A steady state analysis of the nonclassical features and statistical properties of the cavity radiation of a two- photon coherent beat laser is presented. Results show that the degree of two-mode squeezing, detectable...A steady state analysis of the nonclassical features and statistical properties of the cavity radiation of a two- photon coherent beat laser is presented. Results show that the degree of two-mode squeezing, detectable entanglement and intensity of the cavity radiation can increase with the deviation of the phase fluctuations of the laser employed in preparing the atoms, but decrease with the increasing rate at which the induced coherence superposition decays. Although it is found that varying the phase fluctuations and dephasing can lead to modification in the quantum features and statistical properties of the radiation, it does not alter the similarity in the nature of the degree of entanglement detectable by the criteria following from Duan-Giedke-Cirac Zoller and logarithmic negativity in a perceivable manner. Since the intensity and quantum features can be readily enhanced, this system is expected to be a viable source of a strong robust entangled (squeezed) light under various conditions. Moreover, comparison of the mean number of photon pairs with intensity difference shows that the chance of inciting a two-photon process can be enhanced by changing the rate of dephasing and phase fluctuations.展开更多
Hopf bifurcation inducing lasing without inversion has been analyzed by taking into account the effect of phase fluctuation in the driving field based on a closed three level ladder-type atomic model. It is shown that...Hopf bifurcation inducing lasing without inversion has been analyzed by taking into account the effect of phase fluctuation in the driving field based on a closed three level ladder-type atomic model. It is shown that due to the phase fluctuation of the driving field, the necessary threshold increases significantly. Furthermore the area domain to get lasing without inversion decreases as the driving field's linewidth increases.展开更多
Based on the generalized truncated second-order moments,an approximate analytical formula of the beam propagation factor M^2 of high-power laser beams passing through the optical system with multiple hard-edged apertu...Based on the generalized truncated second-order moments,an approximate analytical formula of the beam propagation factor M^2 of high-power laser beams passing through the optical system with multiple hard-edged apertures is deduced.Numerical examples of the beams passing through an aperture-spatial filter are enclosed,and the influences of amplitude modulations(AMs)and phase fluctuations(PFs)on the beam propagation quality of high-power laser beams passing through the multi-apertured ABCD optical system are considered and discussed.It is shown that PFs are able to degrade the beam propagation quality of laser beams more than AMs when the high-power laser beams passing through the aperture-spatial filter,furthermore,one or two aperture-lens optical systems configured appropriate aperture parameters are both able to upgrade the beam propagation quality of high-power laser beams.The M2 factor of Gaussian beam passing through the multi-aperture optical system is a special case in this paper.展开更多
Active-phase engineering is regularly utilized to tune the selectivity of metal nanoparticles (NPs) in heterogeneous catalysis. However, the lack of understanding of the active phase in electrocatalysis has hampered...Active-phase engineering is regularly utilized to tune the selectivity of metal nanoparticles (NPs) in heterogeneous catalysis. However, the lack of understanding of the active phase in electrocatalysis has hampered the development of efficient catalysts for CO2 electroreduction. Herein, we report the systematic engineering of active phases of Pd NPs, which are exploited to select reaction pathways for CO2 electroreduction. In situ X-ray absorption spectroscopy, in situ attenuated total reflection-infrared spectroscopy, and density functional theory calculations suggest that the formation of a hydrogen-adsorbed Pd surface on a mixture of the α- and β-phases of a palladium-hydride core (α+β PdHx@PdHx) above -0.2 V (vs. a reversible hydrogen electrode) facilitates formate production via the HCOO intermediate, whereas the formation of a metallic Pd surface on the β-phase Pd hydride core (β PdHx@Pd) below -0.5 V promotes CO production via the COOH" intermediate. The main product, which is either formate or CO, can be selectively produced with high Faradaic efficiencies (〉90%) and mass activities in the potential window of 0.05 to -0.9 V with scalable application demonstration.展开更多
This paper presents the results of an ongoing investigation into transient pressure pulses using Shan- non entropy. Pressure fluctuations (produced by gas-solid two-phase flow during fluidized dense-phase conveying)...This paper presents the results of an ongoing investigation into transient pressure pulses using Shan- non entropy. Pressure fluctuations (produced by gas-solid two-phase flow during fluidized dense-phase conveying) are recorded by pressure transducers installed at strategic locations along a pipeline. This work validates previous work on identifying the flow mode from pressure signals (Mittal, Mallick, & Wypych, 2014). Two different powders, namely fly ash (median particle diameter 45 μm, particle den- sity 1950 kg/m3. loosely poured bulk density 950 kg/m3) and cement (median particle diameter 15 p,m, particle density 3060 kg/m3, loosely poured bulk density 1070 kg/m3), are conveyed through different pipelines (51 mm I.D. × 70 m length and 63 mm I.D. × 24 m length). The transient nature of pressure fluc- tuations (instead of steady-state behavior) is considered in investigating flow characteristics. Shannon entropy is found to increase along straight pipe sections for both solids and both pipelines. However, Shannon entropy decreases after a bend. A comparison of Shannon entropy among different ranges of superficial air velocity reveals that high Shannon entropy corresponds to very low velocities (i.e. 3-5 m/s) and very high velocities (i.e. 11-14 m/s) while low Shannon entropy corresponds to mid-range velocities (i.e. 6-8 m/s).展开更多
文摘A steady state analysis of the nonclassical features and statistical properties of the cavity radiation of a two- photon coherent beat laser is presented. Results show that the degree of two-mode squeezing, detectable entanglement and intensity of the cavity radiation can increase with the deviation of the phase fluctuations of the laser employed in preparing the atoms, but decrease with the increasing rate at which the induced coherence superposition decays. Although it is found that varying the phase fluctuations and dephasing can lead to modification in the quantum features and statistical properties of the radiation, it does not alter the similarity in the nature of the degree of entanglement detectable by the criteria following from Duan-Giedke-Cirac Zoller and logarithmic negativity in a perceivable manner. Since the intensity and quantum features can be readily enhanced, this system is expected to be a viable source of a strong robust entangled (squeezed) light under various conditions. Moreover, comparison of the mean number of photon pairs with intensity difference shows that the chance of inciting a two-photon process can be enhanced by changing the rate of dephasing and phase fluctuations.
