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Split-Ring Structured All-Inorganic Perovskite Photodetector Arrays for Masterly Internet of Things 被引量:1
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作者 Bori Shi Pingyang Wang +7 位作者 Jingyun Feng Chang Xue Gaojie Yang Qingwei Liao Mengying Zhang Xingcai Zhang Weijia Wen Jinbo Wu 《Nano-Micro Letters》 SCIE EI CAS CSCD 2023年第1期25-42,共18页
Photodetectors with long detection distances and fast response are important media in constructing a non-contact human-machine interface for the Masterly Internet of Things(MIT).All-inorganic perovskites have excellen... Photodetectors with long detection distances and fast response are important media in constructing a non-contact human-machine interface for the Masterly Internet of Things(MIT).All-inorganic perovskites have excellent optoelectronic performance with high moisture and oxygen resistance,making them one of the promising candidates for high-performance photodetectors,but a simple,low-cost and reliable fabrication technology is urgently needed.Here,a dual-function laser etching method is developed to complete both the lyophilic split-ring structure and electrode patterning.This novel split-ring structure can capture the perovskite precursor droplet efficiently and achieve the uniform and compact deposition of CsPbBr3 films.Furthermore,our devices based on laterally conducting split-ring structured photodetectors possess outstanding performance,including the maximum responsivity of 1.44×105 mA W^(−1),a response time of 150μs in 1.5 kHz and one-unit area<4×10-2 mm2.Based on these split-ring photodetector arrays,we realized three-dimensional gesture detection with up to 100 mm distance detection and up to 600 mm s^(−1) speed detection,for low-cost,integrative,and non-contact human-machine interfaces.Finally,we applied this MIT to wearable and flexible digital gesture recognition watch panel,safe and comfortable central controller integrated on the car screen,and remote control of the robot,demonstrating the broad potential applications. 展开更多
关键词 Split-ring DEWETTING perovskite photodetector array Human-machine interface Gesture recognition
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Recent research process on perovskite photodetectors:A review for photodetector——materials,physics,and applications 被引量:2
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作者 Yan Zhao Chenglong Li Liang Shen 《Chinese Physics B》 SCIE EI CAS CSCD 2018年第12期46-56,共11页
The perovskite photodetectors can be used for image sensing, environmental monitoring, optical communication, and chemical/biological detection. In the recent five years, the perovskite photoelectric detectors with va... The perovskite photodetectors can be used for image sensing, environmental monitoring, optical communication, and chemical/biological detection. In the recent five years, the perovskite photoelectric detectors with various devices are welldesigned and have made unprecedented progress of light detection. It is necessary to emphasize the most interesting works and summarize them to provide researchers with systematic information. In this review, we report the recent progress in perovskite photodetectors, including highly sensitive, ultrafast response speed, high gain, low noise, flexibility, and narrowband, concentrating on the photodetection performance of versatile halide perovskites(organic–inorganic hybrid and all inorganic compositions). Currently, organic–inorganic hybrid and all-inorganic halide microcrystals with polycrystalline film, nanoparticle/wire/chip, and block monocrystalline morphology control show important performance in response rate,decomposition rate, noise equivalent power, linear dynamic range, and response speed. It is expected that a comprehensive compendium of the research status of perovskite photodetectors will contribute to the development of this area. 展开更多
关键词 perovskite photodetectors response speed DETECTIVITY linear dynamic range
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Recent advances on organic-inorganic hybrid perovskite photodetectors with fast response 被引量:8
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作者 Yan Zhao Chenglong Li Liang Shen 《InfoMat》 SCIE CAS 2019年第2期164-182,共19页
In the last decade,optoelectronic devices based on organic-inorganic hybrid perovskite(OIHP)materials,which have unique advantages of direct bandgap,large absorption coefficient,low density of defects,long charge carr... In the last decade,optoelectronic devices based on organic-inorganic hybrid perovskite(OIHP)materials,which have unique advantages of direct bandgap,large absorption coefficient,low density of defects,long charge carrier lifetime,diffusion length,and solution processability,have traveled with traditional inorganic semiconductor devices.The state-of-the-art OIHP photodetectors have contributed a comparable performance with Si and III-V compound semiconductor based photodetectors.Large amount of efforts have been focused on improving sensitivity,broadening detection spectra,enlarging linear dynamic range.However,few reports emphasized the important parameter of response speed.In this review,we summarize the progress and applications of OIHP photodetectors with fast response.Based on photovoltaic and photoconductive-type OIHP photodetectors,the working principle and key factors on determining response speed are systematically mentioned.Then,the research progress of response speed,which is composed of resistance-capacitance(RC)time constant and charge carrier transit time is discussed in detail.Subsequently,considering the intrinsic flexibility of perovskite materials,we briefly discuss the flexible photodetectors.Finally,an outlook and potential rules for designing fast-response OIHP photodetectors are further proposed. 展开更多
