The steel industry is a major source of CO_(2) emissions,and thus,the mitigation of carbon emissions is the most pressing challenge in this sector.In this paper,international environmental governance in the steel indu...The steel industry is a major source of CO_(2) emissions,and thus,the mitigation of carbon emissions is the most pressing challenge in this sector.In this paper,international environmental governance in the steel industry is reviewed,and the current state of development of low-carbon technologies is discussed.Additionally,low-carbon pathways for the steel industry at the current time are proposed,emphasizing prevention and treatment strategies.Furthermore,the prospects of low-carbon technologies are explored from the perspective of transitioning the energy structure to a“carbon-electricity-hydrogen”relationship.Overall,steel enterprises should adopt hydrogen-rich metallurgical technologies that are compatible with current needs and process flows in the short term,based on the carbon substitution with hydrogen(prevention)and the CCU(CO_(2) capture and utilization)concepts(treatment).Additionally,the capture and utilization of CO_(2) for steelmaking,which can assist in achieving short-term emission reduction targets but is not a long-term solution,is discussed.In conclusion,in the long term,the carbon metallurgical process should be gradually supplanted by a hydrogen-electric synergistic approach,thus transforming the energy structure of existing steelmaking processes and attaining near-zero carbon emission steelmaking technology.展开更多
Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.Howe...Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.However,two-photon pumped amplified spontaneous emission(ASE)and the corresponding nonlinear optical properties of FAPbBr_(3) NCs are scarcely revealed.Herein,we synthesized colloidal FAPbBr_(3) NCs with different sizes by changing the molar ratio of FABr/PbBr_(2) in the precursor solution,using ligand assisted precipitation(LARP)technology at room temperature.Photoluminescence(PL)and time resolved photoluminescence(TRPL)spectroscopy were measured to characterize their ASE properties.And their nonlinear optical properties were studied through the Zscan technique and the two-photon excited fluorescence method.The stimulated emission properties including oneand two-photon pumped ASE have been realized from FAPbBr_(3) NCs.With large two-photon absorption coefficient(0.27 cm/GW)and high non-linear absorption cross-section(7.52×10^(5) GM),ASE with threshold as low as 9.8μJ/cm^(2) and 487μJ/cm^(2) have been obtained from colloidal FAPbBr_(3) NCs using one-and two-photon excitations.These results indicate that as a new possible green-emitting frequency-upconversion material with low thresholds,FAPbBr_(3) NCs hold great potential in the development of high-performance two-photon pump lasers.展开更多
Recently, researchers in the road field are focusing on the development of green asphalt materials with loweremission of volatile organic compounds (VOCs). The characterization methodology of asphalt VOCs and theinflu...Recently, researchers in the road field are focusing on the development of green asphalt materials with loweremission of volatile organic compounds (VOCs). The characterization methodology of asphalt VOCs and theinfluencing factors on VOCs release have always been the basic issue of asphalt VOCs emission reduction research.Researchers have proposed a variety of asphalt VOCs characterization methodologies, which also have mutuallyirreplaceable characteristics. Asphalt VOCs volatilization is affected by many factors. In this study, asphalt VOCscharacterization methodologies were summarized, including their advantages, disadvantages, characteristics andapplicable requirements. Subsequently, the influencing factors of VOCs release, such as asphalt types and environment conditions, are summarized to provide theoretical support for the emission reduction research. Theclassification and mechanism of newly-development asphalt VOCs emission reduction materials are reviewed. Thereduction efficiencies are also compared to select better materials and put forward the improvement objective ofnew materials and new processes. In addition, the prospects about development of VOCs release mechanism ofasphalt materials during the full life cycle and feasibility research of high-efficiency composite emission reductionmaterials in the future were put forward.展开更多
During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a rest...During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.展开更多
In Fused Filament Fabrication(FFF),the state of material flow significantly influences printing outcomes.However,online monitoring of these micro-physical processes within the extruder remains challenging.The flow sta...In Fused Filament Fabrication(FFF),the state of material flow significantly influences printing outcomes.However,online monitoring of these micro-physical processes within the extruder remains challenging.The flow state is affected by multiple parameters,with temperature and volumetric flow rate(VFR)being the most critical.The study explores the stable extrusion of flow with a highly sensitive acoustic emission(AE)sensor so that AE signals generated by the friction in the annular region can reflect the flow state more effectively.Nevertheless,the large volume and broad frequency range of the data present processing challenges.This study proposes a method that initially selects short impact signals and then uses the Fast Kurtogram(FK)to identify the frequency with the highest kurtosis for signal filtration.The results indicate that this approach significantly enhances processing speed and improves feature extraction capabilities.By correlating AE characteristics under various parameters with the quality of extruded raster beads,AE can monitor the real-time state of material flow.This study offers a concise and efficient method for monitoring the state of raster beads and demonstrates the potential of online monitoring of the flow states.展开更多
Nowadays,presynaptic dopaminergic positron emission tomography,which assesses deficiencies in dopamine synthesis,storage,and transport,is widely utilized for early diagnosis and differential diagnosis of parkinsonism....Nowadays,presynaptic dopaminergic positron emission tomography,which assesses deficiencies in dopamine synthesis,storage,and transport,is widely utilized for early diagnosis and differential diagnosis of parkinsonism.This review provides a comprehensive summary of the latest developments in the application of presynaptic dopaminergic positron emission tomography imaging in disorders that manifest parkinsonism.We conducted a thorough literature search using reputable databases such as PubMed and Web of Science.Selection criteria involved identifying peer-reviewed articles published within the last 5 years,with emphasis on their relevance to clinical applications.The findings from these studies highlight that presynaptic dopaminergic positron emission tomography has demonstrated potential not only in diagnosing and differentiating various Parkinsonian conditions but also in assessing disease severity and predicting prognosis.Moreover,when employed in conjunction with other imaging modalities and advanced analytical methods,presynaptic dopaminergic positron emission tomography has been validated as a reliable in vivo biomarker.This validation extends to screening and exploring potential neuropathological mechanisms associated with dopaminergic depletion.In summary,the insights gained from interpreting these studies are crucial for enhancing the effectiveness of preclinical investigations and clinical trials,ultimately advancing toward the goals of neuroregeneration in parkinsonian disorders.展开更多
