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Transverse relaxation determination based on light polarization modulation for spin-exchange relaxation free atomic magnetometer 被引量:3
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作者 Xue-Jing Liu Ming Ding +3 位作者 Yang Li Yan-Hui Hu Wei Jin Jian-Cheng Fang 《Chinese Physics B》 SCIE EI CAS CSCD 2018年第7期276-280,共5页
A transverse relaxation determination of spin-exchange relaxation free (SERF) magnetometer based on polarization modulation technique is proposed. Compared with the radio-frequency (RF) excitation and light intens... A transverse relaxation determination of spin-exchange relaxation free (SERF) magnetometer based on polarization modulation technique is proposed. Compared with the radio-frequency (RF) excitation and light intensity excitation meth- ods used in SERF magnetometer, the light polarization modulation method has a high stability in low-frequency range, which indicates a more accurate transverse relaxation measurement. 展开更多
关键词 spin-exchange relaxation free (SERF) magnetometer LINEWIDTH optical polarization modulation
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A 3-D Polarization Quadrature Amplitude Modulation Method and Constellation Mapping 被引量:2
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作者 SUN Xuehong ZHANG Haiying +1 位作者 ZENG Zhimin GUO Caili 《China Communications》 SCIE CSCD 2015年第10期16-26,共11页
As a new three-dimensional(3-D)modulation,Polarization Quadrature Amplitude Modulation(PQAM) can be regarded as the combination of Pulse amplitude modulation(PAM) and Quadrature Amplitude Modulation(QAM) Modulation.It... As a new three-dimensional(3-D)modulation,Polarization Quadrature Amplitude Modulation(PQAM) can be regarded as the combination of Pulse amplitude modulation(PAM) and Quadrature Amplitude Modulation(QAM) Modulation.It can better improve the digital communication efficiency and reduce the Symbol error rate(SER) of the system than one-dimensional or two-dimensional modulation scheme.How to design a feasible constellation is the most concerned problem of PQAM currently.This paper first studies the relationship between the SER theoretical value of PQAM and the distribution of M and N,proposes a new M,N allocation scheme.Secondly,a new and straightforward design method of constructing higher-level 3-D signal constellations,which can be matched with the PQAM,and the constellation can divided into three different structures according to the ary for PQAM.Finally,the simulation results show that:in PQAM system,the modulation scheme and the constellation mapping scheme are proposed in this paper which can effectively reduce the system SER and improve the anti-noise performance of the system. 展开更多
关键词 polarization quadrature amplitude modulation minimum euclidean distance symbol error probability 3-D constellation
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Fluorescence emission difference microscopy based on polarization modulation
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作者 Wanjie Dong Yuran Huang +4 位作者 Zhimin Zhang Liang Xu Cuifang Kuang Xiang Hao Xu Liu 《Journal of Innovative Optical Health Sciences》 SCIE EI CAS 2022年第5期83-94,共12页
In this paper,we propose a new fluorescence emission difference microscopy(FED)technique based on polarization modulation.An electro-optical modulator(EOM)is used to switch the excitation beam between the horizontal a... In this paper,we propose a new fluorescence emission difference microscopy(FED)technique based on polarization modulation.An electro-optical modulator(EOM)is used to switch the excitation beam between the horizontal and vertical polarization states at a high frequency,which leads to solid-and donut-shaped beams after spatial light modulation.Experiment on the fluorescent nanoparticles demonstrates that the proposed method can achieve~λ=4 spatial resolution.Using the proposed system,the dynamic imaging of subcellular structures in living cells over time is achieved. 展开更多
关键词 SUPER-RESOLUTION fluorescence emission difference microscopy electro-optical modulator polarization modulation
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Suppression of Soliton Timing Jitters in Fibers with Random Birefringence by Periodical Polarization Modulation
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作者 CHEN Wei-cheng XU Wen-cheng 《Semiconductor Photonics and Technology》 CAS 2006年第4期224-227,237,共5页
