Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-freq...Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-frequency chorus emissions have not been well understood..In this letter, we report an interesting case in which background plasma density lowered the lower cutoff frequency of chorus emissions from above 0.1 f_(ce)(typical ordinary chorus) to 0.02 f_(ce)(extremely low-frequency chorus).Those extremely low-frequency chorus waves were observed in a rather dense plasma, where the number density N_e was found to be several times larger than has been associated with observations of ordinary chorus waves.For suprathermal electrons whose free energy is supplied by anisotropic temperatures, linear growth rates(calculated using in-situ plasma parameters measured by the Van Allen Probes) show that whistler mode instability can occur at frequencies below 0.1 f_(ce) when the background plasma density N_e increases.Especially when N_e reaches 90 cm–3 or more, the lowest unstable frequency can extend to 0.02 f_(ce) or even less, which is consistent with satellite observations.Therefore, our results demonstrate that a dense background plasma could play an essential role in the excitation of extremely lowfrequency chorus waves by controlling the wave growth rates.展开更多
Low-frequency flicker noise is usually associated with material defects or imperfection of fabrication procedure. Up to now, there is only very limited knowledge about flicker noise of the topological insulator, whose...Low-frequency flicker noise is usually associated with material defects or imperfection of fabrication procedure. Up to now, there is only very limited knowledge about flicker noise of the topological insulator, whose topologically protected conducting surface is theoretically immune to back scattering. To suppress the bulk conductivity we synthesize antimony doped Bi2Se3 nanowires and conduct transport measurements at cryogenic temperatures. The low-frequency current noise measurement shows that the noise amplitude at the high-drain current regime can be described by Hooge＇s empirical relationship, while the noise level is significantly lower than that predicted by Hooge＇s model near the Dirac point. Furthermore, different frequency responses of noise power spectrum density for specific drain currents at the low drain current regime indicate the complex origin of noise sources of topological insulator.展开更多
In this work, we designed and synthesized cationic carbon dots(CDs) with a size distribution of 1.6–3.7 nm, which exhibited dark blue fluorescence in the aqueous solution. Based on its excellent luminescence properti...In this work, we designed and synthesized cationic carbon dots(CDs) with a size distribution of 1.6–3.7 nm, which exhibited dark blue fluorescence in the aqueous solution. Based on its excellent luminescence properties, we used it as an energy donor to construct a sequential artificial light-harvesting system(LHS) by employing the energy-matching dyes eosin Y disodium salt(EY) and sulforhodamine101(SR101), which could regulate the white light emission(Commission Internationale de l'Eclairage(CIE) coordinate:(0.30, 0.31)) with the energy transfer efficiency(ΦET) of 53.9% and 20.0%. Moreover, a single-step artificial LHS with white light emission(0.32, 0.28) can be constructed directly using CDs and dye solvent 43(SR) with ΦETand antenna effect(AE) of 48.8% and 6.5, respectively. More importantly,CDs-based artificial LHSs were firstly used in photocatalytic of α-bromoacetophenone, with a yield of90%. This work not only provides a new strategy for constructing CDs-based LHSs, but also opens up a new application for further applying the energy harvested in CDs-based LHSs to the field of the aqueous solution photocatalysis.展开更多
基金supported by the National Natural Science Foundation of China (41874194, 41521063, 41374168)
文摘Low-frequency chorus emissions have recently attracted much attention due to the suggestion that they may play important roles in the dynamics of the Van Allen Belts.However, the mechanism(s) generating these low-frequency chorus emissions have not been well understood..In this letter, we report an interesting case in which background plasma density lowered the lower cutoff frequency of chorus emissions from above 0.1 f_(ce)(typical ordinary chorus) to 0.02 f_(ce)(extremely low-frequency chorus).Those extremely low-frequency chorus waves were observed in a rather dense plasma, where the number density N_e was found to be several times larger than has been associated with observations of ordinary chorus waves.For suprathermal electrons whose free energy is supplied by anisotropic temperatures, linear growth rates(calculated using in-situ plasma parameters measured by the Van Allen Probes) show that whistler mode instability can occur at frequencies below 0.1 f_(ce) when the background plasma density N_e increases.Especially when N_e reaches 90 cm–3 or more, the lowest unstable frequency can extend to 0.02 f_(ce) or even less, which is consistent with satellite observations.Therefore, our results demonstrate that a dense background plasma could play an essential role in the excitation of extremely lowfrequency chorus waves by controlling the wave growth rates.
基金Supported by the National Basic Research Program of China under Grant No 2012CB921703the National Natural Science Foundation of China under Grant Nos 11174357 and 11574379the Strategic Priority Research Program of Chinese Academy of Sciences under Grant No XDB07010300
文摘Low-frequency flicker noise is usually associated with material defects or imperfection of fabrication procedure. Up to now, there is only very limited knowledge about flicker noise of the topological insulator, whose topologically protected conducting surface is theoretically immune to back scattering. To suppress the bulk conductivity we synthesize antimony doped Bi2Se3 nanowires and conduct transport measurements at cryogenic temperatures. The low-frequency current noise measurement shows that the noise amplitude at the high-drain current regime can be described by Hooge＇s empirical relationship, while the noise level is significantly lower than that predicted by Hooge＇s model near the Dirac point. Furthermore, different frequency responses of noise power spectrum density for specific drain currents at the low drain current regime indicate the complex origin of noise sources of topological insulator.
基金the financial support from the National Natural Science Foundation of China (Nos.52205210 and 22002075)the Natural Science Foundation of Shandong Province (Nos.ZR2020MB018 and ZR2022QE033)。
文摘In this work, we designed and synthesized cationic carbon dots(CDs) with a size distribution of 1.6–3.7 nm, which exhibited dark blue fluorescence in the aqueous solution. Based on its excellent luminescence properties, we used it as an energy donor to construct a sequential artificial light-harvesting system(LHS) by employing the energy-matching dyes eosin Y disodium salt(EY) and sulforhodamine101(SR101), which could regulate the white light emission(Commission Internationale de l'Eclairage(CIE) coordinate:(0.30, 0.31)) with the energy transfer efficiency(ΦET) of 53.9% and 20.0%. Moreover, a single-step artificial LHS with white light emission(0.32, 0.28) can be constructed directly using CDs and dye solvent 43(SR) with ΦETand antenna effect(AE) of 48.8% and 6.5, respectively. More importantly,CDs-based artificial LHSs were firstly used in photocatalytic of α-bromoacetophenone, with a yield of90%. This work not only provides a new strategy for constructing CDs-based LHSs, but also opens up a new application for further applying the energy harvested in CDs-based LHSs to the field of the aqueous solution photocatalysis.
基金supported by the National Natural Science Foundation of China (21103135, 21173165, 21073139)Natural Science Basic Research Plan in Shaanxi Province of China (2011JQ2011)+1 种基金Scientific Research Program Funded by Shaanxi Provincial Education Commission, China (12JK0622)Foundation of Xi'an University of Science and Technology, China (2010QDJ030)~~
