Nuclear-spin states of gaseous-state Cs atoms in the ground state are optically manipulated using a Ti:sapphire laser in a magnetic field of 1.516 T, in which optical coupling of the nuclear-spin states is achieved t...Nuclear-spin states of gaseous-state Cs atoms in the ground state are optically manipulated using a Ti:sapphire laser in a magnetic field of 1.516 T, in which optical coupling of the nuclear-spin states is achieved through hyperfine interactions between electrons and nuclei. The steady-state population distribution in the hyperfine Zeeman sublevels of the ground state is detected by using a tunable diode laser. Furthermore, the state population transfer among the hyperfine Zeeman sublevels, which results from the collision-induced modification δa(S·I) of the hyperfine interaction of Cs in the ground state due to stochastic collisions between Cs atoms and buffer-gas molecules, is studied at different buffer-gas pressures. The experimental results show that high-field optical pumping and the small change δa(S · I) of the hyperfine interaction can strongly cause the state population transfer and spin-state interchange among the hyperfine Zeeman sublevels. The calculated results maybe explain the steady-state population in hyperfine Zeeman sublevels in terms of rates of optical-pumping, electron-spin flip, nuclear spin flip, and electron-nuclear spin flip-flop transitions among the hyperfine Zeeman sublevels of the ground state of Cs atoms. This method may be applied to the nuclear-spin-based solid-state quantum computation.展开更多
The high-spin states of 141pro nucleus have been studied by using in-beam v-ray spectroscopy technology through the126Te(19F, 4n) reaction at a beam energy of 90 MeV. The previous level scheme has been extended with...The high-spin states of 141pro nucleus have been studied by using in-beam v-ray spectroscopy technology through the126Te(19F, 4n) reaction at a beam energy of 90 MeV. The previous level scheme has been extended with spin up to 49/2 h. Many new levels and transitions are identified. Five collective band structures are observed. Based on systematic comparison with the neighboring nuclei, two bands with strong AI = 1 M1 transitions inside the bands are proposed as the oblate bands with γ--60°, and three bands with large signature splitting have been suggested as the oblate-triaxial deformation with γ--90°. The characteristics for these bands have been discussed.展开更多
-A truncated shell model approach is presented for studying the properties oflow-lying states as well as the high-spin states in even-even nuclei with the help of thegeneralized boson-fermion expansion technique.The p...-A truncated shell model approach is presented for studying the properties oflow-lying states as well as the high-spin states in even-even nuclei with the help of thegeneralized boson-fermion expansion technique.The primary fermion state space isspanned by the interacting valence protons and neutrons with effective nucleon-nucleonforce.The truncated model space is considered as a direct sum of two subspaces corre-sponding to the configurations of(sd)<sup>N</sup> and(sd)<sup>N-1</sup>,respectively,plus a broken fermionpair.Numerical calculations are carried out for <sup>130~134</sup>Ce isotopes.The calculated spec-trum reproduces the experimental data quite well,especially the backbending appearingin these nuclei.The results suggest that the approach is able to describe the spectroscopyof states with angular momenta up to J≈20.展开更多
A truncated shell model approach is applied to the description of high-spinstates for <sup>162</sup>Hf and <sup>164</sup>Hf isotopes.The backbends of the moment of inertia are repro-duced well ...A truncated shell model approach is applied to the description of high-spinstates for <sup>162</sup>Hf and <sup>164</sup>Hf isotopes.The backbends of the moment of inertia are repro-duced well by the calculation.The results show that the approach is able to investigatethe yrast states of nuclei in rare earth region.展开更多
We study the spatiotemporal Bloch states of a high-frequency driven two-component Bose–Einstein condensate(BEC)with spin–orbit coupling(SOC) in an optical lattice. By adopting the rotating-wave approximation(RWA) an...We study the spatiotemporal Bloch states of a high-frequency driven two-component Bose–Einstein condensate(BEC)with spin–orbit coupling(SOC) in an optical lattice. By adopting the rotating-wave approximation(RWA) and applying an exact trial-solution to the corresponding quasistationary system, we establish a different method for tuning SOC via external field such that the existence conditions of the exact particular solutions are fitted. Several novel features related to the exact states are demonstrated; for example, SOC leads to spin–motion entanglement for the spatiotemporal Bloch states, SOC increases the population imbalance of the two-component BEC, and SOC can be applied to manipulate the stable atomic flow which is conducive to control quantum transport of the BEC for different application purposes.展开更多
