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MXene Hybridized Polymer with Enhanced Electromagnetic Energy Harvest for Sensitized Microwave Actuation and Self‑Powered Motion Sensing
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作者 Yu‑Ze Wang Yu‑Chang Wang +3 位作者 Ting‑Ting Liu Quan‑Liang Zhao Chen‑Sha Li Mao‑Sheng Cao 《Nano-Micro Letters》 SCIE EI CAS 2025年第3期265-279,共15页
Polymeric microwave actuators combining tissue-like softness with programmablemicrowave-responsive deformation hold great promise for mobile intelligentdevices and bionic soft robots. However, their application is cha... Polymeric microwave actuators combining tissue-like softness with programmablemicrowave-responsive deformation hold great promise for mobile intelligentdevices and bionic soft robots. However, their application is challenged by restricted electromagneticsensitivity and intricate sensing coupling. In this study, a sensitized polymericmicrowave actuator is fabricated by hybridizing a liquid crystal polymer with Ti3C2Tx(MXene). Compared to the initial counterpart, the hybrid polymer exhibits unique spacechargepolarization and interfacial polarization, resulting in significant improvements of230% in the dielectric loss factor and 830% in the apparent efficiency of electromagneticenergy harvest. The sensitized microwave actuation demonstrates as the shortenedresponse time of nearly 10 s, which is merely 13% of that for the initial shape memory polymer. Moreover, the ultra-low content of MXene (upto 0.15 wt%) benefits for maintaining the actuation potential of the hybrid polymer. An innovative self-powered sensing prototype that combinesdriving and piezoelectric polymers is developed, which generates real-time electric potential feedback (open-circuit potential of ~ 3 mV) duringactuation. The polarization-dominant energy conversion mechanism observed in the MXene-polymer hybrid structure furnishes a new approachfor developing efficient electromagnetic dissipative structures and shows potential for advancing polymeric electromagnetic intelligent devices. 展开更多
关键词 microwave absorption Electromagnetic response Energy harvest SELF-SENSING Soft actuator
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Magneto‑Dielectric Synergy and Multiscale Hierarchical Structure Design Enable Flexible Multipurpose Microwave Absorption and Infrared Stealth Compatibility
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作者 Chen Li Leilei Liang +2 位作者 Baoshan Zhang Yi Yang Guangbin Ji 《Nano-Micro Letters》 SCIE EI CAS 2025年第2期401-416,共16页
Developing advanced stealth devices to cope with radar-infrared(IR)fusion detection and diverse application scenarios is increasingly demanded,which faces significant challenges due to conflicting microwave and IR clo... Developing advanced stealth devices to cope with radar-infrared(IR)fusion detection and diverse application scenarios is increasingly demanded,which faces significant challenges due to conflicting microwave and IR cloaking mechanisms and functional integration limitations.Here,we propose a multiscale hierarchical structure design,integrating wrinkled MXene IR shielding layer and flexible Fe_(3)O_(4)@C/PDMS microwave absorption layer.The top wrinkled MXene layer induces the intensive diffuse reflection effect,shielding IR radiation signals while allowing microwave to pass through.Meanwhile,the permeable microwaves are assimilated into the bottom Fe_(3)O_(4)@C/PDMS layer via strong magneto-electric synergy.Through theoretical and experimental optimization,the assembled stealth devices realize a near-perfect stealth capability in both X-band(8–12 GHz)and long-wave infrared(8–14μm)wavelength ranges.Specifically,it delivers a radar cross-section reduction of−20 dB m^(2),a large apparent temperature modulation range(ΔT=70℃),and a low average IR emissivity of 0.35.Additionally,the optimal device demonstrates exceptional curved surface conformability,self-cleaning capability(contact angle≈129°),and abrasion resistance(recovery time≈5 s).This design strategy promotes the development of multispectral stealth technology and reinforces its applicability and durability in complex and hostile environments. 展开更多
关键词 microwave absorption Radar-infrared compatible stealth Wrinkled MXene Magneto-dielectric synergy MULTIFUNCTION
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TRIPLET combined with microwave ablation:A novel treatment for advanced hepatocellular carcinoma
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作者 Fei-Yu Zhao Guo-Wei Si Nian-Song Qian 《World Journal of Gastrointestinal Oncology》 SCIE 2025年第1期10-12,共3页
This editorial comments on a study by Zuo et al.The focus is on the efficacy of he-patic arterial infusion chemotherapy combined with camrelizumab and apatinib(the TRIPLET regimen),alongside microwave ablation therapy... This editorial comments on a study by Zuo et al.The focus is on the efficacy of he-patic arterial infusion chemotherapy combined with camrelizumab and apatinib(the TRIPLET regimen),alongside microwave ablation therapy,in treating advanced hepatocellular carcinoma(HCC).The potential application of this combination therapy for patients with advanced HCC is evaluated. 展开更多
关键词 microwave ablation Hepatic arterial infusion chemotherapy Apatinib Camrelizumab Hepatocellular carcinoma
