2 种基金14th Five-year Informatization Plan of Chinese Academy of Sciences,Construction of Scientific Data Center System(WX145XQ07-12)Youth Innovation Promotion Association,CAS(Y201814)the National Youth Talent Support Program of China
文摘The sustainability of the coking industry is supported by reasonable production profit and environmental quality requirements.The traditional measures substantially increased the related costs for enterprises to reach standards.This paper aims to develop a comprehensive cost combined environmental impact assessment method that is necessary for the analysis of wastewater treatment systems.Typical three coking wastewater treatment processes in China were evaluated.Results showed that eutrophication dominantly contributed to the overall environmental effect.Improving effluent quality could significantly reduce the total environmental impact.In terms of an economic perspective,the price of raw materials was the main factor that affected the operating cost of comprehensive treatment.Based on subsystem analysis,the pretreatment stage accounted for the majority of environmental and cost burdens,respectively reaching 64%-78%and 64%-86%.Optimizing the pretreatment process by enhancing the efficiency of high concentration raw material recovery and substituting toxic raw materials for extractant could reduce the environmental impact and economic cost by 43.8%and 57%,respectively,which was an effective way to improve the potential performance of coking wastewater treatment plants(WWTPs).
基金This research was supported financially by the Key Project (No.71033005) from National Natural Science Foundation of China.
文摘The environmental burdens of Chinese copper production have been identified and quantified in the context of typical technologies, materials supplies and environmental emissions by a life cycle approach. Primary and secondary copper production using copper ores and scraps, respectively, were analyzed in detail. The flash and bath smelting approaches and the recycling of copper scraps were selected as representative copper production processes. A quantitative analysis was also conducted to assess the influence of material transport distance in copper production. Life cycle assessment (LCA) results showed that resources depletion and human health contribute significantly to environmental burdens in Chinese copper production. In addition, the secondary copper production has dramatically lower environmental burdens than the primary production. There is no obvious distinction in overall environmental burdens in primary copper production by flash or bath smelting approach. However, resources depletion is lower and the damage to human health is higher for flash smelting approach. Ecosystem quality damage is slight for both approaches. Environ- mental burdens from the mining stage contribute most in all life cycle stages in primary copper production. In secondary copper production, the electrolytic refining stage dominates. Based on the life cycle assessment results, some suggestions for improving environmental performance were proposed to meet the sustainable development of Chinese copper industry.
基金This work was supported by the National Natural Science Foundation of China(Grant Nos.22078266 and 22008198)the Youth Innovation Team construction scientific research Project of Education Ministry of Shaanxi province,China(Grant No.22JP090)+1 种基金the Youth Talent Promotion Program of Shaanxi Association for Science and Technology(Grant No.20220602)Natural Science Basic Research Plan in Shaanxi Province of China(Grant No.2021JQ-555).
文摘China is the largest producer and consumer of HFC-134a(1,1,1,2-tetrafluoroethane)in the world.Coal-based route is mainly adopted to produce HFC-134a,which suffers from large waste and CO_(2) emissions.Natural gas is a low-carbon and clean energy resource,and no research has been found on the environment and economy of producing HFC-134a from natural gas.In this study,CML 2001 method was used to carry out the life cycle assessment of natural gas(partial oxidation)-based and natural gas(plasma cracking)-based routes(abbreviated as gas(O)-based and gas(P)-based routes,respectively),and their environmental performances were compared with coal-based and oil-based routes.Meanwhile,considering that China is vigorously promoting the transformation of energy structure,and the application of electric heating equipment to replace fossil-based heating equipment in industrial field,which has a great impact on the environmental performance of the production processes,the authors conducted a scenario analysis.The results showed that the gas(O)-based route had the most favourable environmental benefits.However,the gas(P)-based route had the highest potential for reducing environmental burdens,and its environmental benefit was the most favourable in scenario 2050.Additionally,the economic performance of the gas(P)-based route was significantly better than that of gas(O)-based and coal-based routes.
基金supported by the National Key R&D Program of China(2017YFB0601801)the National Natural Science Foundation of China(No.51806165)。
文摘The objective of this paper is to understand the benefits that one can achieve for large-scale supercritical CO_(2)(S-CO_(2))coal-fired power plants.The aspects of energy environment and economy of 1000 MW S-CO_(2)coal-fired power generation system and 1000 MW ultra-supercritical(USC)water-steam Rankine cycle coal-fired power generation system are analyzed and compared at the similar main vapor parameters,by adopting the neural network genetic algorithm and life cycle assessment(LCA)methodology.Multi-objective optimization of the 1000 MW S-CO_(2)coal-fired power generation system is further carried out.The power generation efficiency,environmental impact load,and investment recovery period are adopted as the objective functions.The main vapor parameters of temperature and pressure are set as the decision variables.The results are concluded as follows.First,the total energy consumption of the S-CO_(2)coal-fired power generation system is 10.48 MJ/k Wh and the energy payback ratio is 34.37%.The performance is superior to the USC coal-fired power generation system.Second,the resource depletion index of the S-CO_(2)coal-fired power generation system is 4.38μPRchina,90,which is lower than that of the USC coal-fired power generation system,and the resource consumption is less.Third,the environmental impact load of the S-CO_(2)coal-fired power generation system is 0.742 m PEchina,90,which is less than that of the USC coal-fired power generation system,0.783 m PEchina,90.Among all environmental impact types,human toxicity potential HTP and global warming potential GWP account for the most environmental impact.Finally,the investment cost of the S-CO_(2)coal-fired power generation system is generally less than that of the USC coal-fired power generation system because the cost of the S-CO_(2)turbine is only half of the cost of the steam turbine.The optimal turbine inlet temperature T_(5)becomes smaller,and the optimal turbine inlet pressure is unchanged at 622.082°C/30 MPa.
文摘To address current challenges regarding sustainable development of wastewater treatment and provide scientific support in decision procedures towards sustainable solutions, new approaches, frameworks and methodologies about different possible solutions and their potential sustainability implications are needed. One way to facilitate sustainability assessment of wastewater is Life Cycle Assessment (LCA) methodology;however, it fails to map the full scope of wastewater impacts. This paper presents a framework to evaluate the performance of Wastewater Treatment Facilities (WWTF) taking into consideration various factors for insuring environmental sustainability. A total of nine indicators, seven environmental and two economic related to four wastewater treatment facilities, were assessed. Apart from evaluating the sustainability, this study also discussed the link of life cycle approach and social aspects of wastewater. The results show that for the environmental dimension using LCA provides information on different types of environmental activities and different impact categories. LCA can thus be used to quantify and compare the multiple types of impacts caused by one type of use or emission, as well as the various resource uses or emissions that contribute to one type of impacts. For the economic dimension, there is still a need for consistent and robust indicators and methods. The empirical results suggest that the environmental sustainability framework can be used in the first phase of the decision procedure that leads to a strategic choice for sustainable resource recovery from wastewater in developing countries. This motives researchers and decision-makers to consider the whole picture, and not just individual aspects, when considering different futures scenarios.