Ammonia emission is one of the most important pathways of nitrogen loss from agricultural cultivated field. In this paper, we report the measurement of ammonia emission from paddy rice field obtained by surface applic...Ammonia emission is one of the most important pathways of nitrogen loss from agricultural cultivated field. In this paper, we report the measurement of ammonia emission from paddy rice field obtained by surface application of urea fertilizer with water management. The main objective of the present study were to assess the amount of NH3 emission and the loss of nitrogen from paddy field as affected by various N doses, i.e., 0 (control), 90 (N1), 180 (N2), 270 (N3) and 360 (N4) kg ha-1, following field surface application of urea fertilizer with water management. Ammonia emissions were measured by continuous airflow enclosure method from plots fertilized with the application of surface urea. Increase in urea-N dosage increased NH3 emission that was measured from paddy rice field. Ammonia emission started immediately and was almost complete within 12 days after top dressing of urea application to the soils. Ammonia emissions were nearly constant in all treatments from 12 days after fertilizer application. Highest ammonia emission rate was 28 g /day and total amount of ammonia emission was 56.21 kg ha-1 for 360 kg N ha-1 dose. No remarkable observation was found about temperature for ammonia emission. Due to proper water management practices less emission was observed throughout the experiment period. The results also show that N loss through NH3 emission accounted for 11 to 16% during the rice- growing season. These magnitudes of loss of N appear to be most important for environmental point of view.展开更多
This paper takes the climate change and low carbon economy development as the study background, based on the analysis of energy demand and carbon emissions status, which is aimed to provide the low carbon development ...This paper takes the climate change and low carbon economy development as the study background, based on the analysis of energy demand and carbon emissions status, which is aimed to provide the low carbon development path in Chinese cities. The method of scenario analysis can be used to predict long-term strategy for the uncertainty future development, and it was introduced to the field of social forecasting and public policy research, such as the environmental strategic planning, policy analysis, and support of decision in resource management, which can be used to explore the possible development trend and target of the results from the macro perspective. Scenario analysis has been gradually applied to the study area on low carbon economy, energy forecasting and other fields in recent years, and there have been many research results in different aspects. This paper takes the scenario analysis as basic study theory, spreading out the present situation of its application in low carbon city and some issues that need further study. As a tool for predicting the future development in low carbon city, the method of scenario analysis has been providing a powerful reference for policies and their executants.展开更多
Characteristics of electron emission induced by a surface flashover trigger device in a low-pressure trigger switch were investigated. A test method to measure the emitted charges from the trigger device was developed...Characteristics of electron emission induced by a surface flashover trigger device in a low-pressure trigger switch were investigated. A test method to measure the emitted charges from the trigger device was developed, and the factors affecting the emitted charges were analyzed. The results indicated that the major emitted charges from the trigger device were induced by surface plasma generated by surface flashover occurring on the trigger dielectric material. The emitted charges and the peak emission current increased linearly with the change in the trigger voltage and bias voltage. The emitted charges collected from the anode were affected by the gap distance. However, the emitted charges were less affected by the anode diameter. Furthermore, the emitted charges and the peak emission current decreased rapidly with the increase in gas pressure in a range from 0 Pa to 100 Pa, and then remained stable or changed slightly when the increase in gas pressure up to 2400 Pa.展开更多
The study was conducted to investigate the N2O emissions and dissolved N2O in the leachate during the nonflooding period in nongrowing paddy fields.Three kinds of paddy soils were repacked to soil columns and were sup...The study was conducted to investigate the N2O emissions and dissolved N2O in the leachate during the nonflooding period in nongrowing paddy fields.Three kinds of paddy soils were repacked to soil columns and were supersaturated with water initially and dried gradually in a greenhouse to attain the N2O emissions flux during the incubation.Soils with the texture of silty clay-loam (Q and H) produced cracks during the drying of soil,but soil with the texture of silty loam (X) did not form the cracks.Cracked s...展开更多
In order to investigate the effect of hydrogen attack degree on acoustic emission(AE) behavior of low carbon steel during tensiling, specimens made of Low carbon steel was exposed to hydrogen gas of 18 MPa at 450 and ...In order to investigate the effect of hydrogen attack degree on acoustic emission(AE) behavior of low carbon steel during tensiling, specimens made of Low carbon steel was exposed to hydrogen gas of 18 MPa at 450 and 500℃ for 240, 480 and 720 h respectively. Experimental results show that with increase of the hydrogen attack degree, the totally AE activity decreases during tensiling. In addition, the count of AE signals with high amplitude for the specimens with hydrogen attack keeps a constant which is less than that without hydrogen attack. It is concluded that AE signals originate in the specimens with hydrogen attack from intergranular fracture induced by methane blisterings or/and microcracks on grain boundaries.展开更多
Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-freq...Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-frequency chorus emissions have not been well understood..In this letter, we report an interesting case in which background plasma density lowered the lower cutoff frequency of chorus emissions from above 0.1 f_(ce)(typical ordinary chorus) to 0.02 f_(ce)(extremely low-frequency chorus).Those extremely low-frequency chorus waves were observed in a rather dense plasma, where the number density N_e was found to be several times larger than has been associated with observations of ordinary chorus waves.For suprathermal electrons whose free energy is supplied by anisotropic temperatures, linear growth rates(calculated using in-situ plasma parameters measured by the Van Allen Probes) show that whistler mode instability can occur at frequencies below 0.1 f_(ce) when the background plasma density N_e increases.Especially when N_e reaches 90 cm–3 or more, the lowest unstable frequency can extend to 0.02 f_(ce) or even less, which is consistent with satellite observations.Therefore, our results demonstrate that a dense background plasma could play an essential role in the excitation of extremely lowfrequency chorus waves by controlling the wave growth rates.展开更多
The increasing demand for fresh sweet maize (Zea mays L. saccharata) in southern China has prioritized the need to find solutions to the environmental pollution caused by its continuous production and high inputs of...The increasing demand for fresh sweet maize (Zea mays L. saccharata) in southern China has prioritized the need to find solutions to the environmental pollution caused by its continuous production and high inputs of chemical nitrogen fertilizers. A promising method for improving crop production and environmental conditions is to intercrop sweet maize with legumes. Here, a three-year field experiment was conducted to assess the influence of four different cropping systems (sole sweet maize (SS), sole soybean (SB), two rows sweet maize-three rows soybean (S2B3) intercropping, and two rows sweet maize-four rows soybean (S2B4) intercropping), together with two rates of N fertilizer application (300 and 360 kg N ha-1) on grain yield, residual soil mineral N, and soil N2O emissions in southern China. Results showed that in most case, inter- cropping achieved yield advantages (total land equivalent ratio (TLER=0.87-1.25) was above one). Moreover, intercropping resulted in 39.8% less soil mineral N than SS at the time of crop harvest, averaged over six seasons (spring and autumn in each of the three years of the field experiment). Generally, intercropping and reduced-N application (300 kg N ha-1) produced lower cumulative soil N20 and yield-scaled soil N20 emissions than SS and conventionaI-N application (360 kg N ha-l), respectively. $2B4 intercropping with reduced-N rate (300 kg N ha-~) showed the lowest cumulative soil N20 (mean value=0.61 kg ha-1) and yield-scaled soil N20 (mean value=0.04 kg t-1) emissions. Overall, intercropping with reduced-N rate maintained sweet maize production, while also reducing environmental impacts. The system of S2B4 intercropping with reduced-N rate may be the most sustainable and environmentally friendly cropping system.展开更多
Optical emission spectroscopy was used to study a gas mixture glow discharge of CO2 and N2 at a total pressure of 1.2 Torr, a power of 100 W and a flow of 16.5 L/min. The emission bands were measured in the wavelength...Optical emission spectroscopy was used to study a gas mixture glow discharge of CO2 and N2 at a total pressure of 1.2 Torr, a power of 100 W and a flow of 16.5 L/min. The emission bands were measured in the wavelength range of 200 nm to 900 nm. The principal species observed were O2^+ (A^2П→ X^2П), CO^+ (A^2П→X^2∑), N2^+ (B^2∑u+ → X^2∑g^+), CO2^+ (A^2∏ → X^2∏), N2(C^3∏u → B^3∏g), O2(b^1∑g^+→ X^3∑g^-), and CO (a^r3∑→a^3∏). The behavior of the band intensities as a function of the N2 percentage is consistent with recent Monte Carlo simulations. The electron temperature and ion density were determined by a double Langmuir probe. The electron temperature was found in the range of 1.55 eV to 2.93 eV, and the electron concentration in the order of 10^10 cm^-3. The electron temperature and ion density at pure N2 and pure CO2 agree with previous measurements.展开更多
A split-plot experiment in a rice-winter wheat rotation system was performed to study the effects of water regime and wheat straw application in rice-growing season on N2O emission from following wheat growing season....A split-plot experiment in a rice-winter wheat rotation system was performed to study the effects of water regime and wheat straw application in rice-growing season on N2O emission from following wheat growing season. Water regime in the rice-growing season was designed as the conventional irrigation (flooding/drainage cycle) and the permanent flooding. Wheat straw was incorporated with three rates of 0, 225 and 450 g m-2 into the paddy soil for each water regime just before rice was transplanted. N2O emission was measured by static chamber-gas chromatograph method. Results from the variance analysis indicated that the permanent flooding in rice-growing season markedly enhanced N2O emission in following wheat growing season (P=0. 003), and that the effect of straw application on N2O emission was distinguished between two water regimes. Under the conventional irrigation, incoporation of wheat straw reduced N2O emission in the following wheat growing season, while there were no significant differences in the emission for the straw application rates of 225 and 450 g m-2. No significant differences in N2O emissions were observed among the three rates of straw application for the permanent flooding regime. In addition, the seasonal variation of N2O emission was regulated by soil temperature and moisture. The daily N2O flux (Y, mg m-2 d-1) can be quantitatively described by soil temperature (T, ℃) and moisture (W, WFPS %) asY=A0+A1T+A2W+A3W2(n=23, R2 ≥0. 4159** )or y=C0+C1W+C2W2(n=23,R2≥0. 4074** ). Compared with the effect of soil temperature on N2O emission, soil moisture was an important factor regulating the seasonal pattern of N2O emission.展开更多
Based on the revised reduction models of the 14 low-carbon ICT solutions from Chongqing Mobile of the China Mobile Group,the CO2e emission reduction brought about by low-carbon ICTs of the wireless telecom sector of C...Based on the revised reduction models of the 14 low-carbon ICT solutions from Chongqing Mobile of the China Mobile Group,the CO2e emission reduction brought about by low-carbon ICTs of the wireless telecom sector of Chongqing Mobile,the entire China Mobile Group and the whole China in 2009 is calculated.And then the CO2e emission reduction potentials in 2010,2020 and 2030 are calculated in four main important fields of China,i.e.,intelligent transportation,dematerialization,smart work and smart appliances.The ICTs in the telecom sector are mostly dedicated to these fields.It provides a valuable insight into future reduction targets that should be set up for China.展开更多