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Structural and microwave absorption properties of CoFe_(2)O_(4)/residual carbon composites
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作者 Yuanchun Zhang Shengtao Gao +3 位作者 Xingzhao Zhang Dacheng Ma Chuanlei Zhu Jun He 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS 2025年第1期221-232,共12页
Electromagnetic interference,which necessitates the rapid advancement of substances with exceptional capabilities for bsorbing electromagnetic waves,is of urgent concern in contemporary society.In this work,CoFe_(2)O_... Electromagnetic interference,which necessitates the rapid advancement of substances with exceptional capabilities for bsorbing electromagnetic waves,is of urgent concern in contemporary society.In this work,CoFe_(2)O_(4)/residual carbon from coal gasification fine slag(CFO/RC)composites were created using a novel hydrothermal method.Various mechanisms for microwave absorption,including conductive loss,natural resonance,interfacial dipole polarization,and magnetic flux loss,are involved in these composites.Consequently,compared with pure residual carbon materials,this composite offers superior capabilities in microwave absorption.At 7.76GHz,the CFO/RC-2 composite achieves an impressive minimum reflection loss(RL_(min))of-43.99 dB with a thickness of 2.44 mm.Moreover,CFO/RC-3 demonstrates an effective absorption bandwidth(EAB)of up to 4.16 GHz,accompanied by a thickness of 1.18mm.This study revealed the remarkable capability of the composite to diminish electromagnetic waves,providing a new generation method for microwave absorbing materials of superior quality. 展开更多
关键词 coal gasification slag residual carbon hydrothermal method microwave absorption CoFe_(2)O_(4)
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Efficacy and safety of C-arm computed tomography-guided microwave ablation with percutaneous osteoplasty for flat bone metastases
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作者 Zhi-Peng Lin Xu-Gong Zou +4 位作者 Da-Bei Huang Yuan Chen Jia-Wen Lin Xiao-Qun Li Jian Zhang 《World Journal of Clinical Oncology》 2025年第3期40-48,共9页
BACKGROUND Flat bone metastases are common in patients with advanced cancers,often resulting in severe pain,limited mobility,and reduced quality of life(QOL).Traditional treatment options,such as radiotherapy or syste... BACKGROUND Flat bone metastases are common in patients with advanced cancers,often resulting in severe pain,limited mobility,and reduced quality of life(QOL).Traditional treatment options,such as radiotherapy or systemic therapies,often fail to provide sufficient pain relief or improve functional outcomes in these patients.Microwave ablation(MWA)offers advantages,such as shorter pro-cedure times and larger ablation zones,while percutaneous osteoplasty(PO)enhances bone stability and prevents pathological fractures.Despite these be-nefits,the combination of these techniques for treating flat bone metastases re-mains underexplored.AIM To evaluate the efficacy and safety of C-arm computed tomography(CT)-guided MWA combined with PO for managing painful flat bone metastases,focusing on pain relief,functional improvement,and QOL enhancement.METHODS A total of 45 patients with refractory moderate-to-severe pain resulting from flat bone metastases who underwent C-arm CT-guided MWA combined with PO between January 2015 and January 2021 were included.The efficacy of the pro-cedure was assessed by changes in the visual analog scale(VAS),Oswestry disability index(ODI),and QOL,as well as the occurrence of complications.Tumor response was evaluated using RECIST v1.1 and mRECIST criteria,with overall response rate(ORR)and disease control rate(DCR)as the primary end-points.RESULTS No serious complications were observed in any of the patients.A significant reduction in VAS and ODI was noted at 1 week,1 month,and 3 months post-procedure.A marked improvement in QOL was observed at all follow-up points.Bone cement extravasation was observed in 10 patients;however,none exhibited significant clinical symptoms.Based on RECIST v1.1,the ORR was 26.7%and the DCR was 88.9%.The mRECIST evaluation revealed a higher ORR of 51.1%and DCR of 88.9%.CONCLUSION C-arm CT-guided MWA with PO provides a dependable and effective strategy for managing flat bone metastases.It demonstrates significant pain relief,improved functional outcomes,and enhanced QOL.This treatment combination also shows promising tumor response rates with a low complication profile. 展开更多
关键词 microwave ablation Percutaneous osteoplasty Bone metastases EFFICACY SAFETY
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An efficient process for decomposing perfluorinated compounds by reactive species during microwave discharge in liquid
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作者 Shaohua SUN Bing SUN +3 位作者 Zhonglin YU Qiuying WANG Yuanyuan WANG Jinglin LIU 《Plasma Science and Technology》 2025年第1期93-102,共10页