关键词 organic-inorganic hybrid perovskite photodetectors fast response PHOTOCONDUCTIVE PHOTOVOLTAIC
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Self-powered bifunctional perovskite photodetectors with both broadband and narrowband photoresponse 被引量:3
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作者 Wenjie Cheng Wei Tian +1 位作者 Fengren Cao Liang Li 《InfoMat》 SCIE CAS 2022年第11期119-131,共13页
Photodetectors generally operate exclusively in either the broadband or narrowband.Developing bifunctional photodetectors that can detect photons in both broadband and narrowband would bring significant versatility to... Photodetectors generally operate exclusively in either the broadband or narrowband.Developing bifunctional photodetectors that can detect photons in both broadband and narrowband would bring significant versatility to the optoelectronic platform.Nevertheless,the design of bifunctional integrated devices remains challenging due to the differentiated strategies with respect to device structure and material combination.Herein,we propose introducing polyvinylpyrrolidone to increase the viscosity of the perovskite precursor solution,which introduces abundant defects and cavities into the perovskite film while maintaining a relatively low film thickness.Then,we use methylamine gas to postprocess the middle area of the film to promote directional recrystallization and densification,thereby realizing narrowband and broadband dualfunction photodetection in a single device at zero bias.Both ends of the film exhibit a near-infrared peak response at 780 nm with a narrow full-width at half maximum of approximately 30 nm without an external bias.The middle broadband photodetector exhibits a high responsivity of 329 mA W^(-1)and EQE up to 52.46%at 780 nm.We make full use of narrow-band wavelength selective detection and broadband full-spectrum detection to achieve double encryption during signal transmission.This work represents an important step toward the realization of perovskite-based multifunctional integrated devices. 展开更多
关键词 bifunctional device double encryption narrow FWHM perovskite photodetector
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Advances in perovskite photodetectors 被引量:4
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作者 Chenglong Li Yao Ma +2 位作者 Yifan Xiao Liang Shen Liming Ding 《InfoMat》 SCIE CAS 2020年第6期1247-1256,共10页
Perovskite photodetectors have gradually shown preeminent photoelectric performance due to the unique material properties.In recent years,lots of works have been reported in improving the sensitivity,changing detectio... Perovskite photodetectors have gradually shown preeminent photoelectric performance due to the unique material properties.In recent years,lots of works have been reported in improving the sensitivity,changing detection spectrum range and enhancing long-term stability.Herein,we summarize the some efficient strategies for performance improvement and synchronously analyze severe issues exposed in that.Furthermore,some reasonable proposals are put forward to solve future predicted troubles.In addition,more prospective assumptions are proposed on the basis of the development trend in photoelectric detection fields.We hope this perspective will allow researchers to have a clearer understanding of recent studies based on perovskite photodetectors and inspire more meaningful work in the future. 展开更多
关键词 DETECTIVITY perovskite photodetectors response speed STABILITY
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High-quality perovskite MAPbI_3 single crystals for broad-spectrum and rapid response integrate photodetector 被引量:5
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作者 Yunxia Zhang Yucheng Liu +1 位作者 Zhou Yang Shengzhong(Frank)Liu 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2018年第3期722-727,共6页
Organic–inorganic single-crystalline perovskites have attracted significant attentions due to their exceptional progress in intrinsic properties' investigation and applications in photovoltaics and optoelectronics. ... Organic–inorganic single-crystalline perovskites have attracted significant attentions due to their exceptional progress in intrinsic properties' investigation and applications in photovoltaics and optoelectronics. In this study, the large perovskite CH3NH3PbI3 single crystal with the largest length of 80 mm was prepared through the method of inverse-temperature crystallization. Meanwhile, the mass production of integrate photodetectors have been fabricated on the single-crystalline wafer and the photoresponse performances were investigated. The results show that the single-crystalline photodetectors have broad spectrum response to 900 nm, rapid response speed(〈40 μs) and excellent stability. These findings are of great importance for future promising perovskite single crystalline for integrated photoelectronic application. 展开更多