Periodical polarization modulation scheme is proposed to suppress timing jitters induced by frequency fluctuations between two polarization components of solitons. In periodical polarization modulation scheme, the pol... Periodical polarization modulation scheme is proposed to suppress timing jitters induced by frequency fluctuations between two polarization components of solitons. In periodical polarization modulation scheme, the polarization states of the soliton are modulated to excite equally for suppressing timing jitters induced by two unequal polarization components in the soliton trapping. Moreover, polarization modulation can weaken the effect of random birefringence on the soliton pulses in each relay distance. The numerical result shows that the soliton timing jitters are suppressed by our proposed method. 展开更多
关键词 Timing jitter Random birefringence polarization modulation SOLITON
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Super-resolution fluorescence polarization microscopy 被引量:4
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作者 Karl Zhanghao Juntao Gao +2 位作者 Dayong Jin Xuedian Zhang Peng Xi 《Journal of Innovative Optical Health Sciences》 SCIE EI CAS 2018年第1期1-12,共12页
Fluorescence polarization is related to the dipole orientation of chromophores,making fuores-cence polarization microscopy possible to_reveal structures and functions of tagged cellularorganelles and biological macrom... Fluorescence polarization is related to the dipole orientation of chromophores,making fuores-cence polarization microscopy possible to_reveal structures and functions of tagged cellularorganelles and biological macromolecules.Several recent super resolution techniques have beenapplied to fluorescence polarization microscopy,achieving dipole measurement at nanoscale.In this review,we summarize both difraction limited and super resolution fluorescence polari-zation microscopy techniques,as well as their applications in biological imaging. 展开更多
关键词 Fluorescence polarization microscopy super resolution fluorescence anisotropy linear dichroism polarization modulation
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Robust and high-speed rotation control in optical tweezers by using polarization synthesis based on heterodyne interference 被引量:5
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作者 Wei Liu Dashan Dong +2 位作者 Hong Yang Qihuang Gong Kebin Shi 《Opto-Electronic Advances》 2020年第8期23-29,共7页
The rotation control of particles in optical tweezers is often subject to the spin or orbit angular momentum induced optical torque,which is susceptible to the mechanical and morphological properties of individual par... The rotation control of particles in optical tweezers is often subject to the spin or orbit angular momentum induced optical torque,which is susceptible to the mechanical and morphological properties of individual particle.Here we report on a robust and high-speed rotation control in optical tweezers by using a novel linear polarization synthesis based on optical heterodyne interference between two circularly polarized lights with opposite handedness.The synthesized linear polarization can be rotated in a hopping-free scheme at arbitrary speed determined electronically by the heterodyne frequency between two laser fields.The experimental demonstration of a trapped vaterite particle in water shows that the precisely controlled rotation frequency of 300 Hz can be achieved.The proposed method will find promising applications in optically driven micro-gears,fluidic pumps and rotational micro-rheology. 展开更多
关键词 polarization modulation optical heterodyne optical tweezers optical rotation
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Linear polarization holography 被引量:7
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作者 Jinyu Wang Xiaodi Tan +9 位作者 Peiliang Qi Chenhao Wu Lu Huang Xianmiao Xu Zhiyun Huang Lili Zhu Yuanying Zhang Xiao Lin Jinliang Zang Kazuo Kuroda 《Opto-Electronic Science》 2022年第2期10-29,共20页
Polarization holography is a newly researched field,that has gained traction with the development of tensor theory.It primarily focuses on the interaction between polarization waves and photosensitive materials.The ex... Polarization holography is a newly researched field,that has gained traction with the development of tensor theory.It primarily focuses on the interaction between polarization waves and photosensitive materials.The extraordinary capabil-ities in modulating the amplitude,phase,and polarization of light have resulted in several new applications,such as holo-graphic storage technology,multichannel polarization multiplexing,vector beams,and optical functional devices.In this paper,fundamental research on polarization holography with linear polarized wave,a component of the theory of polariz-ation holography,has been reviewed.Primarily,the effect of various polarization changes on the linear and nonlinear po-larization characteristics of reconstructed wave under continuous exposure and during holographic recording and recon-struction have been focused upon.The polarization modulation realized using these polarization characteristics exhibits unusual functionalities,rendering polarization holography as an attractive research topic in many fields of applications.This paper aims to provide readers with new insights and broaden the application of polarization holography in more sci-entific and technological research fields. 展开更多