文摘Hopf bifurcation inducing lasing without inversion has been analyzed by taking into account the effect of phase fluctuation in the driving field based on a closed three level ladder-type atomic model. It is shown that due to the phase fluctuation of the driving field, the necessary threshold increases significantly. Furthermore the area domain to get lasing without inversion decreases as the driving field's linewidth increases.
基金Science Fund from the Shaanxi Provincial Education Department,China(Grant No.18JK0723).
文摘Based on the generalized truncated second-order moments,an approximate analytical formula of the beam propagation factor M^2 of high-power laser beams passing through the optical system with multiple hard-edged apertures is deduced.Numerical examples of the beams passing through an aperture-spatial filter are enclosed,and the influences of amplitude modulations(AMs)and phase fluctuations(PFs)on the beam propagation quality of high-power laser beams passing through the multi-apertured ABCD optical system are considered and discussed.It is shown that PFs are able to degrade the beam propagation quality of laser beams more than AMs when the high-power laser beams passing through the aperture-spatial filter,furthermore,one or two aperture-lens optical systems configured appropriate aperture parameters are both able to upgrade the beam propagation quality of high-power laser beams.The M2 factor of Gaussian beam passing through the multi-aperture optical system is a special case in this paper.
文摘Active-phase engineering is regularly utilized to tune the selectivity of metal nanoparticles (NPs) in heterogeneous catalysis. However, the lack of understanding of the active phase in electrocatalysis has hampered the development of efficient catalysts for CO2 electroreduction. Herein, we report the systematic engineering of active phases of Pd NPs, which are exploited to select reaction pathways for CO2 electroreduction. In situ X-ray absorption spectroscopy, in situ attenuated total reflection-infrared spectroscopy, and density functional theory calculations suggest that the formation of a hydrogen-adsorbed Pd surface on a mixture of the α- and β-phases of a palladium-hydride core (α+β PdHx@PdHx) above -0.2 V (vs. a reversible hydrogen electrode) facilitates formate production via the HCOO intermediate, whereas the formation of a metallic Pd surface on the β-phase Pd hydride core (β PdHx@Pd) below -0.5 V promotes CO production via the COOH" intermediate. The main product, which is either formate or CO, can be selectively produced with high Faradaic efficiencies (〉90%) and mass activities in the potential window of 0.05 to -0.9 V with scalable application demonstration.
文摘This paper presents the results of an ongoing investigation into transient pressure pulses using Shan- non entropy. Pressure fluctuations (produced by gas-solid two-phase flow during fluidized dense-phase conveying) are recorded by pressure transducers installed at strategic locations along a pipeline. This work validates previous work on identifying the flow mode from pressure signals (Mittal, Mallick, & Wypych, 2014). Two different powders, namely fly ash (median particle diameter 45 μm, particle den- sity 1950 kg/m3. loosely poured bulk density 950 kg/m3) and cement (median particle diameter 15 p,m, particle density 3060 kg/m3, loosely poured bulk density 1070 kg/m3), are conveyed through different pipelines (51 mm I.D. × 70 m length and 63 mm I.D. × 24 m length). The transient nature of pressure fluc- tuations (instead of steady-state behavior) is considered in investigating flow characteristics. Shannon entropy is found to increase along straight pipe sections for both solids and both pipelines. However, Shannon entropy decreases after a bend. A comparison of Shannon entropy among different ranges of superficial air velocity reveals that high Shannon entropy corresponds to very low velocities (i.e. 3-5 m/s) and very high velocities (i.e. 11-14 m/s) while low Shannon entropy corresponds to mid-range velocities (i.e. 6-8 m/s).