关键词 Single-crystalline perovskite photodetector Rapid response
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UV soaking for enhancing the photocurrent and response speed of Cs_(2)AgBiBr_(6)-based all-inorganic perovskite photodetectors
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作者 Ye Yuan Genghua Yan +4 位作者 Zhuowei Li Bangqi Jiang Zongcun Liang Hong Jin Fan Wenjie Mai 《Science China Materials》 SCIE EI CAS CSCD 2022年第2期442-450,共9页
The response speed of the reported Cs_(2)AgBiBr_(6)-based photodetectors exhibits a wide variation ranging from microseconds to nanoseconds,while the reason is still unclear.Apart from the conventional approaches such... The response speed of the reported Cs_(2)AgBiBr_(6)-based photodetectors exhibits a wide variation ranging from microseconds to nanoseconds,while the reason is still unclear.Apart from the conventional approaches such as reducing effective area,new regulating approaches for response speed improvement have rarely been reported.On the other hand,it is generally believed that ultraviolet(UV)light has negative impact on perovskite devices resulting in performance degradation.In this work,we demonstrated that the response speed of the photodetector with FTO/Cs_(2)AgBiBr_(6)/Au structure can be effectively regulated by utilizing UV light-soaking effect without reducing the device area.Particularly,the decay time is efficiently modulated from 30.1μs to 340 ns.In addition,the−3 dB bandwidth of the device is extended from 5 to 20 kHz.It is worth mentioning that the light current is remarkably boosted by 15 times instead of any attenuation.Furthermore,we prove the universality of UV soaking treatment on Cs_(2)AgBiBr_(6)-based photodetectors with other all-inorganic structures,i.e.,FTO/TiO_(2)/Cs_(2)AgBiBr_(6)/Au,FTO/Cs_(2)AgBiBr_(6)/TiO_(2)/Au and FTO/TiO_(2)/Cs_(2)AgBiBr_(6)/CuSCN/Au.Our results demonstrate a new method to improve the response speed and light current of Cs_(2)AgBiBr_(6)-based perovskite all-inorganic photodetectors. 展开更多
关键词 UV light all-inorganic perovskite photodetectors Cs_(2)AgBiBr_(6) PHOTOCURRENT response speed
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Improving the interfacial contact between CH_3NH_3PbI_(3–x)Cl_x and Au by LiTFSI solution treatment for efficient photoelectric devices
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作者 Xiang Xia Hongcui Li +2 位作者 Yanhua Li Cailong Liu Xizhe Liu 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2015年第6期693-697,共5页
Organic lead halide compounds with perovskite structure become a promising photovoltaic material for low- cost thin film solar cells in recent years. The property of perovskite/metal interface is a fundamental topic f... Organic lead halide compounds with perovskite structure become a promising photovoltaic material for low- cost thin film solar cells in recent years. The property of perovskite/metal interface is a fundamental topic for the effective charge transfer at metal electrodes. In this work, we develop an interface modification method of lithium bis(trifluoromethane sulfonimide) (LiTFSI) solution treatment, which can effectively decrease the charge transfer resistance at the CH3NHaPbI3_xClx/Au interface. After the solution treatment, uniform nan- odots are formed at the surface of CHaNH3PbI3_xCIx films, and the barrier height at CH3NH3PbI3_xCIx/Au interface reduces from 0.51 V to 0.08 V. As a consequence, the efficiency of hole conductor free solar cells with CH3NHaPbI3-xCIx harvester increase from 4.0% to 7.6% under one sun condition. It is also found that the hole conductor free perovskite solar cell can work in a photodetector mode, which has the same output prop- erties with phototransistors. After the LiTFSI solution treatment, the sensitivity of this photodetector can be improved for about one time. 展开更多
关键词 perovskite solar cells perovskite photodetectors Interfacial contact Barrier height Solution treatment Phototransistor
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Ultrasensitive,flexible perovskite nanowire photodetectors with long-term stability exceeding 5000 h 被引量:3
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作者 Dingjun Wu Yongchang Xu +14 位作者 Hai Zhou Xin Feng Jianqiang Zhang Xiyan Pan Zheng Gao Rui Wang Guokun Ma Li Tao Hanbin Wang Jinxia Duan Houzhao Wan Jun Zhang Liangping Shen Hao Wang Tianyou Zhai 《InfoMat》 SCIE CAS 2022年第9期85-96,共12页