The high spin states of 106pd have been populated through the 100Mo(11B, lp4n)106Pd reaction using a beam energy of 60 MeV provided by the Beijing HI-13 tandem accel- erator at China Institute of Atomic Energy. By a...The high spin states of 106pd have been populated through the 100Mo(11B, lp4n)106Pd reaction using a beam energy of 60 MeV provided by the Beijing HI-13 tandem accel- erator at China Institute of Atomic Energy. By analyzing the V-3' coincidence relation and DCO raios of transitions, 3 rotational bands with 13 new states and 22 new 7 transitions belonging to 106pd were constructed. Bands 2 and 3 with negative parity were supposed to build on the vh1l/297/2 and vh11/2ds/2 configuration, respectively.展开更多
Experiments including C-13 spin-lattice relaxation, C-13 heteronuclear dipolar dephasing and H-1 spin diffusion are performed on poly (2,6-dimethyl-1,4-phenylene oxide) (PPO). The results show that the rotation of the...Experiments including C-13 spin-lattice relaxation, C-13 heteronuclear dipolar dephasing and H-1 spin diffusion are performed on poly (2,6-dimethyl-1,4-phenylene oxide) (PPO). The results show that the rotation of the methyl groups in solid PPO is partially restricted, which results in a surprisingly efficient spin diffusion between the aromatic proton and methyl proton characterized by a diffusion time of 150 mu s. The results also show that the aromatic ring in solid PPO is rigid and twisted, which causes all aromatic carbons to be chemically unequivalent.展开更多
High spin states of 84Sr were populated through the reaction 70Zn(18O,4n)84Sr at 75 MeV beam energy.Measurement of excitation function,γ-γ coincidences,directional correlation from oriented state (DCO) ratios and γ...High spin states of 84Sr were populated through the reaction 70Zn(18O,4n)84Sr at 75 MeV beam energy.Measurement of excitation function,γ-γ coincidences,directional correlation from oriented state (DCO) ratios and γ-transition intensities were performed using eight anticompton HPGe detectors and one planar HPGe detector.Based on the measured results,a new level scheme of 84Sr was established in which 12 new states and nearly 30 new γ-transitions were identified in the present work.The positive-parity states of the new level scheme were compared with the results from calculations in the framework of the projected shell model (PSM).One negative-parity band was extended to spin Iπ=19-and it can be found that in the high spin states,the γ-transition energies show the nature of signature staggering.The negative-parity band levels are in good agreement with deformed configuration-mixing shell model (DCM) calculations.展开更多
The high-spin states in 128I have been studied by using in-beam γ-ray spectroscopy with the 124Sn(7Li,3n)128I reaction at beam energies of 25, 28 and 42 MeV. A new level scheme including 20 new levels and 27 new γ-t...The high-spin states in 128I have been studied by using in-beam γ-ray spectroscopy with the 124Sn(7Li,3n)128I reaction at beam energies of 25, 28 and 42 MeV. A new level scheme including 20 new levels and 27 new γ-transitions for 128I has been established preliminarily.展开更多
Excited states in the odd-A nucleus 71Ga have been studied via the ^(70)Zn(7Li,a2n)^(71)Ga fusion-evaporation reaction with incident beam energies of 30 and 35 MeV.The level scheme is established up to spin I^(n)=(29/...Excited states in the odd-A nucleus 71Ga have been studied via the ^(70)Zn(7Li,a2n)^(71)Ga fusion-evaporation reaction with incident beam energies of 30 and 35 MeV.The level scheme is established up to spin I^(n)=(29/2^(+))and an excitation energy-6.6 MeV.A previously known sequence built on the 9/2^(+) state is extended as a novel rotational band originating from the v(8^(2)_(9/2)alignment.Furthermore,a negative-parity sequence Is also reported.The observed energy levels of Ga have been interpreted in the framework of the nuclear shell model(SM).展开更多
High-spin states of 156Yb have been studied via the 144Sm(16O,4n)156Yb fusion-evaporation reaction at beam energy 102 MeV. The positive-parity yrast band and negative-parity cascade have been extended up to higher-spi...High-spin states of 156Yb have been studied via the 144Sm(16O,4n)156Yb fusion-evaporation reaction at beam energy 102 MeV. The positive-parity yrast band and negative-parity cascade have been extended up to higher-spin states, respectively. The characteristics of the negative-parity sequence above the 25-state may related to the excitation from the nucleon in the Z =64, N =82 core. The E-GOS curve for the positiveparity yrast sequence in 156Yb indicate that this nucleus may undergo an evolution from quasivibrational to quasirotational structure with increasing angular momentum. The Cranked Woods-Saxon-Strutinsky calculations by means of Total-Routhian-Surface (TRS) methods has been made to understand this structure change.展开更多
