In this review we consider the development of optical near-field imaging and nanostructuring by means of laser ablation since its early stages around the turn of the century.The interaction of short,intense laser puls...In this review we consider the development of optical near-field imaging and nanostructuring by means of laser ablation since its early stages around the turn of the century.The interaction of short,intense laser pulses with nanoparticles on a surface leads to laterally tightly confined,strongly enhanced electromagnetic fields below and around the nano-objects,which can easily give rise to nanoablation.This effect can be exploited for structuring substrate surfaces on a length scale well below the diffraction limit,one to two orders smaller than the incident laser wavelength.We report on structure formation by the optical near field of both dielectric and metallic nano-objects,the latter allowing even stronger and more localized enhancement of the electromagnetic field due to the excitation of plasmon modes.Structuring with this method enables one to nanopattern large areas in a one-step parallel process with just one laser pulse irradiation,and in the course of time various improvements have been added to this technique,so that also more complex and even arbitrary structures can be produced by means of nanoablation.The near-field patterns generated on the surface can be read out with high resolution techniques like scanning electron microscopy and atomic force microscopy and provide thus a valuable tool-in conjunction with numerical calculations like finite difference time domain(FDTD)simulations-for a deeper understanding of the optical and plasmonic properties of nanostructures and their applications.展开更多
A windowed very small aperture laser (VSAL) source for use in high resolution near field optical data storage is fabricated.The windowed regions are introduced to avoid shorting the pn junction with metal coating a...A windowed very small aperture laser (VSAL) source for use in high resolution near field optical data storage is fabricated.The windowed regions are introduced to avoid shorting the pn junction with metal coating and suppress the COD effect.It facilitates producing VSAL by simplified technology and improves the laser performance.A VSAL with 400nm small aperture is demonstrated by focused ion beam (FIB) and the output power is 0 3mW at 31mA.展开更多
This article summarizes work at the Laser Thermal Laboratory and discusses related studies on the laser synthesis and functionalization of semiconductor nanostructures and two-dimensional(2D)semiconductor materials.Re...This article summarizes work at the Laser Thermal Laboratory and discusses related studies on the laser synthesis and functionalization of semiconductor nanostructures and two-dimensional(2D)semiconductor materials.Research has been carried out on the laser-induced crystallization of thin films and nanostructures.The in situ transmission electron microscopy(TEM)monitoring of the crystallization of amorphous precursors in nanodomains is discussed herein.The directed assembly of silicon nanoparticles and the modulation of their optical properties by phase switching is presented.The vapor-liquid-solid mechanism has been adopted as a bottom-up approach in the synthesis of semiconducting nanowires(NWs).In contrast to furnace heating methods,laser irradiation offers high spatial selectivity and precise control of the heating mechanism in the time domain.These attributes enabled the investigation of NW nucleation and the early stage of nanostructure growth.Site-and shape-selective,on-demand direct integration of oriented NWs was accomplished.Growth of discrete silicon NWs with nanoscale location selectivity by employing near-field laser illumination is also reported herein.Tuning the properties of 2D transition metal dichalcogenides(TMDCs)by modulating the free carrier type,density,and composition can offer an exciting new pathway to various practical nanoscale electronics.In situ Raman probing of laser-induced processing of TMDC flakes was conducted in a TEM instrument.展开更多
The paper presents second approximation model for optical head in super high-density storage technology firstly and it is an important part for three grades approximate model of ultra-small-size quantum well corn-shap...The paper presents second approximation model for optical head in super high-density storage technology firstly and it is an important part for three grades approximate model of ultra-small-size quantum well corn-shaped laser and simulative calculations. It supplies the important and useful results for the NFOD optical head design with ultra thin active layer and ultra small spot laser.展开更多
The clusters of Eu^3+ ion in Eu(DBM)3Phen-doped polymethyl methacrylate (PMMA) have been studied by three means. The relative fluorescence intensity ratio of the ^5D0 → ^7F2 to ^5D0 → ^7F1 transitions with diff...The clusters of Eu^3+ ion in Eu(DBM)3Phen-doped polymethyl methacrylate (PMMA) have been studied by three means. The relative fluorescence intensity ratio of the ^5D0 → ^7F2 to ^5D0 → ^7F1 transitions with different concentrations of Eu^3+ in Eu(DBM)3Phen-doped PMMA and metastable-state (^5D0) lifetime dependence on Eu^3+ concentration axe analyzed. The analysis indicates that there axe no clustering effects in Eu^3+ ions of Eu(DBM)3Phen-doped PMMA when the Eu^3+ doping concentration is up to 1.0 wt.-%. At the same time, the clustering effect has not been observed by the scanning neax-field optical microscopy (SNOM) in Eu(DBM)3Phen-doped PMMA with 1.0 wt.-% of Eu^3+ ions. The analysis reveals that a high concentration of Eu^3+ can be incorporated into polymer optical fiber (POF) without clustering effect.展开更多
文摘In this review we consider the development of optical near-field imaging and nanostructuring by means of laser ablation since its early stages around the turn of the century.The interaction of short,intense laser pulses with nanoparticles on a surface leads to laterally tightly confined,strongly enhanced electromagnetic fields below and around the nano-objects,which can easily give rise to nanoablation.This effect can be exploited for structuring substrate surfaces on a length scale well below the diffraction limit,one to two orders smaller than the incident laser wavelength.We report on structure formation by the optical near field of both dielectric and metallic nano-objects,the latter allowing even stronger and more localized enhancement of the electromagnetic field due to the excitation of plasmon modes.Structuring with this method enables one to nanopattern large areas in a one-step parallel process with just one laser pulse irradiation,and in the course of time various improvements have been added to this technique,so that also more complex and even arbitrary structures can be produced by means of nanoablation.The near-field patterns generated on the surface can be read out with high resolution techniques like scanning electron microscopy and atomic force microscopy and provide thus a valuable tool-in conjunction with numerical calculations like finite difference time domain(FDTD)simulations-for a deeper understanding of the optical and plasmonic properties of nanostructures and their applications.
