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8MeV中子诱发^(235)U裂变20个产物产额的测定 被引量:1
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作者 李泽 杨毅 +1 位作者 刘永辉 刘大鸣 《青岛大学学报(自然科学版)》 CAS 1997年第2期77-80,共4页
用HPGe直接γ射线能谱法绝对测定热中子和8MeV中子诱发235U裂变的20个产物的产额.其中19个是链产额,1个是独立产额.绝对裂变率是用双裂变室测定的,并测定198Auγ射线的活度检验裂变率测定的可靠性.
关键词 裂变 235 绝对裂变产额 直接γ能谱法
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Calculation of the energy dependence of fission fragments yields and kinetic energy distributions for neutron-induced ^(235)U fission
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作者 Ya-Ning Han Zheng Wei +16 位作者 Yi-Xuan Wang Dong-Ying Huo Peng-Qi Zhang Ming Li Jun Ma Kang Wu Yong-Guang Zheng Yuan He Zhi-Yong Deng Tian-Zhi Jiang Xiang-Lin Zhuo Jin Li Yun Zhang Yu Zhang Jun-Run Wang Xiao-Dong Su Ze-En Yao 《Chinese Physics C》 SCIE CAS CSCD 2024年第8期159-169,共11页
Fission fragments yields and average total kinetic energy are fundamental nuclear data for nuclear energy applications and the study of nuclear devices.Certain fission products,such as ^(95)Zr,^(99)Mo,^(140)Ba,^(144)C... Fission fragments yields and average total kinetic energy are fundamental nuclear data for nuclear energy applications and the study of nuclear devices.Certain fission products,such as ^(95)Zr,^(99)Mo,^(140)Ba,^(144)Ce,and ^(147)Nd,serve as burnup monitors,assessing the number of fissions induced by neutrons on ^(235)U.However,current experimental data for these fission products worldwide are inconsistent,introducing significant uncertainty into related scientific research.In this study,we employed the Potential-driving Model to calculate the independent yields of ^(235)U and evaluate its advantages in such calculations.Additionally,we investigated the energy dependence of independent yields to select important products.Furthermore,we calculated the cumulative yields of ^(95)Zr,^(99)Mo,^(140)Ba,^(144)Ce,and ^(147)Nd,and compared them with existing literature data to explore the energy dependence of fission products for ^(235)U.Given the lack of fission product yield data above 14.8 MeV,we extended our calculated incident neutron energy to 20 MeV,aiming to support future scientific research.The Geant4 physical model does not consider the influence of incident neutron energy on the average total kinetic energy of fission fragments;thus,we introduced the excitation function of the total kinetic energy of fission fragments recommended by Madland et al.,which effectively describes the experimental data of the average total kinetic energy of fragments formed in ^(235)U fission.In this paper,we comprehensively discuss the energy dependence of fission product yields and average total kinetic energy. 展开更多
关键词 ^^(235)u(n f) potential-driving model fission yields kinetic energies energy dependence
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Pre-neutron fragment mass yields for^(235)U(n,f)and^(239)Pu(n,f)reactions at incident energies from thermal up to 20 MeV
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作者 邹方磊 孙小军 +4 位作者 张凯 陈鸿飞 言杰 田俊龙 崔云怡 《Chinese Physics C》 SCIE CAS CSCD 2023年第4期161-167,共7页
Pre-neutron fragment mass yields in the vicinity of the thermal neutron energy are highly important for applications because of the larger fission cross sections of the^(235)U(n,f)and^(239)Pu(n,f)reactions.In this pap... Pre-neutron fragment mass yields in the vicinity of the thermal neutron energy are highly important for applications because of the larger fission cross sections of the^(235)U(n,f)and^(239)Pu(n,f)reactions.In this paper,preneutron fragment mass yields at incident energies from thermal up to 20 MeV are systematically studied using an empirical fission potential(EFP)model,the potential parameters of which are obtained from the measured data.The energy dependences of the peaks and valleys of the pre-neutron fragment mass yields are described by exponential and linear functions for the^(235)U(n,f)and^(239)Pu(n,f)reactions,respectively.The energy dependences of the evaporation neutrons,which play a crucial role in the reasonable description of pre-neutron fragment mass yields,are also obtained from the fission cross sections.The pre-neutron fragment mass yields in this study are not only consistent with the results of previous studies in regions of several Me Vs but also agree well with existing measured data at incident energies from thermal up to 20 MeV.The results show that the feasibility of this EFP model is verified in this extended energy region. 展开更多
关键词 ^^(235)u(n f)reaction ^^(239)Pu(n f)reaction thermal neutron energy empirical fission potential model pre-neutron fragment mass yield
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裂变产额的Z_(p)模型评价方法及燃耗不确定度分析 被引量:1
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作者 舒能川 朱淑瑜 +10 位作者 祖铁军 金永利 卢泽润 曹超维 宿阳 刘丽乐 陈永静 葛智刚 刘萍 黄小龙 续瑞瑞 《原子能科学技术》 EI CAS CSCD 北大核心 2022年第5期927-936,共10页
裂变产额在核科学技术和核工程中有着重要的应用,发展可靠、高效的产额评价方法和相应燃耗计算不确定度分析方法,对于建立高质量的产额数据库具有重要的意义。本文根据裂变产物核衰变模式和衰变分支比,建立独立产额与累积产额的转换矩阵... 裂变产额在核科学技术和核工程中有着重要的应用,发展可靠、高效的产额评价方法和相应燃耗计算不确定度分析方法,对于建立高质量的产额数据库具有重要的意义。本文根据裂变产物核衰变模式和衰变分支比,建立独立产额与累积产额的转换矩阵,用于Z_(p)模型的扩展,使之适用于独立产额和累积产额的统一描述,并以此建立了用于产额统一评价的拟合程序ZpFit。把ZpFit程序应用于中子诱发^(235)U裂变产物产额评价,获得了自洽的独立产额、累积产额和相应的协方差数据,并建立ENDF格式的中子诱发^(235)U裂变的产额数据库。在此基础上,计算了UAM燃耗基准题的TMI-1栅元的k_(inf)、重要核素原子核密度的不确定度,比对了本工作评价的产额数据和ENDF/B-Ⅷ.0评价库中产额数据传递给响应量的相对不确定度,结果基本一致,差异不大。 展开更多
关键词 裂变产额评价 Z_(p)模型 ^n%PLuS%^(235)u 不确定度分析
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分光光度法测定飞来峡水库水中的铀、钍 被引量:10
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作者 陈志东 邓飞 +3 位作者 林清 陈德育 刘瑛 陈福亮 《辐射防护通讯》 2001年第1期38-40,共3页
用 Fe( OH) 3共沉淀淡水样中的铀和钍 ,经硝酸溶解后 ,用 2 3 5 N-环己烷萃取铀钍 ,在盐酸介质中用分光光度法分别测定飞来峡水库水样铀、钍的含量。结果表明 ,铀、钍的回收率稳定在 80 %以上 ,方法稳定可靠 ;飞来峡水利枢纽建成后库区... 用 Fe( OH) 3共沉淀淡水样中的铀和钍 ,经硝酸溶解后 ,用 2 3 5 N-环己烷萃取铀钍 ,在盐酸介质中用分光光度法分别测定飞来峡水库水样铀、钍的含量。结果表明 ,铀、钍的回收率稳定在 80 %以上 ,方法稳定可靠 ;飞来峡水利枢纽建成后库区水体中铀、钍的含量维持在以前的水平。 展开更多
关键词 ^^235n 分光光度法 飞来峡水库 放射性核素 环境水样分析
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