Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in bio...Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in biological subjects.Current semi-implantable devices are mainly based on single-parameter detection.Miniaturized semi-implantable electrodes for multiparameter sensing have more restrictions on the electrode size due to biocompatibility considerations,but reducing the electrode surface area could potentially limit electrode sensitivity.This study developed a semi-implantable device system comprising a multiplexed microfilament electrode cluster(MMEC)and a printed circuit board for real-time monitoring of intra-tissue K^(+),Ca^(2+),and Na^(+)concentrations.The electrode surface area was less important for the potentiometric sensing mechanism,suggesting the feasibility of using a tiny fiber-like electrode for potentiometric sensing.The MMEC device exhibited a broad linear response(K^(+):2–32 mmol/L;Ca^(2+):0.5–4 mmol/L;Na^(+):10–160 mmol/L),high sensitivity(about 20–45 mV/decade),temporal stability(>2weeks),and good selectivity(>80%)for the above ions.In vitro detection and in vivo subcutaneous and brain experiment results showed that the MMEC system exhibits good multi-ion monitoring performance in several complex environments.This work provides a platform for the continuous real-time monitoring of ion fluctuations in different situations and has implications for developing smart sensors to monitor human health.展开更多
Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distr...Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distributed light ions and kappa energy distributed electrons. The extended poincaré-Lighthill-Kuo(e PLK) method is applied for the derivation of two-sided Korteweg–de Vries(KdV) equations(KdVEs). The KdV single-soliton solutions(KdVSSs) are determined using the hyperbolic secant method and the KdV multi-soliton solutions(KdVMSs)are obtained using the Hirota method. The effects of superthermality of electrons, temperature ratios of electron to light ion and heavy ion to electron, and the density ratio of electron to heavy ion on phase shifts are investigated for the head-on collisions between two-soliton HIAWs. The effects of plasma parameters on angular frequency, phase speed, production of multi-soliton structures, and the head-on collisions among single-, double-, triple-, quadruple-, and quintuplesolitons are also studied.展开更多
The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave fr...The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave frequency w, and pitch angle diffusion coefficient Daa were calculated at the center location of the symmetrical ring current： r ≈3.5RE with RE the Earth＇s radius. Emin is found to decrease rapidly from 10 MeV to a few keV with the increase in ca in three bands： H^＋-band, He^＋-band and O^＋-band. Moreover, EMIC waves have substantial potential to scatter energetic （～100 keV） ions （mainly H^＋ and He^＋） into the loss cone and yield precipitation loss, suggesting that wave-particle interactions contribute to ring current decay.展开更多
We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not i...We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not involvethe external degree of freedom.The scheme can be well realized within the current experimental technique.展开更多
Single materials that exhibit efficient and stable white-light emission are highly desirable for lighting applications.This paper reports a novel zero-dimensional perovskite,Rb_(4)CdCl_(6):Sn^(2+),Mn^(2+),which demons...Single materials that exhibit efficient and stable white-light emission are highly desirable for lighting applications.This paper reports a novel zero-dimensional perovskite,Rb_(4)CdCl_(6):Sn^(2+),Mn^(2+),which demonstrates exceptional white-light properties including adjustable correlated color temperature,high color rendering index of up to 85,and near-unity photoluminescence quantum yield of 99%.Using a co-doping strategy involving Sn^(2+)and Mn^(2+),cyan-orange dual-band emission with complementary spectral ranges is activated by the self-trapped excitons and d-d transitions of the Sn^(2+)and Mn^(2+)centers in the Rb_(4)CdCl_(6)host,respectively.Intriguingly,although Mn^(2+)ions doped in Rb_(4)CdCl_(6)are difficult to excite,efficient Mn^(2+)emission can be realized through an ultra-high-efficient energy transfer between Sn^(2+)and Mn^(2+)via the formation of adjacent exchange-coupled Sn–Mn pairs.Benefiting from this efficient Dexter energy transfer process,the dual emission shares the same optimal excitation wavelengths of the Sn^(2+)centers and suppresses the non-radiative vibration relaxation significantly.Moreover,the relative intensities of the dual-emission components can be modulated flexibly by adjusting the fraction of the Sn^(2+)ions to the Sn–Mn pairs.This co-doping approach involving short-range energy transfer represents a promising avenue for achieving high-quality white light within a single material.展开更多
Our previous work on the classical over-barrier ionization model for helium double ionization is extended to the complex multi-electron system of Ne. The total and q-fold ionization cross sections are calculated at en...Our previous work on the classical over-barrier ionization model for helium double ionization is extended to the complex multi-electron system of Ne. The total and q-fold ionization cross sections are calculated at energies ranging from a few tens to several hundred keV/u. The calculation results are in good agreement with the experimental data, and the energy dependence of the cross sections suggests that the multi-ionization of a strong perturbated complex atom is probably the sequential over-barrier ionization process.展开更多
基金The authors would like to acknowledge financial support from the National Key R&D Program of China(Nos.2021YFF1200700 and 2021YFA0911100)the National Natural Science Foundation of China(Nos.T2225010,32171399,and 32171456)+4 种基金the Fundamental Research Funds for the Central Universities,Sun Yat-Sen University(No.22dfx02)Pazhou Lab,Guangzhou(No.PZL2021KF0003)The authors also would like to thank the funding support from the Opening Project of Key Laboratory of Microelectronic Devices&Integrated Technology,Institute of Microelectronics,Chinese Academy of Sciences,and State Key Laboratory of Precision Measuring Technology and Instruments(No.pilab2211)QQOY would like to thank the China Postdoctoral Science Foundation(No.2022M713645)JL would like to thank the National Natural Science Foundation of China(No.62105380)and the China Postdoctoral Science Foundation(No.2021M693686).