A quantitative model was applied to analyze the energy demand and CO2 emissions in China following the Energy Production and Consumption Revolution Strategy(2016e2030)and long-term economic and social development targ...A quantitative model was applied to analyze the energy demand and CO2 emissions in China following the Energy Production and Consumption Revolution Strategy(2016e2030)and long-term economic and social development target China Dream.Results showed that 1)toward the 2050 China Dream target,total final energy consumption is expected to peak at 3.9 Gtce in 2030 and remain stable until 2050,whereas total primary energy consumption is expected to reach an upper platform by 2040 and around 5.8 Gtce by 2050;2)the proportion of non-fossil fuels is expected to reach approximately 50%and that of natural gas to reach more than 16%by 2050;3)CO2 emissions from energy use are expected to peak at 9.6 Gt by no later than 2030 and then gradually decline to 6.7 Gt by 2050.展开更多
To feed an increasing population, large amounts of chemical nitrogen fertilizer have been used to produce much of our food, feed and fiber thereby increasing nitrogen levels in soils, natural waters, crop residues, li...To feed an increasing population, large amounts of chemical nitrogen fertilizer have been used to produce much of our food, feed and fiber thereby increasing nitrogen levels in soils, natural waters, crop residues, livestock wastes,and municipal and agricultural wastes, with national and international concern about its potential adverse effects on environmental quality and public health. To understand these phenomena and problems, first the nitrogen cycle and the environment are described. Then recent trends for nitrogen cycling through the food and feed system, N2O emissions from fertilized upland and paddy soils, and NO-3 pollution in ground water in Japan are reported. Finally, mitigation strategies in Japan for reducing N2O emission and NO-3 pollution are proposed, including nitrification inhibitors, controlled release fertilizers, utilization of plant species that could suppress nitrification, utilizing the toposequence, government policy, and appropriate agricultural practices. Of all the technologies presented, use of nitrification inhibitors and controlled release fertilizers are deemed the most important with further development of these aspects of technologies being expected. These practices, if employed worldwide, could help reduce the load, or environmental deterioration, on the Earth's biosphere.展开更多
Energy consumption increases with intensity of human activities. People consume energy for movement and other activities and the more fossil-fuel based energy used, the more carbon dioxide (CO2) emission. Since carbon...Energy consumption increases with intensity of human activities. People consume energy for movement and other activities and the more fossil-fuel based energy used, the more carbon dioxide (CO2) emission. Since carbon dioxide is the major element of the greenhouse gases (GHG), this phenomenon has a serious implication for global warming and consequent climate change—a scenario that calls for sustainable development. This research considers the emission of CO2 from energy use within the campus of Universiti Teknologi Malaysia. Two major sources of energy consumption were identified, namely: electricity and transport. The emission for electricity was estimated based on electricity meter reading and the conversion rate in accordance with the stand-ardized conversion factors for fuel mix of the purchased electric energy as given by PTM (Pusat Tenaga Malaysia), while the associated CO2 emission for transport was estimated based on the number of miles driven (VMT—Vehicle Miles Travel) within the campus, emissions produced per litre of gasoline, and fuel economy of vehicles plying the campus in line with the Code of Federal Regulations USEPA and consistent with the Inter-governmental Panel on Climate Change (IPCC) guidelines. It was observed that high CO2 emission resulted from electricity energy consumption, and the highest emission in the transport sector was produced by commuting vehicles while emission from service delivery for cooling, lighting and other equipment was similar to national average.展开更多
Optical emission spectroscopy in nitrogen glow discharge plasma is simulated, and the collision excitations and characteristic emissions of the species (N2, N2^+, N^+, N) are investigated by a Monte Carlo model fo...Optical emission spectroscopy in nitrogen glow discharge plasma is simulated, and the collision excitations and characteristic emissions of the species (N2, N2^+, N^+, N) are investigated by a Monte Carlo model for nitrogen molecular gas discharge. The excitation rates of the main excited states are calculated and the corresponding relation and relative magnitude between the distribution of excitation rate of a certain excited state and the distributions of the emission rates of various lines originating from this excited level are also explored. The simulated results are compared with the experimental measurements in two typical discharge conditions. The luminescence mechanism of the line N2^+: 391.4 nm is explained based on the microscopic plasma processes. The cathode glow in N2 discharge is found to be mainly caused by N^+ impact excitation and the intensity of cathode glow decreases with the voltage. The corresponding relation between the emission rate or intensity of the 391.4 nm line and the production rate and the density of N2^+ is also examined.展开更多
文摘The steel industry is a major source of CO_(2) emissions,and thus,the mitigation of carbon emissions is the most pressing challenge in this sector.In this paper,international environmental governance in the steel industry is reviewed,and the current state of development of low-carbon technologies is discussed.Additionally,low-carbon pathways for the steel industry at the current time are proposed,emphasizing prevention and treatment strategies.Furthermore,the prospects of low-carbon technologies are explored from the perspective of transitioning the energy structure to a“carbon-electricity-hydrogen”relationship.Overall,steel enterprises should adopt hydrogen-rich metallurgical technologies that are compatible with current needs and process flows in the short term,based on the carbon substitution with hydrogen(prevention)and the CCU(CO_(2) capture and utilization)concepts(treatment).Additionally,the capture and utilization of CO_(2) for steelmaking,which can assist in achieving short-term emission reduction targets but is not a long-term solution,is discussed.In conclusion,in the long term,the carbon metallurgical process should be gradually supplanted by a hydrogen-electric synergistic approach,thus transforming the energy structure of existing steelmaking processes and attaining near-zero carbon emission steelmaking technology.