关键词 polarization holography tensor theory polarization modulation linear and nonlinear polarization characteristics
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Switchable Optical Ultra-Wideband Pulse Generator Based on Polarization Modulator
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作者 魏志虎 王荣 +2 位作者 蒲涛 孙帼丹 方涛 《China Communications》 SCIE CSCD 2013年第7期113-117,共5页
In order to generate optical Ultra- Wideband (UWB) pulse train with a switchable shape, a novel method based on a Polarization Modulator (PolM), a Polarization Controller (PC) and a delay line, is proposed and e... In order to generate optical Ultra- Wideband (UWB) pulse train with a switchable shape, a novel method based on a Polarization Modulator (PolM), a Polarization Controller (PC) and a delay line, is proposed and experimentally demonstrated. Experimental results show that when a Gaussian pulse is applied to the PolM, under different phase shifts introduced by the PC, a gauss or gauss doublet pulse will be generated at the output of the Polarization Beam Splitter (PBS). If the two- path signals after PBS are properly delayed, Gaussian monocycles or third-order gauss pulses will be generated at the output of the Polarization Beam Combiner (PBC). 展开更多
关键词 optical communication UWB polarization modulation
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Wideband Tunable Frequency-Doubling Optoelectronic Oscillator Using a Polarization Modulator and an Optical Bandpass Filter
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作者 黄庆超 王琪 +3 位作者 杨成悟 陈伟 刘建国 祝宁华 《Chinese Physics Letters》 SCIE CAS CSCD 2017年第8期67-70,共4页
A wideband tunable frequency-doubling optoelectronic oscillator (FD-OEO) is proposed and experimentally demonstrated based on a polarization modulator and an optical bandpass filter (OBPF). The central frequency o... A wideband tunable frequency-doubling optoelectronic oscillator (FD-OEO) is proposed and experimentally demonstrated based on a polarization modulator and an optical bandpass filter (OBPF). The central frequency of the correspondingly fundamental OEO could be adjusted by tuning the bandwidth and central frequency of the OBPF, which could also be regarded as a photonic-assisted tunable microwave filter. The frequency tuning range of the FD-OEO covers from 9.5 to 32.8?GHz, and the single sideband phase noise of the fundamental signal is lower than -100dBc/Hz at an offset of 10?kHz. Moreover, the frequency stability of the generated signal is investigated by measuring its Allan deviation. The Allan deviation of the generated fundamental signal at 10?GHz is 2.39×10^-9. 展开更多
关键词 Wideband Tunable Frequency-Doubling Optoelectronic Oscillator Using a polarization Modulator and an Optical Bandpass Filter FD
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Simulation of Intermediate State Absorption Enhancement in Rare-Earth Ions by Polarization Modulated Femtosecond Laser Field
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作者 Wen-Jing Cheng Shi-Hua Zhao 《Chinese Physics Letters》 SCIE CAS CSCD 2018年第11期23-27,共5页
We extend the third perturbation theory to study the polarization control behavior of the intermediate state absorption in Nd^(3+)ions. The results show that coherent interference can occur between the single-photo... We extend the third perturbation theory to study the polarization control behavior of the intermediate state absorption in Nd^(3+)ions. The results show that coherent interference can occur between the single-photon and three-photon excitation pathways, and depends on the central frequency of the femtosecond laser field. Moreover,single-photon and three-photon absorptions have different polarization control efficiencies, and the relative weight of three-photon absorption in the whole excitation processes can increase with increasing the laser intensity.Therefore, the enhancement or suppression of the intermediate state absorption can be realized and manipulated by properly designing the intensity and central frequency of the polarization modulated femtosecond laser field.This research can not only enrich theoretical research methods for the up-conversion luminescence manipulation of rare-earth ions, but also can provide a clear physical picture for understanding and controlling multi-photon absorption in a multiple energy level system. 展开更多
