We investigated the optical properties of hybrid exciton–plasmon coupling ensembles composed of ZnSe/ZnS quantum dots and Ag nanoparticles in aqueous solution. We modulated their average interval by changing the rati...We investigated the optical properties of hybrid exciton–plasmon coupling ensembles composed of ZnSe/ZnS quantum dots and Ag nanoparticles in aqueous solution. We modulated their average interval by changing the ratio of quantum dots and Ag nanoparticles. The transition from dramatic PL enhancement to PL quenching state was experimentally observed, according to the continuous decrease of the PL lifetime. The PL enhancement rate exceeded 10, with the Purcell factor of 3.5. Meanwhile, the proportion of fast decay increased from 0.3 to 0.6, corresponding to the proportion of slow decay decreased from 0.7 to 0.4. Our experiment is important for the hybrid exciton–plasmon coupling system to be practicable in optoelectronic application.展开更多
高温超导CORC(conductor on round core)电缆失超时的热负荷严重威胁了低温系统和电缆本体的安全稳定运行。受微米级超导薄膜制备工艺等的影响,CORC电缆并绕的多根高温超导带材不均匀。为分析不均匀临界电流对CORC电缆失超特性的影响,...高温超导CORC(conductor on round core)电缆失超时的热负荷严重威胁了低温系统和电缆本体的安全稳定运行。受微米级超导薄膜制备工艺等的影响,CORC电缆并绕的多根高温超导带材不均匀。为分析不均匀临界电流对CORC电缆失超特性的影响,该文搭建了基于三维TA方程的有限元模型。以降维的带材曲面为求解区域,以等效的电流密度为求解变量,失超模型在同一几何中表达超导和常导两种属性,构建电流和电势两种约束。在导体域建立降维的热模型,用以考虑损耗和传热的影响;在全局建立等效的电路模型,用以控制并联导体的分流。进一步地,耦合模型考虑温度依赖的接头电阻以模拟CORC电缆带材的烧断和电流的突变。结果表明,非均匀高温超导带材影响了电流重分配的动态响应,加快了局部失超的发展过程。展开更多
基金Project supported by the National Key R&D Program of China(Grant No.2018YFA0306304)the National Natural Science Foundation of China(Grant No.11674069)
文摘We investigated the optical properties of hybrid exciton–plasmon coupling ensembles composed of ZnSe/ZnS quantum dots and Ag nanoparticles in aqueous solution. We modulated their average interval by changing the ratio of quantum dots and Ag nanoparticles. The transition from dramatic PL enhancement to PL quenching state was experimentally observed, according to the continuous decrease of the PL lifetime. The PL enhancement rate exceeded 10, with the Purcell factor of 3.5. Meanwhile, the proportion of fast decay increased from 0.3 to 0.6, corresponding to the proportion of slow decay decreased from 0.7 to 0.4. Our experiment is important for the hybrid exciton–plasmon coupling system to be practicable in optoelectronic application.
文摘高温超导CORC(conductor on round core)电缆失超时的热负荷严重威胁了低温系统和电缆本体的安全稳定运行。受微米级超导薄膜制备工艺等的影响,CORC电缆并绕的多根高温超导带材不均匀。为分析不均匀临界电流对CORC电缆失超特性的影响,该文搭建了基于三维TA方程的有限元模型。以降维的带材曲面为求解区域,以等效的电流密度为求解变量,失超模型在同一几何中表达超导和常导两种属性,构建电流和电势两种约束。在导体域建立降维的热模型,用以考虑损耗和传热的影响;在全局建立等效的电路模型,用以控制并联导体的分流。进一步地,耦合模型考虑温度依赖的接头电阻以模拟CORC电缆带材的烧断和电流的突变。结果表明,非均匀高温超导带材影响了电流重分配的动态响应,加快了局部失超的发展过程。