文摘Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.However,two-photon pumped amplified spontaneous emission(ASE)and the corresponding nonlinear optical properties of FAPbBr_(3) NCs are scarcely revealed.Herein,we synthesized colloidal FAPbBr_(3) NCs with different sizes by changing the molar ratio of FABr/PbBr_(2) in the precursor solution,using ligand assisted precipitation(LARP)technology at room temperature.Photoluminescence(PL)and time resolved photoluminescence(TRPL)spectroscopy were measured to characterize their ASE properties.And their nonlinear optical properties were studied through the Zscan technique and the two-photon excited fluorescence method.The stimulated emission properties including oneand two-photon pumped ASE have been realized from FAPbBr_(3) NCs.With large two-photon absorption coefficient(0.27 cm/GW)and high non-linear absorption cross-section(7.52×10^(5) GM),ASE with threshold as low as 9.8μJ/cm^(2) and 487μJ/cm^(2) have been obtained from colloidal FAPbBr_(3) NCs using one-and two-photon excitations.These results indicate that as a new possible green-emitting frequency-upconversion material with low thresholds,FAPbBr_(3) NCs hold great potential in the development of high-performance two-photon pump lasers.
基金the National Natural Science Foundation of China(52378460 and 51878526)the Program Fund of Non-metallic Excellent and Innovation Center for Building Materials(Grants 2024TDA-3)Knowledge Innovation Program of Wuhan-Basic Research from the Wuhan Science and Technology Bureau(2022020801010176)are gratefully acknowledged.
文摘Recently, researchers in the road field are focusing on the development of green asphalt materials with loweremission of volatile organic compounds (VOCs). The characterization methodology of asphalt VOCs and theinfluencing factors on VOCs release have always been the basic issue of asphalt VOCs emission reduction research.Researchers have proposed a variety of asphalt VOCs characterization methodologies, which also have mutuallyirreplaceable characteristics. Asphalt VOCs volatilization is affected by many factors. In this study, asphalt VOCscharacterization methodologies were summarized, including their advantages, disadvantages, characteristics andapplicable requirements. Subsequently, the influencing factors of VOCs release, such as asphalt types and environment conditions, are summarized to provide theoretical support for the emission reduction research. Theclassification and mechanism of newly-development asphalt VOCs emission reduction materials are reviewed. Thereduction efficiencies are also compared to select better materials and put forward the improvement objective ofnew materials and new processes. In addition, the prospects about development of VOCs release mechanism ofasphalt materials during the full life cycle and feasibility research of high-efficiency composite emission reductionmaterials in the future were put forward.
基金financially supported by the National Natural Science Foundation of China(Nos.52274315 and 52374320)the Fundamental Research Funds for the Central Universities(Nos.FRF-TP-22-011A1 and FRF-DF22-16)。
文摘During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.
文摘In Fused Filament Fabrication(FFF),the state of material flow significantly influences printing outcomes.However,online monitoring of these micro-physical processes within the extruder remains challenging.The flow state is affected by multiple parameters,with temperature and volumetric flow rate(VFR)being the most critical.The study explores the stable extrusion of flow with a highly sensitive acoustic emission(AE)sensor so that AE signals generated by the friction in the annular region can reflect the flow state more effectively.Nevertheless,the large volume and broad frequency range of the data present processing challenges.This study proposes a method that initially selects short impact signals and then uses the Fast Kurtogram(FK)to identify the frequency with the highest kurtosis for signal filtration.The results indicate that this approach significantly enhances processing speed and improves feature extraction capabilities.By correlating AE characteristics under various parameters with the quality of extruded raster beads,AE can monitor the real-time state of material flow.This study offers a concise and efficient method for monitoring the state of raster beads and demonstrates the potential of online monitoring of the flow states.