关键词 ab Simulation of Intermediate State Absorption Enhancement in Rare-Earth Ions by polarization Modulated Femtosecond Laser Field
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A Golden Decade of Polar Codes:From Basic Principle to 5G Applications 被引量:3
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作者 Kai Niu Ping Zhang +2 位作者 Jincheng Dai Zhongwei Si Chao Dong 《China Communications》 SCIE CSCD 2023年第2期94-121,共28页
After the pursuit of seventy years,the invention of polar codes indicates that we have found the first capacity-achieving coding with low complexity construction and decoding,which is the great breakthrough of the cod... After the pursuit of seventy years,the invention of polar codes indicates that we have found the first capacity-achieving coding with low complexity construction and decoding,which is the great breakthrough of the coding theory in the past two decades.In this survey,we retrospect the history of polar codes and summarize the advancement in the past ten years.First,the primary principle of channel polarization is investigated such that the basic construction,coding method and the classic successive cancellation(SC)decoding are reviewed.Second,in order to improve the performance of the finite code length,we introduce the guiding principle and conclude five design criteria for the construction,design and implementation of the polar code in the practical communication system based on the exemplar schemes in the literature.Especially,we explain the design principle behind the concatenated coding and rate matching of polar codes in 5G wireless system.Furthermore,the improved SC decoding algorithms,such as SC list(SCL)decoding and SC stack(SCS)decoding etc.,are investigated and compared.Finally,the research prospects of polar codes for the future 6G communication system are explored,including the optimization of short polar codes,coding construction in fading channels,polar coded modulation and HARQ,and the polar coded transmission,namely polar processing.Predictably,as a new coding methodology,polar codes will shine a light on communication theory and unveil a revolution in transmission technology. 展开更多
关键词 polar codes channel polarization successive cancellation decoding polar coded modulation polar processing
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Super-resolution dipole orientation mapping via polarization demodulation 被引量:13
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作者 Karl Zhanghao Long Chen +7 位作者 Xu-San Yang Miao-Yan Wang Zhen-Li Jing Hong-Bin Han Michael Q Zhang Dayong Jin Jun-Tao Gao Peng Xi 《Light(Science & Applications)》 SCIE EI CAS CSCD 2016年第1期112-119,共8页
Fluorescence polarization microscopy(FPM)aims to detect the dipole orientation of fluorophores and to resolve structural information for labeled organelles via wide-field or confocal microscopy.Conventional FPM often ... Fluorescence polarization microscopy(FPM)aims to detect the dipole orientation of fluorophores and to resolve structural information for labeled organelles via wide-field or confocal microscopy.Conventional FPM often suffers from the presence of a large number of molecules within the diffraction-limited volume,with averaged fluorescence polarization collected from a group of dipoles with different orientations.Here,we apply sparse deconvolution and least-squares estimation to fluorescence polarization modulation data and demonstrate a super-resolution dipole orientation mapping(SDOM)method that resolves the effective dipole orientation from a much smaller number of fluorescent molecules within a sub-diffraction focal area.We further apply this method to resolve structural details in both fixed and live cells.For the first time,we show that different borders of a dendritic spine neck exhibit a heterogeneous distribution of dipole orientation.Furthermore,we illustrate that the dipole is always perpendicular to the direction of actin filaments in mammalian kidney cells and radially distributed in the hourglass structure of the septin protein under specific labelling.The accuracy of the dipole orientation can be further mapped using the orientation uniform factor,which shows the superiority of SDOM compared with its wide-field counterpart as the number of molecules is decreased within the smaller focal area.Using the inherent feature of the orientation dipole,the SDOM technique,with its fast imaging speed(at sub-second scale),can be applied to a broad range of fluorescently labeled biological systems to simultaneously resolve the valuable dipole orientation information with super-resolution imaging. 展开更多