Microwave discharge plasma in liquid(MDPL)is a new type of water purification technology with a high mass transfer efficiency.It is a kind of low-temperature plasma technology.The reactive species produced by the disc... Microwave discharge plasma in liquid(MDPL)is a new type of water purification technology with a high mass transfer efficiency.It is a kind of low-temperature plasma technology.The reactive species produced by the discharge can efficiently act on the pollutants.To clarify the application prospects of MDPL in water treatment,the discharge performance,practical application,and pollutant degradation mechanism of MDPL were studied in this work.The effects of power,conductivity,pH,and Fe^(2+)concentration on the amount of reactive species produced by the discharge were explored.The most common and refractory perfluorinated compounds(perfluorooctanoic acid(PFOA)and perfluorooctane sulfonate(PFOS)in water environments are degraded by MDPL technology.The highest defluorination of PFOA was 98.8% and the highest defluorination of PFOS was 92.7%.The energy consumption efficiency of 50% defluorination(G_(50-F))of PFOA degraded by MDPL is 78.43 mg/kWh,PFOS is 42.19 mg/kWh.The results show that the MDPL technology is more efficient and cleaner for the degradation of perfluorinated compounds.Finally,the reaction path and pollutant degradation mechanisms of MDPL production were analyzed.The results showed that MDPL technology can produce a variety of reactive species and has a good treatment effect for refractory perfluorinated pollutants. 展开更多
关键词 microwave discharge plasma in liquid reactive species PURIFICATION
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A new Q-band comb-based multi-channel microwave Doppler backward scattering diagnostic developed on the HL-3 tokamak
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作者 Ruihai TONG Yu ZHOU +8 位作者 Wulyu ZHONG Jie WEN Zhongbing SHI Xiaolan ZOU Anshu LIANG Zengchen YANG Min JIANG Xin YU Yuqi SHEN 《Plasma Science and Technology》 2025年第1期23-29,共7页
The Doppler backscattering(DBS)diagnostic is widely used to measure the localized density fluctuations and the propagation velocity of turbulent structures.Microwave is launched at a frequency that approaches a cutoff... The Doppler backscattering(DBS)diagnostic is widely used to measure the localized density fluctuations and the propagation velocity of turbulent structures.Microwave is launched at a frequency that approaches a cutoff layer in the plasma at an angle oblique to the cutoff layer.A new Q-band multichannel DBS system based on a comb generator has been designed and tested for application on the HL-3 tokamak.With the comb generator and heterodyne scheme,the stability and flexibility of the new DBS system are improved.The new DBS diagnostic has a high output power(~10 dBm),good power flatness(<5 dB in Q-band),and frequency stability,and the inter-frequency separation is tunable remotely.This article introduces the system design,laboratory test results,and initial experimental results from the HL-3 tokamak.With the help of the newly developed multichannel DBS,the turbulence information can be studied with high temporal and spatial resolution. 展开更多
关键词 Doppler backscattering(DBS) microwave diagnostic turbulence TOKAMAK
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Microwave irradiation-induced deterioration of rock mechanical properties and implications for mechanized hard rock excavation
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作者 Zheng Yang Ming Tao +2 位作者 Muhammad Burhan Memon Dengdeng Zhuang Yan Zhao 《Journal of Rock Mechanics and Geotechnical Engineering》 2025年第1期275-290,共16页
In this study,a novel microwave-water cooling-assisted mechanical rock breakage method was proposed to address the issues of severe tool wear at elevated temperatures,poor rock microwave absorption,and excessive micro... In this study,a novel microwave-water cooling-assisted mechanical rock breakage method was proposed to address the issues of severe tool wear at elevated temperatures,poor rock microwave absorption,and excessive microwave energy consumption.The investigation object was sandstone,which was irradiated at 4 kW microwave power for 60 s,180 s,300 s,and 420 s,followed by air and water cooling.Subsequently,uniaxial compression,Brazilian tension,and fracture tests were conducted.The evolution of damage in sandstone was measured using active and passive nondestructive acoustic detection methods.The roughness of the fracture surfaces of the specimens was quantified using the box-counting method.The damage mechanisms of microwave heating and water cooling on sandstone were discussed from both macroscopic and microscopic perspectives.The experimental results demonstrated that as the duration of the microwave irradiation increased,the P-wave velocity,uniaxial compressive strength(UCS),elastic modulus(E),tensile strength,and fracture toughness of sandstone exhibited various degrees of weakness and were further weakened by water cooling.Furthermore,an increase in the microwave irradiation duration enhanced the damaging effect of water cooling.The P-wave velocity of the sandstone was proportional to the mechanical parameters.Microwave heating and water cooling weakened the brittleness of the sandstone to a certain extent.The fractal dimension of the fracture surface was correlated with the duration of microwave heating,and the water-cooling treatment resulted in a rougher fracture surface.An analysis of the instantaneous cutting rate revealed that water cooling can substantially enhance the efficiency of microwave-assisted rock breakage. 展开更多
关键词 Hard rock breakage microwave irradiation Water cooling Acoustic testing Fractal dimension Instantaneous cutting rate