基金supported by the Research Project of the Shanghai Health Commission,No.2020YJZX0111(to CZ)the National Natural Science Foundation of China,Nos.82021002(to CZ),82272039(to CZ),82171252(to FL)+1 种基金a grant from the National Health Commission of People’s Republic of China(PRC),No.Pro20211231084249000238(to JW)Medical Innovation Research Project of Shanghai Science and Technology Commission,No.21Y11903300(to JG).
文摘Nowadays,presynaptic dopaminergic positron emission tomography,which assesses deficiencies in dopamine synthesis,storage,and transport,is widely utilized for early diagnosis and differential diagnosis of parkinsonism.This review provides a comprehensive summary of the latest developments in the application of presynaptic dopaminergic positron emission tomography imaging in disorders that manifest parkinsonism.We conducted a thorough literature search using reputable databases such as PubMed and Web of Science.Selection criteria involved identifying peer-reviewed articles published within the last 5 years,with emphasis on their relevance to clinical applications.The findings from these studies highlight that presynaptic dopaminergic positron emission tomography has demonstrated potential not only in diagnosing and differentiating various Parkinsonian conditions but also in assessing disease severity and predicting prognosis.Moreover,when employed in conjunction with other imaging modalities and advanced analytical methods,presynaptic dopaminergic positron emission tomography has been validated as a reliable in vivo biomarker.This validation extends to screening and exploring potential neuropathological mechanisms associated with dopaminergic depletion.In summary,the insights gained from interpreting these studies are crucial for enhancing the effectiveness of preclinical investigations and clinical trials,ultimately advancing toward the goals of neuroregeneration in parkinsonian disorders.
基金the author is wishing to express his gratitude to the National Natural Science Foundation of China(2002CB410807)for subsiding this research.
文摘Ammonia emission is one of the most important pathways of nitrogen loss from agricultural cultivated field. In this paper, we report the measurement of ammonia emission from paddy rice field obtained by surface application of urea fertilizer with water management. The main objective of the present study were to assess the amount of NH3 emission and the loss of nitrogen from paddy field as affected by various N doses, i.e., 0 (control), 90 (N1), 180 (N2), 270 (N3) and 360 (N4) kg ha-1, following field surface application of urea fertilizer with water management. Ammonia emissions were measured by continuous airflow enclosure method from plots fertilized with the application of surface urea. Increase in urea-N dosage increased NH3 emission that was measured from paddy rice field. Ammonia emission started immediately and was almost complete within 12 days after top dressing of urea application to the soils. Ammonia emissions were nearly constant in all treatments from 12 days after fertilizer application. Highest ammonia emission rate was 28 g /day and total amount of ammonia emission was 56.21 kg ha-1 for 360 kg N ha-1 dose. No remarkable observation was found about temperature for ammonia emission. Due to proper water management practices less emission was observed throughout the experiment period. The results also show that N loss through NH3 emission accounted for 11 to 16% during the rice- growing season. These magnitudes of loss of N appear to be most important for environmental point of view.
文摘This paper takes the climate change and low carbon economy development as the study background, based on the analysis of energy demand and carbon emissions status, which is aimed to provide the low carbon development path in Chinese cities. The method of scenario analysis can be used to predict long-term strategy for the uncertainty future development, and it was introduced to the field of social forecasting and public policy research, such as the environmental strategic planning, policy analysis, and support of decision in resource management, which can be used to explore the possible development trend and target of the results from the macro perspective. Scenario analysis has been gradually applied to the study area on low carbon economy, energy forecasting and other fields in recent years, and there have been many research results in different aspects. This paper takes the scenario analysis as basic study theory, spreading out the present situation of its application in low carbon city and some issues that need further study. As a tool for predicting the future development in low carbon city, the method of scenario analysis has been providing a powerful reference for policies and their executants.
基金supported by the New Century Talent Foundation of Ministry of Education of China (NCET-08-0438)
文摘Characteristics of electron emission induced by a surface flashover trigger device in a low-pressure trigger switch were investigated. A test method to measure the emitted charges from the trigger device was developed, and the factors affecting the emitted charges were analyzed. The results indicated that the major emitted charges from the trigger device were induced by surface plasma generated by surface flashover occurring on the trigger dielectric material. The emitted charges and the peak emission current increased linearly with the change in the trigger voltage and bias voltage. The emitted charges collected from the anode were affected by the gap distance. However, the emitted charges were less affected by the anode diameter. Furthermore, the emitted charges and the peak emission current decreased rapidly with the increase in gas pressure in a range from 0 Pa to 100 Pa, and then remained stable or changed slightly when the increase in gas pressure up to 2400 Pa.
基金the National Basic Research Program (973) of China (No.2002CB410807).
文摘The study was conducted to investigate the N2O emissions and dissolved N2O in the leachate during the nonflooding period in nongrowing paddy fields.Three kinds of paddy soils were repacked to soil columns and were supersaturated with water initially and dried gradually in a greenhouse to attain the N2O emissions flux during the incubation.Soils with the texture of silty clay-loam (Q and H) produced cracks during the drying of soil,but soil with the texture of silty loam (X) did not form the cracks.Cracked s...
基金This work was financially supported by the National Science Foundation of China(No.59971011) and the "973" Item of China(No.1999
文摘In order to investigate the effect of hydrogen attack degree on acoustic emission(AE) behavior of low carbon steel during tensiling, specimens made of Low carbon steel was exposed to hydrogen gas of 18 MPa at 450 and 500℃ for 240, 480 and 720 h respectively. Experimental results show that with increase of the hydrogen attack degree, the totally AE activity decreases during tensiling. In addition, the count of AE signals with high amplitude for the specimens with hydrogen attack keeps a constant which is less than that without hydrogen attack. It is concluded that AE signals originate in the specimens with hydrogen attack from intergranular fracture induced by methane blisterings or/and microcracks on grain boundaries.