High-spin states in 161Er have been studied experimentally using the 150Nd(16O, 5n) reaction at a beam energy of 86 MeV. The relatively enhanced E1 transitions between the 5/2+[642] and 3/2-[521] bands are observed...High-spin states in 161Er have been studied experimentally using the 150Nd(16O, 5n) reaction at a beam energy of 86 MeV. The relatively enhanced E1 transitions between the 5/2+[642] and 3/2-[521] bands are observed in 161Er, and the B(E1) values are extracted experimentally. The systematics of the R(E1) values in the N = 93 isotones are presented. It is found that the strength of the E1 transitions obviously exhibits angular momentum dependence, and the occurrence of the relatively enhanced E1 transitions could be attributed to octupole softness.展开更多
The N≈Z nuclei in the mass A^80 region has been researched because of an abundance of nuclear structure phenomena.The projected shell model(PSM)was adopted to investigate the structure of high spin state in proton-ri...The N≈Z nuclei in the mass A^80 region has been researched because of an abundance of nuclear structure phenomena.The projected shell model(PSM)was adopted to investigate the structure of high spin state in proton-rich 74,76,78Kr isotopes including yrast spectra,moment of inertia,electric quadrupole transitions and the behavior of single particle.The calculated results are in good agreement with available data and the shape coexistence in low-spin is also discussed.展开更多
Four new heterotrinuclear complexes have been synthesized and characterized, namely {[Ni(L)2]2[Cu(opba)]}(ClO4)2, where opba denotes o-phenylenebis(oxamato) and L stands for 1,10-phenanthroline(phen) (1), 5-nitro-1,10...Four new heterotrinuclear complexes have been synthesized and characterized, namely {[Ni(L)2]2[Cu(opba)]}(ClO4)2, where opba denotes o-phenylenebis(oxamato) and L stands for 1,10-phenanthroline(phen) (1), 5-nitro-1,10-phenanthroline(NO2-phen) (2), 2,2'-bipyridyl(bpy) (3) and 4,4'-dimethyl-2,2'-bipyridyl(Me2bpy) (4). The temperature dependence of the magnetic susceptibility of {[Ni(phen)2]2[Cu(opba)]}(ClO4)2.3H2O has been studied in the 4-300 K range, giving the exchange integral J=-109 cm-1. The MT vs. T plot exhibits a minimum at about 100 K, characteristic of this kind of coupled polymetallic complex with an irregular spin-state structure.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos 10374103 and 10574143), and the National Basic Research Program of China (Grant No 2001CB309309).
文摘Nuclear-spin states of gaseous-state Cs atoms in the ground state are optically manipulated using a Ti:sapphire laser in a magnetic field of 1.516 T, in which optical coupling of the nuclear-spin states is achieved through hyperfine interactions between electrons and nuclei. The steady-state population distribution in the hyperfine Zeeman sublevels of the ground state is detected by using a tunable diode laser. Furthermore, the state population transfer among the hyperfine Zeeman sublevels, which results from the collision-induced modification δa(S·I) of the hyperfine interaction of Cs in the ground state due to stochastic collisions between Cs atoms and buffer-gas molecules, is studied at different buffer-gas pressures. The experimental results show that high-field optical pumping and the small change δa(S · I) of the hyperfine interaction can strongly cause the state population transfer and spin-state interchange among the hyperfine Zeeman sublevels. The calculated results maybe explain the steady-state population in hyperfine Zeeman sublevels in terms of rates of optical-pumping, electron-spin flip, nuclear spin flip, and electron-nuclear spin flip-flop transitions among the hyperfine Zeeman sublevels of the ground state of Cs atoms. This method may be applied to the nuclear-spin-based solid-state quantum computation.
基金supported by National Natural Science Foundation of China (Nos. 10975082, 10775078)the Major State Basic Research Development Program of China (No. 2007CB815005)the Special Program of Higher Education Science Foundation of China (No. 20070003149)
文摘The high-spin states of 141pro nucleus have been studied by using in-beam v-ray spectroscopy technology through the126Te(19F, 4n) reaction at a beam energy of 90 MeV. The previous level scheme has been extended with spin up to 49/2 h. Many new levels and transitions are identified. Five collective band structures are observed. Based on systematic comparison with the neighboring nuclei, two bands with strong AI = 1 M1 transitions inside the bands are proposed as the oblate bands with γ--60°, and three bands with large signature splitting have been suggested as the oblate-triaxial deformation with γ--90°. The characteristics for these bands have been discussed.
