Two nonstoichiometric UAu_(1-x)Sb_2(x = 0.25, 0.1) single crystals are successfully synthesized using a flux method,and their physical properties are comprehensively studied by measuring the dc-magnetization and elect...Two nonstoichiometric UAu_(1-x)Sb_2(x = 0.25, 0.1) single crystals are successfully synthesized using a flux method,and their physical properties are comprehensively studied by measuring the dc-magnetization and electrical resistivity. Evidence for at least three magnetic phases is found in these samples. In zero field, both samples undergo an antiferromagnetic transition at a relatively high temperature, and with further cooling they pass through another antiferromagnetic phase,before reaching a ferromagnetic ground state. Furthermore, the magnetic order can be tuned by varying the site occupation of Au. Such a tunable magnetic order may provide an opportunity for exploring the potential quantum critical behavior in this system.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11874330,11504342,11504341,and U1630248)the National Key R&D Program of China(Grant No.2017YFA0303104)the Science Challenge Project,China(Grant No.TZ2016004)
文摘Two nonstoichiometric UAu_(1-x)Sb_2(x = 0.25, 0.1) single crystals are successfully synthesized using a flux method,and their physical properties are comprehensively studied by measuring the dc-magnetization and electrical resistivity. Evidence for at least three magnetic phases is found in these samples. In zero field, both samples undergo an antiferromagnetic transition at a relatively high temperature, and with further cooling they pass through another antiferromagnetic phase,before reaching a ferromagnetic ground state. Furthermore, the magnetic order can be tuned by varying the site occupation of Au. Such a tunable magnetic order may provide an opportunity for exploring the potential quantum critical behavior in this system.