文摘A windowed very small aperture laser (VSAL) source for use in high resolution near field optical data storage is fabricated.The windowed regions are introduced to avoid shorting the pn junction with metal coating and suppress the COD effect.It facilitates producing VSAL by simplified technology and improves the laser performance.A VSAL with 400nm small aperture is demonstrated by focused ion beam (FIB) and the output power is 0 3mW at 31mA.
基金The research was performed at the Laser Thermal Laboratory by Drs David J Hwang,Sang-gil Ryu,Eunpa Kim,Jung Bin In,and the current students,Letian Wang,Yoonsoo Rho and Matthew Eliceiri.Professors Andrew M Minor,Junqiao Wu,Oscar D Dubon,Drs Bin Xiang,Frances I Allen,and Changhyun Ko of UCB Materials Science and Engineering,and Dr Carlo Carraro of UCB Chem.Engineering contributed to the work.The research was supported by DARPA/MTO under TBN grant N66001-08-1-2041,the US Department of Energy SBIR grant(DE-FG02-07ER84813),Samsung GRO,and NSF CMMI-1363392.The in situ experiments were performed at the National Center for Electron Microscopy at the Lawrence Berkeley National Laboratory,which is supported by the Office of Science,Office of Basic Energy Sciences,Scientific User Facilities Division,of the US Department of Energy under Contract No.DE-AC02-05CH11231.The laser-induced nanowire growth and doping was conducted on the LACVD apparatus in the UC Berkeley Marvell Nanofabrication Laboratory.
文摘This article summarizes work at the Laser Thermal Laboratory and discusses related studies on the laser synthesis and functionalization of semiconductor nanostructures and two-dimensional(2D)semiconductor materials.Research has been carried out on the laser-induced crystallization of thin films and nanostructures.The in situ transmission electron microscopy(TEM)monitoring of the crystallization of amorphous precursors in nanodomains is discussed herein.The directed assembly of silicon nanoparticles and the modulation of their optical properties by phase switching is presented.The vapor-liquid-solid mechanism has been adopted as a bottom-up approach in the synthesis of semiconducting nanowires(NWs).In contrast to furnace heating methods,laser irradiation offers high spatial selectivity and precise control of the heating mechanism in the time domain.These attributes enabled the investigation of NW nucleation and the early stage of nanostructure growth.Site-and shape-selective,on-demand direct integration of oriented NWs was accomplished.Growth of discrete silicon NWs with nanoscale location selectivity by employing near-field laser illumination is also reported herein.Tuning the properties of 2D transition metal dichalcogenides(TMDCs)by modulating the free carrier type,density,and composition can offer an exciting new pathway to various practical nanoscale electronics.In situ Raman probing of laser-induced processing of TMDC flakes was conducted in a TEM instrument.
基金Supported by the National Natural Science Foundation of China and Doctor Foundation of China
文摘The paper presents second approximation model for optical head in super high-density storage technology firstly and it is an important part for three grades approximate model of ultra-small-size quantum well corn-shaped laser and simulative calculations. It supplies the important and useful results for the NFOD optical head design with ultra thin active layer and ultra small spot laser.
基金This work was supported by the National ScienceFoundation of China (No. 90201013), the Fujian NaturalScience Foundation of China (No. A0510014), and theFujian Educational Department Foundation of China(No. JB03151 and JB04246).
文摘The clusters of Eu^3+ ion in Eu(DBM)3Phen-doped polymethyl methacrylate (PMMA) have been studied by three means. The relative fluorescence intensity ratio of the ^5D0 → ^7F2 to ^5D0 → ^7F1 transitions with different concentrations of Eu^3+ in Eu(DBM)3Phen-doped PMMA and metastable-state (^5D0) lifetime dependence on Eu^3+ concentration axe analyzed. The analysis indicates that there axe no clustering effects in Eu^3+ ions of Eu(DBM)3Phen-doped PMMA when the Eu^3+ doping concentration is up to 1.0 wt.-%. At the same time, the clustering effect has not been observed by the scanning neax-field optical microscopy (SNOM) in Eu(DBM)3Phen-doped PMMA with 1.0 wt.-% of Eu^3+ ions. The analysis reveals that a high concentration of Eu^3+ can be incorporated into polymer optical fiber (POF) without clustering effect.