文摘-A truncated shell model approach is presented for studying the properties oflow-lying states as well as the high-spin states in even-even nuclei with the help of thegeneralized boson-fermion expansion technique.The primary fermion state space isspanned by the interacting valence protons and neutrons with effective nucleon-nucleonforce.The truncated model space is considered as a direct sum of two subspaces corre-sponding to the configurations of(sd)<sup>N</sup> and(sd)<sup>N-1</sup>,respectively,plus a broken fermionpair.Numerical calculations are carried out for <sup>130~134</sup>Ce isotopes.The calculated spec-trum reproduces the experimental data quite well,especially the backbending appearingin these nuclei.The results suggest that the approach is able to describe the spectroscopyof states with angular momenta up to J≈20.
文摘A truncated shell model approach is applied to the description of high-spinstates for <sup>162</sup>Hf and <sup>164</sup>Hf isotopes.The backbends of the moment of inertia are repro-duced well by the calculation.The results show that the approach is able to investigatethe yrast states of nuclei in rare earth region.
基金Project supported by the National Natural Science Foundation of China(Grant No.11475060)
文摘We study the spatiotemporal Bloch states of a high-frequency driven two-component Bose–Einstein condensate(BEC)with spin–orbit coupling(SOC) in an optical lattice. By adopting the rotating-wave approximation(RWA) and applying an exact trial-solution to the corresponding quasistationary system, we establish a different method for tuning SOC via external field such that the existence conditions of the exact particular solutions are fitted. Several novel features related to the exact states are demonstrated; for example, SOC leads to spin–motion entanglement for the spatiotemporal Bloch states, SOC increases the population imbalance of the two-component BEC, and SOC can be applied to manipulate the stable atomic flow which is conducive to control quantum transport of the BEC for different application purposes.
基金supported by the Major State Basic Research Development Program (2007CB815000)by National Natural Science Foundation of China (Nos. 11075214,10927507, 10975191, 10675171, 10105015, 10375092, 10575133, 11175259)
文摘The high spin states of 106pd have been populated through the 100Mo(11B, lp4n)106Pd reaction using a beam energy of 60 MeV provided by the Beijing HI-13 tandem accel- erator at China Institute of Atomic Energy. By analyzing the V-3' coincidence relation and DCO raios of transitions, 3 rotational bands with 13 new states and 22 new 7 transitions belonging to 106pd were constructed. Bands 2 and 3 with negative parity were supposed to build on the vh1l/297/2 and vh11/2ds/2 configuration, respectively.
文摘Experiments including C-13 spin-lattice relaxation, C-13 heteronuclear dipolar dephasing and H-1 spin diffusion are performed on poly (2,6-dimethyl-1,4-phenylene oxide) (PPO). The results show that the rotation of the methyl groups in solid PPO is partially restricted, which results in a surprisingly efficient spin diffusion between the aromatic proton and methyl proton characterized by a diffusion time of 150 mu s. The results also show that the aromatic ring in solid PPO is rigid and twisted, which causes all aromatic carbons to be chemically unequivalent.
基金supported by the Major State Basic Research Development Program in China (Grant No. 2007CB815003)the National Natural Science Foundation of China (Grant Nos. 11065001, 10547140, 10525520,60476043,10675170,10475002 and 10775064)+4 种基金the U.S. National Science Foundation (Grant No. 0500291)the Southeastern Universities Research Association,the Natural Science Foundation of Jiangxi Province (Grant Nos. 0612003 and 2007GZW0476)the LSU - LNNU Joint Research Program (Grant No. 9961)the Foundation of the Education Department of Jiangxi Province (Grant No. [2007]235)the Liaoning Education Department Fund (Grant No. 20060464)
文摘High spin states of 84Sr were populated through the reaction 70Zn(18O,4n)84Sr at 75 MeV beam energy.Measurement of excitation function,γ-γ coincidences,directional correlation from oriented state (DCO) ratios and γ-transition intensities were performed using eight anticompton HPGe detectors and one planar HPGe detector.Based on the measured results,a new level scheme of 84Sr was established in which 12 new states and nearly 30 new γ-transitions were identified in the present work.The positive-parity states of the new level scheme were compared with the results from calculations in the framework of the projected shell model (PSM).One negative-parity band was extended to spin Iπ=19-and it can be found that in the high spin states,the γ-transition energies show the nature of signature staggering.The negative-parity band levels are in good agreement with deformed configuration-mixing shell model (DCM) calculations.