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Microwave ablation for liver metastases from colorectal cancer:A comprehensive review of clinical efficacy and safety
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作者 Fang Li Yuan-Yuan Zhang +1 位作者 Ming Li Sheng-Kai Chen 《World Journal of Gastrointestinal Surgery》 2025年第1期32-40,共9页
Microwave ablation(MWA)is emerging as a highly effective treatment for colorectal liver metastases(CRLMs).This review explores the advantages of MWA compared to other ablative techniques such as radiofrequency ablatio... Microwave ablation(MWA)is emerging as a highly effective treatment for colorectal liver metastases(CRLMs).This review explores the advantages of MWA compared to other ablative techniques such as radiofrequency ablation and cryoablation and highlights its clinical efficacy,safety,and technical considerations.MWA offers significant benefits,including higher intratumoral temperatures,larger ablation zones,and reduced susceptibility to the heat-sink effect,which make it particularly suitable for tumors near large blood vessels.This review details the patient selection criteria,procedural approaches,and the use of advanced imaging techniques to improve the precision and effectiveness of MWA.Clinical outcomes indicate that MWA achieves high rates of complete tumor ablation and long-term survival with a favorable safety profile.This review is significant because it provides updated insights into the expanding role of MWA in treating unresectable CRLM and its potential as an alternative to surgical resection for resectable tumors.By summarizing recent studies and clinical trials,this review highlights the comparative effectiveness,safety,and integration with systemic therapies of MWA.In conclusion,MWA is a promising treatment option for CRLM and offers outcomes comparable to or better than those of other ablative techniques.Future research should focus on optimizing technical parameters,integrating MWA with systemic therapies,and conducting large-scale randomized controlled trials to establish standardized treatment protocols.Advancing our understanding of MWA will enhance its application and improve long-term survival and quality of life for patients with CRLM. 展开更多
关键词 microwave ablation Colorectal liver metastases Thermal ablation techniques Clinical outcomes Tumor ablation safety
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Impact of Linggui Zhugan decoction on microwave ablation outcomes and recurrence in liver cancer
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作者 Rui Huang Jing Cui 《World Journal of Gastrointestinal Oncology》 2025年第2期105-118,共14页
BACKGROUND Liver cancer is one of the most common malignant tumors of the digestive system,and early detection and effective treatment are crucial for improving the prognosis.Microwave ablation(MWA)has shown promising... BACKGROUND Liver cancer is one of the most common malignant tumors of the digestive system,and early detection and effective treatment are crucial for improving the prognosis.Microwave ablation(MWA)has shown promising results as a local therapeutic method for liver cancer;however,further improvement of its efficacy remains a key focus of current research.AIM To evaluate the clinical efficacy of Linggui Zhugan decoction combined with MWA for the treatment of primary liver cancer.METHODS Data were collected from 164 patients with primary liver cancer who underwent MWA at our hospital between March 2019 and April 2021.Among them,79 patients(control group)received routine treatments and 85 patients(research group)received Linggui Zhugan decoction in addition to routine treatment.The clinical efficacy,incidence of adverse reactions,and levels of serum alphafetoprotein(AFP),des-γ-carboxy prothrombin(DCP),AFP-L3,total bilirubin(TBil),alanine aminotransferase(ALT),CD4 cell count,CD8 cell count,and CD4/CD8 ratio were compared between the two groups,before and after treatment.The three-year recurrence rates between the two groups were compared,and independent prognostic factors for recurrence were identified.RESULTS The study results revealed that the objective response rate(ORR)in the research group was significantly higher than that in the control group(P=0.005).After treatment,the CD4 cell count and CD4/CD8 ratio significantly increased,whereas the CD8 cell count and TBil,ALT,AFP,DCP,and AFP-L3 Levels were significantly lower in the research group than in the control group(P<0.001).The Cox regression analysis revealed that the treatment regimen(P=0.003),presence of cirrhosis(P=0.019),tumor diameter(P=0.037),Child-Pugh score(P=0.003),pretreatment AFP level(P=0.006),and AFP-L3 Level(P=0.002)were independent prognostic factors for disease-free survival.CONCLUSION The combination of Linggui Zhugan decoction with MWA significantly improved the clinical efficacy and longterm prognosis of patients with primary liver cancer. 展开更多
关键词 Primary liver cancer microwave ablation Linggui Zhugan decoction Clinical efficacy Disease-free survival Cox regression analysis
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MXene Hollow Spheres Supported by a C–Co Exoskeleton Grow MWCNTs for Efficient Microwave Absorption 被引量:3