关键词 DIPOLE fluorescence polarization microscopy orientation mapping polarization modulation SUPER-RESOLUTION
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A position sensor based on grating projection with spatial filtering and polarization modulation 被引量:3
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作者 胡建明 曾爱军 王向朝 《Chinese Optics Letters》 SCIE EI CAS CSCD 2006年第1期18-20,共3页
A position sensor based on grating projection with spatial filtering and polarization modulation is presented. A grating is projected onto the object to be measured through a 4f optical system with a spatial filter. A... A position sensor based on grating projection with spatial filtering and polarization modulation is presented. A grating is projected onto the object to be measured through a 4f optical system with a spatial filter. After reflected by the object, the grating projection is imaged on a detection grating through another 4f optical system to form moiré fringes, The polarization modulated moiré signal is detected to obtain the position information of the object. In the position sensor, the moiré signal varies sinusoidally with the position of object. The measurement is independent of the incident intensity on the projection grating and the reflectivity of the object to be measured, In experiments, the effectiveness of the position sensor is proved, and the root mean square (RMS) error at each measurement position is less than 13 nm. 展开更多
关键词 A position sensor based on grating projection with spatial filtering and polarization modulation
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Experimental realization to efficiently sort vector beams by polarization topological charge via Pancharatnam–Berry phase modulation 被引量:3
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作者 SHUIQIN ZHENG YING LI +6 位作者 QINGGANG LIN XUANKE ZENG GUOLIANG ZHENG YI CAI ZHENKUAN CHEN SHIXIANG XU DIANYUAN FAN 《Photonics Research》 SCIE EI 2018年第5期385-389,共5页
This paper reports the experimental realization of efficiently sorting vector beams by polarization topological charge (PTC). The PTC of a vector beam can be defined as the repetition number of polarization state ch... This paper reports the experimental realization of efficiently sorting vector beams by polarization topological charge (PTC). The PTC of a vector beam can be defined as the repetition number of polarization state change along the azimuthal axis, while its sign stands for the rotating direction of the polarization. Here, a couple of liquid crystal Pancharatnam-Berry optical dements (PBOEs) have been used to introduce conjugated spatial phase modulations for two orthogonal circular polarization states. Applying these PBOEs in a 4-foptical system, our experiments show the setup can work for PTC sorting with a separation efficiency of more than 58%. This work provides an effective way to decode information from different PTCs, which may be interesting in many fields, especially in optical communication. 展开更多
关键词 Experimental realization to efficiently sort vector beams polarization topological charge via Pancharatnam-Berry phase modulation
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Remote Absolute Roll-Angle Measurement in Range of 180°Based on Polarization Modulation 被引量:1
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作者 Xiuguo Chen Jinbao Liao +3 位作者 Honggang Gu Chuanwei Zhang Hao Jiang Shiyuan Liu 《Nanomanufacturing and Metrology》 2020年第3期228-235,共8页
Remote measurement of object orientation is often required in many applications.Out of the six degrees of freedom(DoF)that determine object orientation in space,the roll angle is the most difficult to measure using op... Remote measurement of object orientation is often required in many applications.Out of the six degrees of freedom(DoF)that determine object orientation in space,the roll angle is the most difficult to measure using optical methods.In this letter,we propose a remote Stokes roll-angle sensor that measures roll angles from the detected Stokes vectors of modulated polarized light retroreflected from a sensing unit comprised simply of a retarder and a planar reflection mirror.Experimental results have shown that the proposed sensor can realize absolute roll angle measurement in an unprecedented range of 180°with a maximum absolute error of less than 0.25°and a measurement resolution of better than 0.01°.The proposed sensor adopts a coaxial design and takes the advantages of compactness,simplicity and low cost,and moreover,can be further expanded to a three-DoF angle sensor due to the sensitivity of the sensing unit to other two kinds of angles(pitch and yaw). 展开更多