基金Supported by Major State Basic Research Development Program (2007CB815000)National Natural Science Foundation of China (10775184, 10675171, 10575133, 10575092, 10375092)
文摘The high-spin states in 128I have been studied by using in-beam γ-ray spectroscopy with the 124Sn(7Li,3n)128I reaction at beam energies of 25, 28 and 42 MeV. A new level scheme including 20 new levels and 27 new γ-transitions for 128I has been established preliminarily.
基金Supported by the National Natural Science Foundation of China(U1932209,11975315,U1867210,11905134)the Leading Innovation Project under Grant(LC192209000701,LC202309000201)+1 种基金the Continuous Basic Scientific Research Project(BJ20002501,WDJC-2019-13)China National Nuclear Corporation(FA18000201)。
文摘Excited states in the odd-A nucleus 71Ga have been studied via the ^(70)Zn(7Li,a2n)^(71)Ga fusion-evaporation reaction with incident beam energies of 30 and 35 MeV.The level scheme is established up to spin I^(n)=(29/2^(+))and an excitation energy-6.6 MeV.A previously known sequence built on the 9/2^(+) state is extended as a novel rotational band originating from the v(8^(2)_(9/2)alignment.Furthermore,a negative-parity sequence Is also reported.The observed energy levels of Ga have been interpreted in the framework of the nuclear shell model(SM).
基金Supported by National Natural Science Foundation of China (10405001, 10775005, 10735010, 10605001, J0730316)Chinese Major State Basic Research Development Program (2007CB815002)
文摘High-spin states of 156Yb have been studied via the 144Sm(16O,4n)156Yb fusion-evaporation reaction at beam energy 102 MeV. The positive-parity yrast band and negative-parity cascade have been extended up to higher-spin states, respectively. The characteristics of the negative-parity sequence above the 25-state may related to the excitation from the nucleon in the Z =64, N =82 core. The E-GOS curve for the positiveparity yrast sequence in 156Yb indicate that this nucleus may undergo an evolution from quasivibrational to quasirotational structure with increasing angular momentum. The Cranked Woods-Saxon-Strutinsky calculations by means of Total-Routhian-Surface (TRS) methods has been made to understand this structure change.
基金Supported by National Natural Science Foundation of China (10825522, 10735010, 10575120)National Basic Research Program of China (2007CB815001)Chinese Academy of Sciences
文摘High-spin states in 161Er have been studied experimentally using the 150Nd(16O, 5n) reaction at a beam energy of 86 MeV. The relatively enhanced E1 transitions between the 5/2+[642] and 3/2-[521] bands are observed in 161Er, and the B(E1) values are extracted experimentally. The systematics of the R(E1) values in the N = 93 isotones are presented. It is found that the strength of the E1 transitions obviously exhibits angular momentum dependence, and the occurrence of the relatively enhanced E1 transitions could be attributed to octupole softness.
基金supported by the National Natural Science Foundation of China(Grant Nos.11305059,11275067,11275068 and 11135005)
文摘The N≈Z nuclei in the mass A^80 region has been researched because of an abundance of nuclear structure phenomena.The projected shell model(PSM)was adopted to investigate the structure of high spin state in proton-rich 74,76,78Kr isotopes including yrast spectra,moment of inertia,electric quadrupole transitions and the behavior of single particle.The calculated results are in good agreement with available data and the shape coexistence in low-spin is also discussed.
基金Project supported by the National Natural Science Foundation of China and 21st Century Youth Foundation of Tianjin,China.
文摘Four new heterotrinuclear complexes have been synthesized and characterized, namely {[Ni(L)2]2[Cu(opba)]}(ClO4)2, where opba denotes o-phenylenebis(oxamato) and L stands for 1,10-phenanthroline(phen) (1), 5-nitro-1,10-phenanthroline(NO2-phen) (2), 2,2'-bipyridyl(bpy) (3) and 4,4'-dimethyl-2,2'-bipyridyl(Me2bpy) (4). The temperature dependence of the magnetic susceptibility of {[Ni(phen)2]2[Cu(opba)]}(ClO4)2.3H2O has been studied in the 4-300 K range, giving the exchange integral J=-109 cm-1. The MT vs. T plot exhibits a minimum at about 100 K, characteristic of this kind of coupled polymetallic complex with an irregular spin-state structure.