A spin model of LiCu2O2 compound with ground state of ellipsoidal helical structure is adopted. Taking into account the interchain coupling and exchange anisotropy, we investigate the magnetoelectric properties in a r...A spin model of LiCu2O2 compound with ground state of ellipsoidal helical structure is adopted. Taking into account the interchain coupling and exchange anisotropy, we investigate the magnetoelectric properties in a rotating magnetic field and perform the Monte Carlo simulation on a two-dimensional lattice. A prominent anisotropic response is observed in both the magnetization curve and the polarization curve, qualitatively coinciding with the behaviors that are detected in the experiment. In addition, the influences of the magnetic field with various magnitudes on polarization are also explored and analyzed in detail. As the magnetic field increases, a much smoother polarization of angle dependence is exhibited, indicating the strong correlation between the magnetic and ferroelectric orders.展开更多
An elastic Ising model for a one-dimensional diatomic spin chain is proposed to explain the ferroelectricity induced by the collinear magnetic order with a low-excited energy state. A statistical theory based on this ...An elastic Ising model for a one-dimensional diatomic spin chain is proposed to explain the ferroelectricity induced by the collinear magnetic order with a low-excited energy state. A statistical theory based on this model is developed to calculate the electrical and magnetic properties of Ca3CoMnO6, a typical quasi-one-dimensional diatomic spin chain system. The calculated ferroelectric polarization and dielectric susceptibility show a good agreement with recently reported data on Ca3Co2-xMnxO6 (x ≈ 0.96) (Phys. Rev. Lett. 100 047601 (2008)), although the predicted magnetic susceptibility does not coincide well with experiment. We also address the rationality and deficiency of this model by including a first-order correction which improves the consistency between the model and experiment.展开更多
基金Project supported by the Academic Scholarship for Doctoral Candidates of China(Grant No.10145201103)the Fundamental Research Funds for the Central Universities of China(Grant No.N110605002)the Shenyang Applied Basic Research Foundation,China(Grant No.F12-277-1-78)
文摘A spin model of LiCu2O2 compound with ground state of ellipsoidal helical structure is adopted. Taking into account the interchain coupling and exchange anisotropy, we investigate the magnetoelectric properties in a rotating magnetic field and perform the Monte Carlo simulation on a two-dimensional lattice. A prominent anisotropic response is observed in both the magnetization curve and the polarization curve, qualitatively coinciding with the behaviors that are detected in the experiment. In addition, the influences of the magnetic field with various magnitudes on polarization are also explored and analyzed in detail. As the magnetic field increases, a much smoother polarization of angle dependence is exhibited, indicating the strong correlation between the magnetic and ferroelectric orders.
基金Project supported by the National Natural Science Foundation of China (Grant Nos 50832002,10674061 and 10874075)the National Key Projects for Basic Research of China (Grant Nos 2006CB921802 and 2009CB623303)
文摘An elastic Ising model for a one-dimensional diatomic spin chain is proposed to explain the ferroelectricity induced by the collinear magnetic order with a low-excited energy state. A statistical theory based on this model is developed to calculate the electrical and magnetic properties of Ca3CoMnO6, a typical quasi-one-dimensional diatomic spin chain system. The calculated ferroelectric polarization and dielectric susceptibility show a good agreement with recently reported data on Ca3Co2-xMnxO6 (x ≈ 0.96) (Phys. Rev. Lett. 100 047601 (2008)), although the predicted magnetic susceptibility does not coincide well with experiment. We also address the rationality and deficiency of this model by including a first-order correction which improves the consistency between the model and experiment.