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作者 Ze Wu Xiuli Tan +4 位作者 Jianqiao Wang Youqiang Xing Peng Huang Bingjue Li Lei Liu 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第6期76-94,共19页
High-performance microwave absorption(MA) materials must be studied immediately since electromagnetic pollution has become a problem that cannot be disregarded. A straightforward composite material, comprising hollow ... High-performance microwave absorption(MA) materials must be studied immediately since electromagnetic pollution has become a problem that cannot be disregarded. A straightforward composite material, comprising hollow MXene spheres loaded with C–Co frameworks, was prepared to develop multiwalled carbon nanotubes(MWCNTs). A high impedance and suitable morphology were guaranteed by the C–Co exoskeleton, the attenuation ability was provided by the MWCNTs endoskeleton, and the material performance was greatly enhanced by the layered core–shell structure. When the thickness was only 2.04 mm, the effective absorption bandwidth was 5.67 GHz, and the minimum reflection loss(RLmin) was-70.70 d B. At a thickness of 1.861 mm, the sample calcined at 700 ℃ had a RLmin of-63.25 d B. All samples performed well with a reduced filler ratio of 15 wt%. This paper provides a method for making lightweight core–shell composite MA materials with magnetoelectric synergy. 展开更多
关键词 MXene C-Co skeleton MWCNTS microwave absorption
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Enhancing Low-Frequency Microwave Absorption Through Structural Polarization Modulation of MXenes 被引量:3
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作者 Bo Shan Yang Wang +1 位作者 Xinyi Ji Yi Huang 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第10期435-452,共18页
Two-dimensional carbon-based materials have shown promising electromagnetic wave absorption capabilities in mid-and high-frequency ranges,but face challenges in low-frequency absorption due to limited control over pol... Two-dimensional carbon-based materials have shown promising electromagnetic wave absorption capabilities in mid-and high-frequency ranges,but face challenges in low-frequency absorption due to limited control over polarization response mecha-nisms and ambiguous resonance behavior.In this study,we pro-pose a novel approach to enhance absorption efficiency in aligned three-dimensional(3D)MXene/CNF(cellulose nanofibers)cavities by modifying polarization properties and manipulating resonance response in the 3D MXene architecture.This controlled polarization mechanism results in a significant shift of the main absorption region from the X-band to the S-band,leading to a remarkable reflection loss value of-47.9 dB in the low-frequency range.Furthermore,our findings revealed the importance of the oriented electromagnetic coupling in influencing electromagnetic response and microwave absorption properties.The present study inspired us to develop a generic strategy for low-frequency tuned absorption in the absence of magnetic element participation,while orientation-induced polarization and the derived magnetic resonance coupling are the key controlling factors of the method. 展开更多
关键词 Hierarchical structure MXene microwave absorption LOW-FREQUENCY
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Compositional and Hollow Engineering of Silicon Carbide/Carbon Microspheres as High-Performance Microwave Absorbing Materials with Good Environmental Tolerance 被引量:4
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作者 Lixue Gai Yahui Wang +5 位作者 Pan Wan Shuping Yu Yongzheng Chen Xijiang Han Ping Xu Yunchen Du 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期128-146,共19页
Microwave absorbing materials(MAMs)characterized by high absorption efficiency and good environmental tolerance are highly desirable in practical applications.Both silicon carbide and carbon are considered as stable M... Microwave absorbing materials(MAMs)characterized by high absorption efficiency and good environmental tolerance are highly desirable in practical applications.Both silicon carbide and carbon are considered as stable MAMs under some rigorous conditions,while their composites still fail to produce satisfactory microwave absorption performance regardless of the improvements as compared with the individuals.Herein,we have successfully implemented compositional and structural engineering to fabricate hollow Si C/C microspheres with controllable composition.The simultaneous modulation on dielectric properties and impedance matching can be easily achieved as the change in the composition of these composites.The formation of hollow structure not only favors lightweight feature,but also generates considerable contribution to microwave attenuation capacity.With the synergistic effect of composition and structure,the optimized SiC/C composite exhibits excellent performance,whose the strongest reflection loss intensity and broadest effective absorption reach-60.8 dB and 5.1 GHz,respectively,and its microwave absorption properties are actually superior to those of most SiC/C composites in previous studies.In addition,the stability tests of microwave absorption capacity after exposure to harsh conditions and Radar Cross Section simulation data demonstrate that hollow SiC/C microspheres from compositional and structural optimization have a bright prospect in practical applications. 展开更多