关键词 Roll angle Angle sensor polarization modulation Stokes polarimeter
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A novel x-ray circularly polarized ranging method
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作者 宋诗斌 许录平 +2 位作者 张华 高娜 申洋赫 《Chinese Physics B》 SCIE EI CAS CSCD 2015年第5期503-513,共11页
Range measurement has found multiple applications in deep space missions. With more and further deep space ex- ploration activities happening now and in the future, the requirement for range measurement has risen. In ... Range measurement has found multiple applications in deep space missions. With more and further deep space ex- ploration activities happening now and in the future, the requirement for range measurement has risen. In view of the future ranging requirement, a novel x-ray polarized ranging method based on the circular polarization modulation is proposed, termed as x-ray circularly polarized ranging (XCPolR). XCPolR utilizes the circular polarization modulation to process x-ray signals and the ranging information is conveyed by the circular polarization states. As the circular polarization states present good stability in space propagation and x-ray detectors have light weight and low power consumption, XCPolR shows great potential in the long-distance range measurement and provides an option for future deep space ranging. In this paper, we present a detailed illustration of XCPolR. Firstly, the structure of the polarized ranging system is described and the signal models in the ranging process are established mathematically. Then, the main factors that affect the ranging accuracy, including the Doppler effect, the differential demodulation, and the correlation error, are analyzed theoretically. Finally, numerical simulation is carded out to evaluate the performance of XCPolR. 展开更多
关键词 x-ray ranging circular polarization modulation deep space regenerative ranging
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Quantum Computation with Nonlinear Optics
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作者 LIU Yang ZHANG Wen-Hong +1 位作者 ZHANG Cun-Lin LONG Gui-Lu 《Communications in Theoretical Physics》 SCIE CAS CSCD 2008年第1期107-110,共4页
We propose a scheme of quantum computation with nonlinear quantum optics. Polarization states of photons are used for qubits. Photons with different frequencies represent different qubits. Single qubit rotation operat... We propose a scheme of quantum computation with nonlinear quantum optics. Polarization states of photons are used for qubits. Photons with different frequencies represent different qubits. Single qubit rotation operation is implemented through optical elements like the Faraday polarization rotator. Photons are separated into different optical paths, or merged into a single optical path using dichromatic mirrors. The controlled-NOT gate between two qubits is implemented by the proper combination of parametric up and down conversions. This scheme has the following features: (1) No auxiliary qubits are required in the controlled-NOT gate operation; (2) No measurement is required in the course of the computation; (3) It is resource efficient and conceptually simple. 展开更多
关键词 quantum computation nonlinear optics parametric up(down)-conversion polarization modulator
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Creation of Multiple Subwavelength Focal Spot Segments Using Phase Modulated Radially Polarized Multi Gaussian Beam
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作者 K.Prabakaran K.B.Rajesh +4 位作者 S.Sumathira M.D.Bharathi R.Hemamalini A.M.Musthafa V.Aroulmoji 《Chinese Physics Letters》 SCIE CAS CSCD 2016年第9期48-51,共4页
Based on the vector diffraction theory, the effect of complex phase filters on intensity distribution of a radially polarized multi Gaussian beam in the focal region of high NA lens is theoretically investigated. It i... Based on the vector diffraction theory, the effect of complex phase filters on intensity distribution of a radially polarized multi Gaussian beam in the focal region of high NA lens is theoretically investigated. It is observed that a properly designed multi belt complex phase filter can generate subwavelength novel focal patterns including splitting of focal spots and generation of multiple focal spot segments such as eight, six and four focal spots along the optical axis are obtained. We expect that such an investigation is useful for optical manipulation and material processing, multiple high refractive index particle trapping technologies. 展开更多