文摘Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in biological subjects.Current semi-implantable devices are mainly based on single-parameter detection.Miniaturized semi-implantable electrodes for multiparameter sensing have more restrictions on the electrode size due to biocompatibility considerations,but reducing the electrode surface area could potentially limit electrode sensitivity.This study developed a semi-implantable device system comprising a multiplexed microfilament electrode cluster(MMEC)and a printed circuit board for real-time monitoring of intra-tissue K^(+),Ca^(2+),and Na^(+)concentrations.The electrode surface area was less important for the potentiometric sensing mechanism,suggesting the feasibility of using a tiny fiber-like electrode for potentiometric sensing.The MMEC device exhibited a broad linear response(K^(+):2–32 mmol/L;Ca^(2+):0.5–4 mmol/L;Na^(+):10–160 mmol/L),high sensitivity(about 20–45 mV/decade),temporal stability(>2weeks),and good selectivity(>80%)for the above ions.In vitro detection and in vivo subcutaneous and brain experiment results showed that the MMEC system exhibits good multi-ion monitoring performance in several complex environments.This work provides a platform for the continuous real-time monitoring of ion fluctuations in different situations and has implications for developing smart sensors to monitor human health.
文摘Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distributed light ions and kappa energy distributed electrons. The extended poincaré-Lighthill-Kuo(e PLK) method is applied for the derivation of two-sided Korteweg–de Vries(KdV) equations(KdVEs). The KdV single-soliton solutions(KdVSSs) are determined using the hyperbolic secant method and the KdV multi-soliton solutions(KdVMSs)are obtained using the Hirota method. The effects of superthermality of electrons, temperature ratios of electron to light ion and heavy ion to electron, and the density ratio of electron to heavy ion on phase shifts are investigated for the head-on collisions between two-soliton HIAWs. The effects of plasma parameters on angular frequency, phase speed, production of multi-soliton structures, and the head-on collisions among single-, double-, triple-, quadruple-, and quintuplesolitons are also studied.
基金National Natural Science Foundation of China (Nos.40874076,40774078,40774079 and 40536029)the Special Fund for Public Welfare Industry (meteorology)GYHY200806072the Visiting Scholar Foundation of State Key Laboratory for Space Weather,Chinese Academy of Sciences
文摘The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave frequency w, and pitch angle diffusion coefficient Daa were calculated at the center location of the symmetrical ring current： r ≈3.5RE with RE the Earth＇s radius. Emin is found to decrease rapidly from 10 MeV to a few keV with the increase in ca in three bands： H^＋-band, He^＋-band and O^＋-band. Moreover, EMIC waves have substantial potential to scatter energetic （～100 keV） ions （mainly H^＋ and He^＋） into the loss cone and yield precipitation loss, suggesting that wave-particle interactions contribute to ring current decay.
基金National Natural Science Foundation of China under Grant Nos.60678022 and 10704001the Specialized Research Fund for the Doctoral Program of Higher Education of Anhui Province under Grant No.20060357008+2 种基金Natural Science Foundation of Anhui Province under Grant No.070412060the Talent Foundation of Anhui UniversityAnhui Key Laboratory of Information Materials and Devices (Anhui University)
文摘We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not involvethe external degree of freedom.The scheme can be well realized within the current experimental technique.
基金support from the National Natural Science Foundation of China(Grant No.61874074)Science and Technology Project of Shenzhen(Grant No.JCYJ20220531100815034)+1 种基金H.L.acknowledges the support from Technology and Innovation Commission of Shenzhen(20200810164814001)Guangdong Basic and Applied Basic Research Foundation(General Program,Grant No.2022A1515012055).
文摘Single materials that exhibit efficient and stable white-light emission are highly desirable for lighting applications.This paper reports a novel zero-dimensional perovskite,Rb_(4)CdCl_(6):Sn^(2+),Mn^(2+),which demonstrates exceptional white-light properties including adjustable correlated color temperature,high color rendering index of up to 85,and near-unity photoluminescence quantum yield of 99%.Using a co-doping strategy involving Sn^(2+)and Mn^(2+),cyan-orange dual-band emission with complementary spectral ranges is activated by the self-trapped excitons and d-d transitions of the Sn^(2+)and Mn^(2+)centers in the Rb_(4)CdCl_(6)host,respectively.Intriguingly,although Mn^(2+)ions doped in Rb_(4)CdCl_(6)are difficult to excite,efficient Mn^(2+)emission can be realized through an ultra-high-efficient energy transfer between Sn^(2+)and Mn^(2+)via the formation of adjacent exchange-coupled Sn–Mn pairs.Benefiting from this efficient Dexter energy transfer process,the dual emission shares the same optimal excitation wavelengths of the Sn^(2+)centers and suppresses the non-radiative vibration relaxation significantly.Moreover,the relative intensities of the dual-emission components can be modulated flexibly by adjusting the fraction of the Sn^(2+)ions to the Sn–Mn pairs.This co-doping approach involving short-range energy transfer represents a promising avenue for achieving high-quality white light within a single material.
基金Project supported the by the National Natural Science Foundation of China (Grant No. 10804039)the Fundamental Research Funds for the Central Universities,China (Grant No. lzujbky-2009-24)
文摘Our previous work on the classical over-barrier ionization model for helium double ionization is extended to the complex multi-electron system of Ne. The total and q-fold ionization cross sections are calculated at energies ranging from a few tens to several hundred keV/u. The calculation results are in good agreement with the experimental data, and the energy dependence of the cross sections suggests that the multi-ionization of a strong perturbated complex atom is probably the sequential over-barrier ionization process.