关键词 SiC/C composites Compositional engineering Hollow engineering microwave absorption Environmental tolerance
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Achieving Ultra-Broad Microwave Absorption Bandwidth Around Millimeter-Wave Atmospheric Window Through an Intentional Manipulation on Multi-Magnetic Resonance Behavior 被引量:3
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作者 Chuyang Liu Lu Xu +6 位作者 Xueyu Xiang Yujing Zhang Li Zhou Bo Ouyang Fan Wu Dong‑Hyun Kim Guangbin Ji 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期291-307,共17页
The utilization of electromagnetic waves is rapidly advancing into the millimeter-wave frequency range,posing increasingly severe challenges in terms of electromagnetic pollution prevention and radar stealth.However,e... The utilization of electromagnetic waves is rapidly advancing into the millimeter-wave frequency range,posing increasingly severe challenges in terms of electromagnetic pollution prevention and radar stealth.However,existing millimeter-wave absorbers are still inadequate in addressing these issues due to their monotonous magnetic resonance pattern.In this work,rare-earth La^(3+)and non-magnetic Zr^(4+)ions are simultaneously incorporated into M-type barium ferrite(BaM)to intentionally manipulate the multi-magnetic resonance behavior.By leveraging the contrary impact of La^(3+)and Zr^(4+)ions on magnetocrystalline anisotropy field,the restrictive relationship between intensity and frequency of the multi-magnetic resonance is successfully eliminated.The magnetic resonance peak-differentiating and imitating results confirm that significant multi-magnetic resonance phenomenon emerges around 35 GHz due to the reinforced exchange coupling effect between Fe^(3+)and Fe^(2+)ions.Additionally,Mosbauer spectra analysis,first-principle calculations,and least square fitting collectively identify that additional La^(3+)doping leads to a profound rearrangement of Zr^(4+)occupation and thus makes the portion of polarization/conduction loss increase gradually.As a consequence,the La^(3+)-Zr^(4+)co-doped BaM achieves an ultra-broad bandwidth of 12.5+GHz covering from 27.5 to 40+GHz,which holds remarkable potential for millimeter-wave absorbers around the atmospheric window of 35 GHz. 展开更多
关键词 microwave absorption Ultra-broad bandwidth M-type barium ferrite Magnetocrystalline anisotropy field Multimagnetic resonance
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Microwave shock motivating the Sr substitution of 2D porous GdFeO_(3) perovskite for highly active oxygen evolution 被引量:1
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作者 Jinglin Xian Huiyu Jiang +10 位作者 Zhiao Wu Huimin Yu Kaisi Liu Miao Fan Rong Hu Guangyu Fang Liyun Wei Jingyan Cai Weilin Xu Huanyu Jin Jun Wan 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第1期232-241,I0006,共11页
The incorporation of partial A-site substitution in perovskite oxides represents a promising strategy for precisely controlling the electronic configuration and enhancing its intrinsic catalytic activity.Conventional ... The incorporation of partial A-site substitution in perovskite oxides represents a promising strategy for precisely controlling the electronic configuration and enhancing its intrinsic catalytic activity.Conventional methods for A-site substitution typically involve prolonged high-temperature processes.While these processes promote the development of unique nanostructures with highly exposed active sites,they often result in the uncontrolled configuration of introduced elements.Herein,we present a novel approach for synthesizing two-dimensional(2D)porous GdFeO_(3) perovskite with A-site strontium(Sr)substitution utilizing microwave shock method.This technique enables precise control of the Sr content and simultaneous construction of 2D porous structures in one step,capitalizing on the advantages of rapid heating and cooling(temperature~1100 K,rate~70 K s^(-1)).The active sites of this oxygen-rich defect structure can be clearly revealed through the simulation of the electronic configuration and the comprehensive analysis of the crystal structure.For electrocatalytic oxygen evolution reaction application,the synthesized 2D porous Gd_(0.8)Sr_(0.2)FeO_(3) electrocatalyst exhibits an exceptional overpotential of 294 mV at a current density of 10 mA cm^(-2)and a small Tafel slope of 55.85 mV dec^(-1)in alkaline electrolytes.This study offers a fresh perspective on designing crystal configurations and the construction of nanostructures in perovskite. 展开更多
关键词 2D materials PEROVSKITE microwave ELECTROCATALYSIS Oxygen evolution reaction
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Microwave-assisted exploration of the electron configuration-dependent electrocatalytic urea oxidation activity of 2D porous NiCo_(2)O_(4) spinel 被引量:1
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作者 Jun Wan Zhiao Wu +11 位作者 Guangyu Fang Jinglin Xian Jiao Dai Jiayue Guo Qingxiang Li Yongfei You Kaisi Liu Huimin Yu Weilin Xu Huiyu Jiang Minggui Xia Huanyu Jin 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第4期226-235,共10页