关键词 of for Creation of Multiple Subwavelength Focal Spot Segments Using Phase Modulated Radially Polarized Multi Gaussian Beam on is in
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Tight Focusing Properties of Phase Modulated Radially Polarized Laguerre Bessel Gaussian Beam
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作者 K.Prabakaran P.Sangeetha +2 位作者 V.Karthik K.B.Rajesh A.M.Musthafa 《Chinese Physics Letters》 SCIE CAS CSCD 2017年第5期56-59,共4页
We propose a new approach for generating a multiple focal spot segment of subwavelength size, by tight focusing of a phase modulated radially polarized Laguerre Bessel Gaussian beam. The focusing properties are invest... We propose a new approach for generating a multiple focal spot segment of subwavelength size, by tight focusing of a phase modulated radially polarized Laguerre Bessel Gaussian beam. The focusing properties are investigated theoretically by .vector diffraction theory. We observe that the focal segment with multiple focal structures is separated with different axial distances and a super long dark channel can be generated by properly tuning the phase of the incident radially polarized Laguerre Bessel Gaussian beam. We presume that such multiple focal patterns and high intense beam may find applications in atom optics, optical manipulations and multiple optical trapping. 展开更多
关键词 Tight Focusing Properties of Phase Modulated Radially Polarized Laguerre Bessel Gaussian Beam
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Plasmonic enhancement and polarization dependence of nonlinear upconversion emissions from single gold nanorod@SiO_(2)@CaF2:Yb^(3+),Er^(3+)hybrid core–shell–satellite nanostructures 被引量:2
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作者 Jijun He Wei Zheng +8 位作者 Filip Ligmajer Chi-Fai Chan Zhiyong Bao Ka-Leung Wong Xueyuan Chen Jianhua Hao Jiyan Dai Siu-Fung Yu Dang Yuan Lei 《Light(Science & Applications)》 SCIE EI CAS CSCD 2016年第1期224-234,共11页
Lanthanide-doped upconversion nanocrystals(UCNCs)have recently become an attractive nonlinear fluorescence material for use in bioimaging because of their tunable spectral characteristics and exceptional photostabilit... Lanthanide-doped upconversion nanocrystals(UCNCs)have recently become an attractive nonlinear fluorescence material for use in bioimaging because of their tunable spectral characteristics and exceptional photostability.Plasmonic materials are often introduced into the vicinity of UCNCs to increase their emission intensity by means of enlarging the absorption cross-section and accelerating the radiative decay rate.Moreover,plasmonic nanostructures(e.g.,gold nanorods,GNRs)can also influence the polarization state of the UC fluorescence—an effect that is of fundamental importance for fluorescence polarization-based imaging methods yet has not been discussed previously.To study this effect,we synthesized GNR@SiO_(2)@CaF2:Yb^(3+),Er^(3+)hybrid core–shell–satellite nanostructures with precise control over the thickness of the SiO_(2) shell.We evaluated the shell thicknessdependent plasmonic enhancement of the emission intensity in ensemble and studied the plasmonic modulation of the emission polarization at the single-particle level.The hybrid plasmonic UC nanostructures with an optimal shell thickness exhibit an improved bioimaging performance compared with bare UCNCs,and we observed a polarized nature of the light at both UC emission bands,which stems from the relationship between the excitation polarization and GNR orientation.We used electrodynamic simulations combined with Förster resonance energy transfer theory to fully explain the observed effect.Our results provide extensive insights into how the coherent interaction between the emission dipoles of UCNCs and the plasmonic dipoles of the GNR determines the emission polarization state in various situations and thus open the way to the accurate control of the UC emission anisotropy for a wide range of bioimaging and biosensing applications. 展开更多
关键词 Förster resonance energy transfer gold nanorods lanthanide-doped upconversion nanocrystals plasmon-enhanced nonlinear fluorescence polarization modulation
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