基金supported by the National Natural Science Foundation of China (41874194, 41521063, 41374168)
文摘Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-frequency chorus emissions have not been well understood..In this letter, we report an interesting case in which background plasma density lowered the lower cutoff frequency of chorus emissions from above 0.1 f_(ce)(typical ordinary chorus) to 0.02 f_(ce)(extremely low-frequency chorus).Those extremely low-frequency chorus waves were observed in a rather dense plasma, where the number density N_e was found to be several times larger than has been associated with observations of ordinary chorus waves.For suprathermal electrons whose free energy is supplied by anisotropic temperatures, linear growth rates(calculated using in-situ plasma parameters measured by the Van Allen Probes) show that whistler mode instability can occur at frequencies below 0.1 f_(ce) when the background plasma density N_e increases.Especially when N_e reaches 90 cm–3 or more, the lowest unstable frequency can extend to 0.02 f_(ce) or even less, which is consistent with satellite observations.Therefore, our results demonstrate that a dense background plasma could play an essential role in the excitation of extremely lowfrequency chorus waves by controlling the wave growth rates.
基金supported by the Key Technologies R&D Program of China during the 12th Five-year Plan period(2012BAD14B16-04)the Science and Technology Development Program of Guangdong,China(2012A020100003 and 2015B090903077)
文摘The increasing demand for fresh sweet maize (Zea mays L. saccharata) in southern China has prioritized the need to find solutions to the environmental pollution caused by its continuous production and high inputs of chemical nitrogen fertilizers. A promising method for improving crop production and environmental conditions is to intercrop sweet maize with legumes. Here, a three-year field experiment was conducted to assess the influence of four different cropping systems (sole sweet maize (SS), sole soybean (SB), two rows sweet maize-three rows soybean (S2B3) intercropping, and two rows sweet maize-four rows soybean (S2B4) intercropping), together with two rates of N fertilizer application (300 and 360 kg N ha-1) on grain yield, residual soil mineral N, and soil N2O emissions in southern China. Results showed that in most case, inter- cropping achieved yield advantages (total land equivalent ratio (TLER=0.87-1.25) was above one). Moreover, intercropping resulted in 39.8% less soil mineral N than SS at the time of crop harvest, averaged over six seasons (spring and autumn in each of the three years of the field experiment). Generally, intercropping and reduced-N application (300 kg N ha-1) produced lower cumulative soil N20 and yield-scaled soil N20 emissions than SS and conventionaI-N application (360 kg N ha-l), respectively. $2B4 intercropping with reduced-N rate (300 kg N ha-~) showed the lowest cumulative soil N20 (mean value=0.61 kg ha-1) and yield-scaled soil N20 (mean value=0.04 kg t-1) emissions. Overall, intercropping with reduced-N rate maintained sweet maize production, while also reducing environmental impacts. The system of S2B4 intercropping with reduced-N rate may be the most sustainable and environmentally friendly cropping system.
基金supported by UAEM 2260/06, UAEM 2362/2006U, PROMEP FE018/2003 of Mexico
文摘Optical emission spectroscopy was used to study a gas mixture glow discharge of CO2 and N2 at a total pressure of 1.2 Torr, a power of 100 W and a flow of 16.5 L/min. The emission bands were measured in the wavelength range of 200 nm to 900 nm. The principal species observed were O2^+ (A^2П→ X^2П), CO^+ (A^2П→X^2∑), N2^+ (B^2∑u+ → X^2∑g^+), CO2^+ (A^2∏ → X^2∏), N2(C^3∏u → B^3∏g), O2(b^1∑g^+→ X^3∑g^-), and CO (a^r3∑→a^3∏). The behavior of the band intensities as a function of the N2 percentage is consistent with recent Monte Carlo simulations. The electron temperature and ion density were determined by a double Langmuir probe. The electron temperature was found in the range of 1.55 eV to 2.93 eV, and the electron concentration in the order of 10^10 cm^-3. The electron temperature and ion density at pure N2 and pure CO2 agree with previous measurements.
基金This work was supported by the Hundred Talents Program launched by the Chinese Academy of Sciencesthe National Key Basic Research Development Foundation of China(G1999011805).
文摘A split-plot experiment in a rice-winter wheat rotation system was performed to study the effects of water regime and wheat straw application in rice-growing season on N2O emission from following wheat growing season. Water regime in the rice-growing season was designed as the conventional irrigation (flooding/drainage cycle) and the permanent flooding. Wheat straw was incorporated with three rates of 0, 225 and 450 g m-2 into the paddy soil for each water regime just before rice was transplanted. N2O emission was measured by static chamber-gas chromatograph method. Results from the variance analysis indicated that the permanent flooding in rice-growing season markedly enhanced N2O emission in following wheat growing season (P=0. 003), and that the effect of straw application on N2O emission was distinguished between two water regimes. Under the conventional irrigation, incoporation of wheat straw reduced N2O emission in the following wheat growing season, while there were no significant differences in the emission for the straw application rates of 225 and 450 g m-2. No significant differences in N2O emissions were observed among the three rates of straw application for the permanent flooding regime. In addition, the seasonal variation of N2O emission was regulated by soil temperature and moisture. The daily N2O flux (Y, mg m-2 d-1) can be quantitatively described by soil temperature (T, ℃) and moisture (W, WFPS %) asY=A0+A1T+A2W+A3W2(n=23, R2 ≥0. 4159** )or y=C0+C1W+C2W2(n=23,R2≥0. 4074** ). Compared with the effect of soil temperature on N2O emission, soil moisture was an important factor regulating the seasonal pattern of N2O emission.