Urea holds promise as an alternative water-oxidation substrate in electrolytic cells.High-valence nickelbased spinel,especially after heteroatom doping,excels in urea oxidation reactions(UOR).However,traditional spine... Urea holds promise as an alternative water-oxidation substrate in electrolytic cells.High-valence nickelbased spinel,especially after heteroatom doping,excels in urea oxidation reactions(UOR).However,traditional spinel synthesis methods with prolonged high-temperature reactions lack kinetic precision,hindering the balance between controlled doping and highly active two-dimensional(2D)porous structures design.This significantly impedes the identification of electron configuration-dependent active sites in doped 2D nickel-based spinels.Herein,we present a microwave shock method for the preparation of 2D porous NiCo_(2)O_(4)spinel.Utilizing the transient on-off property of microwave pulses for precise heteroatom doping and 2D porous structural design,non-metal doping(boron,phosphorus,and sulfur)with distinct extranuclear electron disparities serves as straightforward examples for investigation.Precise tuning of lattice parameter reveals the impact of covalent bond strength on NiCo_(2)O_(4)structural stability.The introduced defect levels induce unpaired d-electrons in transition metals,enhancing the adsorption of electron-donating amino groups in urea molecules.Simultaneously,Bode plots confirm the impact mechanism of rapid electron migration caused by reduced band gaps on UOR activity.The prepared phosphorus-doped 2D porous NiCo_(2)O_(4),with optimal electron configuration control,outperforms most reported spinels.This controlled modification strategy advances understanding theoretical structure-activity mechanisms of high-performance 2D spinels in UOR. 展开更多
关键词 2D materials SPINEL microwave ELECTROCATALYSIS Urea oxidation reaction
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Field test of high-power microwave-assisted mechanical excavation for deep hard iron ore 被引量:1
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作者 Feng Lin Xia-Ting Feng +5 位作者 Shiping Li Xiao Hai Jiuyu Zhang Xiangxin Su Tianyang Tong Jianchun Song 《Journal of Rock Mechanics and Geotechnical Engineering》 SCIE CSCD 2024年第6期1922-1935,共14页
Microwave-assisted mechanical excavation has great application prospects in mines and tunnels,but there are few field experiments on microwave-assisted rock breaking.This paper takes the Sishanling iron mine as the re... Microwave-assisted mechanical excavation has great application prospects in mines and tunnels,but there are few field experiments on microwave-assisted rock breaking.This paper takes the Sishanling iron mine as the research object and adopts the self-developed high-power microwave-induced fracturing test system for hard rock to conduct field experiments of microwave-induced fracturing of iron ore.The heating and reflection evolution characteristics of ore under different microwave parameters(antenna type,power,and working distance)were studied,and the optimal microwave parameters were obtained.Subsequently,the ore was irradiated with the optimal microwave parameters,and the cracking effect of the ore under the action of the high-power open microwave was analyzed.The results show that the reflection coefficient(standing wave ratio)can be rapidly(<5 s)and automatically adjusted below the preset threshold value(1.6)as microwave irradiation is performed.When using a right-angle horn antenna with a working distance of 5 cm,the effect of automatic reflection adjustment reaches the best among other antenna types and working distances.When the working distance is the same,the average temperature of the irradiation surface and the area of the high-temperature area under the action of the two antennas(right-angled and equal-angled horn antenna)are basically the same and decrease with the increase of working distance.The optimal microwave parameters are:a right-angle horn antenna with a working distance of 5 cm.Subsequently,in further experiments,the optimal parameters were used to irradiate for 20 s and 40 s at a microwave power of 60 kW,respectively.The surface damage extended 38 cm×30 cm and 53 cm×30 cm,respectively,and the damage extended to a depth of about 50 cm.The drilling speed was increased by 56.2%and 66.5%,respectively,compared to the case when microwaves were not used. 展开更多
关键词 microwave parameters High power Field experiment Mechanical mining
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Ultra-broadband microwave absorber and high-performance pressure sensor based on aramid nanofiber,polypyrrole and nickel porous aerogel 被引量:1
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作者 Leyi Zhang Hongyu Jin +7 位作者 Hanxin Liao Rao Zhang Bochong Wang Jianyong Xiang Congpu Mu Kun Zhai Tianyu Xue Fusheng Wen 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2024年第8期1912-1921,共10页