Photodetectors(PDs)based on perovskite nanowires are among the most promising next-generation photodetection technologies;however,their poor long-term stability is the biggest challenge limiting their commercial appli... Photodetectors(PDs)based on perovskite nanowires are among the most promising next-generation photodetection technologies;however,their poor long-term stability is the biggest challenge limiting their commercial applica-tion.Herein,an ionic liquid,1-butyl-3 methylimidazolium tetrafuoroborate(BMIMBF_(4)),is incorporated as an additive into methylammonium lead tri-iodide(MAPbI_(3))nanowires;this not only effectively passivates defects to inhibit perovskite degradation but also leads to the formation of nanochannels,enabling fast charge transfer.As a result,the long-term stability and perfor-mance of MAPbI_(3)nanowires are considerably improved.The detectivity,linear detection range,and noise equivalent power of the MA PbI_(3)nanowire PD reach 2.06×10^(13)Jones,160dB,and 1.38×10^(-15)W Hz-^(1/2),respectively,compara-ble to the highest performance of perovskite nanowire PDs reported to date.Moreover,the unencapsulated PD can maintain 100%of its initial performance after being exposed to an open-air environment for more than 5000 h,esta-blishing it as the most stable perovskite nanowire PD reported to date.Nota-bly,the PD exhibits improved diffuse reflection imaging ability when compared with commercial silicon photodiode S2386.This study provides a new strategy for constructing sensitive,stable,and flexible perovskite PDs and will accelerate their commercial application in the future. 展开更多
关键词 diffuse rflction imaging FLEXIBLE ionic liquids long-term stability perovskite nanowire photodetectors
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120 mm Single-crystalline perovskite and wafers: towards viable applications 被引量:10
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作者 Yucheng Liu Xiaodong Ren +13 位作者 Jing Zhang Zhou Yang Dong Yang Fengyang Yu Jiankun Sun Changming Zhao Zhun Yao Bo Wang Qingbo Wei Fengwei Xiao Haibo Fan Hao Deng Liangping Deng Shengzhong (Frank) Liu 《Science China Chemistry》 SCIE EI CAS CSCD 2017年第10期1367-1376,共10页
As the large single-crystalline silicon wafers have revolutionized many industries including electronics and solar cells, it is envisioned that the availability of large single-crystalline perovskite crystals and wafe... As the large single-crystalline silicon wafers have revolutionized many industries including electronics and solar cells, it is envisioned that the availability of large single-crystalline perovskite crystals and wafers will revolutionize its broad applications in photovoltaics, optoelectronics, lasers, photodetectors, light emitting diodes(LEDs), etc. Here we report a method to grow large single-crystalline perovskites including single-halide crystals: CH3NH3PbX3(X=I, Br, Cl), and dual-halide ones:CH3NH3Pb(ClxBr1.x)3 and CH3NH3Pb(BrxI1.x)3, with the largest crystal being 120 mm in length. Meanwhile, we have advanced a process to slice the large perovskite crystals into thin wafers. It is found that the wafers exhibit remarkable features:(1)its trap-state density is a million times smaller than that in the microcrystalline perovskite thin films(MPTF);(2) its carrier mobility is 410 times higher than its most popular organic counterpart P3HT;(3) its optical absorption is expanded to as high as910 nm comparing to 797 nm for the MPTF;(4) while MPTF decomposes at 150 °C, the wafer is stable at high temperature up to270 °C;(5) when exposed to high humidity(75% RH), MPTF decomposes in 5 h while the wafer shows no change for overnight;(6) its photocurrent response is 250 times higher than its MPTF counterpart. A few electronic devices have been fabricated using the crystalline wafers. Among them, the Hall test gives low carrier concentration with high mobility. The trap-state density is measured much lower than common semiconductors. Moreover, the large SC-wafer is found particularly useful for mass production of integrated circuits. By adjusting the halide composition, both the optical absorption and the light emission can be fine-tuned across the entire visible spectrum from 400 nm to 800 nm. It is envisioned that a range of visible lasers and LEDs may be developed using the dual-halide perovskites. With fewer trap states, high mobility, broader absorption, and humidity resistance, it is expected that solar cells with high stable efficiency maybe attainable using the crystalline wafers. 展开更多
关键词 single-crystal growth perovskite wafer IC devices photodetector array
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Enhancement of photodetection based on perovskite/MoS_2 hybrid thin film transistor 被引量:3
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作者 Fengjing Liu Jiawei Wang +3 位作者 Liang Wang Xiaoyong Cai Chao Jiang Gongtang Wang 《Journal of Semiconductors》 EI CAS CSCD 2017年第3期94-99,共6页
Perovskite/MoS2hybrid thin film transistor photodetectors consist of few-layered MoS2and CH3NH3PbI3film with various thickness prepared by two-step vacuum deposition.By implementing perovskite CH3NH3PbI3film onto the ... Perovskite/MoS2hybrid thin film transistor photodetectors consist of few-layered MoS2and CH3NH3PbI3film with various thickness prepared by two-step vacuum deposition.By implementing perovskite CH3NH3PbI3film onto the MoS2flake,the perovskite/MoS2hybrid photodetector exhibited a photoresponsivity of 104A/W and fast response time of about 40 ms.Improvement of photodetection performance is attributed to the balance between light absorption in the perovskite layer and an effective transfer of photogenerated carriers from perovskite entering the MoS2channel.This work may provide guidance to develop high-performance hybrid structure optoelectronic devices. 展开更多
关键词 perovskite MoS2 photodetector
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