基金supported by National Natural Science Foundation of China under Grant No. 71001010Fundamental Research Funds for Central Universities under Grant No.2009RC1001
文摘Based on the revised reduction models of the 14 low-carbon ICT solutions from Chongqing Mobile of the China Mobile Group,the CO2e emission reduction brought about by low-carbon ICTs of the wireless telecom sector of Chongqing Mobile,the entire China Mobile Group and the whole China in 2009 is calculated.And then the CO2e emission reduction potentials in 2010,2020 and 2030 are calculated in four main important fields of China,i.e.,intelligent transportation,dematerialization,smart work and smart appliances.The ICTs in the telecom sector are mostly dedicated to these fields.It provides a valuable insight into future reduction targets that should be set up for China.
基金We thank National Key R&D Program of China(2016YFA0602601),National Natural Science Foundation of China(71573062),China Energy Modeling Forum(CEMF),for support of the study.
文摘A quantitative model was applied to analyze the energy demand and CO2 emissions in China following the Energy Production and Consumption Revolution Strategy(2016e2030)and long-term economic and social development target China Dream.Results showed that 1)toward the 2050 China Dream target,total final energy consumption is expected to peak at 3.9 Gtce in 2030 and remain stable until 2050,whereas total primary energy consumption is expected to reach an upper platform by 2040 and around 5.8 Gtce by 2050;2)the proportion of non-fossil fuels is expected to reach approximately 50%and that of natural gas to reach more than 16%by 2050;3)CO2 emissions from energy use are expected to peak at 9.6 Gt by no later than 2030 and then gradually decline to 6.7 Gt by 2050.
基金Project supported by the Canadian International Development Agency, Canada and the Chinese Academy of Scicences, China (No. KZCX2-413)
文摘To feed an increasing population, large amounts of chemical nitrogen fertilizer have been used to produce much of our food, feed and fiber thereby increasing nitrogen levels in soils, natural waters, crop residues, livestock wastes,and municipal and agricultural wastes, with national and international concern about its potential adverse effects on environmental quality and public health. To understand these phenomena and problems, first the nitrogen cycle and the environment are described. Then recent trends for nitrogen cycling through the food and feed system, N2O emissions from fertilized upland and paddy soils, and NO-3 pollution in ground water in Japan are reported. Finally, mitigation strategies in Japan for reducing N2O emission and NO-3 pollution are proposed, including nitrification inhibitors, controlled release fertilizers, utilization of plant species that could suppress nitrification, utilizing the toposequence, government policy, and appropriate agricultural practices. Of all the technologies presented, use of nitrification inhibitors and controlled release fertilizers are deemed the most important with further development of these aspects of technologies being expected. These practices, if employed worldwide, could help reduce the load, or environmental deterioration, on the Earth's biosphere.
文摘Energy consumption increases with intensity of human activities. People consume energy for movement and other activities and the more fossil-fuel based energy used, the more carbon dioxide (CO2) emission. Since carbon dioxide is the major element of the greenhouse gases (GHG), this phenomenon has a serious implication for global warming and consequent climate change—a scenario that calls for sustainable development. This research considers the emission of CO2 from energy use within the campus of Universiti Teknologi Malaysia. Two major sources of energy consumption were identified, namely: electricity and transport. The emission for electricity was estimated based on electricity meter reading and the conversion rate in accordance with the stand-ardized conversion factors for fuel mix of the purchased electric energy as given by PTM (Pusat Tenaga Malaysia), while the associated CO2 emission for transport was estimated based on the number of miles driven (VMT—Vehicle Miles Travel) within the campus, emissions produced per litre of gasoline, and fuel economy of vehicles plying the campus in line with the Code of Federal Regulations USEPA and consistent with the Inter-governmental Panel on Climate Change (IPCC) guidelines. It was observed that high CO2 emission resulted from electricity energy consumption, and the highest emission in the transport sector was produced by commuting vehicles while emission from service delivery for cooling, lighting and other equipment was similar to national average.
基金Natural Science Foundation of Hebei Province of China(Nos.A2006000123,F2006000183)
文摘Optical emission spectroscopy in nitrogen glow discharge plasma is simulated, and the collision excitations and characteristic emissions of the species (N2, N2^+, N^+, N) are investigated by a Monte Carlo model for nitrogen molecular gas discharge. The excitation rates of the main excited states are calculated and the corresponding relation and relative magnitude between the distribution of excitation rate of a certain excited state and the distributions of the emission rates of various lines originating from this excited level are also explored. The simulated results are compared with the experimental measurements in two typical discharge conditions. The luminescence mechanism of the line N2^+: 391.4 nm is explained based on the microscopic plasma processes. The cathode glow in N2 discharge is found to be mainly caused by N^+ impact excitation and the intensity of cathode glow decreases with the voltage. The corresponding relation between the emission rate or intensity of the 391.4 nm line and the production rate and the density of N2^+ is also examined.