Electronic devices have become ubiquitous in our daily lives,leading to a surge in the use of microwave absorbers and wearable sensor devices across various sectors.A prime example of this trend is the aramid nanofibe... Electronic devices have become ubiquitous in our daily lives,leading to a surge in the use of microwave absorbers and wearable sensor devices across various sectors.A prime example of this trend is the aramid nanofibers/polypyrrole/nickel(APN)aerogels,which serve dual roles as both microwave absorbers and pressure sensors.In this work,we focused on the preparation of aramid nanofibers/polypyrrole(AP15)aerogels,where the mass ratio of aramid nanofibers to pyrrole was 1:5.We employed the oxidative polymerization method for the preparation process.Following this,nickel was thermally evaporated onto the surface of the AP15 aerogels,resulting in the creation of an ultralight(9.35 mg·cm^(-3)).This aerogel exhibited a porous structure.The introduction of nickel into the aerogel aimed to enhance magnetic loss and adjust impedance matching,thereby improving electromagnetic wave absorption performance.The minimum reflection loss value achieved was-48.7 dB,and the maximum effective absorption bandwidth spanned 8.42 GHz with a thickness of 2.9 mm.These impressive metrics can be attributed to the three-dimensional network porous structure of the aerogel and perfect impedance matching.Moreover,the use of aramid nanofibers and a three-dimensional hole structure endowed the APN aerogels with good insulation,flame-retardant properties,and compression resilience.Even under a compression strain of 50%,the aerogel maintained its resilience over 500 cycles.The incorporation of polypyrrole and nickel particles further enhanced the conductivity of the aerogel.Consequently,the final APN aerogel sensor demonstrated high sensitivity(10.78 kPa-1)and thermal stability.In conclusion,the APN aerogels hold significant promise as ultra-broadband microwave absorbers and pressure sensors. 展开更多
关键词 porous aerogel aramid nanofibers microwave absorbers pressure sensor porous structure
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Fusion SST from Infrared and Microwave Measurement of FY-3D Meteorological Satellite 被引量:1
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作者 张淼 徐娜 陈林 《Journal of Tropical Meteorology》 SCIE 2024年第1期89-96,共8页
Sea surface temperature(SST)is one of the important parameters of global ocean and climate research,which can be retrieved by satellite infrared and passive microwave remote sensing instruments.While satellite infrare... Sea surface temperature(SST)is one of the important parameters of global ocean and climate research,which can be retrieved by satellite infrared and passive microwave remote sensing instruments.While satellite infrared SST offers high spatial resolution,it is limited by cloud cover.On the other hand,passive microwave SST provides all-weather observation but suffers from poor spatial resolution and susceptibility to environmental factors such as rainfall,coastal effects,and high wind speeds.To achieve high-precision,comprehensive,and high-resolution SST data,it is essential to fuse infrared and microwave SST measurements.In this study,data from the Fengyun-3D(FY-3D)medium resolution spectral imager II(MERSI-II)SST and microwave imager(MWRI)SST were fused.Firstly,the accuracy of both MERSIII SST and MWRI SST was verified,and the latter was bilinearly interpolated to match the 5km resolution grid of MERSI SST.After pretreatment and quality control of MERSI SST and MWRI SST,a Piece-Wise Regression method was employed to correct biases in MWRI SST.Subsequently,SST data were selected based on spatial resolution and accuracy within a 3-day window of the analysis date.Finally,an optimal interpolation method was applied to fuse the FY-3D MERSI-II SST and MWRI SST.The results demonstrated a significant improvement in spatial coverage compared to MERSI-II SST and MWRI SST.Furthermore,the fusion SST retained true spatial distribution details and exhibited an accuracy of–0.12±0.74℃compared to OSTIA SST.This study has improved the accuracy of FY satellite fusion SST products in China. 展开更多
关键词 SST data fusion FY3 INFRARED microwave
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Abnormal uterine bleeding successfully treated via ultrasoundguided microwave ablation of uterine myoma lesions: Three case reports 被引量:1
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作者 Toshiyuki Kakinuma Kaoru Kakinuma +3 位作者 Rora Okamoto Kaoru Yanagida Michitaka Ohwada NobuhiroTakeshima 《World Journal of Clinical Cases》 SCIE 2024年第5期980-987,共8页
BACKGROUND Microwave endometrial ablation(MEA)is a minimally invasive treatment method for heavy menstrual bleeding.However,additional treatment is often required after recurrence of uterine myomas treated with MEA.Ad... BACKGROUND Microwave endometrial ablation(MEA)is a minimally invasive treatment method for heavy menstrual bleeding.However,additional treatment is often required after recurrence of uterine myomas treated with MEA.Additionally,because this treatment ablates the endometrium,it is not indicated for patients planning to become pregnant.To overcome these issues,we devised a method for ultrasound-guided microwave ablation of uterine myoma feeder vessels.We report three patients successfully treated for heavy menstrual bleeding,secondary to uterine myoma,using our novel method.CASE SUMMARY All patients had a favorable postoperative course,were discharged within 4 h,and experienced no complications.Further,no postoperative recurrence of heavy menstrual bleeding was noted.Our method also reduced the myoma’s maximum diameter.CONCLUSION This method does not ablate the endometrium,suggesting its potential appli-cation in patients planning to become pregnant. 展开更多
关键词 Uterine myoma microwave Heavy menstrual bleeding DYSMENORRHEA Fertility preservation Case report
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